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Multimodal Machine Learning Guides Low Carbon Aeration Strategies in Urban Wastewater Treatment

Engineering 2024年第5期36卷 51-62页

作者： Hong-Cheng wang Yu-Qi wang Xu wang Wan-Xin Yin Ting-Chao Yu Chen-Hao Xue ai-jie wang State Key Laboratory of Urban Water Resource and Environment School of Civil and Environmental EngineeringHarbin Institute of Technology(Shenzhen)Shenzhen 518055China Key Laboratory of Drinking Water Safety and Distribution Technology of Zhejiang Province College of Civil Engineering and ArchitectureZhejiang UniversityHangzhou 310058China

The potential for reducing greenhouse gas(GHG)emissions and energy consumption in wastewater treatment can be realized through intelligent control,with machine learning(ML)and multimodality emerging as a promising ***,we introduce an ML technique based on multimodal strategies,focusing specifically on intelligent aeration control in wastewater treatment plants(WWTPs).The generalization of the multimodal strategy is demonstrated on eight ML *** results demonstrate that this multimodal strategy significantly enhances model indicators for ML in environmental science and the efficiency of aeration control,exhibiting exceptional performance and *** random forest with visual models achieves the highest accuracy in forecasting aeration quantity in multimodal models,with a mean absolute percentage error of 4.4%and a coefficient of determination of *** testing in a full-scale plant reveals that the multimodal model can reduce operation costs by 19.8%compared to traditional fuzzy control *** potential application of these strategies in critical water science domains is *** foster accessibility and promote widespread adoption,the multimodal ML models are freely available on GitHub,thereby eliminating technical barriers and encouraging the application of artificial intelligence in urban wastewater treatment.

关键词： Wastewater treatment Multimodal machine learning Deep learning Aeration control Interpretable machine learning

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Digital Twins for Wastewater Treatment:A Technical Review

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Engineering 2024年第5期36卷 21-35页

作者： ai-jie wang Hewen Li Zhejun He Yu Tao Hongcheng wang Min Yang Dragan Savic Glen TDaigger Nanqi Ren School of Civil and Environmental Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090China Department of Civil and Environmental Engineering Cornell UniversityIthacaNY 14850USA BIOMATH Department of Data Analysis and Mathematical ModellingGhent UniversityGhent 9000Belgium KWR Water Research Institute Nieuwegein 3430 BBNetherlands Centre for Water Systems University of ExeterExeter EX44QFUK Department of Civil and Environmental Engineering University of MichiganAnn ArborMI 48109USA

The digital twins concept enhances modeling and simulation through the integration of real-time data and *** review elucidates the foundational elements of digital twins,covering their concept,entities,domains,and key *** specifically,we investigate the transformative potential of digital twins for the wastewater treatment engineering *** discussion highlights the application of digital twins to wastewater treatment plants(WWTPs)and sewage networks,hardware(i.e.,facilities and pipes,sensors for water quality and activated sludge,hydrodynamics,and power consumption),and software(i.e.,knowledge-based and data-driven models,mechanistic models,hybrid twins,control methods,and the Internet of Things).Furthermore,two cases are provided,followed by an assessment of current challenges in and perspectives on the application of digital twins in *** review serves as an essential primer for wastewater engineers navigating the digital paradigm shift.

关键词： Digital twins Urban water systems Wastewater treatment

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Efficient treatment of azo dye containing wastewater in a hybrid acidogenic bioreactor stimulated by biocatalyzed electrolysis

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Journal of Environmental Sciences 2016年第1期28卷 198-207页

作者： Hong-Cheng wang Hao-Yi Cheng Shu-Sen wang Dan Cui Jing-Long Han Ya-Ping Hu Shi-Gang Su ai-jie wang Key Laboratory of Environmental Biotechnology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences State Key Laboratory of Urban Water Resource and Environment Harbin Institute of Technology

In this study, a novel scaled-up hybrid acidogenic bioreactor（HAB） was designed and adopted to evaluate the performance of azo dye（acid red G, ARG） containing wastewater treatment. Principally, HAB is an acidogenic bioreactor coupled with a biocatalyzed electrolysis module. The effects of hydraulic retention time（HRT） and ARG loading rate on the performance of HAB were investigated. In addition, the influent was switched from synthetic wastewater to domestic wastewater to examine the key parameters for the application of HAB. The results showed that the introduction of the biocatalyzed electrolysis module could enhance anoxic decolorization and COD（chemical oxygen demand） removal. The combined process of HAB-CASS presented superior performance compared to a control system without biocatalyzed electrolysis（AB-CASS）. When the influent was switched to domestic wastewater, with an environment having more balanced nutrients and diverse organic matters, the ARG, COD and nitrogen removal efficiencies of HAB-CASS were further improved, reaching 73.3% ± 2.5%, 86.2% ± 3.8% and 93.5% ± 1.6% at HRT of 6 hr, respectively, which were much higher than those of AB-CASS（61.1% ± 4.7%,75.4% ± 5.0% and 82.1% ± 2.1%, respectively）. Moreover, larger TCV/TV（total cathode volume/total volume） for HAB led to higher current and ARG removal. The ARG removal efficiency and current at TCV/TV of 0.15 were 39.2% ± 3.7% and 28.30 ± 1.48 mA,respectively. They were significantly increased to 62.1% ± 2.0% and 34.55 ± 0.83 mA at TCV/TV of 0.25. These results show that HAB system could be used to effectively treat real wastewater.

关键词： HAB(hybrid acidogenic bioreactor) Scale-up Azo dye Domestic wastewater Cyclic activated sludge system(CASS)

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A model reduction approach for discrete-time linear time-variant systems with delayed inputs

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Science China(Information Sciences) 2024年第4期67卷 197-217页

作者： ai-Guo WU Guang-Ren DUAN Yu wang jie ZHANG School of Mechanical Engineering and Automation Harbin Institute of Technology(Shenzhen) HIT Wuhu Robot Technology Research Institute Center for Control Science and Technology Southern University of Science and Technology

A model reduction approach is presented for discrete-time linear time-variant input-delayed systems. According to this proposed approach, a dynamical variable is constructed by taking advantage of the current state and historical information of input. It is revealed that the behavior of this dynamical variable is governed by a discrete-time linear delay-free system. It is worth noting that the presented variable transformation does not require the system matrix to be invertible. Based on the reduced delay-free models,stabilizing control laws can be easily obtained for the original delayed system. For the case with a single input delay, the constructed variable is an exact prediction for the future state, and thus the stabilizing control law could be designed by replacing the future state with its prediction. Finally, three discrete-time periodic systems with delayed input are employed to illustrate how to utilize the presented model reduction approaches.

关键词： reduction approach predictor-based feedback time-varying systems delayed input periodic system

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Efficiency,mechanism and microbial community of Cd(Ⅱ)removal by mixed bacteria enriched from heavy metals mine soil

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Transactions of Nonferrous Metals Society of China 2022年第10期32卷 3404-3419页

作者： Tao-tao ZENG Xiao-ling ZHANG Hai-du NONG Qing HU Liang-qin wang ai-jie wang Hunan Provincial Key Laboratory of Pollution Control and Resources Reuse Technology University of South ChinaHengyang 421001China Key Laboratory of Environmental Biotechnology Chinese Academy of SciencesBeijing 100085China

Mixed bacteria were enriched from heavy metals mine soil for cadmium(Cd(Ⅱ))-containing wastewater treatment. Batch adsorption experiment results showed that the optimal pH, temperature, initial Cd(Ⅱ) concentration, and biomass dosage were 6.0, 30 ℃, 20 mg/L, and 1 g/L, respectively. Living biomass exhibited better Cd(Ⅱ) removal efficiency(91.97%) than autoclaved biomass(79.54%) under optimal conditions. The isotherms and kinetics of living biomass conformed to the Langmuir isotherm model and pseudo-first-order kinetic model, respectively. FTIR results implied that amine groups, hydroxyl groups and phosphoric acid play an important role in the Cd(Ⅱ) adsorption process, while XRD results showed that crystalline Cd(OH)and CdO were obtained. After Cd(Ⅱ)-containing wastewater treatment exposure, the dominant bacteria genera included Comamonas(39.94%), unclassified_f__Enterobacteriaceae(34.96%), Ochrobactrum(14.07%), Alcaligenes(4.84%), Bordetella(2.07%), Serratia(1.04%), and Bacillus(1.01%). Function prediction showed that the abundance of metabolic genes changed significantly. This study proposes the potential application of mixed bacteria for Cd(Ⅱ)-containing wastewater treatment.

关键词： Cd(Ⅱ) wastewater treatment bacterial community function prediction

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Ordered mesoporous carbon as an efficient heterogeneous catalyst to activate peroxydisulfate for degradation of sulfadiazine

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Chinese Chemical Letters 2022年第5期33卷 2747-2752页

作者： Zhi-Ling Li Di Cao Hao Cheng Fan Chen Jun Nan Bin Liang Kai Sun Cong Huang ai-jie wang State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China School of Civil&Environmental Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China School of Ecology and Environment Northwestern Polytechnical UniversityXi’an 710129China Key Lab of Structures Dynamic Behavior and Control of China Ministry of Education School of Civil EngineeringHarbin Institute of TechnologyHarbin 150090China National Technology Innovation Center of Synthetic Biology Tianjin Institute of Industrial BiotechnologyChinese Academy of SciencesTianjin 300308China

Catalytic potential of carbon nanomaterials in peroxydisulfate(PDS)advanced oxidation systems for degradation of antibiotics remains poorly *** study revealed ordered mesoporous carbon(type CMK)acted as a superior catalyst for heterogeneous degradation of sulfadiazine(SDZ)in PDS sys-tem,with a first-order reaction kinetic constant(k)and total organic carbon(TOC)mineralization efficiency of 0.06 min^(–1) and 59.67%±3.4%within 60min,*** catalyzed PDS system exhibited high degradation efficiencies of five other sulfonamides and three other types of antibiotics,verifying the broad-degradation capacity of *** neutral pH conditions,the optimal catalytic parameters were an initial SDZ concentration of 44.0mg/L,CMK dosage of 0.07g/L,and PDS dosage of 5.44mmol/L,respectively.X-ray photoelectron spectroscopy and Raman spectrum analysis confirmed that the defect structure at edge of CMK and oxygen-containing functional groups on surface of CMK were major active sites,contributing to the high catalytic *** radical quenching analysis revealed that both SO_(4)•−and•OH were generated and participated in catalytic *** addition,direct electron transfer by CMK to activate PDS also occurred,further promoting catalytic *** of SDZ molecule was optimized using density functional theory,and the possible reaction sites in SDZ molecule were calculated using Fukui *** ultra-high-performance liquid chromatography(UPLC)–mass spectrometry(MS)/MS analysis,three potential degradation pathways were proposed,including the direct removal of SO_(2)molecules,the 14S-17N fracture,and the 19C-20N and 19C-27N cleavage of the SDZ *** study demonstrated that ordered mesoporous carbon could work as a feasible catalytic material for PDS advanced oxidation during removal of antibiotics from wastewater.

关键词： Ordered mesoporous carbon CMK Sulfadiazine Peroxydisulfate Degradation pathway Density functional theory Physicochemical properties

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Classifying hepatitis B therapies with insights from covalently closed circular DNA dynamics

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Virologica Sinica 2024年第1期39卷 9-23页

作者： jie-Li Hu ai-Long Huang Key Laboratory of Molecular Biology on Infectious Diseases Ministry of EducationChongqing Medical UniversityChongqing400016China

The achievement of a functional cure for chronic hepatitis B(CHB)remains limited to a minority of patients treated with currently approved *** primary objective in developing new anti-HBV drugs is to enhance the functional cure rates for CHB.A critical prerequisite for the functional cure of CHB is a substantial reduction,or even eradication of covalently closed circular DNA(cccDNA).Within this context,the changes in cccDNA levels during treatment become as a pivotal *** have previously analyzed the factors influencing cccDNA dynamics and introduced a preliminary classification of hepatitis B treatment strategies based on these *** this review,we employ a systems thinking perspective to elucidate the fundamental aspects of the HBV replication cycle and to rationalize the classification of treatment strategies according to their impact on the dynamic equilibrium of *** upon this foundation,we categorize current anti-HBV strategies into two distinct groups and advocate for their combined use to significantly reduce cccDNA levels within a well-defined timeframe.

关键词： Hepatitis B cccDNA Functional cure Dynamics Treatment Strategy

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Inkjet-Printing Controlled Phase Evolution Boosts the Efficiency of Hole Transport Material Free and Carbon-Based CsPbBr3 Perovskite Solar Cells Exceeding 9%

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Energy & Environmental Materials 2024年第2期7卷 213-224页

作者： Lihua Zhang Shi Chen jie Zeng Zhengyan Jiang Qian ai Xianfu Zhang Bihua Hu Xingzhu wang Shihe Yang Baomin Xu Department of Materials Science and Engineering and Shenzhen Engineering Research and Development Center for Flexible Solar Cells Southern University of Science and Technology Department of Chemistry The Hong Kong University of Science and Technology Henan Key Laboratory of Photovoltaic Materials Henan University Guangdong Key Lab of Nano-Micro Material Research School of Chemical Biology and Biotechnology Shenzhen Graduate School Peking University Key University Laboratory of Highly Efficient Utilization of Solar Energy and Sustainable Development of Guangdong Southern University of Science and Technology Guangdong-Hong Kong-Macao Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices Southern University of Science and Technology

Hole transport material free carbon-based all-inorganic CsPbBr3perovskite solar cells（PSCs） are promising for commercialization due to its low-cost,high open-circuit voltage(Voc) and superior *** to the different solubility of PbBr2and CsBr in conventional solvents,CsPbBr3films are mainly obtained by multi-step spin-coating through the phase evolution from PbBr2to CsPb2Br5and then to *** scalable fabrication of highquality CsPbBr3films has been rarely ***,an inkjet-printing method is developed to prepare high-quality *** formation of long-range crystalline CsPb2Br5phase can effectively improve phase purity and promote regular crystal stacking of ***,the inkjetprinted CsPbBr3C-PSCs realized PCEs up to 9.09%,8.59% and 7.81% with active areas of 0.09,0.25,and 1 cm2,respectively,demonstrating the upscaling potential of our fabrication method and *** high performance is mainly ascribed to the high purity,strong crystal orientation,reduced surface roughness and lower trap states density of the as-printed *** work provides insights into the relationship between the phase evolution mechanisms and crystal growth dynamics of cesium lead bromide halide films.

关键词： all-inorganic perovskite solar cells CsPbBr3 inkjet-printing phase evolution

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Effective electrocatalytic hydrodechlorination of 2,4,6-trichlorophenol by a novel Pd/MnO_(2)/Ni foam cathode

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Chinese Chemical Letters 2022年第8期33卷 3823-3828页

作者： Zi-Meng Zhang Rui Cheng Jun Nan Xue-Qi Chen Cong Huang Di Cao Cai-Hua Bai Jing-Long Han Bin Liang Zhi-Ling Li ai-jie wang State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China National Technology Innovation Center of Synthetic Biology Tianjin Institute of Industrial BiotechnologyChinese Academy of SciencesTianjin 300308China State Key Laboratory of Urban Water Resource and Environment School of Civil&Environmental EngineeringHarbin Institute of Technology ShenzhenShenzhen 518055China

Pd modified electrodes possess problems such as easy agglomeration and low electrolytic ability,and the use of manganese dioxide(MnO_(2)) to facilitate Pd reduction of organic pollutants is just ***,there is still a limited understanding of how to match the Pd load and MnO_(2) to realize optimal dechlorination efficiency at minimum ***,a Pd/MnO_(2)/Ni foam cathode was successfully fabricated and applied for the efficient electrochemical dechlorination of 2,4,6-trichlorophenol(2,4,6-TCP).The optimal electrocatalytic hydrodechlorination(ECH)performance with 2,4,6-TCP dechlorination efficiency(92.58%in 180 min)was obtained when the concentration of PdCl_(2) precipitation was 1 mmol/L,the deposition time of MnO_(2) was 300 s and cathode potential was-0.8 *** influenced by the exogenous factors(e.g.,initial pH and coexisted ions)were further *** was found that the neutral pH was the most favorable for ECH and a reduction in dechlorination efficiency(6%~47.6%)was observed in presence of 5 mmol/L of NO_(2)^(-),NO_(3)^(-),S^(2-)or SO_(3)^(2-).Cyclic voltammetry(CV)and quenching experiments verified the existence of three hydrogen species on Pd surface,including adsorbed atomic hydrogen(H^(*)_(ads)),absorbed atomic hydrogen(H^(*)_(abs)),and molecular hydrogen(H_(2)).And the introduction of MnO_(2)promoted the generation of atomic H^(*).Only adsorbed atomic hydrogen(H^(*)_(ads)) was confirmed that it truly facilitated the ECH *** H^(*)_(ads) induced reduction,the direct reduction by cathode electrons also participated in the 2,4,6-TCP dechlorination ***/MnO_(2)/Ni foam cathode shows excellent dechlorination performance,fine stability and recyclable potential,which provides strategies for the effective degradation of persistent halogenated organic pollutants in groundwater.

关键词： Pd/MnO_(2)/Ni foam cathode 2 4 6-Trichlorophenol Electrocatalytic hydrodechlorination Dechlorination pathway Atomic H^(*)generation and utilization

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Infrared microspectroscopy beamline BL06B at SSRF

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Nuclear Science and Techniques 2024年第1期35卷 10-17页

作者： Te Ji Hua-Chun Zhu Wei-Wei Peng jie wang Hong-Wei Zhao ai-Guo Li Min Chen Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210China

The infrared microspectroscopy beamline(BL06B) is a phase Ⅱ beamline project at the Shanghai Synchrotron Radiation Facility(SSRF). The construction and optical alignment of BL06B were completed by the end of 2020. By 2021, it became accessible to users. The synchrotron radiation infrared(SRIR) source included edge radiation(ER) and bending magnet radiation(BMR). The extracted angles in the horizontal and vertical directions were 40 and 20 mrad, respectively. The photon flux, spectral resolution, and focused spot size were measured at the BL06B endstation, and the experimental results were consistent with theoretical calculations. SRIR light has a small divergence angle, high brightness, and a wide wavelength range. As a source of IR microscopy, it can easily focus on a diffraction-limited spatial resolution with a high signal-to-noise ratio(SNR). The BL06B endstation can be applied in a wide range of research fields, including materials, chemistry, biology, geophysics, and pharmacology.

关键词： Synchrotron radiation Infrared beamline Infrared microspectroscopy

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