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Rare Metals 2024年第7期43卷 3107-3117页

作者： Xin-Yang Liu Jing-Wei Liu Gang Li Jing-xiang Zhao College of Chemistry and Chemical Engineering Harbin Normal UniversityHarbin 150025China

Subnanometer metal clusters play an increasingly important role in heterogeneous catalysis due to their high catalytic activity and *** this work,by means of the density functional theory(DFT) calculations,the catalytic activities of transition metal clusters with precise numbers of atoms supported on graphdiyne(TM_(1-4)@GDY,TM=V,Cr,Mn,Fe,Co,Ni,Cu,Ru,Rh,Pd,Ir,Pt) were investigated for oxygen evolution reactions(OER),oxygen reduction reactions(ORR) and hydrogen evolution reactions(HER).The computed results reveal that the Pd_(2),Pd_(4) and Pt_(1) anchored graphdiyne can serve as trifunctional catalysts for OER/ORR/HER with the overpotentials of 0.49/0.37/0.06,0.45/0.33/0.12 and 0.37/0.43/0.01 V,respectively,while Pd_(1) and Pt_(2)@graphdiyne can exhibit excellent catalytic performance for water splitting(OER/HER) with the overpotentials of 0.55/0.17 and 0.43/0.03 *** addition,Ni_(1) and Pd_(3) anchored GDY can perform as bifunctional catalysts for metal-air cells(OER/ORR) and fuels cells(ORR/HER) with the overpotentials of 0.34/0.32 and 0.42/0.04 V,***,by precisely controlling the numbers of atoms in clusters,the TM_(1-4) anchored graphdiyne can serve as promising multifunctional electrocatalysts for OER/ORR/HER,which may provide an instructive strategy to design catalysts for the energy conversation and storage devices.

关键词： Density functional theory Graphdiyne Single-cluster catalysts Multifunctional electrocatalysts Overpotential

Learning a Mixture of Conditional Gating Blocks for Visual Question Answering

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Journal of Computer Science & Technology 2024年第4期39卷 912-928页

作者： Qiang Sun Yan-Wei Fu xiang-Yang Xue School of Statistics and Information Shanghai University of International Business and EconomicsShanghai 201620China Academy for Engineering and Technology Fudan UniversityShanghai 200433China School of Data Science Fudan UniversityShanghai 200433China School of Computer Science Fudan UniversityShanghai 200433China

As a Turing test in multimedia,visual question answering(VQA)aims to answer the textual question with a given ***,the“dynamic”property of neural networks has been explored as one of the most promising ways of improving the adaptability,interpretability,and capacity of the neural network ***,despite the prevalence of dynamic convolutional neural networks,it is relatively less touched and very nontrivial to exploit dynamics in the transformers of the VQA tasks through all the stages in an end-to-end ***,due to the large computation cost of transformers,researchers are inclined to only apply transformers on the extracted high-level visual features for downstream vision and language *** this end,we introduce a question-guided dynamic layer to the transformer as it can effectively increase the model capacity and require fewer transformer layers for the VQA *** particular,we name the dynamics in the Transformer as Conditional Multi-Head Self-Attention block(cMHSA).Furthermore,our questionguided cMHSA is compatible with conditional ResNeXt block(cResNeXt).Thus a novel model mixture of conditional gating blocks(McG)is proposed for VQA,which keeps the best of the Transformer,convolutional neural network(CNN),and dynamic *** pure conditional gating CNN model and the conditional gating Transformer model can be viewed as special examples of *** quantitatively and qualitatively evaluate McG on the CLEVR and VQA-Abstract *** experiments show that McG has achieved the state-of-the-art performance on these benchmark datasets.

关键词： visual question answering Transformer dynamic network

Detection of LAMA2 c.715C>G:p.R239G mutation in a newborn with raised creatine kinase: A case report

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World Journal of Clinical Cases 2024年第14期12卷 2445-2450页

作者： Jing Yuan xiang-Ming Yan Department of Pediatric Children’s Hospital of Soochow UniversitySuzhou 215025Jiangsu ProvinceChina Department of Surgery Children's Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina

BACKGROUND We report a rare case of primary clinical presentation featuring elevated creatine kinase(CK)levels in a neonate,which is associated with the LAMA2 *** this case,a heterozygous mutation in exon5 of the LAMA2 gene,c.715C>G(resulting in a change of nucleotide number 715 in the coding region from cytosine to gua-nine),induced an amino acid alteration p.R239G(No.239)in the patient,repre-senting a missense *** observation may be elucidated by the neonatal creatine monitoring mechanism,a phenomenon not previously *** SUMMARY We analysed the case of a neonate presenting solely with elevated CK levels who was eventually discharged after supportive *** chief complaint was identification of increased CK levels for 15 d and higher CK values for 1 ***-mission occurred at 18 d of age,and despite prolonged treatment with creatine and vitamin C,the elevated CK levels showed limited *** exo-me sequencing revealed the presence of a c.715C>G mutation in LAMA2 in the newborn,correlating with a clinical ***,the available informa-tion offers insufficient evidence for clinical *** Mutations in LAMA2 are associated with the clinical phenotype of increased neonatal CK levels,for which no specific treatment *** genome sequen-cing facilitates early diagnosis.

关键词： Creatine kinase LAMA2 Gene mutation Neonate Case report

Linear shallow neural network to accelerate transmitter dispersion eye closure quaternary(TDECQ) assessment

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Science China(Information Sciences) 2024年第4期67卷 337-338页

作者： Junjiang xiang Zejun CHEN Yijun CHENG Hailin YANG Xuancheng HUO Meng xiang Gai ZHOU Yuwen QIN Songnian FU Institute of Advanced Photonics Technology School of Information EngineeringGuangdong University of Technology School of Optical and Electronic Information Huazhong University of Science and Technology Key Laboratory of Photonic Technology for Integrated Sensing and Communication Ministry of Education of ChinaGuangdong University of Technology Guangdong Provincial Key Laboratory of Information Photonics Technology Guangdong University of Technology

To support the ever-emerging capacity requirement of datacenter interconnection(DCI) applications, transmitter dispersion eye closure quaternary(TDECQ) has been proposed by IEEE802.3 standard [1], which is specifically employed for the four-level pulse amplitude modulation(PAM-4) signals. However, the traditional scheme of TDECQ assessment needs several iterative operations,

关键词： IEEE Standards

All-trans retinoic acid alleviates transmissible gastroenteritis virus-induced intestinal inflammation and barrier dysfunction in weaned piglets

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Journal of Animal Science and Biotechnology 2024年第3期15卷 1131-1144页

作者： Junning Pu Daiwen Chen Gang Tian Jun He Ping Zheng Zhiqing Huang xiangbing Mao Jie Yu Yuheng Luo Junqiu Luo Hui Yan aimin Wu Bing Yu Institute of Animal Nutrition Sichuan Agricultural UniversityChengdu 611130SichuanPeople’s Republic of China Key Laboratory of Animal Disease-Resistance Nutrition Ministry of EducationMinistry of Agriculture and Rural AffairsKey Laboratory of Sichuan Province611130 ChengduSichuanPeople’s Republic of China

Background Transmissible gastroenteritis virus(TGEV)is one of the main pathogens causing severe diarrhea of *** pathogenesis of TGEV is closely related to intestinal ***-trans retinoic acid(ATRA)is the main active metabolite of vitamin A,which has immunomodulatory and anti-inflammatory ***,it is unclear whether ATRA can alleviate TGEV-induced intestinal inflammation and barrier dysfunction in *** study aimed to investigate the effects of ATRA on growth performance,diarrhea,intestinal inflammation and intesti-nal barrier integrity of TGEV-challenged *** In a 19-d study,32 weaned piglets were randomly divided into 4 treatments:Control group(basal diet),TGEV group(basal diet+TGEV challenge),TGEV+ATRA5 group(basal diet+5 mg/d ATRA+TGEV challenge)and TGEV+ATRA15 group(basal diet+15 mg/d ATRA+TGEV challenge).On d 14,piglets were orally administered TGEV or the sterile *** Feeding piglets with 5 and 15 mg/d ATRA alleviated the growth inhibition and diarrhea induced by TGEV(P<0.05).Feeding piglets with 5 and 15 mg/d ATRA also inhibited the increase of serum diamine oxidase(DAO)activ-ity and the decrease of occludin and claudin-1 protein levels in jejunal mucosa induced by TGEV,and maintained intestinal barrier integrity(P<0.05).Meanwhile,5 mg/d ATRA feeding increased the sucrase activity and the expres-sions of nutrient transporter related genes(GLUT2 and SLC7A1)in jejunal mucosa of TGEV-challenged piglets(P<0.05).Furthermore,5 mg/d ATRA feeding attenuated TGEV-induced intestinal inflammatory response by inhibit-ing the release of interleukin(IL)-1β,IL-8 and tumor necrosis factor-α(TNF-α),and promoting the secretion of IL-10 and secretory immunoglobulin A(sIgA)(P<0.05).Feeding 5 mg/d ATRA also down-regulated the expressions of Toll-like receptors and RIG-I like receptors signaling pathway related genes(TLR3,TLR4,RIG-I,MyD88,TRIF and MAVS)and the phosphorylation level of nuclear factor-κB-p65(NF-κB p65),and

关键词： All-trans retinoic acid Inflammation Intestinal barrier Piglets Transmissible gastroenteritis virus

Isoindigo nanoparticles for photoacoustic imaging-guided tumor photothermal therapy

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Chinese Journal of Chemical Engineering 2024年第8期72卷 19-25页

作者： Yao Pei Ran Wang xiang Rong xiang Xia Hexiang Wang Zongwei Zhang Tian Qiu Saran Long Jianjun Du Jiangli Fan Wen Sun Xiaojun Peng State Key Laboratory of Fine Chemicals Frontiers Science Center for Smart Materials Oriented Chemical EngineeringDalian University of TechnologyDalian 116024China Ningbo Institute of Dalian University of Technology Ningbo 315016China

The key factor in photothermal therapy lies in the selection of photothermal *** photothermal agents generally have problems such as poor photothermal stability and low photothermal conversion ***,we have designed and synthesized an isoindigo(IID)*** used isoindigo as the molecular center and introduced common triphenylamine and methoxy groups as *** order to improve the photothermal stability and tumor targeting ability,we encapsulated IID into *** a result,the nanoparticles exhibited high photothermal stability and photothermal conversion efficiency(67%)upon 635 nm laser ***,the nanoparticles demonstrated a significant inhibitory effect on live tumors in photothermal therapy guided by photoacoustic imaging and provided a viable strategy to overcome the treatment challenges.

关键词： Photothermal therapy Isoindigo Nanoparticles Photoacoustic imaging

NFXL1 functions as a transcriptional activator required for thermotolerance at reproductive stage in Arabidopsis

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Journal of Integrative Plant Biology 2024年第1期66卷 54-65页

作者： Qiao‐Yun Zhu Lin‐Lin Zhang Jian‐xiang Liu State Key Laboratory of Plant Environmental Resilience College of Life SciencesZhejiang UniversityHangzhou 310027China

Plants are highly susceptible to abiotic stresses,particularly heat stress during the reproductive ***,the specific molecular mechanisms underlying this sensitivity remain largely *** the current study,we demonstrate that the Nuclear Transcription Factor,X-box Binding Protein 1-Like 1(NFXL1),directly regulates the expression of DEHYDRATION-RESPONSIVE ELEMENT-BINDING PROTEIN 2A(DREB2A),which is crucial for reproductive thermotolerance in ***1 is upregulated by heat stress,and its mutation leads to a reduction in silique length(seed number)under heat stress ***-Seq analysis reveals that NFXL1 has a global impact on the expression of heat stress responsive genes,including DREB2A,Heat Shock Factor A3(HSFA3)and Heat Shock Protein 17.6(HSP17.6)in flower ***,NFXL1 is enriched in the promoter region of DREB2A,but not of either HSFA3 or *** experiments using electrophoretic mobility shift assay have confirmed that NFXL1 directly binds to the DNA fragment derived from the DREB2A ***,effector-reporter assays have shown that NFXL1 activates the DREB2A *** DREB2A mutants are also heat stress sensitive at the reproductive stage,and DEREB2A is epistatic to NFXL1 in regulating thermotolerance in flower *** is known that HSFA3,a direct target of DREB2A,regulates the expression of heat shock proteins genes under heat stress ***,our findings establish NFXL1 as a critical upstream regulator of DREB2A in the transcriptional cassette responsible for heat stress responses required for reproductive thermotolerance in Arabidopsis.

关键词： Arabidopsis DREB2A heat stress NFXL1 reproductive thermotolerance

Securing offshore resources development: A mathematical investigation into gas leakage in long-distance flexible pipes

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Petroleum Science 2024年第4期21卷 2734-2744页

作者： xiang-An Lu Liang-Liang Jiang Jian-Sheng Zhang Min-Gui Wang Guangling College of Yangzhou University Department of Chemical and Petroleum Engineering University of Calgary Department of Energy and Power Engineering Tsinghua University

Gas flexible pipes are critical multi-layered equipment for offshore oil and gas development. Under high pressure conditions, small molecular components of natural gas dissolve into the polymer inner liner of the flexible pipes and further diffuse into the annular space, incurring annular pressure build-up and/or production of acidic environment, which poses serious challenges to the structure and integrity of the flexible pipes. Gas permeation in pipes is a complex phenomenon governed by various factors such as internal pressure and temperature, annular structure, external temperature. In a long-distance gas flexible pipe, moreover, gas permeation exhibits non-uniform features, and the gas permeated into the annular space flows along the metal gap. To assess the complex gas transport behavior in long-distance gas flexible pipes, a mathematical model is established in this paper considering the multiphase flow phenomena inside the flexible pipes, the diffusion of gas in the inner liner, and the gas seepage in the annular space under varying permeable properties of the annulus. In addition, the effect of a variable temperature is accounted. A numerical calculation method is accordingly constructed to solve the coupling mathematical equations. The annular permeability was shown to significantly influence the distribution of annular pressure. As permeability increases, the annular pressure tends to become more uniform, and the annular pressure at the wellhead rises more rapidly. After annular pressure relief followed by shut-in, the pressure increase follows a convex function. By simulating the pressure recovery pattern after pressure relief and comparing it with test results, we deduce that the annular permeability lies between 123 and 512 m D. The results help shed light upon assessing the annular pressure in long distance gas flexible pipes and thus ensure the security of gas transport in the emerging development of offshore resources.

关键词： Offshore resources development Transport security Long-distance flexible pipes Gas leakage Heat and mass transfer model Finite difference calculation

Intelligent responsive self-assembled micro-nanocapsules: Used to delay gel gelation time

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Petroleum Science 2024年第4期21卷 2433-2443页

作者： Chuan-Hong Kang Ji-xiang Guo Dong-Tao Fei Wyclif Kiyingi Unconventional Petroleum Research Institute China University of Petroleum

In the application of polymer gels to profile control and water shutoff,the gelation time will directly determine whether the gel can "go further" in the formation,but the most of the methods for delaying gel gelation time are complicated or have low *** is an urgent need for an effective method for delaying gel gelation time with intelligent *** by the slow-release effect of drug capsules,this paper uses the self-assembly effect of gas-phase hydrophobic SiO2in aqueous solution as a capsule to prepare an intelligent responsive self-assembled *** capsule slowly releases the cross-linking agent under the stimulation of external conditions such as temperature and pH value,thus delaying gel gelation *** the pH value is 2 and the concentration of gas-phase hydrophobic SiO2particles is 10%,the gelation time of the capsule gel system at 30,60,90,and 120℃ is12.5,13.2,15.2,and 21.1 times longer than that of the gel system without containing capsule,*** with other methods,the yield stress of the gel without containing capsules was 78 Pa,and the yield stress after the addition of capsules was 322 *** intelligent responsive self-assembled micronanocapsules prepared by gas-phase hydrophobic silica nanoparticles can not only delay the gel gelation time,but also increase the gel *** slow release of cross-linking agent from capsule provides an effective method for prolongating the gelation time of polymer gels.

关键词： Profile control and water shutoff Polymer gel Delayed gelation time Intelligent response Self-assembled Micro-nanocapsules

LLM4CP:Adapting Large Language Models for Channel Prediction

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Journal of Communications and Information Networks 2024年第2期9卷 113-125页

作者： Boxun Liu Xuanyu Liu Shijian Gao xiang Cheng Liuqing Yang State Key Laboratory of Advanced Optical Communication Systems and Networks School of ElectronicsPeking UniversityBeijing 100871China Internet of Things Thrust The Hong Kong University of Science and Technology(Guangzhou)Guangzhou 511400China Internet of Things Thrust and Intelligent Transportation Thrust The Hong Kong University of Science and Technology(Guangzhou)Guangzhou 511400China Department of Electronic and Computer Engineering and Department of Civil and Environmental Engineering The Hong Kong University of Science and TechnologyHong KongChina

Channel prediction is an effective approach for reducing the feedback or estimation overhead in massive multi-input multi-output (m-MIMO) systems. However, existing channel prediction methods lack precision due to model mismatch errors or network generalization issues. Large language models (LLMs) have demonstrated powerful modeling and generalization abilities, and have been successfully applied to cross-modal tasks, including the time series analysis. Leveraging the expressive power of LLMs, we propose a pre-trained LLM-empowered channel prediction(LLM4CP)method to predict the future downlink channel state information (CSI) sequence based on the historical uplink CSI sequence. We fine-tune the network while freezing most of the parameters of the pre-trained LLM for better cross-modality knowledge transfer. To bridge the gap between the channel data and the feature space of the LLM,preprocessor, embedding, and output modules are specifically tailored by taking into account unique channel characteristics. Simulations validate that the proposed method achieves state-of-the-art (SOTA) prediction performance on full-sample, few-shot, and generalization tests with low training and inference costs.

关键词： channel prediction massive multi-input multi-output(m-MIMO) large language models(LLMs) fine-tuning time-series