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化工学报 2003年第Z1期54卷 62-66页

作者： GUO Guangjun,ZHANG Yigang and ZHAO Yajuan institute of geology and geophysics,chinese academy of {5. beijing 100029,chinese institute of geology and geophysics Chinese Academy of Sciences Beijing 100029 China

Molecular dynamics simulations are performed to observe the evolutions of 5.2 and 5.262 cage-like water clusters filled with or without a methane molecule immersed in bulk liquid water at 25. K and 230 K. The lifetimes of these clusters are calculated according to their Lindemann index δ (t) using the criteria of δ≥0.07. For both the filled and empty clusters, we find the dynamics of bulk water determines the lifetimes of cage-like water clusters, and that the lifetime of 5.2 62 cage-like cluster is the same as that of 5.2 cage-like cluster. Although the methane molecule indeed makes the filled cage-like cluster more stable than the empty one, the empty cage-like cluster still has chance to be long-lived compared with the filled clusters. These observations support the labile cluster hypothesis on the formation mechanisms of gas hydrates.

关键词： like in time that were MOLECULAR DYNAMICS SIMULATIONS OF FILLED AND EMPTY CAGE-LIKE WATER CLUSTERS IN LIQUID WATER AND THEIR SIGNIFICANCE TO GAS HYDRATE FORMATION MECHANISMS of cage GAS

The deep thermal characteristic of continental margin of the northern South china Sea

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chinese Science Bulletin 2000年第18期45卷 1717-1722页

作者： ZHANG Jian & WANG Jiyang1. Graduate School, University of Science and Technology of china, chinese academy of sciences, beijing 100039, china 2. institute of {5., chinese academy of sciences, beijing 100029, china Graduate School University of Science and Technology of China Chinese Academy of Sciences Beijing China institute of geology Chinese Academy of Sciences Beijing China

Heat flow plays an important role in the study ot thermal structure and thermal evolutionof continental margin of the northern South china Sea. The analysis of heat flow value shows that margin heat flow in the northern South china Sea is relatively high setting, but the percentage of crustal heat flow is lower than 35. in terrestrial heat flow. The terrestrial heat flow exhibited a current of rise from the Northern Continental Margin to the Southern Central Basin. However, the proportion of crustal heat flow in terrestrial heat flow slowly dropped down in the same direction. It is suggested that the main factor causing high heat flow setting is the moving up of hot material from asthenosphere.

关键词： margin of northern South china Sea terrestrial heat flow thermal structures.

DMTB:A comprehensive online resource of 16S rRNA genes,ecological metadata,oligonucleotides,and magnetic properties of magnetotactic bacteria

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chinese Science Bulletin 2011年第6期56卷 476-478页

作者： LIN Wei1,2, LI Bi1,2 & PAN YongXin1,2 1 Paleomagnetism and Geochronology Laboratory, Key Laboratory of the Earth’s Deep Interior, institute of geology and geophysics, chinese academy of sciences, beijing 100029,{5. 2 France-china Bio-Mineralization and Nano-Structures Laboratory, institute of geology and geophysics, chinese academy of sciences, beijing 100029,{5. Paleomagnetism and Geochronology Laboratory Key Laboratory of the Earth’s Deep Interior Institute of Geology and Geophysics Chinese Academy of Sciences Beijing China France-china Bio-Mineralization and Nano-Structures Laboratory Institute of Geology and Geophysics Chinese Academy of Sciences Beijing China

Magnetotactic bacteria (MTB) are of interest in microbiology, biomineralization, advanced magnetic materials, and bio-geo-sciences because of their ability to form highly ordered intracellular magnetic minerals. Great strides for MTB studies have been made in the past four decades. In this paper we complied the first internet-accessible database for MTB, Database of Magnestotactic Bacteria (DMTB). It contains information of 16S rRNA gene sequences, corresponding ecological metadata, oligonucleotides, and magnetic properties of MTB. The comprehensive information contained in DMTB will provide a very useful data resource for researchers from different disciplines. The website of DMTB is at http://***/.

关键词： rRNA基因序列趋磁细菌 16S 网上资源寡核苷酸磁学性质生态磁性材料

Research progress in studies on the coalbed gas geochemistry

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Progress in Natural Science:Materials International 2006年第3期16卷 215-220页

作者： TAO Mingxin (College of Resources sciences & Technology, beijing Normal University, beijing 100875. china Key Laboratory of Gas Geochemistry, institute of {5. and geophysics, chinese academy of sciences, Lanzhou 730000, china) College of Resources sciences and Technology Beijing Normal University Beijing 100875 China Key Laboratory of Gas Geochemistry Institute of Geology and Geophysics Chinese Academy of Sciences Lanzhou 730000 China

The current situation of geochemical studies on coalbed gas is reviewed in this paper. Generally, coalbed gas is composi-tionally dominated by methane with δ13C1 values ranging approximately from - 80‰ to - 10‰. However, few isotopic studies have been carried out on other components of coalbed gas except for hydrogen and carbon dioxide, whose δDCH4 values available for utilization vary from - 333‰ to - 117‰, and δ13CCO2 values from - 29. 4‰ to + 18. 6‰. Two major types of coalbed gas, thermogenic gas and secondary biogenic gas, have been identified, and there are also some other classification criteria. Compared with conventional natural gases, coalbed gas has a wide distribution range of δ13C1 and δ13CCO2 values, especially possessing some extremely heavy values. Current problems that remain unsolved in the coalbed gas geochemistry include the variation mechanism, controlling factors and application of carbon and hydrogen isotopes of methane, the relation between the values of δ13C1 and Ro, the systematic classification scheme and criterion of genetic types, and the application of the coalbed gas geochemistry in evaluating target districts of the coalbed gas exploration.

关键词： coalbed gas geochemistry isotopic composition genetic type novel resource.

General regularity of dynamic responses of slopes under dynamic input

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Science china(Technological sciences) 2003年第Z1期46卷 120-132页

作者： QI Shengwen, WU Faquan & SUN Jinzhong institute of geology and geophysics, chinese academy of sciences, beijing 100029,{5. College of Engineering Technique,{5. University of Geosciences, beijing 100083,{5. chinese Acad Sci Inst Geol & Geophys Beijing 100029 Peoples R China china Univ Geosci Coll Engn Techn Beijing 100083 Peoples R China

Through lots of numerical simulations with FLAC3D, dynamic responses of slopes are comprehensively studied in this paper and the general regularities of the isoline of the coefficient of the displacement, velocity and acceleration of the slope section are reached. Given a certain material slope, if the height of the slope is less than a certain value, the displacement, velocity and acceleration linearly enlarge with elevation in the vertical direction; if the height of the slope surpasses the certain value, the displacement,velocity and acceleration do not linearly enlarge with elevation any more, on the other hand, they fluctuate with a certain rhythm. At the same time, the rhythm appears in the horizontal direction, and the displacement, velocity and acceleration of the slope surface enlarge near the slope surface. The distribution form of the isoline of the coefficient of displacement, velocity and acceleration in the section of the slope is remarkably affected by the slope angle. In the certain area near the slope surface, the isoline of displacement,velocity and acceleration is parallel to the surface of the slope; in the mean time the strike direction of the extremum area is parallel to the surface of the slope, too. The charts of the slope dynamic responses can be depicted with two indexes, one is the strike direction of the isoline, and the other is the number of the rhythm extremum area of the direction parallel to the surface of the slope.

关键词： slope, dynamic response, regularity, rhythm.

Geochemical research on C-O and Sr-Nd isotopes of mantle-derived rocks from Shandong Province, china

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Science china Earth sciences 2004年第2期47卷 171-180页

作者： LIU Jianming, ZHANG Hongfu, SUN Jinggui & YE Jie1. institute of geology and geophysics, chinese academy of sciences, beijing 100029,{5. 2. School of Earth Science, Jilin University, Changchun 130061,{5. Correspondence should be addressed to Liu Jianming (email: jmliu@***) institute of geology and geophysics Chinese Academy of Sciences Beijing China School of Earth Science Jilin University Changchun China

This paper presents systematic studies on the C-O and Sr-Nd isotopic compositions for Cretaceous Badou carbonatites, Fangcheng basalts, and Jiaodong lamprophyres and Paleozoic Mengyin kimberlites in Shandong Province, china. Paleozoic kimberlites have normal and uniform C-O isotopic compositions with δ13C and δ18O in the range of -4.8‰--7.6‰ and +9.9‰-+13.2‰, respectively. However, Cretaceous three different types of mantle-derived rocks have quite different C-O isotopic compositions, indicating that the mantle sources are probably partially contaminated with organic carbon-bearing crustal materials. These Cretaceous rocks show uniform and EMII-like Sr-Nd isotopic compositions and also indicate that the mantle sources were affected by recycled crustal materials. Comparative studies of C-O and Sr-Nd isotopes reveal that the lithospheric mantle beneath the eastern North china Craton had different isotope characteristics in the Paleozoic, the early Cretaceous, and the Tertiary time. This demonstrates that the lithospheric mantle beneath the region underwent at least twice reconstructions since the Paleozoic. Available data imply that the first reconstruction mainly happened during the Triassic-Jurassic time with gradual changes and the second in the Cretaceous with abrupt changes. Results also show that the early Cretaceous (especially at 120-130 Ma) was perhaps the key period leading to the dramatic change of the Mesozoic geodynamics on the eastern North china Craton.

关键词： mantle-derived rocks, carbonate minerals, C-O isotope, Sr-Nd isotope, lithospheric mantle, Shandong.

Garnet Sm-Nd and U-Pb systems: A case study of a granulite from the European Variscan belt

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chinese Science Bulletin 2002年第15期47卷 1284-1288页

作者： CHEN FukunInstitut fur Mineralogie, Petrologie und Geochemie, Universitat Tubingen, 72074 Tubingen, Germany institute of geology and geophysics, chinese academy of sciences, beijing 100029,{5. Institut für Mineralogie Petrologie und Geochemie Universität Tübingen Tübingen Germany institute of geology and geophysics Chinese Academy of Sciences Beijing China

This study presents zircon and garnet ages of a mafic granulite from the high-grade Variscan basement of the Black Forest, Germany and discuss isotope closure temperature of garnet Sm-Nd and U-Pb systems. Zircon grains yield 207Pb/206Pb ages between -340 and -414 Ma by the U-Pb and evaporation methods. In contract, garnet dating gives Sm-Nd and Pb-Pb isochron ages of (398±3) Ma and (411±14) Ma, respectively, which are older than most of zircon ages. These data imply that most of zircons lost radiogenic Pb, probably due to metamictization or recrystallisa-tion during the granulite-facies metamorphism (-800°C) at -340 Ma. Garnet Sm-Nd and U-Pb systems preserve chronological information of pro-grade metamorphism, probably profiting from a fluid-absence metamorphic environment. These results demonstrate that garnet mineral can be a better candidate than zircon mineral to date high-grade metamorphism by the U-Pb and Sm-Nd methods in some cases.

关键词： Variscan granulite garnet Sm-Nd U-Pb.

δ^13Csc values of the loess-paleosol sequence in Dali area, Shaanxi Province, china, and paleoenvironmental implications

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chinese Science Bulletin 2003年第9期48卷 902-907页

作者： LI Yumei & LIU Dongsheng (LIU Tungsheng)institute of geology and geophysics, chinese academy of sciences, beijing 100029 (e-mail: liyrney@***) institute of geology and geophysics Chinese Academy of Sciences Beijing 100029 China

The carbon isotopic ratios of carbonate in the two profiles of the Dali area were analyzed and some new understandings on the influencing factors of the δ13CSC value of the loess-paleosol sequence and its paleoenvironmental implications were discussed preliminarily in this report. The 13CSC value of the Dali loess-paleosol sequence is synchronizing with the variance of magnetic susceptibility basically and the negative peaks of the δ13CSC curves are corresponding to the different developmental periods of the paleosol. It is believed that the intervention of the CO2 produced by plants will cause the decrease of the δ13CSC value, the amplitude of which may be relevant to the paleovegetation density and the ancient humidity. The relative biomass of C4 plants in the vegetation will affect the sublevel change of the δ13CSC. Low δ13CSC value by and large indicates the environmental conditions of the relatively abundant vegetation and humid climate. During the last 25.000 years, the period with the sparsest vegetation and the most arid climate is the phase of the loess in L2 depositing and the period with the most abundant vegetation and the most humid climate is the last interglacial period. The δ13CSC curves of Dali also show that the High Temperature and Large Precipitation Event of the Qinghai-Tibetan Plateau during 40-30 kaBP had affected the Central Shaanxi Plain with relatively humid climate, and had apparent influence on the local vegetation and humidity.

关键词：古环境大理地区黄土陕西湿润气候碳同位素植被高温天气

Neogene eolian deposits within the West Qinling Mountains:Climatic and tectonic implications

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chinese Science Bulletin 2010年第15期55卷 1483-1487页

作者： GE JunYi 1,2 & GUO ZhengTang 3 1 State Key Laboratory of Loess and Quaternary geology (SKLLQG),institute of Earth Environment,chinese academy of sciences,Xi’an 710075.{5. 2 Graduate University of chinese academy of sciences,beijing 100049,{5. 3 Key Laboratory of Cenozoic geology and Environment,institute of geology and geophysics,chinese academy of sciences,beijing 100029,{5. State Key Laboratory of Loess and Quaternary geology (SKLLQG) Institute of Earth Environment Chinese Academy of Sciences Xi’an China Graduate University of chinese academy of sciences Beijing China Key Laboratory of Cenozoic geology and Environment Institute of Geology and Geophysics Chinese Academy of Sciences Beijing China

The Qinling Mountains constitute a key climate barrier between southern and northern *** recent investigations revealed widely spread eolian deposits of Neogene age mantling the piedmont highlands of the intermountain basins within West ***-mammalian fossils dated a 15..2 m section (NL-VI) near Xihe for the late Miocene to Pliocene (～10-4 Ma).Soil micromorphology,grain-size and geochemical analysis consistently define typical loess-soil alternations for the upper (0-66 m) and lower (98-15..2 m) parts of the section,with the middle section (66-98 m) having been affected by episodic slope *** results add important insights to the earlier studies about the widespread eolian deposition in northern china during the Miocene,prior to 8 *** also suggest that the basic configuration of the ridges and inter-ridge basins of West Qinling has already formed by ～10 *** well-preserved eolian deposits are unlikely to support intense substratum deformation and rapid uplift of West Qinling since the late Miocene.

关键词：秦岭山脉风尘堆积构造意义气候新近纪晚中新世地球化学分析风尘沉积

^(14)C measurement of forest soils in Dinghushan Biosphere Reserve

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chinese Science Bulletin 1999年第3期44卷 251-256页

作者： SHEN Chengde , LIU Dongsheng (LIU Tungsheng) , PENG Shaolin, SUN Yanmin , JIANG Mantao , Yl Weixi , XING Changping , GAO Quanzhou , LI Zhi’an and ZHOU Guoyi Guangzhou institute of Geochemisry, chinese academy of sciences, Guangzhou 5.0640, china institute of geology, chinese academy of sciences , beijing 100029, china South china institute of Botany, chinese academy of sciences, Guangzhou 5.065., china Guannzhou institute of Geochemisry Chinese Academy of Sciences Guanazhou China institute of geology Chinese Academy of Sciences Beijing China South china institute of Botany Chinese Academy of Sciences Guangzhou China

Organic carbon in forest soils of Qingyunsi and Wukesong profiles can be divided into fast and slow components. Δ14C values of these profiles decrease with increasing of depth. The Δ14C values in 30—40 cm depth interval of Wukesong profile are decreasing sharply until a very low value,showing that a strong geological environment change occurred about 1 5.0 years ago. The 14C apparent ages of Wukesong profile show that the coniferous and broad-leaf mixed forests around Wukesong profile have been developing since 425.a BP, which is consistent with historical documents. The penetrating depths of "bomb 14C" in Qingyunsi and Wukesong profiles are 10 and 20 cm, respectively.

关键词： Dinghushan forest soil 14C tracing 14C apparent age.