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New Applications of Zirconium Phosphate Nanomaterials

Accounts of Materials Research 2021年第9期2卷 793-803页

作者： Mario V.Ramos-Garcés Julissa González-Villegas aleannette lópez-cubero Jorge l.Colón Cain Department of Chemical Engineering Louisiana State UniversityBaton RougeLouisiana 70803United States Department of Chemistry University of Puerto RicoSan JuanPuerto Rico 00925-2537United States

CONSPECTUS:The 2-D layers of the inorganic ion exchangerα-zirconium phosphate(Zr(HPO_(4))2·H_(2)O,α-ZrP)make this compound particularly stable to low pH,high temperature,and ionizing *** studied for its ion exchange properties,once the conditions for its synthesis in crystalline form was accomplished by James Stynes and Abraham Clearfield in 1964,numerous other types of studies and applications *** studies in the 1960s and 1970s on the thermodynamics of ion exchange led to insights into the intercalation mechanism of this *** Clearfield group solved the crystal structure in 1968 and refined it in *** methods were pioneered by the Clearfield group to solve the structure of this type of *** 1968 Giulio Alberti reported means to prepare zirconium phosphonates expanding the chemistry of these layered *** phases of ZrP were also discovered(e.g.,γ,θ,λ,τ)and the applications ranged from heterogeneous catalysis to intercalation chemistry and solid-state proton *** to exfoliate the layers of ZrP were developed in the 1990s as interest grew in new applications of these types of *** example,protein and enzyme intercalation was accomplished starting in the 1990s by the Mclendon,Mallouk,and Kumar *** the early 2000s,the Colon group pioneered the use of théθphase of ZrP for the direct intercalation of large inorganic metal complexes that could not be directly intercalated into theα*** studies in the Colon group ranged from applications of these directly intercalated ZrP derivatives in photophysics and photochemistry,́amperometric biosensors,vapochromism,and *** the past decade,new applications of these materials have been developed in anticancer drug delivery and electrocatalysis of the oxygen evolution reaction(OER).ZrP has now proven to be a promising drug nanocarrier and its unique chemical microenvironment provided by theα-type layers and the interlay

关键词： properties zirconium inorganic

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