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Tailoring spontaneous infrared emission of HgTe quantum dots with laser-printed plasmonic arrays

light(Science & Applications) 2020年第1期9卷 1870-1879页

作者： A.A.Sergeev D.V.Pavlov A.A.Kuchmizhak M.V.lapine W.K.Yiu Y.Dong N.Ke S.Juodkazis N.Zhao S.V.Kershaw a.l.rogach Institute of Automation and Control Processes Far Eastern BranchRussian Academy of SciencesVladivostok 690041Russia Far Eastern Federal University Vladivostok 690090Russia University of Technology Sydney NSW 2007 SydneyAustralia Department of Materials Science and Engineering and Centre for Functional Photonics(CFP)City University of Hong KongKowloonHong Kong SARChina Engineering Research Center of Nano-Geomaterials of Ministry of Education Faculty of Material Science and ChemistryChina University of GeosciencesWuhan 430074China Department of Electronic Engineering The Chinese University of Hong KongShatinNew TerritoriesHong Kong SARChina Swinburne University of Technology John St.HawthornVIC 3122Australia Melbourne Centre for Nanofabrication ANFF151 Wellington RoadClaytonVIC 3168Australia

Chemically synthesized near-infrared to mid-infrared(IR)colloidal quantum dots(QDs)offer a promising platform for the realization of devices including emitters,detectors,security,and sensor ***,at longer wavelengths,the quantum yield of such QDs decreases as the radiative emission rate drops following Fermi’s golden rule,while non-radiative recombination channels compete with light *** over the radiative and non-radiative channels of the IR-emitting QDs is crucially important to improve the performance of IR-range ***,we demonstrate strong enhancement of the spontaneous emission rate of near-to mid-IR HgTe QDs coupled to periodically arranged plasmonic nanoantennas,in the form of nanobumps,produced on the surface of glasssupported Au films via ablation-free direct femtosecond laser *** enhancement is achieved by simultaneous radiative coupling of the emission that spectrally matches the first-order lattice resonance of the arrays,as well as more efficient photoluminescence excitation provided by coupling of the pump radiation to the local surface plasmon resonances of the isolated ***,coupling of the HgTe QDs to the lattice plasmons reduces the influence of non-radiative decay losses mediated by the formation of polarons formed between QD surface-trapped carriers and the IR absorption bands of dodecanethiol used as a ligand on the QDs,allowing us to improve the shape of the emission spectrum through a reduction in the spectral dip related to this ligand *** the ease of the chemical synthesis and processing of the HgTe QDs combined with the scalability of the direct laser fabrication of nanoantennas with tailored plasmonic responses,our results provide an important step towards the design of IR-range devices for various applications.

关键词： quantum radiative coupling

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Enhancing crystal integrity and structural rigidity of CsPbBr_(3) nanoplatelets to achieve a narrow colorsaturated blue emission

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light(Science & Applications) 2024年第5期13卷 985-997页

作者： Qianqian Huang Wenxu Yin Bo Gao Qingsen Zeng Dong Yao Hao Zhang Yinghe Zhao Weijia Zheng Jiaqi Zhang Xuyong Yang Xiaoyu Zhang Andrey l.rogach Key laboratory of Automobile Materials MOE School of Materials Science&Engineeringand Jilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsJilin UniversityChangchunChina. State Key laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchunChina. State Key laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhanHubeiChina. Department of Chemistry University of VictoriaVictoriaBCCanada. Key laboratory of Advanced Display and System Applications of Ministry of Education Shanghai UniversityShanghaiChina. Department of Materials Science and Engineering and Centre for Functional Photonics(CFP)City University of Hong KongHong Kong S.A.RChina

Quantum-confined CsPbBr_(3) perovskites are promising blue emitters for ultra-high-definition displays,but their soft lattice caused by highly ionic nature has a limited ***,we endow CsPbBr_(3) nanoplatelets(NPls)with atomic crystal-like structural rigidity through proper surface engineering,by using strongly bound N-dodecylbenzene sulfonic acid(DBSA).A stable,rigid crystal structure,as well as uniform,orderly-arranged surface of these NPls is achieved by optimizing intermediate reaction stage,by switching from molecular clusters to mono-octahedra,while interaction with DBSA resulted in formation of a Cs_(x)O monolayer shell capping the NPl *** a result,both structural and optical stability of the CsPbBr3 NPls is enhanced by strong covalent bonding of DBSA,which inhibits undesired phase transitions and decomposition of the perovskite phase potentially caused by ligand ***,rather small amount of DBSA ligands at the NPl surface results in a short inter-NPl spacing in their closely-packed films,which facilitates efficient charge injection and *** photoluminescence of the produced CsPbBr_(3) NPls is bright(nearly unity emission quantum yield)and peaks at 457 nm with an extremely narrow bandwidth of 3.7 nm at 80 K,while the bandwidth of the electroluminescence(peaked at 460 nm)also reaches a record-narrow value of 15 nm at room *** value corresponds to the CIE coordinates of(0.141,0.062),which meets Rec.2020 standards for ultra-high-definition displays.

关键词： temperature stability narrow

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ligand density control boosts the efficiency of all-inorganic CsPbBr3 perovskite nanocrystal based light emitting diodes

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Science Bulletin 2017年第5期62卷 314-315页

作者： Andrey l. rogach Department of Physics and Materials Science Centre for Functional Photonics (CFP) City University of Hong Kong Hong Kong China

lead halide perovskites attracted a lot of attention in the last several years,with a focus gradually shifting from the record power conversion efficiencies reported for photovoltaic devices based on thin perovskite f... 详细信息

关键词： lEDs ligand density control boosts the efficiency of all-inorganic Cs Pb Br3 perovskite nanocrystal based light emitting diodes Cs Pb Br

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Chiral carbon dots:synthesis,optical properties,and emerging applications

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light(Science & Applications) 2022年第4期11卷 542-564页

作者： Aaron Doring Elena Ushakova Andrey l.rogach Department of Materials Science and Engineering and Centre for Functional Photonics(CFP)City University of Hong Kong83 Tat Chee AvenueKowloonHong Kong SARChina. Center of Information Optical Technologies ITMO UniversitySaint Petersburg 197101Russia. Shenzhen Research Institute City University of Hong Kong518057 ShenzhenChina

Carbon dots are luminescent carbonaceous nanoparticles that can be endowed with chiral properties,making them particularly interesting for biomedical applications due to their low cytotoxicity and facile *** recent years,synthetic efforts leading to chiral carbon dots with other attractive optical properties such as two-photon absorption and circularly polarized light emission have *** start this review by introducing examples of molecular chirality and its origins and providing a summary of chiroptical spectroscopy used for its *** approaches used to induce chirality in nanomaterials are *** the main part of this review we focus on chiral carbon dots,introducing their fabrication techniques such as bottom-up and top-down chemical syntheses,their morphology,and optical/chiroptical *** then consider emerging applications of chiral carbon dots in sensing,bioimaging,and catalysis,and conclude this review with a summary and future challenges.

关键词： properties synthesis chiral

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Towards next generation white lEDs:opticselectronics synergistic effect in a single-layer heterophase halide perovskite

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light(Science & Applications) 2021年第3期10卷 310-312页

作者： Andrey l.rogach Departm ent of Materials Science and Engineering and Centre for Functional Photonics(CFP)City University of Hong KongHong Kong SARPR China

A novel concept of the heterophase optics-electronics synergistic effect has been demonstrated in a single-layerα/δ-heterophase perovskite CsPbl3 in order to realize white lEDs featuring only one broadband emissive ... 详细信息

关键词： optics synergistic white

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On the functions of astrocyte-mediated neuronal slow inward currents

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Neural Regeneration Research 2024年第12期19卷 2602-2612页

作者： Balázs Pál Department of Physiology Faculty of MedicineUniversity of DebrecenDebrecenHungary

Slow inward currents are known as neuronal excitatory currents mediated by glutamate release and activation of neuronal extra synaptic N-met hyl-D-aspartate receptors with the contribution of *** events are significantly slower than the excitatory postsynaptic *** of slow inward currents are determined by seve ral factors including the mechanisms of astrocytic activation and glutamate release,as well as the diffusion pathways from the release site towards the extra synaptic recepto *** are stimulated by neuronal network activity,which in turn excite neurons,forming an astrocyte-neuron feedback *** as a consequence of brain edema,astrocytic swelling can also induce slow inward currents under pathological *** is a growing body of evidence on the roles of slow inward currents on a single neuron or local network *** events often occur in synchro ny on neurons located in the same astrocytic *** synchronization of neuronal excitability,slow inward currents also set synaptic strength via eliciting timing-dependent synaptic *** addition,slow inward currents are also subject to non-synaptic plasticity triggered by long-la sting stimulation of the excitatory *** note,there might be important regionspecific differences in the roles and actions triggering slow inward *** greater networks,the pathophysiological roles of slow inward currents can be better understood than physiological *** inward currents are identified in the pathophysiological background of autism,as slow inward currents drive early hypersynchrony of the neural *** inward currents are significant contributors to paroxysmal depolarizational shifts/interictal *** events are related to epilepsy,but also found in Alzheimer's disease,Parkinson's disease,and stroke,leading to the decline of cognitive *** with features overlapping with slow inward currents(excitatory,N-methyl-Dasp

关键词： astrocyte cortical spreading depolarization gliotransmission glutamate neural synchronization NMDA receptor paroxysmal depolarizational shift slow inward current

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On calculating glacial isostatic adjustment

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Geodesy and Geodynamics 2024年第5期15卷 441-452页

作者： l.M.Cathles Cornell University IthacaNY 14853USA

Modeling the earth's fluid and elastic response to the melting of the glaciers of the last ice age is the most direct way to infer the earth's radial viscosity ***,we compare two methods for calculating the viscoelastic response to surface *** one,the elastic equation of motion is converted to a viscoelastic equation using the Correspondence *** the other,elastic deformation is added to the viscous flow as isostatic adjustment *** two modeling methods predict adjustment histories that are different enough to potentially impact the interpretation of the observed glacial isostatic adjustment(GIA).The differences arise from buoyancy and whether fluid displacements are subjected to hydrostatic *** methods agree if they use the same equations and boundary *** origin of the differences is determined by varying the boundary conditions and pre-stress application.

关键词： Glacial isostatic adjustment Viscoelastic normal modes Hydrostatic pre-stress Elastic buoyancy Correspondence principle

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Effect of radiative loss mechanisms on FIR thermometric parameters of Nd^(3+)-doped lithium tellurite glasses

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Journal of Rare Earths 2024年第7期42卷 1250-1257,I0002页

作者： C.Y.Morassuti A.P.l Silva l.A.O.Nunes S.M.lima l.H.C.Andrade Optical and Photothermal Spectroscopy Group(GEOF) Center for Studies in Natural Resources(CERNA)State University of Mato Grosso do Sul(UEMS)C.P.351DouradosMSBrazil Renato Archer Information Technology Center Dom Pedro I Highway(SP-65)Km 1436-Chácaras Campos dos AmaraisCampinasSPBrazil Institute of Physics of São Carlos University of São PauloSão CarlosSPBrazil

Nd^(3+)-doped tellurite glasses are promising materials for thermometers based on the fluorescence intensity ratio(FIR)***,at high Nd^(3+)concentrations,energy transfer(ET)processes such as optical reabsorption and cross-relaxation can affect the Nd^(3+)emission,which has been little explored in the ***,the present work investigated the use of Nd^(3+)-doped tellurite glass(samples doped with Nd^(3+)at 0.2 mol%,0.5 mol%,2.0 mol%,and 4.0 mol%)in fluorescence thermometers,in the temperature range from 299 to 371 *** results indicate a strong dependence of the FIR parameters on the Nd^(3+)concentration,due to changes in the emission band profiles caused by optical reabsorption of the Nd^(3+)emissions and cross-relaxation processes.A decrease of the relative sensitivity of the ratio^(4)F_(5/2)→^(4)I_(9/2)/^(4)F_(3/2)→^(4)I_(9/2)is observed for samples doped with higher amounts of Nd^(3+).The maximum relative sensitivity at 299 K is 3.00%/K,which is the highest value among the reported Nd^(3+)ions.

关键词： Nd^(3+)-doped tellurite glass Fluorescence intensity ratio Optical thermometry Judd-Ofelt Rare earths

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Quantum vortices get stretched

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Frontiers of physics 2024年第3期19卷 225-227页

作者： Emanuel A.l.Henn São Carlos Institute of Physics University of São Paulo-PO Box 36913560-970São CarlosBrazil

Since its discovery, superfluidity [1,2] remains one of the most remarkable phenomena in quantum physics. The onset of the quantum regime in liquid helium is visually striking, when the fluid flows without dissipation or detaches from a rotating bucket, remaining still upon soft rotations. The same phenomenon is present in the context of ultracold bosonic quantum gases where, most of the time, superfluidity walks hand-in-hand with the transition to Bose−Einstein condensation [3].

关键词： quantum rotating rotation

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Time-inconsistent stochastic linear-quadratic control problem with indefinite control weight costs

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Science China Mathematics 2024年第1期67卷 211-236页

作者： Qi lü Bowen Ma School of Mathematics Sichuan UniversityChengdu 610064China

A time-inconsistent linear-quadratic optimal control problem for stochastic differential equations is *** introduce conditions where the control cost weighting matrix is possibly *** such conditions,we obtain a family of closed-loop equilibrium strategies via multi-person differential *** result extends Yong’s work(2017) in the case of stochastic differential equations,where a unique closed-loop equilibrium strategy can be derived under standard conditions(namely,the control cost weighting matrix is uniformly positive definite,and the other weighting coefficients are positive semidefinite).

关键词： linear-quadratic optimal control problem time-inconsistent cost functional generalized Riccati equation indefinite control weight cost closed-loop equilibrium strategy

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