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“Zero‑Strain” NiNb_(2)O_(6) Fibers for All‑Climate Lithium Storage

Nano-Micro Letters 2025年第1期17卷 348-360页

作者： Yan Zhao Qiang Yuan Liting Yang Guisheng Liang Yifeng cheng Limin Wu Chunfu Lin Renchao che College of Physics Donghua UniversityShanghai 201620People’s Republic of China School of Materials Science and engineering Institute of Materials for Energy and EnvironmentQingdao UniversityQingdao 266071People’s Republic of China Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Zhejiang Laboratory Hangzhou 311100People’s Republic of China Inner Mongolia University Hohhot 010021People’s Republic of China

Niobates are promising all-climate Li^(+)-storage anode material due to their fast charge transport,large specific capacities,and resistance to electrolyte ***,their moderate unit-cellvolume expansion(generally 5%–10%)during Li^(+)storage causes unsatisfactory long-term ***,“zero-strain”NiNb_(2)O_(6) fibers are explored as a new anode material with comprehensively good electrochemical *** Li^(+)storage,the expansion of electrochemical inactive NiO_(6) octahedra almost fully offsets the shrinkage of active NbO_(6) octahedra through reversible O *** superior volume-accommodation capability of the NiO_(6) layers guarantees the“zero-strain”behavior of NiNb_(2)O_(6) in a broad temperature range(0.53%//0.51%//0.74%at 25//−10//60℃),leading to the excellent cyclability of the NiNb_(2)O_(6) fibers(92.8%//99.2%//91.1%capacity retention after 1000//2000//1000 cycles at 10C and 25//−10//60℃).This NiNb_(2)O_(6) material further exhibits a large reversible capacity(300//184//318 mAh g−1 at 0.1C and 25//−10//60℃)and outstanding rate performance(10 to 0.5C capacity percentage of 64.3%//50.0%//65.4%at 25//−10//60℃).Therefore,the NiNb_(2)O_(6) fibers are especially suitable for large-capacity,fast-charging,long-life,and all-climate lithium-ion batteries.

关键词： NiNb_(2)O_(6)porous fiber “Zero-strain”mechanism electrochemical property Harsh-temperature operation Operando characterization

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Spontaneous Orientation Polarization of Anisotropic equivalent Dipoles Harnessed by entropy engineering for Ultra‑Thin electromagnetic Wave Absorber

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Nano-Micro Letters 2025年第1期17卷 424-438页

作者： Honghan Wang Xinyu Xiao Shangru Zhai Chuang Xue Guangping Zheng Deqing Zhang Renchao che Junye cheng Liaoning Key Lab of Lignocellulose chemistry and BioMaterials Liaoning Collaborative Innovation Center for Lignocellulosic BiorefinerySchool of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034People’s Republic of China School of Life Science and Biotechnology Dalian University of TechnologyDalian 116024People’s Republic of China Department of Mechanical engineering Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China School of Materials Science and engineering Qiqihar UniversityQiqihar 161006People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Department of Materials Science Shenzhen MSU-BIT UniversityShenzhen 517182People’s Republic of China

The synthesis of carbon supporter/nanoscale high-entropy alloys(HeAs)electromagnetic response composites by carbothermal shock method has been identified as an advanced strategy for the collaborative competition engineering of conductive/dielectric *** migration modes within HeAs as manipulated by the electronegativity,valence electron configurations and molar proportions of constituent elements determine the steady state and efficiency of equivalent ***,enlightened by skin-like effect,a reformative carbothermal shock method using carbonized cellulose paper(CCP)as carbon supporter is used to preserve the oxygencontaining functional groups(O·)of carbonized cellulose fibers(CCF).Nucleation of HeAs and construction of emblematic shell-core CCF/HeAs heterointerfaces are inextricably linked to carbon metabolism induced by O·.Meanwhile,the electron migration mode of switchable electronrich sites promotes the orientation polarization of anisotropic equivalent *** virtue of the reinforcement strategy,CCP/HeAs composite prepared by 35%molar ratio of Mn element(CCP/HeAs-Mn_(2.15))achieves efficient electromagnetic wave(eMW)absorption of−51.35 dB at an ultra-thin thickness of 1.03 *** mechanisms of the resulting dielectric properties of HeAs-based eMW absorbing materials are elucidated by combining theoretical calculations with experimental characterizations,which provide theoretical bases and feasible strategies for the simulation and practical application of electromagnetic functional devices(e.g.,ultra-wideband bandpass filter).

关键词： High-entropy alloys Carbothermal shock Switchable electron migration modes emblematic shell-core heterointerfaces Ultra-thin thickness

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Designing electronic Structures of Multiscale Helical Converters for Tailored Ultrabroad electromagnetic Absorption

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Nano-Micro Letters 2025年第1期17卷 439-455页

作者： Zhaobo Feng Chongbo Liu Xin Li Guangsheng Luo Naixin Zhai Ruizhe Hu Jing Lin Jinbin Peng Yuhui Peng Renchao che Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle School of Environmental and Chemical EngineeringNanchang Hangkong UniversityNanchang 330063People’s Republic of China School of Physics and Materials Nanchang UniversityNanchang 330031People’s Republic of China Key Laboratory of Nondestructive Testing Ministry of EducationNanchang Hangkong UniversityNanchang 330063People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering and TechnologyFudan UniversityShanghai 200438People’s Republic of China

Atomic-scale doping strategies and structure design play pivotal roles in tailoring the electronic structure and physicochemical property of electromagnetic wave absorption(eMWA)***,the relationship between configuration and electromagnetic(eM)loss mechanism has remained ***,drawing inspiration from the DNA transcription process,we report the successful synthesis of novel in situ Mn/N co-doped helical carbon nanotubes with ultrabroad eMWA *** calculation and eM simulation confirm that the orbital coupling and spin polarization of the Mn–N4–C configuration,along with cross polarization generated by the helical structure,endow the helical converters with enhanced eM *** a result,HMC-8 demonstrates outstanding eMWA performance,achieving a minimum reflection loss of−63.13 dB at an ultralow thickness of 1.29 *** precise tuning of the graphite domain size,HMC-7 achieves an effective absorption bandwidth(eAB)of 6.08 GHz at 2.02 mm ***,constructing macroscale gradient metamaterials enables an ultrabroadband eAB of 12.16 GHz at a thickness of only 5.00 mm,with the maximum radar cross section reduction value reaching 36.4 dB *** innovative approach not only advances the understanding of metal–nonmetal co-doping but also realizes broadband eMWA,thus contributing to the development of eMWA mechanisms and applications.

关键词： Metal-nonmetal co-doping 3d-2p orbital coupling Spin polarization Helical structure Broadband eM wave absorption

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Finite Projective Geometries and Classification of the Weight Hierarchies of Codes(Ⅰ)

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Acta Mathematica Sinica,english Series 2004年第2期20卷 333-348页

作者： WenDecheN TorleivKLφve LaboratoryofSystemsandControl CenterofInformationSecurityAcademyofMathematicsandSystemsScienceChineseAcademyofSciencesBeijing100080P.R.China Departmentoflnformatics UniversityofBergenBergenHighTechnologyCenterN-5020BergenNorway

The weight hierarchy of a binary linear [n, k] code C is the sequence (d 1, d 2, . . . , d k ), where d r is the smallest support of an r-dimensional subcode of C. The codes of dimension 4 are collected in classes and the possible weight hierarchies in each class is determined by finite projective geometries. The possible weight hierarchies in class A, B, C, D are determined in Part (I). The possible weight hierarchies in class e, F, G, H, I are determined in Part (II).

关键词： Weight hierarchy Support weight Finite projective geometries Binary linear code Chain condition Difference sequence

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压应力激活SOST/Wnt/β-catenin 通路诱导软骨终板细胞退变

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中国组织工程研究 2025年第5期29卷 951-957页

作者：项攀车艳军罗宗平苏州大学附属第一医院骨科研究所江苏省苏州市215006 南京医科大学附属苏州医院骨科与运动医学中心江苏省苏州市215000

背景:在许多可以导致椎间盘退变的因素中(衰老、营养匮乏、机械因素等),力学负荷被认为是极其重要的因素,但其机制尚不清楚。目的:探讨硬骨素和Wnt/β-catenin信号通路在压应力诱导终板软骨退变中的作用。方法:提取4周龄雄性SD大鼠软骨... 详细信息

背景:在许多可以导致椎间盘退变的因素中(衰老、营养匮乏、机械因素等),力学负荷被认为是极其重要的因素,但其机制尚不清楚。目的:探讨硬骨素和Wnt/β-catenin信号通路在压应力诱导终板软骨退变中的作用。方法:提取4周龄雄性SD大鼠软骨终板细胞,体外利用力学加载仪器对终板软骨细胞施加压应力,于压缩细胞1,3,5,7 d,采用CCK-8法测定细胞活力;Western blot、RT-qPCR及细胞免疫荧光等检查终板软骨细胞内软骨标记物(聚集蛋白聚糖、Ⅱ型胶原)、钙化相关因子(Runx2、骨钙素)、细胞外基质降解酶及信号通路基因(硬骨素、β-catenin)等表达。结果与结论:①压应力作用下,终板软骨细胞活力会随着压应力时间、强度增加而降低;②终板软骨细胞的软骨标记物(聚集蛋白聚糖、Ⅱ型胶原)表达下降,而钙化相关因子(Runx2、骨钙素)表达上升;③压应力能促进终板软骨细胞的细胞外基质降解,基质金属蛋白酶3、基质金属蛋白酶13表达量增加;④细胞内Wnt/β-catenin信号通路表达出现异常,其特异性抑制因子硬骨素伴随着β-catenin的异常积累而表达下降。结果说明:在压应力作用下,终板软骨细胞内硬骨素的表达下降,导致Wnt/β-catenin信号通路激活,促进软骨终板的钙化、退变与细胞外基质的降解,进而促进椎间盘退变。

关键词：软骨终板软骨细胞 SOST Wnt/β-catenin 压应力椎间盘退变

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Combating with extremely noisy samples in weakly supervised slot filling for automatic diagnosis

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Frontiers of Computer Science 2023年第5期17卷 67-73页

作者： Xiaoming SHI Wanxiang che School of Computer Science and Technology Harbin Institute of TechnologyHarbin 150001China

Slot filling,to extract entities for specific types of information(slot),is a vitally important modular of dialogue systems for automatic *** responses can be regarded as the weak supervision of patient *** this way,a large amount of weakly labeled data can be obtained from unlabeled diagnosis dialogue,alleviating the problem of costly and time-consuming data ***,weakly labeled data suffers from extremely noisy *** alleviate the problem,we propose a simple and effective Co-WeakTeaching *** method trains two slot filling models *** two models learn from two different weakly labeled data,ensuring learning from two ***,one model utilizes selected weakly labeled data generated by the other,*** model,obtained by the Co-WeakTeaching on weakly labeled data,can be directly tested on testing data or sequentially fine-tuned on a small amount of human-annotated *** results on these two settings illustrate the effectiveness of the method with an increase of 8.03%and 14.74%in micro and macro f1 scores,respectively.

关键词： dialogue system slot filling co-teaching

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Searching for QCD critical point with light nuclei

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Nuclear Science and Techniques 2023年第5期34卷 192-195页

作者： che Ming Ko Cyclotron Institute and Department of Physics and Astronomy Texas A&M UniversityCollege StationTexas 77843‑3366USA

Density fluctuations and correlations due to a first-order quark-gluon plasma to hadronic matter phase transition and its critical end point,if they remain present after the hadronic evolution in a heavy ion collisions,can lead to an enhanced production of light nuclei in these *** would then result in a non-monotonic collision energy dependence of the yield ratio NtNp∕Nd2of proton number Np,deuteron number Nd,and triton number *** of this yield ratio as a function of collision energy thus provides the possibility to probe the equation of state of strong-interaction matter and its phase diagram.

关键词： critical collision light

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Solid and liquid phase equilibria in mixtures of N, N-dimethylacetamide with chlorinated hydrocarbons

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Chinese Science Bulletin 1997年第11期42卷 918-921页

作者： che, GQ Peng, WL che, B Department of chemistry Zhongshan University Guangzhou China

IN refs.[1,2],we studied the solid and liquid phase equilibria in mixtures of tetra-chloromethane with oxygen and nitrogen-containing compounds,intermolecular interactionswith the formation of solid molecular addition... 详细信息

关键词： phase diagram solid and liquid equilibrium N N-dimethylacetamide.

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estimating thermohaline variability of the equatorial Pacific Ocean from satellite altimetry

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Science China earth Sciences 2016年第11期59卷 2213-2222页

作者： SUN che MA Xiao Institute of Oceanology Chinese Academy of Sciences Qingdao 266071 China National Laboratory for Marine Science and Technology Qingdao 266071 China State Key Laboratory of Satellite Ocean environment Dynamics Second Institute of Oceanography State Oceanic Administration Hangzhou 310012 China

The vertical thermohaline structure in the western equatorial Pacific is examined with a Gravest empirical Mode(GeM)diagnosis of in-situ mooring measurements. The poor GeM performance in estimating deep thermohaline variability from satellite altimetry confirms a lack of vertical coherence in the equatorial ocean. Mooring observation reveals layered equatorial water with phase difference up to 6 months between thermocline and sub-thermocline variations. The disjointed layers reflect weak geostrophy and resemble pancake structures in non-rotating stratified turbulence. A coherency theorem is then proved, stating that traditional stationary GeM represents in-phase coherent structure and can not describe vertically out-of-phase variability. The fact that stationary GeM holds both spatial and temporal coherence makes it a unique tool to diagnose vertical coherent structure in geophysical flows. The study also develops a non-stationary GeM projection that captures more than 40% of the thermohaline variance in the equatorial deep water.

关键词： equatorial Pacific TRITON buoys Satellite altimetry GeM vertical coherence

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enhanced release of the poorly soluble drug itraconazole loaded in ordered mesoporous silica

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Science China chemistry 2015年第3期58卷 400-410页

作者： Xiao Liu Shunai che State Key Laboratory of Metal Matrix Composites School of chemistry and chemical engineering Shanghai Jiao Tong University

It is known that the energy of the amorphous state of itraconazole loaded in ordered mesoporous materials is high relative to that of the crystalline state and is responsible for enhanced solubility and dissolution rate. We investigated the effects of particle size(0.7–5μm), mesostructure(2D p6 mm, cubic Ia-3d and cubic Fm-3m) and pore size(2.2–15.4 nm) of mesoporous silicas on the release performance of itraconazole. Results indicated that the release performance was not influenced by the particle sizes tested here, that the release performance increased with increasing pore diameter due to the lower probability of drug molecules colliding to recrystallize in large pores, and that the release performance was decreased in the cage-type pore structure(Fm-3m) compared to that in the cylindrical pore structures(p6mm and Ia-3d) because of the small entrance to the cagelike pores that retards the drug release.

关键词： itraconazole poorly soluble enhanced release mesoporous silica

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