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Structural disruption of melanin-like polymers with boosted UV protection

Science China Chemistry 2024年第5期67卷 1653-1663页

作者： zhen Yang Xianheng Wang Wanjie Bai Zikun Zou Haoxing Wu Yiwen Li department of Radiology Huaxi MR Research CenterFunctional and Molecular Imaging Key Laboratory of Sichuan ProvinceNational Clinical Research Center for GeriatricsWest China HospitalSichuan UniversityChengdu 610041China College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu 610065China

Manipulating the energy structure of materials represents an efficient way to regulate their light absorption behaviors. For example, constructing donor-acceptor(d-A) structures to increase the polarizability and reduce the energy bandgap of local molecules has been widely used in the field of organic photovoltaics with ordered structures. Remarkably, even in disordered and chaotic systems such as melanin-like polydopamine(PdA), visible and near-infrared light absorption can be significantly improved using this strategy. However, there has been a noticeable dearth of research on the ultraviolet(UV) light absorption regulation of bioinspired polymers with disordered and chaotic architectures by tailoring the d-A microstructures. In this study, a series of benzoheterocyclic molecules with strong electron-donating features screened by molecular simulation calculations were involved in disrupting the d-A structures within PdA. The destruction of d-A structures promoted the increase of the energy band gap and finally boosted the UV absorption of PdA. The resulting PdA nanoparticles with enhanced UV absorption were further employed to fabricate UV shielding composite films to protect the growth of plants from harmful UV radiation. This research may open up new avenues for structural disruption of bioinspired polymers for enhanced photoprotection applications.

关键词： melanin-like polymers polydopamine d-A structure UV absorption photoprotection

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Set Stabilization of Large-Scale Stochastic Boolean Networks:A distributed Control Strategy

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IEEE/CAA Journal of Automatica Sinica 2024年第3期11卷 806-808页

作者： Lin Lin Jinde cao Jianquan Lu Leszek Rutkowski the department of Mechanical Engineering the University of Hong KongHong Kong China the School of Mathematics Southeast UniversityNanjing 210096China IEEE the School of Mathematics and the Frontiers Science Center for Mobile Information Communication and Security Southeast UniversityNanjing 210096China the School of Mathematics the Southeast UniversityNanjing 210096 the School of Electronic Information and Electrical Engineering Chengdu UniversityChengdu 610106China the Systems Research Institute of the Polish Academy of Sciences Warsaw 01-447 the Institute of Computer Science AGH University of Science and TechnologyKraków 30-059 the Information Technology Institute University of Social SciencesŁódź90-113Poland

dear Editor,This letter deals with the set stabilization of stochastic Boolean control networks(SBCNs)by the pinning control strategy,which is to realize the full control for systems by imposing control inputs on a fr... 详细信息

关键词： Boolean stabilization letter

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Physics-constrained graph modeling for building thermal dynamics

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Energy and AI 2024年第2期16卷 150-157页

作者： Ziyao Yang Amol d.Gaidhane Ján drgoňa Vikas Chandan Mahantesh M.Halappanavar Frank Liu Yu cao School of Electrical Computer and Energy EngineeringArizona State UniversityTempeAZ 85287USA Pacific Northwest National Laboratory RichlandWA 99354USA Oak Ridge National Laboratory Oak RidgeTN 37830USA

In this paper,we propose a graph model embedded with compact physical equations for modeling the thermal dynamics of *** principles of heat flow across various components in the building,such as walls and doors,fit the message-passing strategy used by Graph Neural networks(GNNs).The proposed method is to represent the multi-zone building as a graph,in which only zones are considered as nodes,and any heat flow between zones is modeled as an edge based on prior knowledge of the building ***,the thermal dynamics of these components are described by compact models in the *** are further employed to train model parameters from collected *** model training,our proposed method enforces physical constraints(e.g.,zone sizes and connections)on model parameters and propagates the penalty in the loss function of *** constraints are essential to ensure model robustness and *** evaluate the effectiveness of the proposed modeling approach on a realistic dataset with multiple *** results demonstrate a satisfactory accuracy in the prediction of multi-zone ***,we illustrate that the new model can reliably learn hidden physical parameters with incomplete data.

关键词： Physics-constrained learning Graph Neural Networks Compact model Building thermal dynamics

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Numerical investigation of dynamic characteristics of dual throat nozzle and bypass dual throat nozzle in thrust vectoring starting process

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Chinese Journal of Aeronautics 2024年第10期37卷 184-206页

作者： Yuqi ZHANG Jinglei XU Minglei cao Ruifeng PAN Shuai HUANG Key Laboratory of Inlet and Exhaust System Technology of Ministry of Education Nanjing University of Aeronautics and AstronauticsNanjing 210016China College of Energy and Power Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China State Key Laboratory of Mechanics and Control of Aeronautics and Astronautics Structures Nanjing 210016China

The Bypass dual Throat Nozzle(BdTN)is a novel fluidic Thrust Vectoring(TV)nozzle,it switches to TV state by opening the valve in the *** greatly manipulate the BdTN,the dynamic characteristics in the TV starting process should be *** paper conducts numerical simulations to grasp the variation processes of performances and the flow field evolution of BdTN and dual Throat Nozzle(dTN).The dynamic responses of TV starting in typical dTN models are investigated at ***,the TV starting processes of BdTN in different Nozzle Pressure Ratio(NPR)conditions are simulated,and the valve opening durations(T)are also *** the expected TV direction is achieved in the dTN,the jet is deflected to the opposite direction at the beginning of the dynamic process,which is called the reverse TV ***,this phenomenon disappears in the *** larger injection width of dTN intensifies unsteady oscillations,and the reverse TV phenomenon is *** the BdTN,T determines the delay degree of performance variations compared to the static results,which is called hysteresis *** NPR=10,the hysteresis affects the final stable performance of *** study analyses the dynamic characteristics in dTN and BdTN,laying a foundation for further design of nozzles and control strategies.

关键词： dual Throat Nozzle(dTN) Bypass dual Throat Nozzle(BdTN) dynamic characteristic Thrust vectoring starting process Cavity vortex Hysteresis effect

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Mechanism investigation of A-site doping on modulating electronic band structure and photocatalytic performance towards CO_(2) reduction of LaFeO_(3) perovskite

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Nano Research 2024年第5期17卷 3733-3744页

作者： Chi cao Jinshuo Li Yang Hu Lin Zhang Wensheng Yang State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012China Engineering Research Center for Nanomaterials Henan UniversityKaifeng 475004China

Three kinds of metal atoms with different valence electronic configurations,Bi(6s^(2)6p^(3)),Y(4d^(1)5s^(2)),and Ce(4f^(1)5d^(1)6s^(2)),were selected to investigate the effect of A-site(La^(3+))doping on electronic band structure,photoelectric properties,and photocatalytic performance of LaFeO_(3) *** was identified that the Bi doped LaFeO_(3) presented significantly improved photocatalytic activity towards the reduction of CO_(2),while the Y or Ce doped LaFeO_(3) displayed decreased photocatalytic activity compared to the pristine LaFeO_(3).It was revealed that doping of all the three metal atoms resulted in narrowed band gap and thus extended light absorption of LaFeO_(3) by lowering its conduction band minimum(CBM).The recombination rate and mobility of the charge carriers were represented by the relative effective mass(d)between holes and electrons for pristine and A-site doped LaFeO_(3).The doping of Bi resulted in increased d value,attributed to the Bi 6s electron states at the valence band maximum(VBM),and thus promoted separation and transfer of the charge carriers and improved photocatalytic activity of LaFeO_(3).In contrast,the doping of Ce resulted in significantly decreased d value,induced by the highly localized Ce 4f hole states at the CBM,and thus higher recombination rate of the charge carriers and decreased photocatalytic activity of LaFeO_(3).Furthermore,the Y doped LaFeO_(3) with a slightly decreased d value presented slightly increased recombination rate of the charge carriers and thus decreased photocatalytic *** a work provides new insights into the A-site doping in LaFeO_(3) perovskite,which should be helpful for optimizing the electronic band structure and activity of perovskite-type photocatalysts at atomic level.

关键词： A-site doping electronic band structure charge carrier behavior photocatalytic CO_(2)reduction perovskite-type photocatalytsts

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Effects of Heat Transfer on Laminar-to-Turbulent Transition over a Compressor Blade Operating at Low Reynolds Number

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Journal of Thermal Science 2024年第5期33卷 1826-1838页

作者： LU Lehan WANG Mingyang ZHANG Yanfeng SUN Shuang HUANG zhen WANG Maomao department of aviation Engineering Civil Aviation University of ChinaTianjin 300300China Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China State Key Laboratory of Aerodynamics CARDCMianyang 621000China

To control the transition process in a laminar separation bubble(LSB)over an ultra-high load compressor blade at a Re of 1.5×10^(5),the effects of wall heat transfer were considered and numerically investigated by large eddy simulations(LES).Compared with the adiabatic wall condition,the local kinematic viscosity of airflow was reduced by wall cooling;thus the effects of turbulent dissipation on the growth of fluctuations were *** such,the transition occurred much earlier,and the size of LSB became *** the cooled surface,the spanwise vortices deformed much more rapidly and the size of hairpin vortex structures was ***,the rolling-up of 3d hairpin vortices and the ejection and sweeping process very close to the blade surface was ***,the aerodynamic losses of the compressor blade were reduced by 18.2%and 38.4%for the two cooled wall *** results demonstrated the feasibility of wall cooling in controlling the transition within an LSB and reducing the aerodynamic loss of an ultra-highly loaded compressor blade.

关键词： heat transfer compressor blade laminar-to-turbulent transition loss generation

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Sustainable production of high-energy-density jet fuel via cycloaddition reactions

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Journal of Energy Chemistry 2024年第8期95卷 712-722,I0016页

作者： Yan-Cheng Hu Yingying Zhao Ning Li Jing-Pei cao School of Chemical Engineering and Technology China University of Mining and TechnologyXuzhou 221116JiangsuChina School of Education Science Jiangsu Normal UniversityXuzhou 221116JiangsuChina CAS Key Laboratory of Science and Technology on Applied Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023LiaoningChina

developing an energy supply-chain based on renewable biomass holds great potential to build a low carbon ***-energy-density(HEd)jet fuel,featuring unique fused/strained cycloalkanes,is of great significance for volume-limited military aircrafts,as their high density and combustion heat can extend flight duration and increase the ***,the exploration of biomass-based routes towards HEd fuel has drawn much attention over the past *** reaction features rapid construction of various carbocycles in an atom-and step-economical *** elegant strategy has been widely applied in the manufacture of sustainable HEd *** we carefully summarize the progress achieved in this fascinating area and the review is categorized by the cycloaddition patterns including[4+2],[2+2],[4+4],and[2+1]***,the energy densities of the as-prepared biofuels and petroleumbased fuels(conventional Jet-A and advanced JP-10)are also *** review will provide important insights into rational design of new HEd fuel with different ring-types/sizes and inspire the chemists to turn those literature studies into practical applications in military field.

关键词： High-energy-density fuel Biomass-based chemicals Cycloaddition Cycloalkanes Catalysis

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Cascading multi-segment rupture process of the 2023 Turkish earthquake doublet on a complex fault system revealed by teleseismic P wave back projection method

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Earthquake Science 2024年第2期37卷 158-173页

作者： Bonan cao Zengxi Ge department of Geophysics School of Earth and Space SciencesPeking UniversityBeijing 100871China Hebei Hongshan National Geophysical Observatory for Thick Sediments and Seismic Hazards Peking UniversityBeijing 100871China

In this study,the vertical components of broadband teleseismic P wave data recorded by China Earthquake Network are used to image the rupture processes of the February 6th,2023 Turkish earthquake doublet via back projection *** in two frequency bands(0.5-2 Hz and 1-3 Hz)are used in the imaging *** results show that the rupture of the first event extends about 200 km to the northeast and about 150 km to the southwest,lasting~90 s in *** southwestern rupture is triggered by the northeastern rupture,demonstrating a sequential bidirectional unilateral rupture *** rupture of the second event extends approximately 80 km in both northeast and west directions,lasting~35 s in total and demonstrates a typical bilateral rupture *** cascading ruptures on both sides also reflect the occurrence of selective rupture behaviors on bifurcated *** addition,we observe super-shear ruptures on certain fault sections with relatively straight fault structures and sparse aftershocks.

关键词： 2023 Turkish earthquake doublet back projection method cascading segmented rupture process coseismic triggering super-shear ruptures

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Mucosal immune responses to Ichthyophthirius multifiliis in the ocular mucosa of rainbow trout(Oncorhynchus mykiss,Walbaum),an ancient teleost fish

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Marine Life Science & Technology 2024年第2期6卷 266-279页

作者： Weiguang Kong Guangyi ding Gaofeng Cheng Peng Yang zhen Xu Key Laboratory of Breeding Biotechnology and Sustainable Aquaculture Institute of HydrobiologyChinese Academy of SciencesWuhan 430072China department of Aquatic Animal Medicine College of FisheriesHuazhong Agricultural UniversityWuhan 430070China

The eye,as a specialized visual organ,is directly exposed to the external environment,and,therefore,it faces constant chal-lenges from external pathogenic organisms and *** the ocular mucosa(OM)of mammals,mucosal-associated lymphoid tissues(MALTs)constitute the primary line of ***,the immune defense role of the OM remains unknown in aquatic *** gain insights into the immune processes within the OM of teleost fish,we developed an infection model of rainbow trout(Oncorhynchus mykiss)OM using a parasite,Ichthyophthirius multifiliis(Ich).Immunofluorescence,qPCR,and H&E staining revealed that Ich successfully infiltrates the OM of rainbow trout,leading to pathological struc-tural changes,as evidenced by A&B ***,the qPCR results indicate an up-regulation of immune-related genes following Ich infection in the ***,transcriptome analyses were conducted to detect immune responses and impairments in eye function within the OM of rainbow trout with Ich *** results of the transcriptome analysis that Ich infection can cause an extensive immune response in the OM,ultimately affecting ocular *** the best of our knowledge,our findings represent for the first time that the teleost OM could act as an invasion site for parasites and trigger a strong mucosal immune response to parasitic infection.

关键词： Ocular mucosa Mucosal immunity Transcriptome analysis Oncorhynchus mykiss Ichthyophthirius multifiliis

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Research on Performance Optimization of Spark distributed Computing Platform

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Computers, Materials & Continua 2024年第5期79卷 2833-2850页

作者： Qinlu He Fan Zhang Genqing Bian Weiqi Zhang zhen Li School of Information and Control Engineering Xi’an University of Architecture and TechnologyXi’an710054China Shaanxi Institute of Metrology Science Xi’an710043China

Spark,a distributed computing platform,has rapidly developed in the field of big *** in-memory computing feature reduces disk read overhead and shortens data processing time,making it have broad application prospects in large-scale computing applications such as machine learning and image ***,the performance of the Spark platform still needs to be *** a large number of tasks are processed simultaneously,Spark’s cache replacementmechanismcannot identify high-value data partitions,resulting inmemory resources not being fully utilized and affecting the performance of the Spark *** address the problem that Spark’s default cache replacement algorithm cannot accurately evaluate high-value data partitions,firstly the weight influence factors of data partitions are modeled and ***,based on this weighted model,a cache replacement algorithm based on dynamic weighted data value is proposed,which takes into account hit rate and data *** integration and usage strategies are implemented based on LRU(LeastRecentlyUsed).Theweight update algorithm updates the weight value when the data partition information changes,accurately measuring the importance of the partition in the current job;the cache removal algorithm clears partitions without useful values in the cache to releasememory resources;the weight replacement algorithm combines partition weights and partition information to replace Rdd partitions when memory remaining space is ***,by setting up a Spark cluster environment,the algorithm proposed in this paper is experimentally *** have shown that this algorithmcan effectively improve cache hit rate,enhance the performance of the platform,and reduce job execution time by 7.61%compared to existing improved algorithms.

关键词： Spark memory optimization memory replacement strategy

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