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Fluorescence dynamics of interactions between polyamide PyPyPyβDp and DNA

Science China Chemistry 2006年第1期49卷 75-80页

作者： ZHANG Huijuan1,2. WANG Jin3. WU Yishi1, YUAN Gu3. AI Xicheng1, WANG Li4 & ZHANG Jianping1 1. State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, Chinese academy of sciences,{2., China 2. {3. of Life Science and Technology, beijing Institute of Technology, beijing 100081, China 3. College of Chemistry and Molecular Engineering, Peking University,{2., China 4. Center for Condensed Matter Physics, Institute of Physics, Chinese academy of sciences,{2., China Correspondence should be addressed to Ai Xicheng and Zhang Jianping 1. State Key Laboratory for Structural Chemistry of Unstable and Stable Species Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China 2. school of Life Science and Technology Beijing Institute of Technology Beijing 100081 China 3. College of Chemistry and Molecular Engineering Peking University Beijing 100080 China 4. Center for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Beijing 100080 China

The photophysical properties of the polyamide PyPyPyβDp (PPP) were investigated by means of steady-state absorption and fluorescence spectroscopies, as well as time-resolved fluo-rescence spectroscopy. It was found that the excited-state properties of PPP are very sensitive to solvents. In TKMC buffer PPP exhibited weak fluorescence with a decay time constant of 16 ps, while with the decrease of the solvent polarity PPP showed the blue-shifted peak position, increased inten-sity and lengthened life-time for its fluorescence behavior. In the presence of calf thymus DNA, it was observed that the fluorescence intensity was enhanced and the fluorescence lifetime increased from 16 to 3.0}ps for PPP, which verified that PPP bound into the minor groove of DNA duplex.

关键词： polyamide (PPP), calf thymus DNA (ctDNA), time-resolved fluorescence spectroscopy, recognition dynamics.

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Study on growth and properties of novel γ-LiAlO_2.substrate

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Science China(Technological sciences) 2006年第2期49卷 188-193页

作者： ZOU Jun1,2. ZHOU Shengming1, XU Jun1 & ZHANG Rong3.1. Shanghai Institute of Optics and Fine Mechanics, Chinese academy of sciences, Shanghai 2.1800, China 2. {2. {3. of Chinese academy of sciences, beijing 10003., China 3. Laboratory of Solid State Microstructures and Department of Physics, Nanjing University, Nanjing 2.0093. China 1. Shanghai Institute of Optics and Fine Mechanics Chinese Academy of Sciences Shanghai 201800 China 2. graduate school of Chinese {2. of {3. Beijing 100039 China 3. Laboratory of Solid State Microstructures and Department of Physics Nanjing University Nanjing 210093 China

Transparent γ-LiAlO2.single crystal has been grown by Temperature Gradient technique. The surface of the wafer annealed in O2.atmosphere at 1100°C for 70 h became opaque and Li-poor phase (LiAl5O8); while, that annealed in Li-rich atmosphere kept transparent and smooth. The full-width at half maximum value dropped to 3. arcsecs when the wafer was annealed in Li-rich atmosphere. That annealed in O2.atmosphere increased to 78 arcsec. Compared with absorption spectra, we can conclude that the 196 nm absorption peak was caused by Li vacancies and the 73. nm peak was caused by O vacancies.

关键词： γ-LiAlO2 crystal, scanning electron micrograph (SEM), absorption spectra.

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Characteristics and geological significance of olivine xenocrysts in Cenozoic volcanic rocks from western Qinling

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Progress in Natural Science:Materials International 2006年第12期16卷 1300-1306页

作者： SU Benxun~ 1,2.**, ZHANG Hongfu~1, XIAO Yan~ 1,2.and ZHAO Xinmiao~ 1,2.(1. State Key Laboratory of Lithospheric Evolution, Institute of Geology and Geophysics, Chinese {3. of sciences, {2. 10002., China 2. {3. school of Chinese {3. of sciences, {2. 10003., China) [a]State Key Laboratory of Lithospheric Evolution Institute of Geology and Geophysics Chinese Academy of Sciences Beijing China [b]graduate school of Chinese {2. of {3. Beijing China

Cenozoic volcanic rocks from the Haoti, Dangchang County of the western Qinling Mountains, contain a few clearly-zoned olivines. These olivines are relatively big in grain sizes and usually have cracks or broken features. Their cores have similar compositions （Mg#=90.4-91.0） to those for the peridotitic xenoliths entrained in host volcanic rocks and their rims are close to the compositions of olivine phenocrysts （Mg#=85.5-81.9）. The CaO contents in these zoned olivines are lower than 0.1%. These features demonstrate that the clearly-zoned olivines are xenocrysts and disaggregated from mantle peridotites. The zoned texture was the result of the interaction between the olivine and host magma. Available data show that the volcanic rocks would have been derived from the mantle source metasomatized by subducted hydrathermally-altered oceanic crust. The formation of these Cenozoic volcanic rocks was perhaps related to the rapid uplift of the Tibetan Plateau.

关键词： Western Qinling Dangchang Haoti Cenozoic volcanic rocks olivine xenocrysts zoned texture.

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Cotton pixel identification with CBERS-02.CCD data based on spectral knowledge

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Science China(Technological sciences) 2005年第S2期48卷 129-144页

作者： LI Jing1,2.3. LIU Qinhuo1,3. LIU Qiang1, CHEN Liangfu1, BO Junhua3.& LI Shaokun3.1. State Key Laboratory of Remote Sensing Science, IRSA, Chinese academy of sciences, {2. 100101, China 2. {3. University of Chinese academy of sciences, {2. 100049, China 3. The Key Oasis Eco-agriculture Laboratory of Xinjiang Production and Construction Corps, Shi Hezi 83.0}00, China 1. State Key Laboratory of Remote Sensing Science IRSA Chinese Academy of Sciences 100101 Beijing China 2. graduate University of Chinese academy of {2. 100049 Beijing China 3. The Key Oasis Eco-agriculture Laboratory of Xinjiang Production and Construction Corps 832000 Shi Hezi China

In this paper the in-situ experiment data are collected from the Spectral Library to estimate the possible values of the primary structural parameters in each cotton growing season by statistics. Based on these values the spectra of the cotton major growing seasons were simulated and analyzed using the canopy reflectance model, SAILH. In this way we also simulated the cotton pixel spectra corresponding to CBERS-02.CCD and took them as the reference spectra for spectra fitting. Then No.143.Regiment of No.8 Agricultural Division of Xinjiang Production and Construction Corps (XPCC) was chosen as the study area, and two spectra fitting methods, Mahalanobis distance and spectra angle, were used to identify cotton pixel from CBERS-02.CCD image of the study area. At last we analyzed the effect of the calibration coefficients error on cotton identifying. The results showed that within 4% error the spectral angle classifier can still have a good performance.

关键词： CBERS-02 cotton pixel identification spectra fitting.

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The regular representation and regular covariant representation of crossed products of Woronowicz C^(*)-algebras

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Science China Mathematics 2005年第9期48卷 1245-1259页

作者： ZHANG Xiaoxia~(1,2. & GUO Maozheng~(1,3. 1. school of Mathematical sciences,Peking University,{2. 100871,China 2. Department of Mathematics,Yantai University,Yantai 2.4005,China 3. LMAM,Peking University,{2. 100871,China 1. school of Mathematical sciences Peking University 100871 Beijing China 2. Department of Mathematics Yantai University 264005 Yantai China 3. LMAM Peking University 100871 Beijing China

In this paper,it is shown that the regular representation and regular covariant representation of the crossed products A×α G correspond to the twisted multiplicative unitary operators,where A is a Woronowicz C~*-algebra acted upon by a discrete group ***,it is also shown that the regular covariant C~*-algebra is the Woronowicz C~*-algebra which corresponds to a multiplicative ***,an explicit description of the multiplicative unitary operator for C(SU_q(2. )×α (?) is given in terms of those of the Woronowicz C~*-algebra C(SU_q(2. ) and the discrete group G.

关键词： multiplicative unitary operator, Woronowicz C*-algebra, crossed product.

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Analysis and Modeling on the Spatial Structure of Urban Land Use: A Case of Jinan, China

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Chinese Journal of Population,Resources and Environment 2007年第2期5卷 34-40页

作者： Zhao Huixia1, 3. Zhang Zulu2. Jiang Luguang 1 1. Institute of Geographical sciences and Natural Resources Research, Chinese academy of sciences, {3. 100101, China 2. College of Population, Resources and Environment, Shandong Normal University, Jinan Shandong 2.0014, China 3. graduate school of the Chinese academy of sciences, {3. 10003., China Institute of Geographical sciences and Natural Resources Research Chinese Academy of Sciences Beijing 100101 China graduate school of the Chinese {2. of {3. Beijing 100039 China College of Population Resources and Environment Shandong Normal University Jinan Shandong 250014 China

Based on the data of urban land use obtained by remote sensing interpretation from aero images in 1986 and 2.04, the spatial structure of Jinan is studied in this paper with the method of Geographic Information System (GIS). According to the proportion of land for residence, industry and commerce, the urban district can be distinguished into three rings. Compared with the traditional theory of the ring structure in Western coun- tries, they have many distinctive characteristics. The main func- tions of the inner ring include residence, business and banking, but the proportion of residential land (more than 50%) is considerably higher than that of the cities in Western countries. The land proportion for residence and industry in the intermediate ring is equal on the whole. The main land of the outside ring is for industrial use. From 1986 to 2.04, great changes have taken place on the land proportion of different types of use. In the inner ring, the land for residential and industrial use has shrunk much while the land for commercial use has increased. In the intermediate ring, the changes of the three types of land use were not very much and the temporal variation was relatively stable. On the contrary, the structure in the outside ring varies acutely. Though most of it is also for industrial use, the proportion of residential land has in- creased much. The three rings can also be divided into several sectors respectively, according to the function of land use clusters. New trends and mechanisms of the changes of land use impacting the urban structure were proposed in the end of the paper.

关键词： urban land use ring structure sector structure Jinan

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The onset and advance of the Asian summer monsoon

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Science Bulletin 2006年第1期51卷 80-88页

作者： Lü Junmei1,2.4, ZHANG Qingyun1, TAO Shiyan1 & JU Jianhua3.1. State Key Laboratory of Numerical Modeling for Atmospheric Sci- ences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese academy of sciences, {2. 10002., China 2. Department of Atmospheric sciences, Yunnan University, Kunming 650091, China 3. China Meteorological Administration Training Centre, {2. 100081, China 4. graduate school of Chinese academy of sciences, {2. 10003., China State Key Laboratory of Numerical Modeling for Atmospheric sciences and Geophysical Fluid Dynamics Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China Department of Atmospheric sciences Yunnan University Kunming 650091 China graduate school of Chinese {2. of {3. Beijing 100039 China China Meteorological Administration Training Centre Beijing 100081 China

Based on the daily outgoing longwave radiation (OLR) data from National Oceanic and At- mospheric Administration (NOAA) satellites, the Cli- mate Prediction Center’s merged analysis of pre- cipitation (CMAP) data and the National Centers for Environmental Prediction/National Center for At- mospheric Research (NCEP/NCAR) reanalysis dataset, the mean intraseasonal variability of the Asian summer monsoon (ASM) is investigated by using power spectrum analysis, band-pass filter, and diagnostic analyses. The processes of the onset and advance of monsoon over the southern part of Indo- china Peninsula, the east coast of Bay of Bengal, the South China Sea and the Indian subcontinent are explored. It is found that there is an abrupt change in OLR, precipitation and zonal wind during the onset and advance of the ASM. It is also indicated that the southern part of Indochina Peninsula and the adja- cent Andaman Sea is the region where the earliest onset of the ASM occurs in the 2.d pentad of May.

关键词： Asian summer monsoon intraseasonal variability onset advance.

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The biomarkers of 2.6,10,15, 19-pentamethylicosenes and their carbon isotopic composition in the sediments from the Gulf of Mexico

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Chinese Science Bulletin 2006年第14期51卷 1736-1740页

作者： SONG Zhiguang1,2.& WANG Cuiping1,3.. State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese academy of sciences, Guangzhou 510640, China 2. Guangzhou Research Center of Gas Hydrate, Chinese academy of sciences, Guangzhou 510640, China 3. graduate school of Chinese academy of sciences, beijing 10003., China State Key Laboratory of Organic Geochemistry Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China Guangzhou Research Center of Gas Hydrate Chinese Academy of Sciences Guangzhou 510640 China graduate school of Chinese {2. of {3. Beijing 100039 China

A group of 2.6,10,15,19-pentamethyli- cosenes (PMIΔ) containing 1―5 unsaturated double bonds has been identified in the sea floor sediments from the Gulf of Mexico at the Green Canyon 2.8 *** PMIΔ compounds are distributed between nC2. and nC2. on the mass chromatogram of aliphatic fraction. Their δ 13. values are very much depleted in 13. and in the range of ?86.7‰ to ?115.5‰, whereas the δ 13. values of companion n-alkanes range from ?2..4‰ to ?3..6‰. These unsaturated PMIΔ com-pounds are typical biomarkers derived from the an-aerobic oxidation of methane mediated by meth-ane-oxidizing archaeal bacteria and indicative of the gas seeps or even the occurrence of gas hydrates in the deep sea sediments.

关键词：生物标志墨西哥湾沉积物 PMIA 天然气水化物

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A new principle of synthetic cascade utilization of chemical energy and physical energy

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Science China(Technological sciences) 2005年第2期48卷 163-179页

作者： JIN Hongguang1, HONG Hui1,2. WANG Baoqun1,2. HAN Wei1,2.& LIN Rumou1,2.1. Institute of Engineering Thermophysics, Chinese academy of sciences,{2., China 2. {3. school of the Chinese academy of sciences, beijing 10003., China 1. Institute of Engineering Thermophysics Chinese Academy of Sciences 100080 Beijing China 2. graduate school of the Chinese {2. of {3. 100039 Beijing China

We propose a new principle of the cascade utilization of both chemical energy and physical energy in energy systems with the integration of chemical processes and thermal cycles. Particularly, a general equation of energy levels of substance, Gibbs free energy of chemical reaction and physical energy is explicitly founded. On the basis of this equation, a chemical-looping combustion and an indirect combustion are investigated. Furthermore, a mechanism of energy release, with the combination of decreasing the energy level of Gibbs free energy and upgrading the energy level of low or middle- temperature thermal energy, is clarified. The promising results obtained here establish a theoretical basis for the further investigation of multi-function systems in which energy and the environment are compatible, and create a new approach to improve the performance of traditional thermal cycles.

关键词： chemical energy, cascade utilization, exergy, energy conversion.

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Threshold quantum secure direct communication without entanglement

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Science China(Physics,Mechanics & Astronomy) 2008年第2期51卷 176-183页

作者： YANG YuGuang1,3.& WEN QiaoYan2.1 College of Computer Science and Technology, beijing University of Technology, beijing 10002., China 2.{2. of Science, beijing University of Posts and Telecommunications, beijing 100876, China 3.State Key Laboratory of Information Security (graduate {2. of Chinese academy of sciences), beijing 100049, China 1. College of Computer Science and Technology Beijing University of Technology Beijing 100022 China 3. State Key Laboratory of Information Security (graduate school of Chinese {2. of {3.) Beijing 100049 China 2. school of Science Beijing University of Posts and Telecommunications Beijing 100876 China

For the first time, a threshold quantum secure direct communication (TQSDC) scheme is presented. Similar to the classical Shamir's secret sharing scheme, the sender makes n shares, S1, …, Sn of secret key K and each receiver keeps a share secretly. If the sender wants to send a secret message M to the receivers, he en-codes the information of K and M on a single photon sequence and sends it to one of the receivers. According to the secret shares, the t receivers sequentially per-form the corresponding unitary operations on the single photon sequence and ob-tain the secret message M. The shared shares may be reusable if it can be judged that there is no eavesdropper in line. We discuss that our protocol is feasible with current technology.

关键词： quantum secure direct communication threshold secure direct communication quantum secret sharing

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