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Rational molecular design of efficient yellow-red dendrimer TADF for solution-processed OLEDs: a combined effect of substitution position and strength of the donors

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Science China Chemistry 2024年第5期67卷 1613-1623页

作者： Changfeng Si Dianming Sun Tomas Matulaitis David b.Cordes Alexandra M.z.Slawin Eli zysman-Colman Organic Semiconductor Centre EaStCHEM School of ChemistryUniversity of St AndrewsSt AndrewsKY169STUK

The development of high-performance solution-processed red organic light-emitting diodes(OLEDs) remains a challenge,particularly in terms of maintaining efficiency at high luminance. Here, we designed and synthesized four novel orange-red thermally activated delayed fluorescence(TADF) dendrimers that are solution-processable: 2GCz bP, 2DPACz bP, 2FbP2GCz and 2FbP2DPACz. We systematically investigated the effect of substitution position and strength of donors on the optoelectronic properties. The reverse intersystem crossing rate constant(kRISC) of the emitters having donors substituted at positions 11and 12 of the dibenzo[a,c]phenazine(bP) is more than 10-times faster than that of compounds substituted having donors substituted at positions 3 and 6. Compound 2DPACz bP, containing stronger donors than 2GCz bP, exhibits a red-shifted emission and smaller singlet-triplet energy splitting, ΔE_(ST), of 0.01 e v. The solution-processed OLED with 10 wt% 2DPACz bP doped in m CP emitted at 640 nm and showed a maximum external quantum efficiency(EQE_(max)) of 7.8%, which was effectively maintained out to a luminance of 1,000 cd m-2. Such a device's performance at relevant display luminance is among the highest for solution-processed red TADF OLEDs. The efficiency of the devices was improved significantly by using 4Cz IPN as an assistant dopant in a hyperfluorescence(HF) configuration, where the 2DPACz bP HF device shows an EQEmaxof 20.0% at λEL of 605 nm and remains high at 11.8% at a luminance of 1,000 cd m-2, which makes this device one of the highest efficiency orange-to-red HF SP-OLEDs to date.

关键词： thermally activated delayed fluorescence solution-processing red OLEDs dibenzo[a,c]phenazine dendrimers

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b-L model with D_(4)×z_(4)×z_(2)symmetry for fermion mass hierarchies and mixings

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Chinese Physics C 2024年第6期48卷 11-30页

作者： v.v.vien Department of Physics Tay Nguyen UniversityDaklakVietnam

We constructed a gauge b-L model with D_(4)×z_(4)×z_(2)symmetry to explain the quark and lepton mass hierarchies and their mixings with realistic CP phases via the type-I seesaw *** quark mases,three quark mixing angles,and the CP phase in the quark sector take the central values whereas Yukawa couplings in the quark sector are diluted in a range of difference of three orders of magnitude by the perturbation theory at the first *** the neutrino sector,a small neutrino mass is achieved by the type-I seesaw *** inverted and normal neutrino mass hierarchies are consistent with the experimental *** predicted sum of neutrino masses for normal and inverted hierarchies,the effective neutrino masses,and the Dirac CP phase are also consistent with recently reported limits.

关键词： flavor symmetries quark and lepton masses and mixing extensions of electroweak gauge sector neutrino mass and mixing non-standard-model neutrinos right-handed neutrinos D4 discrete symmetry

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SANC Monte Carlo programs for small-angle bhabha scattering

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Chinese Physics C 2024年第4期48卷 14-19页

作者： a.b.arb.z.v S.G.bondarenko I.R.boyko L.v.Kalinovskaya A.A.Kampf R.R.Sadykov v.L.Yermolchyk bogoliubov Laboratory of Theoretical Physics JINRDubna141980 Russia Dzhelepov Laboratory of Nuclear Problems JINRDubna141980 Russia Dubna State University Dubna141982 Russia

Luminosity monitoring at e^(+)e^(−)colliders was investigated using SANC Monte Carlo event generator ReneSANCe and integrator MCSANC for simulation of bhabha scattering at low *** are presented for center-of-mass energies of the z boson resonance and at 240 Gev for the conditions of typical luminosity *** is shown that bremsstrahlung events with extremely low electron scattering angles are relevant to match the precision tags of future electron-positron colliders.

关键词： luminosity bhabha scattering QED Monte Carlo simulation

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The Radcliffe Wave Parameters from Data on Open Star Clusters

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Research in Astronomy and Astrophysics 2024年第3期24卷 106-109页

作者： v.v.bobylev A.T.bajkova Pulkovo Astronomical Observatory St-Petersburg 196140Russia

A spectral analysis of the vertical positions and velocities of 374 open star clusters(OSCs)was carried *** took these OSCs from the Hunt and Reffert catalog;they have an average age of about 10 million years,and are located on the galactic plane XY in a narrow zone inclined by 25°to the galactic axis *** following estimates of the parameters of the Radcliffe wave were obtained:(a)the maximum value in periodic perturbations of vertical coordinates z_(max)=92±10pc with the wavelength of these perturbations λ_(z)=4.82±0.09 kpc;(b)the maximum value of the velocity of vertical disturbances Wmax=4.36±0.12km s^(-1) with disturbance wavelengthλ_(W)=1.78±0.02 *** that the results of the vertical velocity analysis are first-class in accuracy and completely new.

关键词： (Galaxy) local interstellar matter-Galaxy structure-(Galaxy) solar neighborhood

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Gradient-induced long-range optical pulling force based on photonic band gap

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Light(Science & Applications) 2024年第5期13卷 865-874页

作者： Wenlong Lu Alexey v.Krasavin Sheng Lan Anatoly v.zayats Qiaofeng Dai Guangdong basic Research Center of Excellence for Structure and Fundamental Interactions of Matter Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and DevicesSchool of Information and Optoelectronic Science and EngineeringSouth China Normal UniversityGuangzhou 510006China Department of Physics and London Centre for Nanotechnology King’s College LondonLondon WC2R 2LSUK

Optical pulling provides a new degree of freedom in optical *** is generally believed that long-range optical pulling forces cannot be generated by the gradient of the incident ***,we theoretically propose and numerically demonstrate the realization of a long-range optical pulling force stemming from a self-induced gradient field in the manipulated *** analogy to potential barriers in quantum tunnelling,we use a photonic band gap design in order to obtain the intensity gradients inside a manipulated object placed in a photonic crystal waveguide,thereby achieving a pulling *** the usual scattering-type optical pulling forces,the proposed gradient-field approach does not require precise elimination of the reflection from the manipulated *** particular,the Einstein-Laub formalism is applied to design this unconventional gradient *** magnitude of the force can be enhanced by a factor of up to 50 at the optical resonance of the manipulated object in the waveguide,making it insensitive to *** developed approach helps to break the limitation of scattering forces to obtain longrange optical pulling for manipulation and sorting of nanoparticles and other *** developed principle of using the band gap to obtain a pulling force may also be applied to other types of waves,such as acoustic or water waves,which are important for numerous applications.

关键词： optical waveguide scattering

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STCF conceptual design report (volume 1): Physics & detector

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Frontiers of physics 2024年第1期19卷 1-154页

作者： M.Achasov X.C.Ai L.P.An R.Aliberti Q.An X.z.bai Y.bai O.bakina A.barnyakov v.blinov v.bobrovnikov D.bodrov A.bogomyagkov A.bondar I.boyko z.H.bu F.M.Cai H.Cai J.J.Cao Q.H.Cao X.Cao z.Cao Q.Chang K.T.Chao D.Y.Chen H.Chen H.X.Chen J.F.Chen K.Chen L.L.Chen P.Chen S.L.Chen S.M.Chen S.Chen S.P.Chen W.Chen X.Chen X.F.Chen X.R.Chen Y.Chen Y.Q.Chen H.Y.Cheng J.Cheng S.Cheng T.G.Cheng J.P.Dai L.Y.Dai X.C.Dai D.Dedovich A.Denig I.Denisenko J.M.Dias D.z.Ding L.Y.Dong W.H.Dong v.Druzhinin D.S.Du Y.J.Du z.G.Du L.M.Duan D.Epifanov Y.L.Fan S.S.Fang z.J.Fang G.Fedotovich C.Q.Feng X.Feng Y.T.Feng J.L.Fu J.Gao Y.N.Gao P.S.Ge C.Q.Geng L.S.Geng A.Gilman L.Gong T.Gong b.Gou W.Gradl J.L.Gu A.Guevara L.C.Gui A.Q.Guo F.K.Guo J.C.Guo J.Guo Y.P.Guo z.H.Guo A.Guskov K.L.Han L.Han M.Han X.Q.Hao J.b.He S.Q.He X.G.He Y.L.He z.b.He z.X.Heng b.L.Hou T.J.Hou Y.R.Hou C.Y.Hu H.M.Hu K.Hu R.J.Hu W.H.Hu X.H.Hu Y.C.Hu J.Hua G.S.Huang J.S.Huang M.Huang Q.Y.Huang W.Q.Huang X.T.Huang X.J.Huang Y.b.Huang Y.S.Huang N.Hüsken v.Ivanov Q.P.Ji J.J.Jia S.Jia z.K.Jia H.b.Jiang J.Jiang S.z.Jiang J.b.Jiao z.Jiao H.J.Jing X.L.Kang X.S.Kang b.C.Ke M.Kenzie A.Khoukaz I.Koop E.Kravchenko A.Kuzmin Y.Lei E.Levichev C.H.Li C.Li D.Y.Li F.Li G.Li G.Li H.b.Li H.Li H.N.Li H.J.Li H.L.Li J.M.Li J.Li L.Li L.Li L.Y.Li N.Li P.R.Li R.H.Li S.Li T.Li W.J.Li X.Li X.H.Li X.Q.Li X.H.Li Y.Li Y.Y.Li z.J.Li H.Liang J.H.Liang Y.T.Liang G.R.Liao L.z.Liao Y.Liao C.X.Lin D.X.Lin X.S.Lin b.J.Liu C.W.Liu D.Liu F.Liu G.M.Liu H.b.Liu J.Liu J.J.Liu J.b.Liu K.Liu K.Y.Liu K.Liu L.Liu Q.Liu S.b.Liu T.Liu X.Liu Y.W.Liu Y.Liu Y.L.Liu z.Q.Liu z.Y.Liu z.W.Liu I.Logashenko Y.Long C.G.Lu J.X.Lu N.Lu Q.F.Lü Y.Lu Y.Lu z.Lu P.Lukin F.J.Luo T.Luo X.F.Luo Y.H.Luo H.J.Lyu X.R.Lyu J.P.Ma P.Ma Y.Ma Y.M.Ma F.Maas S.Malde D.Matvienko z.X.Meng R.Mitchell A.Nefediev Y.Nefedov S.L.Olsen Q.Ouyang P.Pakhlov G.Pakhlova X.Pan Y.Pan E.Passemar Y.P.Pei H.P.Peng L.Peng X.Y.Peng X.J.Peng K.Peters S.Pivovarov E.Pyata b.b.Qi Y.Q.Qi W.b.Qian Y.Qian C.F.Qiao J.J.Qin J.J.Qin L.Q.Qin X.S.Qin T.L.Qiu J.Rademacker C.F.Redmer H.Y.Sang Anhui University Hefei 230039China beihang University Beijing 100191China budker Institute of Nuclear Physics Novosibirsk 630090Russia CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China Cavendish Laboratory University of CambridgeJJ Thomson AveCambridge CB30HEUnited Kingdom Central China Normal University Wuhan 430079China Central South University Changsha 410083China China University of Geosciences Wuhan 430074China China University of Mining and Technology Xuzhou 221116China École Polytechnique Fédérale de Lausanne(EPFL) LausanneSwitzerland Fudan University Shanghai 200433China Goethe University Frankfurt D-60325 Frankfurt am MainGermany Guangxi Normal University Guilin 541004China Guangxi Uninversity Nanning 530004China Hangzhou Institute for Advanced Study UCASHangzhou 310024China Hebei Normal University Shijiazhuang 050024China Hebei University Baoding 071002China Hefei University of Technology Hefei 230601China Helmholtz Institute Mainz Staudinger Weg 18D-55099 MainzGermany Henan Normal University Xinxiang 453007China Henan University Kaifeng 475004China High Energy Physics Center Chung-Ang UniversitySeoul 06974Korea Higher School of Economy 11 Pokrovsky bulvar Moscow 109028Russia Huangshan University Huangshan 245000China Hubei University of Automotive Technology Shiyan 442002China Hunan Normal University Changsha 410081China Hunan University of Science and Technology Xiangtan 411201China Hunan University Changsha 410082China Indiana University BloomingtonIndiana 47405USA Inner Mongolia University Hohhot 010021China Institute of Advanced Science Facilities Shenzhen 518107China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China Institute of Physics Academia SinicaTaipeiTaiwan 11529China Institute of Theoretical Physics Chinese Academy of SciencesBeijing 100190China Jilin University Changch

The superτ-charm facility(STCF)is an electron–positron collider proposed by the Chinese particle physics *** is designed to operate in a center-of-mass energy range from 2 to 7 Gev with a peak luminosity of 0.5×10^(35) cm^(–2)·s^(–1) or *** STCF will produce a data sample about a factor of 100 larger than that of the presentτ-charm factory—the bEPCII,providing a unique platform for exploring the asymmetry of matter-antimatter(charge-parity violation),in-depth studies of the internal structure of hadrons and the nature of non-perturbative strong interactions,as well as searching for exotic hadrons and physics beyond the Standard *** STCF project in China is under development with an extensive R&D *** document presents the physics opportunities at the STCF,describes conceptual designs of the STCF detector system,and discusses future plans for detector R&D and physics case studies.

关键词： electron–positron collider tau-charm region high luminosity STCF detector conceptual design

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Neuroprotective effects of Shaoyao Gancao decoction against excitatory damage in PC12 cells based on the Src-NR2-nNOS pathway

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Journal of Traditional Chinese Medical Sciences 2024年第3期11卷 293-302页

作者： Fan X. Ma H. zhou T. Fu M. Qiao z. Feng Y. Wang z. Shen Y. Wang J. School of Traditional Chinese Medicine Beijing University of Chinese Medicine Beijing 102488 China These authors have contributed equally to this work. School of Traditional Chinese Medicine Xinjiang Medical University Urumqi 830017 China The Centre for Translational biology Research Institute of McGill University Health Centre Montréal H4A 3J1 Canada

Objective: To explore the neuroprotective effects of the Shaoyao Gancao decoction (SGD) against excitatory damage in PC12 cells and the role of the Src-NR2-nNOS pathway mediation by SGD in regulating γ-aminobutyric acid (GAbA)-glutamate (Glu) homeostasis. Methods: N-Methyl-D-aspartic acid (NMDA) was used to establish a PC12 cell excitability injury model. To investigate the neuroprotective effect of SGD, a cell counting kit-8 (CCK-8) assay was used to determine PC12 cell viability, Annexin v/Propidium Iodide (Annexin v/PI) double staining was used to determine PC12 cell apoptosis, and Ca2+ concentration was observed using laser confocal microscopy. GAbA receptor agonists and antagonists were used to analyze the neuroprotective interactions between γ-aminobutyric acid (GAbA) and NMDA receptors. Additionally, molecular biology techniques were used to determine mRNA and protein expression in the Src-NR2-nNOS pathway. We analyzed the correlations between the regulatory sites of GAbA and NMDA interactions, excitatory neurotoxicity, and brain damage at the molecular level. Results: NMDA excitotoxic injury manifested as a significant decrease in cell activity, increased apoptosis and caspase-3 protein expression, and a significant increase in intracellular Ca2+ concentration. Administration of SGD, a GAbAA receptor agonist (muscimol), or a GAbAb receptor agonist (baclofen) decreased intracellular Ca2+ concentrations, attenuated apoptosis, and reversed NMDA-induced upregulation of caspase-3, Src, NMDAR2A, NMDAR2b, and nNOS. Unexpectedly, a GAbAA receptor antagonist (bicuculline) and a GAbAb receptor antagonist (saclofen) failed to significantly increase excitatory neurotoxicity. Conclusions: Taken together, these results not only provide an experimental basis for SGD administration in the clinical treatment of central nervous system injury diseases, but also suggest that the Src-NR2A-nNOS pathway may be a valuable target in excitotoxicity treatment. © 2024 beijing Universit

关键词： N-Methyl-D-aspartic acid (NMDA) nNOS PC12 Shaoyao Gancao decoction Src γ-aminobutyric acid (GAbA)

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Synthesis,characterization and application of PvA/ionic liquid mixed matrix membranes for pervaporation dehydration of isopropanol

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Chinese Journal of Chemical Engineering 2017年第10期25卷 1402-1411页

作者： Ganesh b.Thorat Smita Gupta z.v.P.Murthy Department of Chemical Engineering Sardar Vallabhbhai National Institute of Technology Surat 395007 Gujarat India

In this study,polyvinyl alcohol(PvA)–ionic liquid(IL) membranes were prepared for the separation of isopropyl alcohol(IPA)–water azeotropic mixtures by ***-IL composite membranes were prepared by simple solvent evaporation method using four ILs,viz.,1-n-butyl-3-methylimidazolium chloride(bMIMCl),1-hexyl-3-methylimidazolium chloride(HMIMCl),1-hexyl-3-methylimidazolium tetra fluoroborate(HMIMbF4) and 1-octyl-3-methylimidazolium chloride(OMIMCl).Three ILs were used to study the effect of alkyl chain on the pervaporation *** study had focused on the effect feed water concentration from 10%–40%and effect of feed temperature from 50–80°*** properties of all the membranes were studied using Fourier transform infrared spectroscopy(FTIR),scanning electron microscopy(SEM) and contact angle *** Arrhenius activation energies for permeation were estimated to be in the range 4–12 kJ·mol-1 from the temperature dependent permeation values.

关键词： Composite membranes Ionic liquids Dehydration Isopropanol Pervaporation

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Synthesis gas production on glass cloth catalysts modified by Ni and Co oxides

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Journal of Energy Chemistry 2013年第5期22卷 811-818页

作者： G.b.Aldashukurova A.v.Mironenko z.A.Mansurov N.v.Shikina S.A.Yashnik v.v.Kuznetsov z.R.Ismagilov Institute for Problems in Combustion boreskov Institute of Catalysis of Sb RAS Institute of Coal Chemistry and Material Science of Sb RAS

The catalytic activity of nanostructured low percent (1%) Co-Ni catalysts on the basis of glass fiber (GF) prepared by a"solution combustion" (SC) method was *** catalytic activity of the prepared samples was studied in the reaction of dry reforming of methane (DRM) with *** obtained samples were characterized by a number of physico-chemical methods,including XRD,SEM,TEM,TGA and *** active component was shown to be dispersed in the near-surface layer of the support as nanoparticles of 10—20 nm in *** active component showed a Co3O4 or(Co,Ni)Co2O4 spinel structure,depending on the catalyst *** spinel structure of the active component interacted strongly with the carrier,providing resistance to carbonization,high catalytic activity toward DRM,and high activity and stability in oxidation reactions.

关键词： dry reforming of methane Co-Ni-catalyst glass fiber catalyst self-propagating high temperature synthesis

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Tight Focusing Properties of Radially Polarized Gaussian beams with Pair of vortices

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Chinese Physics Letters 2016年第12期33卷 73-76页

作者： *** K.b.Rajesh M.Udhayakumar z.Jaroszewicz T.v.S.Pillai Department of Physics St.Xavier's Catholic College of EngineeringNagercoilIndia Department of Physics Chikkanna Government Arts College Department of Physical Optics Institute of Applied OpticsPolandand National Institute of Telecommunications Department of Physics University College of EngineeringNagercoilIndia

The tight focusing properties of a radially polarized Gaussian beam with a nested pair of vortices having a radial wave front distribution are investigated theoretically by the vector diffraction theory. The results show that the optical intensity in the focal region can be altered considerably by changing the location of the vortices nested in a radially polarized Gaussian beam. It is noted that focal evolution from one annular focal pattern to a highly confined focal spot in the transverse direction is observed corresponding to the change in the location of the optical vortices in the input plane. It is also observed that the generated focal hole or spot lead to a focal shift along the optical axis remarkably under proper radial phase modulation. Hence the proposed system may be applied to construct tunable optical traps for both high and low refractive index particles.

关键词： of is on in for Tight Focusing Properties of Radially Polarized Gaussian beams with Pair of vortices with

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