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Simulated perturbation in the sea-to-air flux of dimethylsulfi de and the impact on polar climate

Journal of Oceanology and Limnology 2021年第1期39卷 110-121页

作者： Bo QU albert jgabric Rebecca JACKSON School of Science Nantong UniversityNantong 226219China School of Environment and Science Griffi th UniversityBrisbane 4111QLDAustralia

Marine biogenic emission of dimethylsulfi de(DMS)has been well recognized as the main natural source of reduced sulfur to the remote marine atmosphere and has the potential to aff ect climate,especially in the polar *** used a global climate model(GCM)to investigate the impact on atmospheric chemistry from a change to the contemporary DMS fl ux to that which has been projected for the late 21 st *** perturbed simulation corresponded to conditions that pertained to a tripling of equivalent CO 2,which was estimated to occur by year 2090 based on current worst-case greenhouse gas emission *** changes in zonal mean DMS fl ux were applied to 50°S–70°S Antarctic(ANT)and 65°N–80°N Arctic(ARC)*** results indicate that there are clearly diff erent impacts after perturbation in the southern and northern polar *** quantities related to the sulfur cycle show a higher increase in ***,most sulfur compounds have higher peaks in *** perturbation in DMS fl ux leads to an increase of atmospheric DMS of about 45%in ANT and 33.6%in *** sulfur dioxide(SO 2)vertical integral increases around 43%in ANT and 7.5%in ***(SO 4)vertical integral increases by 17%in ANT and increases around 6%in *** emissions increases by 21%in ANT and increases by 9.7%in ***,oxidation of DMS by OH increases by 38.2%in ARC and by 15.17%in *** optical depth(AOD)increases by 4%in the ARC and by 17.5%in the ANT,and increases by 22.8%in austral *** importance of the perturbation of the biogenic source to future aerosol burden in polar regions leads to a cooling in surface temperature of 1 K in the ANT and 0.8 K in the ***,polar regions in the Antarctic Ocean will have a higher off setting eff ect on warming after DMS fl ux perturbation.

关键词： dimethylsulfi de(DMS) sulfur dioxide DMS sea-to-air fl ux perturbation global climate model(GCM) polar region

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Comparison Between Early and Late 21stC Phytoplankton Biomass and Dimethylsulfide Flux in the Subantarctic Southern Ocean

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Journal of Ocean University of China 2020年第1期19卷 151-160页

作者： QU Bo albert jgabric JIANG Limei LI Chunyue School of Science Nantong UniversityNantong 226019China School of Environment and Science Griffith UniversityNathan Qld 4111Australia Nantong Chong Chuan School Nantong 226000China Marketing Thermo Fisher ScientificShanghai 201206China

Time-series of chlorophyll-a(CHL),a proxy for phytoplankton biomass,and various satellite-derived climate indicators are compared in a region of the Subantarctic Southern Ocean(40°-60°S,110°-140°E)for years *** reached a minimum in winter(June)and a maximum in late summer(early February).Zonal mean CHL decreased towards the *** sea surface temperature(SST)ranged between 8℃and 15℃and peaked in late *** and SST were positively correlated from March to June,negatively correlated from July to *** and wind speed(WIND)were negatively correlated with peak WIND occurred in *** direction(WIRD)was mostly in the southwest to westerly *** Antarctic Oscillation index(AAO)and CHL were negatively correlated(R=−0.58),indicating that as synoptic wind systems move southwards,CHL increases,and conversely when wind systems move northwards,CHL decreases.A genetic algorithm is used to calibrate the biogeochemical DMS model’s key *** 4×CO2(after year 2100)Regional mean SST increases 12%-17%,WIND increases 1.2ms−1,Cloud Cover increases 4.8%and mixed layer depth(MLD)decreases *** annual CHL increases 6.3%.The annual mean DMS flux increase 25.2%,increases 37%from day 1 to day 280 and decrease 3%from day 288 to day *** general increase of DMS flux under 4×CO2 conditions indicates the Subantarctic regional climate would be affected by changes in the DMS flux,with the potential for a cooling effect in the austral summer and autumn.

关键词： wind speed phytoplankton dimethylsulfide flux climate change subantarctic Southern Ocean

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