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Al-modified yolk-shell silica particle-supported NiMo catalysts for ultradeep hydrodesulfurization of dibenzothiophene and 4.6-dimethyldibenzothiophene:Efficient accessibility of active sites and suitable acidity

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Petroleum Science 2024年第1期21卷 654-666页

作者： Ke Yu Wei-Min Kong Zhen Zhao Ai-Jun Duan Lian Kong xi-Long Wang State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing102249China Institute of Catalysis for Energy and Environment College of Chemistry and Chemical EngineeringShenyang Normal UniversityShenyang 110034LiaoningChina

Yolk-shell SiO2 particles(YP)with center-radial meso-channels were fabricated through a simple and effective ***-containing YP-supported NiMo catalysts with different Al amounts(NiMo/AYP-x,x=Si/Al molar proportion)were prepared and dibenzothiophene(DBT)and 4.6-dimethyl-dibenzothiophene(4.6-DMDBT)were employed as the probes to evaluate the hydrodesulfurization(HDS)catalytic *** as-prepared AYP-x carriers and corresponding catalysts were characterized by some advanced characterizations to obtain deeper correlations between physicochemical properties and the HDS *** average pore sizes of series AYP-x supports are above 6.0 nm,which favors the mass transfer of organic *** cavity between the yolk and the shell is beneficial for the enrichment of S-containing compounds and the accessibility between reactants and active *** embedded into the silica framework could facilitate the formation of Lewis(L)and Brønsted(B)acid sites and adjust the metal-support interaction(MSI).Among all the as-synthesized catalysts,NiMo/AYP-20 catalyst shows the highest HDS *** improved HDS activity of NiMo/AYP-20 catalyst is attributed to the perfect combination of excellent structural properties of the yolk-shell mesoporous silica,enhanced acidity,moderate MSI,and good accessibility/dispersion of active components.

关键词： Al-containing yolk-shell silica particles Accessibility Acidity Metal-support interaction Hydrodesulfurization

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Low-energy-consumption temperature swing system for CO_(2) capture by combining passive radiative cooling and solar heating

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Green Energy & Environment 2024年第3期9卷 507-515页

作者： Ying-xi Dang Peng Tan Bin Hu Chen Gu xiao-Qin Liu Lin-Bing Sun State Key Laboratory of Materials-Oriented Chemical engineering Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)College of Chemical EngineeringNanjing Tech UniversityNanjing211816China

Temperature-swing adsorption(TSA)is an effective technique for CO_(2) capture,but the temperature swing procedure is ***,we report a low-energy-consumption system by combining passive radiative cooling and solar heating for the uptake of CO_(2) on commercial activated carbons(CACs).During adsorption,the adsorbents are coated with a layer of hierarchically porous poly(vinylidene fluoride-co-hexafluoropropene)[P(VdF-HFP)HP],which cools the adsorbents to a low temperature under sunlight through radiative *** desorption,CACs with broad absorption of the solar spectrum are exposed to light irradiation for *** heating and cooling processes are completely driven by solar *** tests under mimicked sunlight using the CACs show that the performance of this system is comparable to that of the traditional ***,under real sunlight irradiation,the adsorption capacity of the CACs can be well maintained after multiple *** present work may inspire the development of new temperature swing procedures with little energy consumption.

关键词： CO_(2)capture Solar heating Passive radiative cooling Temperature swing adsorption

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Improvements in energy saving and thermal comfort for electric vehicles in summer through coupled electrochromic and radiative cooling smart windows

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Building Simulation 2024年第8期17卷 1231-1251页

作者： Zhoujie Duan Shuangdui Wu Hongli Sun Borong Lin Pei Ding Tao Cui Jeremy To xi Zhang college of Architectureand Environment Sichuan UniversityChengdu610065China Department of Building Science Tsinghua UniversityBejing 100084China KeyLaboratoryofEco Planning&Green Building MinistryofEducationTsinghua UniversityBeijing100084China State Key Laboratory of Hydraulics and Mountain River engineering Sichuan UniversityChengdu 610065China School of EmergencyManagement Xihua UniversityChengdu 610039China Department of PSVD Mercedes-benz Group China Ltd.Beijing 100102China

In hot climates,the large amount of cooling load in electric vehicle(EV)results in a lot of battery energy consumption,leading the decrease of driving *** the widespread application of windows in EV,the electrochromic glass(EC)shows great prospect in lowering the cooling ***,researches on the application of EC in EV lack the consideration of both passive cooling measures and passenger comfort,which limits the further application of *** this paper,we proposed an idea combining the novel techniques of both electrochromism and radiative *** fluid dynamics(CFD)is modeled to simulate the application of electrochromic and radiative cooling coupled smart windows in hot parking conditions,exploring the improvement effect of the window on the thermal environment,comfort and energy saving of the *** results indicate that,under the intense sunlight with an outdoor temperature of 33℃,activating the air conditioning to maintain an average interior temperature of 26℃,the coupled windows reduced the cooling capacity of the air conditioning by 762 W compared to regular windows,which can further increase the range of ***,compared to simple electrochromic fully colored glass,the integration of radiative cooling technology can lower the window surface temperature by up to 10.7℃.Moreover,compared to regular windows,the coupled windows lowered the standard effective temperature(SET*)for passengers by approximately 7℃,significantly improving *** research findings are expected to provide guidance for optimizing window design and enhancing the performance of EV.

关键词： electrochromism radiative cooling smart windowel ectric vehicle cabin thermal comfort energy saving

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Rain Erosion Behavior of Silicon Dioxide Films Prepared on Sapphire

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Journal of Materials Science & Technology 2005年第6期21卷 883-886页

作者： Liping FENG+, Zhengtang LIU and Wenting LIU Laboratory of Functional Materials, college of Materials Science and engineering, Northwestern Polytechnical university, xi’an710072, china Laboratory of Functional Materials College of Materials Science and Engineering Northwestern Polytechnical University Xi'an 710072 China

Silicon dioxide （SiO2） films were prepared on sapphire （α-Al2O3） by radio frequency magnetron reactive sputtering in order to increase both transmission and rain erosion resistant performance of infrared domes of sapphire. Composition and structure of SiO2 films were analyzed by X-ray photoelectron spectroscopy （XPS） and X-ray diffraction （XRD）, respectively. The transmittance of uncoated and coated sapphire was measured using a Fourier transform infrared （FTIR） spectrometer. Rain erosion tests of the uncoated and coated sapphire were performed at 211 m/s impact velocity with an exposure time ranging from 1 to 8 min on a whirling arm rig. Results show that the deposited films can greatly increase the transmission of sapphire in mid-wave IR. After rain erosion test, decreases in normalized transmission were less than 1% for designed SiO2 films and the SiO2 coating was strongly bonded to the sapphire substrate. In addition, sapphires coated with SiO2 films had a higher transmittance than uncoated ones after rain erosion.

关键词： Silicon dioxide films Sapphire Magnetron reactive sputtering Rain erosion

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Recent Development of Heat Transfer and Fluid Flow of Supercritical CO2 in Tubes:Mechanisms and Applications

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Journal of Thermal Science 2024年第06期33卷 2274-2298页

作者： ZHANG xirui SHAO Qihan LIU Jian xi Wenxiong LIU Chaoyang SUNDEN Bengt Research Institute of Aerospace Technology Central South University college of Aerospace Science and engineering National University of Defense Technology Department of Energy Sciences Lund University

With the advantages of low cost,excellent ability of heat and mass transfer and easy accessibility to the supercritical point,supercritical CO2has been applied in many engineering devices *** of the sharply-varying thermophysical properties near the supercritical point,heat transfer and flow behavior of supercritical CO2in tubes become complex and have received a lot of research *** main purpose of this paper is to summarize the findings of the published works related to flow phenomena and heat transfer characteristics of supercritical ***,influence parameters related to boundary conditions of supercritical CO2flowing in a smooth tube are ***,commonly-used turbulence and mathematic models dealing with internal flows of supercritical CO2are ***,research works on geometric effects of design parameters,shapes and configurations are *** practical applications of supercritical CO2in recent years are ***,developments and future challenges of supercritical CO2in tubes are analyzed and *** paper provides basic knowledge of heat transfer and fluid flow mechanisms and related practical applications of supercritical CO2in tubes.

关键词： developments and challenges flow behavior heat transfer practical applications supercritical CO2

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THE VELOCITY FIELD OF MULTIPHASE FLOW AND EFFICIENCY OF BIOLOGICAL AERATION FILTER

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Journal of Hydrodynamics 2010年第2期22卷 260-264页

作者： CHENG Wen HU Bao-wei YANG Chun-di CHENG Wen-juan Environment Research Institute Xian University of Technology Xi＇an 710048 China State Key Laboratory of Multiphase Flow in Power engineering Xi＇ an Jiaotong University Xi＇an 710049 China Key Laboratory of Northwest Water Resources and Environmental Ecology of Education Ministry Xi＇anUniversity of Technology Xi＇an 710048 China Yuanpei college Shaoxing University Shaoxing 312000 China Environment Research Institute Xi＇an University of Technology Xi＇an 710048 China

Aeration is an important factor affecting the biological aeration *** a set of experiment device specially designed for the purpose,and the particle image velocimetry technique,the velocity field of the gas-liquid two-phase flow is studied under different *** various simulated aeration states were actually applied to the experimental device of sewage treatment,and the results of the numerical simulation were *** final experimental results indicate that the most efficient state occurs when the ratio of water in aeration tank h / w =1,the diameter of capillary tubes d=0.6mm and the velocity of bubbles v=0.3m/s.

关键词： ratio of water diameter of capillary tube bubbles velocity sewage disposal efficiency

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Precise determination of GNSS trajectory in the Antarctic airborne kinematic positioning

Precise determination of GNSS trajectory in the Antarctic ai...

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第三届中国卫星导航学术年会

作者： Yan Xu1,Yuanxi Yang2,Guochang Xu3 1 changAn university,college of {4. engineering and geomatics,xi''an 710054,china

The airborne kinematic GNSS positioning in the Antarctic region has different characteristics with those in the internal *** with the Asian internal continent（***）,more satellites are visible so that lower PDOP of the polar regional GNSS positioning can be *** PDOP in the polar region may reduce 22%compared with that of ***,the VDOP in the polar region is weaker because of lacking of satellites with high elevation *** that basis,the significance of the Beidou Compass system for the Antarctic survey is quantitatively *** simulation result shows,comparing with using a single navigation system,that using Compass and GPS combined system may raise the positioning precision up to 4.%（in case of the elevation cut-off angle is 15 degrees）.Finally,the Antarctic GPS data are processed in different ways and the internal and external precision are *** show that the kinematic GNSS positioning can obtain a precision of cm by using precise point positioning technology.

关键词： Antarctic kinematic positioning GPS Compass accuracy analysis

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Synthesis,Structure and Antitumor Activities of Tridccapeptide PSPP3 from Papaver Somniferum Pollen

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Chinese Chemical Letters 1999年第2期10卷 115-116页

作者： Jia xi XU Sheng JIN(college of Chemistry and Molecular engineering, Peking university, Beijing 100871) Coll. of Chem. and Molec. Eng. Peking University Beijing 100871 China

Five analogs and five segments of the Papavor Somniferum pollen tridecapeptidePSPP3 were designed and synthesized by using solid-phase peptide synthesis method. Theirinhibitive activities to human liver tumor cell Bel-74.2 were assayed by MTT method and theirsecondary structures in solution were determined by CD spectra. The relationship of the structureand activity was discussed.

关键词： Pollen peptide anti-tumor activity structure and activity

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Effects of ABA Content on the Development of Abscission Zone and Berry Falling After Harvesting of Grapes

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Agricultural Sciences in china 2009年第1期8卷 59-67页

作者： ZHANG You-lin and ZHANG Run-guang college of Food engineering and Nutritional Science,Shaanxi Normal university,xi’an 710062,P.R.china [a]college of Food engineering and Nutritional Science Shaanxi Normal University Xi'an 710062 P. R. China

The commodity price of grape reduces as berry falling after harvest. It is crucial to prevent grape from berry falling during storage. In this article, the structure change of grape cells in the abscission zone was observed, the ABA content and the activities of cellulase and polygalacturonase （PG） were measured, and the relationship of ABA and berry falling was investigated. The results suggest that cells in the abscission zone grow into a separation layer soon after the grapes are cut off. According to the level of development, we designed 6 grades to sort the different development stages. The grade 3 plays an important role in berry falling. ABA enhances the activities of cellulase and polygalacturonase, and accelerates the decomposition of cellulose and pectin, which determines the level of development of abscission zone and berry falling. If ABA ratio is less than 20 ng g-i flesh weight （FW）, the abscission zone is not developed to the grade 3, and the berry falling is effectively stopped. We treated grape bunches with nine plant growth regulators and two chemicals. The results indicated that 2,3,5-triiodobenzoic acid （TIBA） can （a） inhibit the generation of ABA significantly, （b） inactivate the activities of cellulase and PG, （c） delay the development of the grade 3 of abscission zone, and （d） stop berry falling. Indole acetic acid （IAA）, gibberellic acid （GA3）, naphthalene acetic acid （NAA）, 6-benzylaminopurine （6-BA）, calcium chloride （CaCl2）, and potassium permanganate （KMnO4. caused similar results as TIBA. Chlorocholine chloride （CCC）, dimethyl amino succinamic acid （B9）, chloroethylphosphonic acid （CEPA） and exogenous ABA showed opposite effects.

关键词： grape phytohormone enzyme berry falling

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Upgrade and separation of Co from solution with low-grade Co

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中南工业大学学报：英文版 2001年第4期8卷 249-251页

作者： ZHONG Shi an,ZHOU Chun shan,OU Yang xi,CHENG Ben cheng(college of Chemistry and Chemical engineering, Central South university, changsha 4.0083,{4.) 1. college of Chemistry and Chemical engineering Central South University 410083 Changsha China

Upgrade and separation of Co from solution with low grade Co were studied. In the solution, the content of Co is about 1 g·L -1 , while that of Ni, Zn, Mn, Mg, Si and Ca is 0.14., 1.108, 0.119, 6.672, 0.026 and 0.200 g·L -1 , respectively. After absorbed with absorbent G-1, the content of Co in the solution is less than 1 mg·L -1 , the average loss rate of Co is 0.07%, while the average loss rate of Mg is 67.92%. It is demonstrated that the absorbent has selectivity to absorb Co. After the absorbent was eluted with HCl at room temperature, the solution with higher content of Co was obtained. Through being evaporated and concentrated, the contant of Co in the solution can be upgraded to 26.6 g·L -1 . At the same time, most of Si, Mg is removed, the total recovery of Co can reach as high as 98.7%. The content of Pb, Ni, Cu, Zn, Mn in the discharge solution is 1.00, 0.26, 0.21, 0.09, 0.15 mg·L -1 , respectively, and the discharge solution can reach the national discharge standard. CoCl 2 solid can be obtained and can reach chemical purity.

关键词： Co upgrade separation

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