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Electric field-induced phase transition from the glasslike to paraelectric phase and dielectric spectra hardening in PMN single crystal

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Journal of Advanced Dielectrics 2023年第2期13卷 1-5页

作者： E.Koroleva a.molokov S.Vakhrushev Ioffe Institute Polytekhnicheskaya 26194021St.-PetersburgRussia

One of the key points in the physics of the relaxors is their response to the applied DC *** studies of this topic were made,in particular on the influence of the field on the dielectric ***,practically,in all the cases,the measurements were performed at a fixed frequency and usually with the change in the temperature at the fixed field *** this paper,we report the evolution of the dielectric spectra at low frequencies(0.1 Hz<ω<1 kHz)at fixed temperature 246 K on changing the DC electric field applied in(111)from 1 kV to 7 ***-Cole function was used to describe the spectra and the field dependences of the mean relaxation timeτ,the oscillation strengthΔεand the width parameterαwere *** obtainedτ(E)andΔε(E)provide evidence of the field-induced transition from the nonpolar glass-like phase to the nonpolar paraelectric phase at around 1.5 kV/*** the paraelectric phase,very fast hardening of the spectra was observed withτchanging from 10 s to about 10−4 *** performed analysis demonstrated that the earlier reported positive C-V effect is completely determined by the spectra hardening,whileΔεdoes not show any change in the glass-like phase and monotonously decreases with a field increase in the paraelectric *** complete understanding of the microscopic origin of the observed phenomena,a detailed study on the short-and long-range structures at the same condition is necessary.

关键词： Relaxor ferroelectrics dielectric spectroscopy phase transition lead magnoniobate

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Effect of interface carbonization on dielectric properties of potassium nitrate nanocomposite based on porous glasses

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Journal of Advanced Dielectrics 2022年第4期12卷 42-48页

作者： a.molokov A.Sysoeva A.Naberezhnov R.Kumar E.Koroleva S.Vakhrushev Peter the Great St.-Petersburg Polytechnical University Polytechnicheskaya 29195251 St.-PetersburgRussia Ioffe Institute Polytekhnicheskaya 26194021 St.-PetersburgRussia Laboratory for High Performance Ceramics Department of Metallurgical and Materials Engineering Indian Institute of Technology-Madras(IIT Madras)Chennai 600036India

Dielectric properties and structure of pure and carbon-modified nanocomposites on the base of porous glasses with an average pore diameter of 6 nm(PG6)with embedded KNO3 have been studied at the temperature diapason of 300-430 K and at fre-quencies of 0.1-3×10^(6) Hz on cooling.X-ray diffraction studies of these samples have shown,that in modified and unmodified composites there is a mixture of the low-temperature paraelectric phase(α-phase)and the ferroelectricγ-*** modified composites,a decrease in permittivity and conductivity is *** response has been analyzed in the framework of modern theoretical *** relaxation processes have been identified and their origin has been *** has been found that the main contribution to the dielectric response of nanocomposite material PG6+KNO3 is provided by charge polarization on interfaces,which can be governed by modifying the inner pore ***-conductivity of both composites has been estimated and the activation energies have been *** energy change observed in a vicinity of 360 K is attributed to the phase transformation and the appearance of KNO3α-phase.

关键词： Nanocomposites ferroelectrics potassium nitrate porous glasses dielectric properties

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