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Recent progress on MOF/MXene nanoarchitectures:A new era in coordination chemistry for energy storage and conversion

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Journal of Energy Chemistry 2023年第11期86卷 409-436,I0009页

作者： Sada Venkateswarlu Sowjanya Vallem Muhammad Umer N.V.V.Jyothi anam giridhar babu Saravanan Govindaraju Younghu Son Myung Jong Kim Minyoung Yoon Department of Chemistry and Green-Nano Materials Research Center Kyungpook National UniversityDaegu 41566Republic of Korea Department of Chemistry Gachon UniversitySeongnam 1320Republic of Korea Department of Physics Gachon UniversitySeongnam 13120Republic of Korea Center for Superfunctional Materials Department of ChemistryUlsan National Institute of Science and Technology(UNIST)Ulsan 44919Republic of Korea Department of Chemistry Sri Venkateswara UniversityTirupati 517502Andhra PradeshIndia Department of Civil Engineering Yeungnam UniversityGyeongsan 38541GyeongbukRepublic of Korea Department of Bionanotechnology Gachon UniversitySeongnam 13120Republic of Korea

The development of urbanization and industrialization leads to rapid depletion of fossil ***,the production of fuel from renewable resources is highly *** energy conversion and storage is a benign technique with reliable output and is *** an exceptional electrochemical catalyst with tunable properties like a huge specific surface area,porous channels,and abundant active sites is critical ***,Metal-organic frameworks(MOFs)and two-dimensional(2D)transition-metal carbides/nitrides(MXenes)have been extensively investigated in the field of electrochemical energy conversion and ***,advances in the research on MOFs are hampered by their limited structural stability and conventionally low electrical conductivity,whereas the practical electrochemical performance of MXenes is impeded by their low porosity,inadequate redox sites,and ***,researchers have been designing MOF/MXene nanoarchitectures to overcome the limitations in electrochemical energy conversion and *** review explores the recent advances in MOF/MXene nanoarchitectures design strategies,tailoring their properties based on the morphologies(0D,1D,2D,and 3D),and broadening their future opportunities in electrochemical energy storage(batteries,supercapacitors)and catalytic energy conversion(HER,OER,and ORR).The intercalation of MOF in between the MXene layers in the nanoarchitectures functions synergistically to address the issues associated with bare MXene and MOF in the electrochemical energy storage and *** review gives a clear emphasis on the general aspects of MOF/MXene nanoarchitectures,and the future research perspectives,challenges of MOF/MXene design strategies and electrochemical applications are highlighted.

关键词： Metal-organicframework MXene MoF/MXene nanoarchitecture Battery Supercapacitor Electrochemical catalysis

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