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Rare Metals 2024年第3期43卷 1275-1287页

作者： Shao-Le Song Run-Qing Liu Miao-Miao Sun ai-Gang zhen Fan-zhen Kong Yue Yang School of Minerals Processing and Bioengineering Central South UniversityChangsha410083China Zhejiang Tianneng New Materials Co. Ltd.Huzhou313103China

The recycling of cathode materials from spent lithium-ion battery has attracted extensive attention,but few research have focused on spent blended cathode *** reality,the blended materials of lithium iron phosphate and ternary are widely used in electric vehicles,so it is critical to design an effective recycling *** this study,an efficient method for recovering Li and Fe from the blended cathode materials of spent LiFePO_(4)and LiNi_(x)Co_(y)Mn_(1-x-y)O_(2)batteries is ***,87%A1 was removed by alkali ***,91.65%Li,72.08%Ni,64.6%Co and 71.66%Mn were further separated by selective leaching with H_(2)SO_(4)and H_(2)O_(2).Li,Ni,Co and Mn in solution were recovered in the form of Li_(2)CO_(3)and hydroxide ***,98.38%Fe was leached from the residue by two stage process,and it is recovered as FePO_(4)·2H_(2)O with a purity of 99.5%by *** and P were present in FePO_(4)·2H_(2)O in amounts of 28.34%and 15.98%,***,the drift and control of various components were discussed,and cost-benefit analysis was used to assess the feasibility of potential application.

关键词： Spent lithium-ion battery Blended cathode materials Recovery Lithium carbonate Iron phosphate

Characterization of cancer stem-like cells in the side population cells of human gastric cancer cell line MKN-45

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2013年第3期14卷 216-223页

作者： Hai-hong ZHANG ai-zhen ca Xue-ming WEI Li DING Feng-zhi LI ai-ming zhenG Da-jiang Dai Rong-rong HUANG Hou-jun caO Hai-yang ZHOU Jian-mei WANG Xue-jing WANG Wei SHI Heng ZHU Xiao-ying YUAN Lin CHEN Department of General Surgery General Hospital of the Air ForcePLA Department of General Surgery Chinese PLA General Hospital Department of Cell Biology Institute of Basic Medical SciencesAcademy of Military Medical Sciences

Objective:Side population(SP) cells may play a crucial role in tumorigenesis and the recurrence of *** kinds of cell lines and tissues have demonstrated the presence of SP cells,including several gastric cancer cell *** study is aimed to identify the cancer stem-like cells in the SP of gastric cancer cell line ***:We used fluorescence activated cell sorting(FACS) to sort SP cells in the human gastric carcinoma cell line MKN-45(cells labeled with Hoechst 33342) and then characterized the cancer stem-like properties of SP ***:This study found that the SP cells had higher clone formation efficiency than major population(MP) *** stemness-related gene expression profiles,including OCT-4,SOX-2,NANOG,CD44,and adenosine triphosphate(ATP)-binding cassette transporters gene ABCG2,were tested in SP and MP cells using quantitative real-time reverse transcription polymerase chain reaction(RT-PCR).Western blot was used to show the difference of protein expression between SP and MP *** results show that there was significantly higher protein expression in SP cells than in MP *** inoculated into non-obese diabetic/severe combined immunodeficiency(NOD/SCID) mice,SP cells show higher tumorigenesis tendency than MP ***:These results indicate that SP cells possess cancer stem cell properties and prove that SP cells from MKN-45 are gastric cancer stem-like cells.

关键词： ATP-binding cassette transporters Side population cells Stem cells Benzimidazole (Hoechst 33342),Stomach neoplasm

Al-modified yolk-shell silica particle-supported NiMo catalysts for ultradeep hydrodesulfurization of dibenzothiophene and 4,6-dimethyldibenzothiophene:Efficient accessibility of active sites and suitable acidity

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Petroleum Science 2024年第1期21卷 654-666页

作者： Ke Yu Wei-Min Kong zhen Zhao ai-Jun Duan Lian Kong Xi-Long Wang State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing102249China Institute of catalysis for Energy and Environment College of Chemistry and Chemical EngineeringShenyang Normal UniversityShenyang 110034LiaoningChina

Yolk-shell SiO2 particles(YP)with center-radial meso-channels were fabricated through a simple and effective ***-containing YP-supported NiMo catalysts with different Al amounts(NiMo/AYP-x,x=Si/Al molar proportion)were prepared and dibenzothiophene(DBT)and 4,6-dimethyl-dibenzothiophene(4,6-DMDBT)were employed as the probes to evaluate the hydrodesulfurization(HDS)catalytic *** as-prepared AYP-x carriers and corresponding catalysts were characterized by some advanced characterizations to obtain deeper correlations between physicochemical properties and the HDS *** average pore sizes of series AYP-x supports are above 6.0 nm,which favors the mass transfer of organic *** cavity between the yolk and the shell is beneficial for the enrichment of S-containing compounds and the accessibility between reactants and active *** embedded into the silica framework could facilitate the formation of Lewis(L)and Brønsted(B)acid sites and adjust the metal-support interaction(MSI).Among all the as-synthesized catalysts,NiMo/AYP-20 catalyst shows the highest HDS *** improved HDS activity of NiMo/AYP-20 catalyst is attributed to the perfect combination of excellent structural properties of the yolk-shell mesoporous silica,enhanced acidity,moderate MSI,and good accessibility/dispersion of active components.

关键词： Al-containing yolk-shell silica particles Accessibility Acidity Metal-support interaction Hydrodesulfurization

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关于儿科学发展融入叙事医学理念的思考

中国当代儿科杂志 2024年第4期26卷 325-330页

作者：金贞爱延边大学附属医院围产新生儿/儿童家庭门诊吉林延吉133000

医学是不断进步的科学,是多学科融合的科学,归根结底是关于“人”的科学。半个世纪以来,国内外掀起重塑医学人文精神的热潮。叙事医学是高度融合医学专业性和人文普世性的新兴学科。近十几年来,我国叙事医学从无到有、从点到面,发展迅... 详细信息

医学是不断进步的科学,是多学科融合的科学,归根结底是关于“人”的科学。半个世纪以来,国内外掀起重塑医学人文精神的热潮。叙事医学是高度融合医学专业性和人文普世性的新兴学科。近十几年来,我国叙事医学从无到有、从点到面,发展迅猛。该文通过介绍叙事医学在国内外的发展历程,阐述如何正确理解中国叙事医学体系的内涵以及实践叙事医学的意义,剖析当前在临床实践、教育教学、科学研究、医患共识及社会认可等方面存在的问题,并提出努力方向,即在“大健康”和“新医科”语境下,叙事医学赋能,助力构建和谐医疗叙事生态,促进儿科学高质量发展,也为医科院校教育创新和人才培养贡献人文力量和智慧。

关键词：叙事医学儿科学发展

Nuclear charge radius predictions by kernel ridge regression with odd-even effects

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Nuclear Science and Techniques 2024年第2期35卷 94-102页

作者： Lu Tang zhen-Hua Zhang Mathematics and Physics Department North China Electric Power UniversityBeijing 102206China Hebei Key Laboratory of Physics and Energy Technology North China Electric Power UniversityBaoding 071000China

The extended kernel ridge regression(EKRR)method with odd-even effects was adopted to improve the description of the nuclear charge radius using five commonly used nuclear *** are:(i)the isospin-dependent A^(1∕3) formula,(ii)relativistic continuum Hartree-Bogoliubov(RCHB)theory,(iii)Hartree-Fock-Bogoliubov(HFB)model HFB25,(iv)the Weizsacker-Skyrme(WS)model WS*,and(v)HFB25**** the last two models,the charge radii were calculated using a five-parameter formula with the nuclear shell corrections and deformations obtained from the WS and HFB25 models,*** each model,the resultant root-mean-square deviation for the 1014 nuclei with proton number Z≥8 can be significantly reduced to 0.009-0.013 fm after considering the modification with the EKRR *** best among them was the RCHB model,with a root-mean-square deviation of 0.0092 *** extrapolation abilities of the KRR and EKRR methods for the neutron-rich region were examined,and it was found that after considering the odd-even effects,the extrapolation power was improved compared with that of the original KRR *** strong odd-even staggering of nuclear charge radii of ca and Cu isotopes and the abrupt kinks across the neutron N=126 and 82 shell closures were also calculated and could be reproduced quite well by calculations using the EKRR method.

关键词： Nuclear charge radius Machine learning Kernel ridge regression method

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16世纪中国博古图与西方静物画中的物比较

艺术百家 2024年第2期40卷 1-8页

作者：倪爱珍江西省社会科学院文学与文化研究所江西南昌330077

中国博古图与西方静物画的兴盛都始于16世纪前后,都以静物为表现对象,但又有所不同。从物的属性来看,博古图中的物与人们的精神需求紧密相关,其主要功能经历了从宋代的正经补史到明代的雅文化象征再到清代的吉祥文化寓意的变迁;在西方... 详细信息

中国博古图与西方静物画的兴盛都始于16世纪前后,都以静物为表现对象,但又有所不同。从物的属性来看,博古图中的物与人们的精神需求紧密相关,其主要功能经历了从宋代的正经补史到明代的雅文化象征再到清代的吉祥文化寓意的变迁;在西方静物画发展史上具有节点意义的罗马静物画、荷兰静物画、夏尔丹静物画的繁荣都与特定时期物质生活的变化紧密相关。从物的审美来看,博古图因物喻志,以志为本,体现了中国传统诗学的比兴理论;静物画观物绘形,以物为本,使被忽视或熟视无睹的事物变得陌生、反常,体现了陌生化的审美追求。从物的感知来看,两者体现了中西文化中感物与观物两种不同的美学传统及其背后的感官倚重的不同。但由于艺术有其自身的特征和发展规律,所以两者的这些不同只是相对的。

关键词：博古图静物画感物观物

Analysis of level structure and monopole effects in ca isotopes

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NUCLEAR SCIENCE AND TECHNIQUES 2024年第10期35卷 1-7页

作者： Li, Jin Chen, ai-Xi Jalili, Amir Wang, Han-Kui Zhejiang Sci Tech Univ Sch Sci Hangzhou 310018 Peoples R China

Understanding the properties of nuclei near the double magic nucleus 40ca is crucial for both nuclear theory and experiments. In this study, ca isotopes were investigated using an extended pairing-plus-quadrupole model with monopole corrections. The negative-parity states of 44ca were coupled with the intruder orbital g9/2\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$g_{9/2}$$\end{document} at 4 MeV. The values of E4+\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$E_{4+}$$\end{document}/E2+\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$E_{2+}$$\end{document} agree well with experimental trend from 42ca to 50ca, considering monopole effects between nu f7/2\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$\nu f_{7/2}$$\end{document} and nu p3/2\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$\nu p_{3/2}$$\end{document}(nu f5/2\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$\nu f_{5/2}$$\end{docume

关键词： Shell model Doubly magic Isotopes Monopole effects Level structure BETA-DEcaY MODEL

ca_(2)MnO_(4)-layered perovskite modified by NaNO_(3)for chemical-looping oxidative dehydrogenation of ethane to ethylene

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Chinese Journal of Chemical Engineering 2024年第4期68卷 53-64页

作者： Weixiao Ding Kun Zhao Shican Jiang zhen Huang Fang He College of Chemistry and Bioengineering Guilin University of TechnologyGuilin 541006China Guangzhou Institute of Energy Conversion Chinese Academy of SciencesGuangzhou 510640China School of Chemistry and Chemical Engineering Nanjing University of Science and TechnologyNanjing 210094China

Chemical-looping oxidative dehydrogenation(CL-ODH)is a process designed for the conversion of alkanes into olefins through cyclic redox reactions,eliminating the need for gaseous O_(2).In this work,we investigated the use of ca_(2)MnO_(4)-layered perovskites modified with NaNO_(3) dopants,serving as redox catalysts(also known as oxygen carriers),for the CL-ODH of ethane within a temperature range of 700-780℃.Our findings revealed that the incorporation of NaNO_(3) as a modifier significantly-nhanced the selectivity for-thylene generation from ca_(2)MnO_(4).At 750℃and a gas hourly space velocity of 1300 h^(-1),we achieved an-thane conversion up to 68.17%,accompanied by a corresponding-thylene yield of 57.39%.X-ray photoelectron spectroscopy analysis unveiled that the doping NaNO_(3) onto ca_(2)MnO_(4) not only played a role in reducing the oxidation state of Mn ions but also increased the lattice oxygen content of the redox ***,formation of NaNO_(3) shell on the surface of ca_(2)MnO_(4) led to a reduction in the concentration of manganese sites and modulated the oxygen-releasing behavior in a step-wise *** modulation contributed significantly to the enhanced selectivity for ethylene of the NaNO_(3)-doped ca_(2)MnO_(4) *** findings provide compelling evidence for the potential of ca_(2)MnO_(4)-layered perovskites as promising redox catalysts in the context of CL-ODH reactions.

关键词： Chemical-looping oxidative dehydrogenation Ethane Ethylene NaNO_(3)-doped ca_(2)MnO_(4)redox catalyst Layered perovskites

The Bright Single Pulse Emission from PSR B1133+16

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Research in Astronomy and Astrophysics 2024年第4期24卷 253-261页

作者： Jun Tan Zhi-Gang Wen zhen Wang Xue-Feng Duan Hong-Guang Wang Na Wang Vishal Gajjar Jian-Ping Yuan Rai Yuen Wen-Ming Yan Jian-Ling Chen Wei Han Hui Wang Cheng-Bing Lyu ai-Jun Dong Maths and Information Technology School Yuncheng UniversityYuncheng 044000China Xinjiang Astronomical Observatory Chinese Academy of SciencesUrumqi 830011China Xinjiang Key Laboratory of Radio Astrophysics Urumqi 830011China School of Physics and Materials Science Guangzhou UniversityGuangzhou 510006China Space Science Laboratory University of CaliforniaBerkeley 94710USA Department of Physics and Electronic Engineering Yuncheng UniversityYuncheng 044000China School of Physics and Electronic Science Guizhou Normal UniversityGuiyang 550025China

We have conducted a comprehensive investigation into the bright single pulse emission from PSR B1133+16using the Giant Metrewave Radio *** time resolution data(61μs)were obtained at a center frequency of 322 MHz with a bandwidth of 32 MHz over a continuous observation period of 7.45 hr.A total of 1082 bright pulses were sporadically detected with peak flux densities ranging from 10 to 23 times stronger than the average pulse ***,no giant pulse-like emission with a relative pulse energy larger than 10 and extremely short duration was detected,indicating that these bright pulses cannot be categorized as giant pulse *** majority of these bright pulses are concentrated in pulse phases at both the leading and trailing windows of the average pulse profile,with an occurrence ratio of approximately *** pulse energy distribution for all individual pulses can be described by a combination of two Gaussian components and a cutoff power-law with an index of α=-*** updated nulling fraction of 15.35%±0.45% was determined from the energy *** emission of individual pulses follows a log-normal distribution in peak flux density *** is imperative that regular phase drifting in bright pulse sequence is identified in both the leading and trailing components for the first *** physical mechanisms are discussed in detail to provide insights into these observations.

关键词： (stars:)pulsars:general (stars:)pulsars:individual(PSR B1133+16) methods:observational methods:data analysis

Stress relaxation properties of calcium silicate hydrate:a molecular dynamics study

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第2期25卷 97-115页

作者： Zhicheng GENG Shengwen TANG Yang WANG Hubao A zhen HE Kai WU Lei WANG State Key Laboratory of Water Resources Engineering and Management Wuhan UniversityWuhan430072China Key Laboratory of Advanced Civil Engineering Materials of Ministry of Education School of Materials Science and EngineeringTongji UniversityShanghai200092China College of Materials Science and Engineering Xi’an University of Architecture and TechnologyXi’an710055China

The time-dependent viscoelastic response of cement-based materials to applied deformation is far from fully understood at the atomic *** silicate hydrate(C-S-H),the main hydration product of Portland cement,is responsible for the viscoelastic mechanism of cement-based *** this study,a molecular model of C-S-H was developed to explain the stress relaxation characteristics of C-S-H at different initial deformation states,ca/Si ratios,temperatures,and water contents,which cannot be accessed *** stress relaxation of C-S-H occurs regardless of whether it is subjected to initial shear,tensile,or compressive deformation,and shows a heterogeneous *** plays a crucial role in the stress relaxation process.A large ca/Si ratio and high temperature reduce the cohesion between the calcium-silicate layer and the interlayer region,and the viscosity of the interlayer region,thereby accelerating the stress relaxation of *** effect of the hydrogen bond network and the morphology of C-S-H on the evolution of the stress relaxation characteristics of C-S-H at different water contents was elucidated by nonaffine mean squared *** results shed light on the stress relaxation characteristics of C-S-H from a microscopic perspective,bridging the gap between the microscopic phenomena and the underlying atomic-level mechanisms.

关键词： calcium silicate hydrate(C-S-H) Stress relaxation ca/Si ratio Temperature Water content Atomic simulation