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Computational Design of Azo-anthraquinone Schiff Base Mn Complexes as Mediators for Biofuel Cell Cathode

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Journal of Chemistry and Chemical Engineering 2019年第1期13卷 23-33页

作者： Kazuto Kajiwara Shinsuke Yamane Tomoyuki Haraguchi Sayantan Pradhan Chittaranjan Sinha Rakesh Parida Santanab giri Gourisankar Roymahaptra Dohyun Moon Takashiro Akitsu Department of Chemistry Faculty of Science Tokyo University of Science Tokyo Japan Chemical Sciences Division Saha Institute of Nuclear Physics Kolkata West Bengal India Department of Chemistry Jadavpur University Kolkata West Bengal India Department of Chemistry National Institute of Technology Rourkela India Department of Applied Sciences Haldia Institute of Technology Haldia West Bengal India Beamline Department Pohang Accelerator Laboratory Pohang Korea

The cathode of biofuel cell reduces molecular oxygen to water using four electrons, an enzyme of multicopper oxidase family, laccase, is contained, though its electron transfer efficiency from the electrode resulted in rate determining process. To improve this electron, transfer via mediators, we have investigated several mediator metal complexes between the electrode and laccase, in particular hydrophobic pocket on the surface. We have discussed DFT computational results and selected experimental data of new Mn(III/II) Schiff base complexes having redox active (anthraquinone) ligands and photochromic (azobenzene) ligands about azobenzene moiety at the sole molecular level. Moreover, we carried out computational docking simulation of laccase and complexes considering trans-cis photoisomerization (electronic states) and Weigert effect (molecular orientation to fit better) of azobenzene moiety. Additionally, actual experimental data also presented to indicate the expected merits for mediators.

关键词： Laccase Schiff base Mn complex anthraquinone azobenzne computational chemistry

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口服胺碘酮可预防心脏手术后心房纤颤

国外医学（护理学分册） 2001年第9期20卷 440-440页

作者： giri S 计惠民黄敏捷

据报道，心脏直视手术后心房纤颤的发生率约为２７％～４０％。美国Ｈａｒｔｆｏｒｄ医院科研人员近年的一项研究结果表明，心脏直视手术病人在围手术期口服胺碘酮和β阻滞剂，可有效降低手术后发生各种心房纤颤、脑血管意外和心动过速... 详细信息

据报道，心脏直视手术后心房纤颤的发生率约为２７％～４０％。美国Ｈａｒｔｆｏｒｄ医院科研人员近年的一项研究结果表明，心脏直视手术病人在围手术期口服胺碘酮和β阻滞剂，可有效降低手术后发生各种心房纤颤、脑血管意外和心动过速的危险性。这项随机、双盲、安慰剂对照试验的对象，是从１９９８年２月至１９９９年４月间住院病人中选择的２２０例已服用β阻滞剂需接受心脏直视手术者，年龄均在６０岁以上，平均年龄为７３岁。其中１２０例病人口服胺碘酮，为实验组；其余１００例病人服用安慰剂，为对照组。实验组中距手术日≥５ｄ的６４例病人，在手术前５ｄ内每日服用胺碘酮３次，每次２００ｍｇ；手术后１～４ｄ每日服用胺碘酮２次，每次４００ｍｇ。对照组中距手术日≥５ｄ的５６例病人服用安慰剂。实验组中距手术日不足５ｄ但超过１ｄ的５６例病人，在手术前１ｄ服用胺碘酮４次，每次４００ｍｇ，手术日服用胺碘酮２次，每次６００ｍｇ。对照组中距手术日不足５ｄ但超过１ｄ的４４例病人服用安慰剂。研究结果表明，口Ｂｉｏ碘酮的实验组病人，其心脏直视手术后各种心房纤颤的发生率明显低于眼用安慰剂的对照组（２２．５％对３８．０％，Ｐ—０．０１）；症状性房颤（４．２％对１８．０％...

关键词：心脏直视手术并发症心房纤颤胺碘酮预防

疫苗性脊灰病毒的排泄量可确定印度口服疫苗儿童血清中和抗体应答的滴度

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微生物学免疫学进展 2019年第6期47卷 46-46页

作者：李安敏陈锦荣(校) giri S 不详

口服脊灰疫苗(OPV)在肠道内的复制(即疫苗接种)与血清阳转和抗脊髓灰质炎的保护作用有关。作者用定量聚合酶链反应分析法测定300名 6~11 月龄血清阴性婴儿和218名1~4岁血清阴性幼儿,在接受单价或双价OPV后 7 d他们的疫苗排泄情况。发现... 详细信息

口服脊灰疫苗(OPV)在肠道内的复制(即疫苗接种)与血清阳转和抗脊髓灰质炎的保护作用有关。作者用定量聚合酶链反应分析法测定300名 6~11 月龄血清阴性婴儿和218名1~4岁血清阴性幼儿,在接受单价或双价OPV后 7 d他们的疫苗排泄情况。发现排苗的数量与疫苗接种后21、28 d测得的血清中和抗体应答量相关。这提示,对OPV的免疫应答是连续性的,而不是全或无表象,免疫应答取决于疫苗病毒的有效复制。

关键词：定量聚合酶链反应脊髓灰质炎排泄情况疫苗接种免疫应答脊灰病毒 OPV 口服疫苗

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应用田口设计法探讨影响地毯压缩性能的因素

国际纺织导报 2018年第9期46卷 14-14页

作者： R.K.Verma A.Agarwal P.Srivastava S.K.giri 刘书惠(译) 孟粉叶(校) 印度地毯技术研究所(IICT) 印度不详

为满足客户对产品高品质与快速可靠的交付要求，新的加工制造技术正飞速发展，这也促进了新产品的开发与制造工艺的改进。地毯主要可分为机制地毯和手工地毯两类，机制地毯有时也称动力制造地毯。各种机制地毯通常可通过针刺与黏合技术... 详细信息

为满足客户对产品高品质与快速可靠的交付要求，新的加工制造技术正飞速发展，这也促进了新产品的开发与制造工艺的改进。地毯主要可分为机制地毯和手工地毯两类，机制地毯有时也称动力制造地毯。各种机制地毯通常可通过针刺与黏合技术制备。

关键词：手工地毯压缩性能设计法加工制造技术田口应用制造工艺机制

Measurement of the integrated luminosity of the Phase 2 data of the Belle Ⅱ experiment

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Chinese Physics C 2020年第2期44卷 1-12页

作者： F.Abudinén I.Adachi P.Ahlburg H.Aihara N.Akopov A.Aloisio F.Ameli L.Andricek N.Anh Ky D.M.Asner H.Atmacan T.Aushev V.Aushev T.Aziz K.Azmi V.Babu S.Baehr S.Bahinipati A.M.Bakich P.Bambade Sw.Banerjee S.Bansal V.Bansal M.Barrett J.Baudot A.Beaulieu J.Becker P.K.Behera J.V.Bennett E.Bernieri F.U.Bernlochner M.Bertemes M.Bessner S.Bettarini V.Bhardwaj F.Bianchi T.Bilka S.Bilokin D.Biswas G.Bonvicini A.Bozek M.Bračko P.Branchini N.Braun T.E.Browder A.Budano S.Bussino M.Campajola L.Cao G.Casarosa C.Cecchi D.Červenkov M.-C.Chang P.Chang R.Cheaib V.Chekelian Y.Q.Chen Y.-T.Chen B.G.Cheon K.Chilikin H.-E.Cho K.Cho S.Cho S.-K.Choi S.Choudhury D.Cinabro L.Corona L.M.Cremaldi S.Cunliffe T.Czank F.Dattola E.De La Cruz-Burelo G.De Nardo M.De Nuccio G.De Pietro R.de Sangro M.Destefanis S.Dey A.De Yta-Hernandez F.Di Capua S.Di Carlo J.Dingfelder Z.Doležal I.Domínguez Jiménez T.V.Dong K.Dort S.Dubey S.Duell S.Eidelman M.Eliachevitch T.Ferber D.Ferlewicz G.Finocchiaro S.Fiore A.Fodor F.Forti A.Frey B.G.Fulsom M.Gabriel E.Ganiev M.Garcia-Hernandez R.Garg A.Garmash V.Gaur A.Gaz U.Gebauer A.Gellrich J.Gemmler T.Geßler R.Giordano A.giri B.Gobbo R.Godang P.Goldenzweig B.Golob P.Gomis P.Grace W.Gradl E.Graziani D.Greenwald C.Hadjivasiliou S.Halder K.Hara T.Hara O.Hartbrich K.Hayasaka H.Hayashii C.Hearty M.T.Hedges I.Heredia de la Cruz M.Hernández Villanueva A.Hershenhorn T.Higuchi E.C.Hill H.Hirata M.Hoek S.Hollitt T.Hotta C.-L.Hsu Y.Hu K.Huang T.Iijima K.Inami G.Inguglia J.Irakkathil Jabbar A.Ishikawa R.Itoh M.Iwasaki Y.Iwasaki S.Iwata P.Jackson W.W.Jacobs D.E.Jaffe E.-J.Jang H.B.Jeon S.Jia Y.Jin C.Joo J.Kahn H.Kakuno A.B.Kaliyar G.Karyan Y.Kato T.Kawasaki H.Kichimi C.Kiesling B.H.Kim C.-H.Kim D.Y.Kim S.-H.Kim Y.K.Kim Y.Kim T.D.Kimmel K.Kinoshita C.Kleinwort B.Knysh P.Kodyš T.Koga I.Komarov T.Konno S.Korpar D.Kotchetkov N.Kovalchuk T.M.G.Kraetzschmar P.Križan R.Kroeger J.F.Krohn P.Krokovny W.Kuehn T.Kuhr M.Kumar R.Kumar K.Kumara S.Kurz A.Kuzmin Y.-J.Kwon S.Lacaprara Y.-T.Lai C.La Licata K.Lalwani L.Lanceri J.S.Lange K.Lautenbach I.-S.Le Beihang University Beijing 100191 Brookhaven National Laboratory UptonNew York 11973 Budker Institute of Nuclear Physics SB RAS Novosibirsk 630090 Centro de Investigacion y de Estudios Avanzados del Instituto Politecnico Nacional Mexico City 07360 Faculty of Mathematics and Physics Charles University12116 Prague Chiba University Chiba 263-8522 Consejo Nacional de Ciencia y Tecnología Mexico City 03940 Deutsches Elektronen–Synchrotron 22607 Hamburg Duke University DurhamNorth Carolina 27708 Earthquake Research Institute University of TokyoTokyo 113-0032 Forschungszentrum Jülich 52425 Jülich Department of Physics Fu Jen Catholic UniversityTaipei 24205 Key Laboratory of Nuclear Physics and Ion-beam Application(MOE)and Institute of Modern Physics Fudan UniversityShanghai 200443 II.Physikalisches Institut Georg-August-Universität Göttingen37073 Göttingen Gifu University Gifu 501-1193 The Graduate University for Advanced Studies(SOKENDAI) Hayama 240-0193 Gyeongsang National University Jinju 52828 Department of Physics and Institute of Natural Sciences Hanyang UniversitySeoul 04763 High Energy Accelerator Research Organization(KEK) Tsukuba 305-0801 J-PARC Branch KEK Theory CenterHigh Energy Accelerator Research Organization(KEK)Tsukuba 305-0801 Indian Institute of Science Education and Research Mohali SAS Nagar140306 Indian Institute of Technology Bhubaneswar Satya Nagar 751007 Indian Institute of Technology Hyderabad Telangana 502285 Indian Institute of Technology Madras Chennai 600036 Indiana University BloomingtonIndiana 47408 Institute for High Energy Physics Protvino 142281 Institute of High Energy Physics Vienna 1050 Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049 Institute of Particle Physics(Canada) VictoriaBritish Columbia V8W 2Y2 Institute of Physics Hanoi Instituto de Fisica Corpuscular Paterna 46980 INFN Laboratori Nazionali di Frascati I-00044 Frascati INFN Sezione di Napoli I-80126 Napoli INFN Sezione di Padova I-35131 Padova INFN Sezione di Perugia I-06123 Perugia

From April to July 2018,a data sample at the peak energy of the T(4 S) resonance was collected with the Belle Ⅱ detector at the SuperKEKB electron-positron *** is the first data sample of the Belle Ⅱ *** Bhabha and digamma events,we measure the integrated luminosity of the data sample to be(496.3±0.3±3.0) pb-1,where the first uncertainty is statistical and the second is *** work provides a basis for future luminosity measurements at Belle Ⅱ.

关键词： luminosity Bhabha digamma Belle II