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Nitric oxide assists nitrogen reduction reaction on 2D MBene: A theoretical study

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Chinese Chemical Letters 2024年第5期35卷 428-433页

作者： Chaozheng He jia Wang Ling Fu Wei Wei Henan Engineering Center of New Energy Battery Materials College of Chemistry and Chemical EngineeringShangqiu Normal UniversityShangqiu 476000China School of Chemistry and Chemical Engineering Shandong Provincial Key Laboratory/Collaborative Innovation Center of Chemical Energy Storage&Novel Cell TechnologyLiaocheng UniversityLiaocheng 252059China Institute of Environment and Energy Catalysis Shaanxi Key Laboratory of Optoelectronic Functional Materials and DevicesSchool of Materials Science and Chemical EngineeringXi’an Technological UniversityXi’an 710021China College of Resources and Environmental Engineering Tianshui Normal UniversityTianshui 741001China

Electrocatalytic synthesis of ammonia as an environment-friendly and sustainable development method has received widespread attention in recent ***-dimensional(2D)materials are a promising catalyst for ammonia synthesis due to their large surface *** this work,we have constructed a series of 2D metal borides(MBenes)with transition metal(TM)defects(TMd-MBenes)and comprehensively calculated the reactivity of electrocatalytic synthesis of ammonia-based on density functional *** results have demonstrated that the TMd-MBenes can effectively activate nitrogen oxide(NO)and nitrogen(N2)molecules *** interesting,the co-chemisorption of O atoms,dissociated from NO,can facilitate the spilled of the inert N2 molecules into single N atoms,which can further hydrogenate into ammonia easily with an ultralow limiting potential of 0.59 V on *** research has not only provided clues for catalyst design for experimental study but also paved the way for the industrial application of electrocatalytic ammonia synthesis.

关键词： 2D mbenes Nitrogen electro-reduction DFT N_(2)activation Ammonia synthesis

Improving the Short-Range Precipitation Forecast of Numerical Weather Prediction through a Deep Learning-Based Mask Approach

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Advances in Atmospheric Sciences 2024年第8期41卷 1601-1613页

作者： jiaqi ZHENG Qing LING jia LI Yerong FENG School of Computer Science and Engineering/Guangdong Provincial Key Laboratory of Computational Science Sun Yat-Sen UniversityGuangzhou 510006China School of Mathematics Sun Yat-Sen UniversityGuangzhou 510275China Guangzhou Institute of Tropical and Marine Meteorology/Guangdong Provincial Key Laboratory of Regional Numerical Weather Prediction Guangzhou 510641China Shenzhen Institute of Meteorological Innovation Shenzhen 518038China

Due to various technical issues,existing numerical weather prediction(NWP)models often perform poorly at forecasting rainfall in the first several *** correct the bias of an NWP model and improve the accuracy of short-range precipitation forecasting,we propose a deep learning-based approach called UNet Mask,which combines NWP forecasts with the output of a convolutional neural network called *** UNet Mask involves training the UNet on historical data from the NWP model and gridded rainfall observations for 6-hour precipitation *** overlap of the UNet output and the NWP forecasts at the same rainfall threshold yields a *** UNet Mask blends the UNet output and the NWP forecasts by taking the maximum between them and passing through the mask,which provides the corrected 6-hour rainfall *** evaluated UNet Mask on a test set and in real-time *** results showed that UNet Mask outperforms the NWP model in 6-hour precipitation prediction by reducing the FAR and improving CSI *** tests also showed that different small rainfall thresholds applied to the UNet and the NWP model have different effects on UNet Mask's forecast *** study shows that UNet Mask is a promising approach for improving rainfall forecasting of NWP models.

关键词： deep learning numerical weather prediction(NWP) 6-hour quantitative precipitation forecast

Noise-induced phase transition in the Vicsek model through eigen microstate methodology

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Chinese Physics B 2024年第9期33卷 327-338页

作者： Yongnan jia jiali Han Qing Li School of Automation and Electrical Engineering University of Science and Technology BeijingBeijing 100083China

This paper presents a comprehensive framework for analyzing phase transitions in collective models such as theVicsek model under various noise types. The Vicsek model, focusing on understanding the collective behaviors of socialanimals, is known due to its discontinuous phase transitions under vector noise. However, its behavior under scalar noiseremains less conclusive. Renowned for its efficacy in the analysis of complex systems under both equilibrium and nonequilibriumstates, the eigen microstate method is employed here for a quantitative examination of the phase transitions inthe Vicsek model under both vector and scalar noises. The study finds that the Vicsek model exhibits discontinuous phasetransitions regardless of noise type. Furthermore, the dichotomy method is utilized to identify the critical points for thesephase transitions. A significant finding is the observed increase in the critical point for discontinuous phase transitions withescalation of population density.

关键词： Vicsek model phase transitions eigen microstate method noise

Constructing the metabolic network of wheat kernels based on structure-guided chemical modification and multi-omics data

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Journal of Genetics and Genomics 2024年第7期51卷 714-722页

作者： Zhitao Tian Jingqi jia Bo Yin Wei Chen National Key Laboratory of Crop Genetic Improvement and National Center of Plant Gene Research(Wuhan) Huazhong Agricultural UniversityWuhanHubei 430070China Hubei Hongshan Laboratory WuhanHubei 430070China

Metabolic network construction plays a pivotal role in unraveling the regulatory mechanism of biological activities,although it often proves to be challenging and labor-intensive,particularly with non-model *** this study,we develop a computational approach that employs reaction models based on the structure-guided chemical modification and related compounds to construct a metabolic network in *** construction results in a comprehensive structure-guided network,including 625 identified metabolites and additional 333 putative reactions compared with the Kyoto Encyclopedia of Genes and Genomes *** a combination of gene annotation,reaction classification,structure similarity,and correlations from transcriptome and metabolome analysis,a total of 229 potential genes related to these reactions are identified within this *** validate the network,the functionality of a hydroxycinnamoyltransferase(TraesCS3D01G314900)for the synthesis of polyphenols and a rhamnosyltransferase(TraesCS2D01G078700)for the modification of flavonoids are verified through in vitro enzymatic studies and wheat mutant tests,*** research thus supports the utility of structure-guided chemical modification as an effective tool in identifying causal candidate genes for constructing metabolic networks and further in metabolomic genetic studies.

关键词： Metabolic network Chemical modification Genetic study Wheat kernel Multi-omics

长春花感染黄龙病菌多酚氧化酶基因的表达及活性分析

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华南农业大学学报 2017年第2期38卷 63-68页

作者：李亚贾奥琳鲍敏丽许美容邓晓玲广东海洋大学农学院广东湛江524088 华南农业大学农学院/广东省微生物信号与作物病害防控重点试验室广东广州510642

【目的】分析长春花Catharanthus roseus受黄龙病菌Candidatus Liberibacter asiaticus侵染后多酚氧化酶(PPO)基因的表达及活性变化。【方法】根据不同作物多酚氧化酶基因PPO序列的相似性,筛选出长春花多酚氧化酶基因Pw PPO引物,PCR扩增... 详细信息

【目的】分析长春花Catharanthus roseus受黄龙病菌Candidatus Liberibacter asiaticus侵染后多酚氧化酶(PPO)基因的表达及活性变化。【方法】根据不同作物多酚氧化酶基因PPO序列的相似性,筛选出长春花多酚氧化酶基因Pw PPO引物,PCR扩增得Pw PPO基因片段,运用qRT-PCR和生理生化方法分析长春花嫁接黄龙病芽后,不同时间长春花叶、主茎和根中Pw PPO基因的表达量和酶活性变化。【结果】长春花受黄龙病菌侵染后,叶、主茎和根中Pw PPO基因的表达分别在嫁接后30、35和40 d上调表达4.23、12.64和33.80倍,不同组织中Pw PPO基因上调表达的时间和幅度不同。染病长春花的叶、主茎和根中PPO活性分别在嫁接后30、35和45 d为对照的2.87、2.10和1.89倍。【结论】Pw PPO基因表达量与PPO活性成正比,与长春花抵抗黄龙病菌侵染的能力密切相关。

关键词：长春花黄龙病菌多酚氧化酶基因表达多酚氧化酶(PPO)活性

Mutual Information Maximization via Joint Power Allocation in Integrated Sensing and Communications System

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China Communications 2024年第2期21卷 129-142页

作者： jia Zhu Junsheng Mu Yuanhao Cui Xiaojun Jing School of Information and Communication Engineering Beijing University of Posts and TelecommunicationsBeijing 100876China

In this paper, we focus on the power allocation of Integrated Sensing and Communication(ISAC) with orthogonal frequency division multiplexing(OFDM) waveform. In order to improve the spectrum utilization efficiency in ISAC, we propose a design scheme based on spectrum sharing, that is,to maximize the mutual information(MI) of radar sensing while ensuring certain communication rate and transmission power constraints. In the proposed scheme, three cases are considered for the scattering off the target due to the communication signals,as negligible signal, beneficial signal, and interference signal to radar sensing, respectively, thus requiring three power allocation schemes. However,the corresponding power allocation schemes are nonconvex and their closed-form solutions are unavailable as a consequence. Motivated by this, alternating optimization(AO), sequence convex programming(SCP) and Lagrange multiplier are individually combined for three suboptimal solutions corresponding with three power allocation schemes. By combining the three algorithms, we transform the non-convex problem which is difficult to deal with into a convex problem which is easy to solve and obtain the suboptimal solution of the corresponding optimization problem. Numerical results show that, compared with the allocation results of the existing algorithms, the proposed joint design algorithm significantly improves the radar performance.

关键词： coexistence communications multicarrier radar mutual information spectrum sharing

Aagab is required for zebrafish larval development by regulating neural activity

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Journal of Genetics and Genomics 2024年第6期51卷 630-641页

作者： Shihui Ding Tursunjan Aziz Anming Meng Shunji jia State Key Laboratory of Membrane Biology Tsinghua-Peking Center for Life SciencesSchool of Life SciencesTsinghua UniversityBeijing 100084China Guangzhou Laboratory GuangzhouGuangdong 510320China State Key Laboratory of Molecular Developmental Biology Institute of Genetics and Developmental BiologyChinese Academy of SciencesBeijing 100101China

Clathrin-mediated endocytosis has been implicated in various physiological processes,including nutrient uptake,signal transduction,synaptic vesicle recycling,maintenance of cell polarity,and antigen *** prior knowledge of its importance as a key regulator in promoting clathrin-mediated endocytosis,the physiological function of α-and γ-adaptin binding protein(aagab)remains *** this study,we investigate the biological function of aagab during zebrafish *** establish a loss-of-function mutant of aagab in zebrafish,revealing impaired swimming and early larval *** the high expression level of aagab in the brain,we probe into its physiological role in the nervous *** mutants display subdued calcium responses and local field potential in the optic tectal neurons,aligning with reduced neurotransmitter release(e.g.,norepinephrine)in the tectal neuropil of aagab *** aagab mRNA or nervous stimulant treatment in mutants restores neurotransmitter release,calcium responses,swimming ability,and ***,our observations show delayed release of FM 1-43 in AAGAB knockdown differentiated neuroblastoma cells,pointing towards a probable link to defective clathrin-mediated synaptic vesicle *** conclusion,our study underscores the significance of Aagab in neurobiology and suggests its potential impacts on neurological disorders.

关键词： Aagab Endocytosis Neural activity Synaptic transmitter release Zebrafish

Colorimetric Detection of Acid Phosphatase and Malathion Using NiCo_(2)O_(4)Nanosheets as Peroxidase-Mimicking Activity

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Journal of Analysis and Testing 2024年第2期8卷 170-179页

作者： jia Chen Zerong Long Yan Li Hongdeng Qiu Xinjiang Uygur Autonomous Product Quality Supervision and Inspection Institute Urumqi830000China CAS Key Laboratory of Chemistry of Northwestern Plant Resources and Key Laboratory for Natural Medicine of Gansu Province Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China

The establishment of a low-cost and facile approach for the assay of acid phosphatase(ACP)and its inhibitor is a research *** this paper,we successfully synthesized NiCo_(2)O_(4)nanosheets with peroxidase-mimicking activity in alkaline deep eutectic solvents(DESs)composed of NaOH and PEG-200,which can catalyze 3,3',5,5'-tetramethylbenzidine(TMB)to the oxidation state TMB(ox-TMB)in the presence of *** to L-ascorbic acid-2-phosphate can be hydrolyzed into ascorbic acid by ACP,the peroxidase-like activity of NiCo_(2)O_(4)nanosheets is ***,the addition of malathion,an inhibitor of ACP,can inhibit the activity of ACP and thus limit the production of ascorbic acid(AA).Therefore,a colorimetric approach can be established for highly sensitive and selective detection of ACP and malathion with detection limits of 0.032 U/L and 0.65 nmol/L,*** importantly,this method can be successfully applied to malathion detection in environmental samples tap water and food cucumber juice,indicating that it has potential application prospects in environmental and agricultural fields.

关键词： NiCo_(2)O_(4)nanosheets Acid phosphatase Malathion Peroxidase-mimicking activity Colorimetric

Impact of Media Information on Social Response in Disasters:A Case Study of the Freezing‑Rain and Snowstorm Disasters in Southern China in 2008

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International Journal of Disaster Risk Science 2024年第1期15卷 73-87页

作者： jia He Wenjing Duan Yuxuan Zhou Yun Su College of Geographic Science and Tourism Xinjiang Normal UniversityUrumqi 830054China Xinjiang Laboratory of Lake Environment and Resources in Arid Zone Urumqi 830054China Faculty of Geographical Science Beijing Normal UniversityBeijing 100875China Key Laboratory of Environmental Change and Natural Disaster Ministry of EducationBeijing Normal UniversityBeijing 100875China

Disaster information content is an objective mapping of disaster situations,social response,and public *** response to emergency is an important mechanism for implementing and guaranteeing emergency management of major natural hazard-related *** how disaster information content affects social response to emergencies is helpful for managing risk communication and efficient disaster *** on the 2008 freezing-rain and snowstorm disasters in southern China,this study used Python to extract 7,857 case-related media reports and applied natural language processing for text *** used three typical cases to identify and analyze disaster media report content and the relationship between these reports and the social response to the *** categories of disaster response-such as prewarning and forecasting,announcements by the authorities,and social mobilization-appeared in the disaster information in the media,along with disaster impact information,that is,real-time disaster *** response information and an appropriate amount of disaster impact information played important roles in prewarning,disaster relief,public opinion guidance,and social stability maintenance and can serve important functions in communicating with all stakeholders of emergency management,assisting or influencing emergency departments or individuals in decision making,and eliminating "information islands." Empathy caused the general public to become "disaster responders" through receiving *** and an excess of negative information may have a perverse amplification effect on public opinion and increase the unpredictability of the disaster situation and the risk of social crisis.

关键词： Emergency management Freezing-rain and snowstorm disasters Media reports on disasters Social response to emergencies China