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Generation of brain vascular heterogeneity:recent advances from the perspective of angiogenesis

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Neural Regeneration Research 2025年第7期20卷 2013-2014页

作者： Nathanael j.lee Ryota l.Matsuoka Department of Neurosciences Lerner Research InstituteCleveland ClinicClevelandOHUSA Department of Molecular Medicine Cleveland Clinic Lerner College of MedicineCase Western Reserve UniversityClevelandOHUSA

Heterogeneous proper t i es of vascular endothelial cells in the brain:The brain displays large energy dynamics and consumption,and this high level of metabolic demands is fulfilled by a continuous supply of glucose and oxygen through its vascular *** vasculature consists of highly divergent blood vessel branches,giving rise to a dense network of capillaries that supply blood to all cells across the *** elaborated vascular network is thought to develop via angiogenesis,a process in which new blood vessels grow from pre-existing *** capillaries exhibit organotypic features distinct from other tissues and are formed primarily by two major endothelial cell(EC)types:those that form the semi-permeable blood-brain barrier(BBB)and those that develop highly permeable pores known as fenestrae(Matsuoka et al.,2022).The structural and functional differences between BBB and fenestrated vascular ECs represent a fundamental feature of brain vasculature and form the foundation for both brain function and homeostasis.

关键词： angiogenesis homeostasis network

Tuning the porosity of {Co12IICo8III（μ3-OH）24（X）}11+ supramolecular frameworks by reaction time for D2/H2 separation

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science China Chemistry 2025年

作者： Zhuozhou Xie Zhu Zhuo Zi-Ang Nan Qing li Xiufang li Zi-Xiu lu linzhe lü jin liu luyao liu Wenjing Wang Wei Wang Daqiang Yuan You-Gui Huang state Key laboratory of structure Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences University of Chinese Academy of sciences Xiamen Key laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth Materials Haixi InstitutesChinese Academy of Sciences state Key laboratory of Physical Chemistry of solid surfaces Department of Chemistry College of Chemistry and Chemical EngineeringXiamen University

systematicly tuning the porosities of porous materials is crucial for targeted gas mixture separation,yet it remains a longstanding *** a common strategy,altering the phenylene ring count in the organic building units has been exploited to adjust pore apertures in metal organic frameworks （MOFs） and covalent organic frameworks （COFs）,resulting in only a stepwise pore size variation of approximately 2.8?.Unlike MOFs and COFs,the porosities for supramolecular assembly frameworks are highly dependent on the packings of the molecular building units in the *** above strategy cannot be applied to supramolecular assembly frameworks and other strategies are required to adjust pore apertures in supramolecular frameworks,especially to achieve porous materials with the optimal pore size for D2/H2separation （～3?）.Here,we successfully modulate the porosity of supramolecular frameworks of[CoII1+12CoIII8l12（μ3-OH）24（X）]1clusters （l=mono-deprotonated 1-iminoisoindole-3-amine,X=ClO?4or Cl?） by controlling the duration of self-assembly *** simply adjusting the reaction time,we obtain three[CoII12CoIII8l12（μ3-OH）24（X）]11+supramolecular frameworks:[CoII12CoIII8（μ3-OH）24（ClO4）l12)]·（Cl）4·（HCO2）7（1）,[CoII12CoIII8l12（μ3-OH）24（Cl）]·（ClOI4）4·（Cl）6·（HCO2）·（H2O）10（2）,and[CoI12CoIII8l12（μ3-OH）24（Cl）]·（Cl）11·（H2O）12（3）.The different stacking patterns of the[CoII12CoIII8l12（μ3-OH）24（X）]11+clusters in these frameworks lead to significantly varied stabilities and *** 1 exhibits permanent porosity with interconnected channels and maintains stability under harsh *** contrast,compound 2 is nearly nonporous,and compound 3 becomes unstable upon *** pores of compound 1 show higher affinity to D2than H2,and the pore aperture diameter of compound 1 （～3.06?） meets the optimal porosity for D2/***,compound 1 demonstrates moderate D2/H2separation at 77 K (retention time:～7 min/g for D2/H2/Ne （10/10/80 vol%） in a flow of 5 ml

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Boosting bidirectional sulfur conversion enabled by introducing boron-doped atoms and phosphorus vacancies in Ni2P for lithium-sulfur batteries

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journal of Energy Chemistry 2025年第1期100卷 760-769页

作者： lin Peng Yu Bai Hang li Meixiu Qu Zhenhua Wang Kening sun Advanced Research Institute of Multidisciplinary science Beijing Institute of Technology Beijing Key laboratory of Chemical Power source and Green Catalysis School of Chemistry and Chemical Engineering Beijing Institute of Technology

lithium-sulfur （li-s） batteries have gained great attention due to the high theoretical energy density and low cost,yet their further commercialization has been obstructed by the notorious shuttle effect and sluggish redox ***,we supply a strategy to optimize the electron structure of Ni2P by concurrently introducing B-doped atoms and P vacancies in Ni2P （Vp-B-Ni2P）,thereby enhancing the bidirectional sulfur *** study indicates that the simultaneous introduction of B-doped atoms and P vacancies in Ni2P causes the redistribution of electron around Ni atoms,bringing about the upward shift of d-band center of Ni atoms and effective d-p orbital hybridization between Ni atoms and sulfur species,thus strengthening the chemical anchoring for lithium polysulfides （liPss） as well as expediting the bidirectional conversion kinetics of sulfur ***,theoretical calculations reveal that the incorporation of B-doped atoms and P vacancies in Ni2P selectively promotes li2s dissolution and nucleation ***,the li-s batteries with Vp-B-Ni2P-separators present outstanding rate ability of 777 m A h g-1at 5 C and high areal capacity of 8.03 mA h cm-2under E/s of 5μl mg-1and sulfur loading of 7.20 mg *** work elucidates that introducing heteroatom and vacancy in metal phosphide collaboratively regulates the electron structure to accelerate bidirectional sulfur conversion.

关键词： lithium sulfur batteries

Apples to oranges:environmentally derived,dynamic regulation of serotonin neuron subpopulations in adulthood?

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Neural Regeneration Research 2025年第9期20卷 2596-2597页

作者： Christopher j.O’Connell Matthew j.Robson Department of Genetics College of MedicineHarvard UniversityBostonMAUSA james l.Winkle College of Pharmacy Division of Pharmaceutical SciencesUniversity of CincinnatiCincinnatiOHUSA Neuroscience Graduate Program College of MedicineUniversity of CincinnatiCincinnatiOHUSA

Traumatic brain injury(TBI)is a public health problem with an undue economic burden that impacts nearly every age,ethnic,and gender group across the globe(Capizzi et al.,2020).TBIs are often sustained during a dynamic range of exposures to energetic environmental forces and as such outcomes are typically heterogeneous regarding severity and pathology(Capizzi et al.,2020).

关键词： sustained orange dynamic

Pulsed dynamic electrolysis enhanced PEMWE hydrogen production:Revealing the effects of pulsed electric fields on protons mass transport and hydrogen bubble escape

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journal of Energy Chemistry 2025年第1期100卷 201-214页

作者： Xuewei Zhang Wei Zhou Yuming Huang liang Xie Tonghui li Huimin Kang lijie Wang Yang Yu Yani Ding junfeng li jiaxiang Chen Miaoting sun shuo Cheng Xiaoxiao Meng jihui Gao Guangbo Zhao school of Energy science and Engineering Harbin Institute of Technology China Datang Technology Innovation Co. Ltd

The transition of hydrogen sourcing from carbon-intensive to water-based methodologies is underway,with renewable energy-powered proton exchange membrane water electrolysis （PEMWE） emerging as the preeminent pathway for hydrogen *** remarkable advancements in this field,confronting the sluggish electrochemical kinetics and inherent high-energy consumption arising from deteriorated mass transport within PEMWE systems remains a formidable *** impediment stems primarily from the hindered protons mass transfer and the untimely hydrogen bubbles *** address these challenges,we harness the inherent variability of electrical energy and introduce an innovative pulsed dynamic water electrolysis *** to constant voltage electrolysis (hydrogen production rate:51.6 m l h-1,energy consumption:5.37 kWh Nm-3H2),this strategy (hydrogen production rate:66 m l h-1,energy consumption:3.83 kWh Nm-3H2) increases the hydrogen production rate by approximately 27%and reduces the energy consumption by about 28%.Furthermore,we demonstrate the practicality of this system by integrating it with an off-grid photovoltaic （PV） system designed for outdoor operation,successfully driving a hydrogen production current of up to 500 mA under an average voltage of approximately 2 *** combined results of in-situ characterization and finite element analysis reveal the performance enhancement mechanism:pulsed dynamic electrolysis （PDE） dramatically accelerates the enrichment of protons at the electrode/solution interface and facilitates the release of bubbles on the electrode *** such,PDE-enhanced PEMWE represents a synergistic advancement,concurrently enhancing both the hydrogen generation reaction and associated transport *** promising technology not only redefines the landscape of electrolysis-based hydrogen production but also holds immense potential for broadening its application across a diverse spectrum of electrocatalytic endeavors.

关键词： Electrolysis

Effect of solidification Condition and Carbon Content on the Morphology of MC Carbide in Directionally solidified Nickel-base superalloys

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journal of Materials science & Technology 2014年第12期30卷 1296-1300页

作者： X.W.li l.Wang j.s.Dong l.H.lou superalloys Division Institute of Metal Research Chinese Academy of Sciences

Evolution of the morphology of MC carbides with the change of cooling rate and carbon content in two kinds of nickel-base superalloys, K417 G and DD33, has been investigated. The morphology of MC carbides evolves from faceted to script-like with increasing cooling rate. Varying the carbon content from 40X10-6 to 320X10-6, the morphology of carbides changes from blocky, rod-like into script-like. scanning electron microscopy observation of deep-etched samples indicates that these carbides evolve from octahedral to dendritic and then into welldeveloped dendrites accordingly in a three-dimensional manner. The morphology evolution is discussed from the viewpoint of the preferential growth orientation of fcc crystals and the carbide growth rate during directional solidification.

关键词： Carbides morphology Directional solidification Three-dimensional microstructure Nickel-base superalloys

Improved mechanical properties in titanium matrix composites reinforced with quasi-continuously networked graphene nanosheets and in-situ formed carbides

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journal of Materials science & Technology 2022年第1期96卷 85-93页

作者： Q.Yan B.Chen l.Cao K.Y.liu s.li l.jia K.Kondoh j.s.li state Key laboratory of solidification Processing Northwestern Polytechnical UniversityXi’an 710072China school of Materials science and Engineering Xi’an University of TechnologyXi’an 710048China joining and Welding Research Institution Osaka University11-1 MihogaokaIbarakiOsaka 567-0047Japan

In order to construct quasi-continuously networked reinforcement in titanium(Ti)matrix composites,in this study,Ti-6 Al-4 V spherical powders were uniformly coated with a graphene nanosheet(GNs)layer by high energy ball milling and then consolidated by spark plasma *** showed that the GNs layer on the powder surface inhibited continuous metallurgy bonding between powders during sintering,which led to the formation of quasi-networked hybrid reinforcement structure consisting of insitu Ti C and remained *** networked GNss/Ti64 composite possessed noticeably higher tensile strength but similar ductility to the Ti64 alloy,leading to both better tensile strength and ductility than the GNss/Ti composite with randomly dispersed GNss and Ti *** formation mechanism and the fracture mechanism of the networked hybrid reinforcement were *** results provided a method to fabricate Ti matrix composites with high strength and good ductility.

关键词： Titanium matrix composites(TMCs) Graphene Network structure strength Ductility

Formation process and oxidation behavior of MCrAlY+AlsiY composite coatings on a Ni-based superalloy

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journal of Materials science & Technology 2022年第25期120卷 65-77页

作者： s.M.li l.B.Fu W.l.Zhang W.li j.sun T.G.Wang s.M.jiang j.Gong C.sun school of Materials science and Engineering University of Science and Technology of ChinaShenyang 110016China shi-changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Advanced Research Institute for Multidisciplinary science Qilu University of Technology(Shandong Academy of Sciences)Jinan 250353China Tianjin Key laboratory of High speed Cutting and Precision Machining Tianjin University of Technology and EducationTianjin 300222China

An AlsiY coating and two MCrAlY+AlsiY composite coatings with different thickness of MCrAlY interlayer were prepared by arc ion plating(AIP)and vacuum *** isothermal oxidation behavior of coatings at 1100℃ for 300 h was also investigated to characterize the microstructure evolution of coatings during *** composite coatings exhibited a better high-temperature oxidation resistance at 1100℃ .The reason is that the addition of MCrAlY layer can greatly contribute to prevent the diffusion of refractory elements to the outer *** inhibition of Al inward diffusion can be much stronger,as the si content increases in the outer layer during annealing.

关键词： Composite coating Annealing Arc ion plating sEM Oxidation

Compression stability of Reversed Austenite in 9Ni steel

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journal of Materials science & Technology 2012年第6期28卷 558-561页

作者： s.H.Chen M.j.Zhao X.Y.li l.j.Rong Institute of Metal Research Chinese Academy of SciencesShenyang 110016China

The effect of compressive stress on the stability of reversed austenite in gNi steel was investigated by uni- axial and hydrostatic compression. It was found that the uniaxial compressive pressure promoted the Υ-α transformation, while the hydrostatic pressure suppressed the -Υ-α transformation. The pressure dependent transformation behavior can be explained according to thermodynamic analysis.

关键词： 9Ni steel Martensite Reversed austenite Hydrostatic pressure Uniaxial compressive pressure