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Templated synthesis of transition metal phosphide electrocatalysts for oxygen and hydrogen evolution reactions

Journal of Energy Chemistry 2024年第2期89卷 646-669,I0014页

作者： Rose anne Acedera Alicia Theresse Dumlao DJ Donn Matienzo Maricor Divinagracia Julie anne del Rosario Paraggua Po-Ya Abel Chuang Joey Ocon Laboratory of Electrochemical Engineering(LEE) Department of Chemical EngineeringUniversity of the PhilippinesDilimanQuezon City 1101Philippines Mechanical Engineering University of CaliforniaMercedCA 95343USA Energy Engineering Program College of EngineeringUniversity of the PhilippinesDilimanQuezon City 1101Philippines

Transition metal phosphides(TMPs)have been regarded as alternative hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)catalysts owing to their comparable activity to those of noble metal-based *** have been produced in various morphologies,including hollow and porous nanostructures,which are features deemed desirable for electrocatalytic *** synthesis routes are often responsible for such *** paper reviews the latest advances and existing challenges in the synthesis of TMP-based OER and HER catalysts through templated methods.A comprehensive review of the structure-property-performance of TMP-based HER and OER catalysts prepared using different templates is *** discussion proceeds according to application,first by HER and further divided among the types of templates used-from hard templates,sacrificial templates,and soft templates to the emerging dynamic hydrogen bubble *** catalysts are then reviewed and grouped according to their ***,prospective research directions for the synthesis of hollow and porous TMP-based catalysts,such as improvements on both activity and stability of TMPs,design of environmentally benign templates and processes,and analysis of the reaction mechanism through advanced material characterization techniques and theoretical calculations,are suggested.

关键词： OER HER Transition metal phosphide Templated synthesis Electrocatalysts

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Comparative study of the effects of terlipressin versus splenectomy on liver regeneration after partial hepatectomy in rats

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Hepatobiliary & Pancreatic Diseases International 2017年第5期16卷 506-511页

作者： Tom Florian Ulmer anne Weiland Georg Lurje Christian Klink anne Andert Hamid Alizai Christoph Heidenhain Ulf Neumann Department of General Visceral and Transplantation Surgery RWTH Aachen University Hospital Aachen Germany Department of Urology Helios Hospital Berlin-Buch Germany

BACKGROUND: Post-hepatectomy liver failure as a result of insufficient liver remnant is a feared complication in liver surgery. Efforts have been made to find new strategies to support liver regeneration. The aim of this study was to investigate the effects of terlipressin versus splenectomy on postoperative liver function and liver regeneration in rats undergoing 70%partial hepatectomy. METHODS: Seventy-two male Wistar rats were randomly assigned into three groups(n=24 in each group): 70% partial hepatectomy as control(PHC), 70% partial hepatectomy with splenectomy(PHS) or 70% partial hepatectomy with a micropump for terlipressin administration(PHT). Eight rats in each group were sacrificed on postoperative day(POD) 1,3 and 7. To assess liver regeneration, immunohistochemical analysis of liver tissue using bromodeoxyuridine(BrdU) and Ki-67 labeling was performed. Portal venous pressure, serum concentrations of creatinine, urea, albumin, bilirubin and prothrombin time as well as liver-, body-weight and their ratio were determined on POD 1, 3 and ***: The liver-, body-weight and their ratio were not statistically different among the groups. On POD 1, 3 and 7 portal venous pressure in the intervention groups(PHT:8.13 ±1.55, 10.38±1.30, 6.25±0.89 cm H2O and PHS: 7.50±0.93,8.88 ±2.42, 5.75±1.04 cm H2O) was lower compared to the control group(PHC: 8.63±2.06, 10.50±2.45, 6.50±2.67 cmH2O). Hepatocyte proliferation in the intervention groups was delayed, especially after splenectomy on POD 1(Brd U: PHS vs PHC, 20.85% ±13.05% vs 28.11%±10.10%; Ki-67, 20.14%±14.10% vs 23.96% ±11.69%). However, none of the differences were statistically ***: Neither the administration of terlipressin nor splenectomy improved liver regeneration after 70% partial hepatectomy in rats. Further studies assessing the regulation of portal venous pressure as well as extended hepatectomy animal models and liver function tests will help to further investigate mechanisms of live

关键词： liver regeneration liver failure terlipressin splenectomy hepatectomy

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Segmentation of Images from Fourier Spectral Data

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Communications in Computational Physics 2009年第2期5卷 326-349页

作者： anne Gelb Dennis Cates Department of Mathematics and Statistics Arizona State UniversityTempeArizona 85287 USA

This paper designs a segmentation method for an image based on its Fourier spectral *** edge map is generated directly from the Fourier coefficients without first reconstructing the image in pixelated *** the internal boundaries of the edge map are not blurred by any(filtered)Fourier *** edge map is then processed with an edge linking segmentation *** include examples from magnetic resonance imaging(MRI).Our results illustrate some potential benefits of using high order methods in imaging.

关键词： Fourier coefficients edge detection segmentation

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Potential risk factors for constipation in the community

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World Journal of Gastroenterology 2021年第21期27卷 2795-2817页

作者： Barry L Werth Sybele-anne Christopher Susan Wakil School of Nursing and Midwifery Faculty of Medicine and HealthUniversity of SydneySydney 2006New South WalesAustralia

Constipation is a common community health *** are many factors that are widely thought to be associated with constipation but real-world evidence of these associations is difficult to *** potential risk factors may be categorised as demographic,lifestyle and health-related *** review presents the available evidence for each factor by an assessment of quantitative data from cross-sectional studies of community-dwelling adults published over the last 30 *** appears that there is evidence of an association between constipation and female gender,residential location,physical activity and some health-related factors such as self-rated health,some surgery,certain medical conditions and certain *** available evidence for most other factors is either conflicting or ***,further research is necessary to determine if each factor is truly associated with constipation and whether it can be regarded as a potential risk *** is recommended that studies investigating a broad range of factors are conducted in populations in community *** analyses should be performed to account for all possible confounding *** this way,valuable evidence can be accumulated for a better understanding of potential risk factors for constipation in the community.

关键词： Adults Constipation Epidemiology Factors Community

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Xerotolerant foliar endophytic fungi of Populus euphratica from the Tarim River basin,Central China are conspecific to endophytic ITS phylotypes of Populus tremula from temperate Europe

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Fungal Diversity 2012年第3期54卷 133-142页

作者： Martin Unterseher anne Petzold Martin Schnittler Institute of Botany and Landscape Ecology Department of Systematic BotanyErnst-Moritz-Arndt UniversityGrimmer Str.8817487 GreifswaldGermany

Fungal research on non-lichenized taxa in xeric and other unusual habitats for fungi is comparatively scarce but constantly reveal an enormous ecological and functional adaptiveness of these organisms to *** holds true in the topmost forest canopies as well as in marine,arctic,antarctic or desert *** the present study dried leaves of Populus euphratica from a continental desert area in Central China were investigated for endophytic fungi 6 weeks after sampling by cultivation of small leaf ***-five species,many of them well-known from extreme environments,were delimitated from as few as 58 isolates by a combined analysis of morphotypes,micromorphology and ITS ***-analyses revealed pronounced conspecificity to endophytes from Populus tremula leaves,but significant differences to foliar endophytic assemblages in Pinus monticola and Fagus *** deduced high similarity of endophytic communities on both Populus species compared with that on Pinus and Fagus suggests that many fungal phyllosphere species show a well-pronounced host preference,at least for their endophytic *** addition,it demonstrates that leaving leaves as a microhabitat might provide similar conditions such as constantly high relative humidity,regardless of the surrounding climatic *** evolution of extremotolerance might be of particular importance for retaining competitiveness of foliar endophytes in deciduous host trees after loss of pathogenicity.

关键词： Frost-drought tolerance Extremophile Alternaria Cladosporium Penicillium Evolution of endophytism

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ACCURATE AND EFFICIENT IMAGE RECONSTRUCTION FROM MULTIPLE MEASUREMENTS OF FOURIER SAMPLES

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Journal of Computational Mathematics 2020年第5期38卷 797-826页

作者： T.Scarnati anne Gelb Air Force Research Laboratory WPAFBOH 45433USA Dartmouth College HanoverNH 03755USA

Several problems in imaging acquire multiple measurement vectors(MMVs)of Fourier samples for the same underlying *** recovery techniques from MMVs aim to exploit the joint sparsity across the measurements in the sparse *** is typically accomplished by extending the use of`1 regularization of the sparse domain in the single measurement vector(SMV)case to using`2,1 regularization so that the“jointness”can be accounted *** effective,the approach is inherently coupled and therefore computationally *** method also does not consider current approaches in the SMV case that use spatially varying weighted`1 regularization *** recently introduced variance based joint sparsity(VBJS)recovery method uses the variance across the measurements in the sparse domain to produce a weighted MMV method that is more accurate and more efficient than the standard`2,1 *** efficiency is due to the decoupling of the measurement vectors,with the increased accuracy resulting from the spatially varying *** by these results,this paper introduces a new technique to even further reduce computational cost by eliminating the requirement to first approximate the underlying image in order to construct the *** this preprocessing step moreover reduces the amount of information lost from the data,so that our method is more *** examples provided in the paper verify these benefits.

关键词： Multiple measurement vectors Joint sparsity Weighted`1 Edge detection Fourier data

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Evaluation of the Heat,Entropy,and Rotational Changes Produced by Gravitational Segregation during Core Formation

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Journal of Earth Science 2015年第1期26卷 124-133页

作者： anne M.Hofmeister Robert E.Criss Department of Earth and Planetary Sciences Washington University

Core formation by gravitational segregation allegedly released sufficient interior heat to melt the Earth. Analysis of the energetics, which compare gravitational potential energy （Ug） of a fictitious, homogeneous reference state to Earth＇s current layered configuration, needs updating to correct errors and omissions, and to accommodate recent findings：（1） An erroneous positive sign was used for Ug while maintaining the reference value of 0 at infinity, which results in an incorrect sign fur AUg, which is crucial in determining whether a process is endothermic or exothermic. （2） The value of Ug for Earth＇s initial state is uncertain. （3） Recent meteorite evidence indicates that core formation began before the Earth was full-sized, which severely limits AUg. （4） Inhomogeneous accretion additionally reduced AUg. （5） The potentially large effect of differential rotation between the core and the mantle was not accounted for. （6） Entropy changes associated with creating order were neglected. Accordingly, we revise values of Ug, evaluate uncertainties, and show that AUg was converted substantially to eonfigurational energy （TAS）. These considerations limit the large sources of primordial heat to impacts and radioactivity. Although these processes may play a role in core formation, their energies are independent of gravitational segregation, which produces order and rotational energy, not internal heat. Instead, gravitational segregation promotes planetary cooling mainly because it segregates lithophilic radioactive elements upward, increasing surface heat flux while shortening the distance over which radiogenic heat diffuses outwards.

关键词： core formation primordial heat configurational energy thermodynamics rotational energy.

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How virtual reality can help visualise and assess geohazards

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International Journal of Digital Earth 2019年第2期12卷 173-189页

作者： Hans-Balder Havenith Philippe Cerfontaine anne-Sophie Mreyen Georisk and Environment Department of GeologyUniversity of LiegeLiègeBelgium

Geohazard research requires extensive spatiotemporal understanding based on an adequate multi-scale representation of modelling *** most commonly applied representation basis for collected data is still the one of a 2D plane,typically a *** maps of spatial data can be visualised and processed by using Geographic Information *** is far less common to use 3D geomodels for the analysis and visualisation of spatial *** the visualisation of both spatial and temporal hazard components,there are no standardised *** claim that a full geohazard assessment is only possible inside a new type of geoscientific and technological environment that is at the same time multi-dimensional,spatiotemporal,integrated,fully interactive(tele-)immersive,and *** and subsurface processes are interacting at various scales that are difficult to be overviewed at *** Reality(VR)technology could provide an attractive solution to overcome the multi-dimensional and spatiotemporal *** review of geoscientific applications using VR technology developed by multiple teams around the world shows that some solutions have already been developed many years ago,but widespread use was not *** is clearly changing now and soon we will see if VR can contribute to a better understanding of geo-processes.

关键词： 4D geospace spatiotemporal analysis virtual environments immersive visualisation collaboration

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How Properties that Distinguish Solids from Fluids and Constraints of Spherical Geometry Suppress Lower Mantle Convection

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Journal of Earth Science 2018年第1期29卷 1-20页

作者： anne M. Hofmeister Everett M. Criss Department of Earth and Planetary Sciences Washington University St. Louis MO 63130 USA Panasonic Avionics Corporation Lake Forest CA 92630 USA

The large magnitude of the dimensionless Rayleigh number （Ra-10^8） for Earth＇s -3 000 km thick mantle is considered evidence of whole mantle convection. However, the current formulation assumes behavior characteristic of gases and liquids and also assumes Cartesian geometry. Issues arising from neglecting physical properties unique to solids and ignoring the spherical shapes for planets include：（1） Planet radius must be incorporated into Ra, in addition to layer thickness, to conserve mass during radial displacements. （2） The vastly different rates for heat and mass diffusion in solids, which result from their decoupled transport mechanisms, promote stability. （3） Unlike liquids, sub- stantial stress is needed to deform solids, which independently promotes stability. （4） High interior compression stabilizes the mantle in additional minor ways. Therefore, representing conditions for convection in solid, self-gravitating spheroids, requires modifying formulae developed for bottom- heated fluids near ambient conditions under an invariant gravitational field. To derive stability criteria appropriate to solid spheres, we use dimensional analysis, and consider the effects of geometry, force competition, and microscopic behavior. We show that internal heating has been improperly ac- counted for in the Ra. We conclude that the lower mantle is stable for two independent reasons： heat diffusion far outpaces mass diffusion （creep） and yield strength of solids at high pressure exceeds the effective deviatoric stress. We discuss the role of partial melt in lubricating plate motion, and explain why the Ra is not applicable to the multi-component upper mantle. When conduction is insufficient to transport heat in the Earth, melt production and ascent are expected, not convection of solid rock.

关键词： plasticity diffusion mantle convection stability criteria dimensional analysis geometry.

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Ependymal cells and multiple sclerosis: proposing a relationship

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Neural Regeneration Research 2020年第2期15卷 263-264页

作者： Dale Hatrock Nina Caporicci-nucci Jo anne Stratton The Montreal Neurological Institute McGill UniversityMontrealCanada Integrated Program in Neuroscience McGill UniversityMontrealCanada

Multiple sclerosis (MS) currently affects ~2.5 million people worldwide. MS is typically diagnosed in young adults and is usually not fatal, meaning people live long lives with MS. Affected individuals usually suffer from progressive physical and/or cognitive disability, often including fatigue (89.6%), depression (53.9%), memory loss (49.0%), motor or sensory dysfunction (76.4%, 70.4%) and urinary incontinence (50.8%).

关键词： multiple sclerosis relationship dysfunction

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