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Metal-organic frameworks (MOFs) in aqueous batteries (ABs):unlocking potential through innovative materials design

Science China Chemistry 2025年

作者： Bo Han Erhai Hu Bei-Er Jia Ziyang Liu Shuen Tso afriyant. sumboja Ivandini T.Anggraningrum Anne Zulfia Syahrial Qingyu Yan SCARCE Laboratory Energy Research Institute NTU (ERIN) Nanyang Technological University School of Materials Science and Engineering Nanyang Technological University Material Science and Engineering Research Group Faculty of Mechanical and Aerospace Engineering Institut Teknologi Bandung Department of Chemistry University of Indonesia Metallurgical & Materials Engineering Department Fakultas Teknik Universitas Indonesia

Metal-organic frameworks (MOFs) represent a revolutionary class of materials in the field of energy storage,particularly for aqueous batteries (ABs).Distinguished by their large surface area,tuneable porosity,and adaptable chemical activity,MOFs offer significant advantages over conventional materials in battery *** article provides a thorough analysis of the crucial role that MOFs play in improving the efficiency of *** includes a concise review of the current research progress,emphasizing the fundamental processes by which MOFs enhance electrochemical ***,the review examines the synthesis and design strategies for the structure of MOFs to maximize ion transport,improve conductivity,and enhance *** structural advantages,chemical versatility,stability,durability and functionalization potential of MOFs are comprehensively ***,we explore the distinct advantages of MOFs in overcoming common challenges encountered in ABs,such as declining capacity,inadequate cycling stability,and limited energy *** paper also highlights the future research directions needed to fully harness their *** goal is to develop a fundamental understanding and stimulate further progress in the use of MOFs for advanced energy storage solutions.

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FeCo Nanoparticle-Loaded Nutshell-Derived Porous Carbon as Sustainable Catalyst in Al-Air Batteries

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Energy Material Advances 2021年第1期2021卷 273-284页

作者： A.sumboja B.Prakoso Y.Ma F.R.Irwan J.J.Hutani A.Mulyadewi M.A.A.Mahbub Y.Zong Z.Liu Material Science and Engineering Research Group Faculty of Mechanical and Aerospace EngineeringInstitut Teknologi BandungJl.Ganesha 10Bandung 40132Indonesia National Centre for Sustainable Transportation Technology(NCSTT) Jl.Ganesha 10Bandung 40132Indonesia Department of Materials Science and Engineering National University of SingaporeSingapore 117574 Institute of Materials Research and Engineering(IMRE) ASTAR(Agency for Science Technology and Research)2 Fusionopolis WayInnovisSingapore#08-03138634

Developing a high-performance ORR(oxygen reduction reaction)catalyst at low cost has been a challenge for the commercialization of high-energy density and low production cost aluminium-air ***,we report a catalyst,prepared by pyrolyzing the shell waste of peanut or pistachio,followed by concurrent nitrogen-doping and FeCo alloy nanoparticle *** surface area(1246.4m2 g-1)of pistachio shell-derived carbon can be obtained by combining physical and chemical treatments of the *** a large surface area carbon eases nitrogen doping and provides more nucleation sites for FeCo alloy growth,furnishing the resultant catalyst(FeCo/N-C-Pistachio)with higher content of N,Fe,and Co with a larger electrochemically active surface area as compared to its peanut shell counterpart(FeCo/N-C-Peanut).The FeCo/N-CPistachio displays a promising onset potential of 0.93V *** and a high saturating current density of 4.49mAcm-2,suggesting its high ORR *** aluminium-air battery,with FeCo/N-C-Pistachio catalyst on the cathode and coupled with a commercial aluminium 1100 anode,delivers a power density of 99.7mWcm-2 and a stable discharge voltage at 1.37V over 5 h of *** high-performance,low-cost,and environmentally sustainable electrocatalyst shows potential for large-scale adoption of aluminium-air batteries.

关键词： cost Porous particle

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