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Physical mechanisms of plant roots affecting weathering and leaching of loess soil

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Science china Earth sciences 2006年第9期49卷 1002-1008页

作者： LI Yong1,2, ZHANG Qingwen1,2, WAN Guojiang3. HUANG Ronggui3. PIAO Hechun3. BAI Lingyu2 & LI Lu2 1. State Key Laboratory of Soil Erosion and Dryland Farming on the Loess Plateau, institute of Soil and Water Conservation, chinese academy of sciences, Yangling 712100, china 2. institute of Agro-Environment and Sustainable Development, chinese academy of Agricultural sciences, Beijing 100081, china 3. institute of Geochemistry, chinese academy of sciences, guiyang 550002. china State Key Laboratory of Soil Erosion and Dryland Farming on the Loess Plateau Institute of Soil and Water Conservation Chinese Academy of Sciences Yangling China institute of Agro-Environment and Sustainable Development Chinese Academy of Agricultural Sciences Beijing China institute of Geochemistry Chinese Academy of Sciences Guiyang China

Plant roots have potential impacts on soil mineral weathering and *** objective is to understand the physical mechanisms of plant roots affecting weathering andleaching of loess soil. Root densities were measured through the method of a large-size dug profile,and transport fluxes of soil elements were determined using an undisturbed monolith soilinfiltration device on the hilly and gully regions of the chinese Loess Plateau. The results showthat the improvement effects of soil environment by plant roots are mainly controlled by the densityand weight of the fibrous roots with the diameters less than 1 mm. Plant roots have the strongereffects on soil physical properties than chemical properties. The principal components analysis(PCA) indicates that soil physical properties by plant roots account for 56.7% of variations in soilenvironment whereas soil chemical properties and pH contribute about 24.2% of the soil *** roles of plant roots in controlling soil weathering and leaching increased in the followingorder: infiltration enhancement > increase of bio-active substance > stabilization of soilstructure. The effects of plant roots on soil mineral weathering and leaching can be quantifiedusing the multiple regression models with the high prediction accuracies developed in this study.

关键词： plant roots, soil weathering and leaching rates, soil environment field, principal components analysis (PCA), chinese Loess Plateau.

PREPARATION AND PROPERTIES OF ETHYL-CYANOETHYL CELLULOSE/POLYACRYLIC ACID COMPOSITE FILMS WITH REFLECTION COLORS

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chinese Journal of Polymer Science 2001年第3期19卷 277-282页

作者： Yong Huang institute of chemistry, chinese academy of sciences, Beijing 100080 {3. Laboratory of Cellulose and Lignocellulosics chemistry Guangzhou institute of chemistry chinese academy of sciences, Guangzhou 510650, {3. 中科院化学所北京

Ethyl-cyanoethyl cellulose [(E-CE)C]/acrylic acid (AA) becomes a cholesteric liquid crystalline solution withvivid colors when the (E-CE)C concentration is 42 wt%～52 wt%. (E-CE)C/polyacrylic acid (PAA) composites withcholesteric structure were prepared by polymerzing AA in (E-CE)C/AA liquid crystalline solutions. The layers of orderedpolymer chains in the cholesteric phase were inclined during polymerization and the degree of the inclination depended onthe polymerization temperature and the concentration of the solution before polymerization. The cholesteric structure in thecomposites could not be changed when temperature was lower than 100℃. Cross-linking of the PAA in compositesimproved their water-resistance. The cholesteric order of the composites without cross-linking was destroyed when theywhere immersed in water. The color derived from the selective reflection of the cholesteric phase of the cross-linkedcomposites turned from blue to red after the composites absorbed water. The color of the composites could be returned to theoriginal one when the absorbed water was removed from the swollen composites.

关键词： Cholesteric structure Composites Selective reflection Liquid crystalline solutions

Advances in geochemical research on nanometer materials

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Progress in Natural Science:Materials International 2006年第4期16卷 331-337页

作者： ZHU Xiaoqing and WANG Zhonggang Key Laboratory of Ore Deposit Geochemistry, institute of Geochemistry,{3., guiyang 550002. china Key Laboratory of Ore Deposit Geochemistry Institute of Geochemistry Chinese Academy of Sciences Guiyang 550002 China

Important advances have been made in the field of geochemistry since nanometer science and technology were introduced into the field of geoscience. The nanometer particulates have been discovered in naturally-occurring ore deposits, volcano-eruptive materials and geo-gases, and a more detailed exploration of the metallogenic mechanism of endogenic metallic ore deposits has been conducted. It is considered that some ore-forming metals may transport in the form of native particulates. Because they have very strong capabilities of adsorption, adsorption is always regarded as an important mechanism of metallogenesis under supergenic and low temperature conditions. Therefore, a new technology of ore exploration has also been developed. This paper attempts to review the new advances in geochemical research on nanometer materials, as well as its perspectivess.

关键词： nanometer geochemistry adsorption metallogenic theory prospecting method.

SYNTHESIS AND CHARACTERIZATION OF NEW STABILIZERS WITH OPTIMAL MOLECULAR WEIGHT

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chinese Journal of Polymer Science 2001年第4期19卷 341-350页

作者： Jiang-qing Pan institute of chemistry chinese academy of sciences, Beijing 100080 {3. 中科院化学所北京

Over 2 x 10(8) tons of polymers are produced every year, and a large portion of polymers faces the degradation problem. There are many effective methods to protect polymers against degradation and the addition of stabilizers to polymer remains the most convenient and effective way of enhancing polymer life and performance. In this article, a series of effective stabilizers with optimal molecular weight (MW), including common, monomeric and polymeric stabilizers (antioxidant and light stabilizer) were synthesized using isocyanation, controlled isocyanation, hydrosilylation, epoxide addition, macroreaction of stabilizing functional compounds and polymerization of monomeric stabilizers. The structure and performance of these new stabilizers were characterized by using IR, NMR, MS, UV-spectra, XPS and elemental analysis. The current development of stabilizer synthesis was also reviewed.

关键词： preparation of stabilizer antioxidant hindered amine light stabilizer isocyanation hydrosilylation

Evidence of acid nature of ore-forming solutions

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chinese Science Bulletin 1999年第S2期44卷 199-201页

作者： CHEN Fu institute of Geochemistry, chinese academy of sciences,{3. institute of Geochemistry Chinese Academy of Sciences Guiyang 550002 China

THE author thinks that the ore-forming solution is formed not by the near-neutral brine but by the strongacid solutions. Some evidence are the following: （i） The simulating experiments showed that, all near-neutral supergenic water as volcanic hotspring water of Tengchong, K-brine of Mengyejing, seawater of Qingdao, oil-gasses-bearing water of Chitianhua, rain water of guiyang and CO2-bearing rain cannot form metal-bearing solutions by heating mixedabove-mentioned supergenic water with ore-source rocks as basalt, ore-bearing carbonate, sandstone andshale. The most content of Cu, Pb, Zn, Hg, Sb, As, Ag in solutions is only （0.3.0.5）×10-6.They cannot form any ore deposit. Oppositely, the acid solution of pH=1.0 is easy to form metal-bearingsolutions with every ore-source rocks. The most content of metal in solution is n×10-n×1000 × 10-6i.e. rose in 3.5 grades. The content of metals in humic acid-bearing solutions is variable, perhaps dueto the changes of humic components and content and due to easy-decomposition by oxidation or *** the best one in solutions to form ore-forming solution is only the acidic water.

关键词： ore-forming solution acid solution in nature genesis of brine.

Mantle-derived sulfur and its time constraints on gold mineralization of Ailaoshan gold belt, china

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chinese Science Bulletin 1999年第S2期44卷 242-244页

作者： BI Xianwu institute of Geochemistry, chinese academy of sciences,{3. institute of Geochemistry Chinese Academy of Sciences Guiyang 550002 China

IN the previous studies of hydrothermal deposits much attention was paid to their material sources ratherthan the mechanisms of dynamic association of ore-forming fluids. In recent years many studies haveshown that ore-forming elements were transferred into ore-forming solutions after some suitable mineralizerwas incorporated into hydrothermal solutions. Therefore, the time at which the mineralizer is incorporated into hydrothermal solutions could, to a great extent, reflect the time of ore deposition. In the dynamic study of the origin of ore deposits on a trial basis the author took the Ailaoshan gold belt in YunnanProvince as an example and carried out investigations into the sources of mineralizers (the anion coordinates of stable complexes of gold in hydrothermal solutions) in ore-forming hydrothermal solutions and theconstraints of relevant geological events on gold mineralization.

关键词： sulfur isotope mantle-derived sulfur dating gold mineralization Ailaoshan gold belt.

Epithermal gold deposits in china and potential assessment

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chinese Science Bulletin 1999年第S2期44卷 164-166页

作者： QIU Yuzhuo institute of Geochemistry, chinese academy of sciences,{3. institute of Geochemistry Chinese Academy of Sciences Guiyang 550002 China

THE epithermal gold deposit (epi-gold) is one of the most important types in various gold deposits all overthe world. The discovery of several superlarge deposits of this type around the circum-Pacific Rim duringthe 1980s, greatly stimulated the interest in searching for epi-golds in the world as well as in china. Theepi-gold has become a major target in gold exploration in china during last two-decade "Golden *** discovery of the Zijinshan Cu (Au) deposit in SE china and the Axi and other Au deposits in NWchina is the significant success in gold prospecting in this field. The author suggested that it is the timeto do an overview and the potential assessment of epi-golds in china Some people are holding an optimistic idea on this topic mainly based on the following considerations: (i) as a host rock, the subaerial volcanic rocks of Mesozoic are widespread in East china; (ii)

关键词： epithermal gold deposit china potential assessment.

Experimental measurement of the electrical conductivity of single crystal olivine at high temperature and high pressure under different oxygen fugacities

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Progress in Natural Science:Materials International 2006年第4期16卷 387-393页

作者： DAI Lidong, LI Heping, LIU Congqiang, CUI Tongdi, SHAN Shuangming, YANG Changjun, LIU Qingyou and DENG Heming Laboratory of the Earth’s Interior Materials and Fluid Geochemistry, institute of Geochemistry,{3., guiyang 550002. china Graduate School of the{3., Beijing 10003., china institute of Geochemistry,{3., guiyang 550002. china Guizhou University, guiyang 550004, china Laboratory of the Earth's Interior Materials and Fluid Geochemistry Institute of Geochemistry Chinese Academy of Sciences Guiyang 550002 China Graduate School of the chinese academy of sciences Beijing 100039 China institute of Geochemistry chinese academy of sciences Guiyang 550002 China Guizhou University Guiyang 550004 China

At 1.0-4.0 GPa and 1123.1473.K and under oxygen fugacity-controlled conditions (Ni + NiO, Fe + Fe3.4, Fe + FeO and Mo+ M0O2 buffers), a YJ-3.00t Model six-anvil solid high-pressure apparatus and a Sarltron-1260 Impedance/Gain-Phase analyzer were employed to conduct an in situ measurement of the electrical conductivity of single crystal olivine. Experimental results showed that: (1) within the range of experimentally selected frequencies (103.106 Hz), the electrical conductivity of the sample is of great dependence on the frequency; (2) with the rise of temperature ( T), the electrical conductivity (σ) will increase, and the Arrenhius linear relationship is established between lgσ and 1/T; (3. under the control of oxygen buffer Fe+ Fe3.4, with the rise of pressure, the electrical conductivity tends to decrease whereas the activation enthalpy and independent-of-temperature preexponential factor tend to increase, with the activation energy and activation volume of the sample estimated at (1. 25 ± 0.08) eV and (0.105 ±0.025) cm3.mol, respectively; (4) under given pressure and temperature conditions, the electrical conductivity tends to increase whereas the activation energy tends to decrease with increasing oxygen fugacity; and ( 5) the mechanism of electrical conduction of small polarons can provide insight into the behavior of electrical conduction of olivine under high pressure and high temperature.

关键词： olivine high temperature and high pressure electrical conductivity oxygen fugacity small polaron.

Oxygen isotopic (^(17)O-^(18)O) heterogeneity in Archaean continental nucleus, North china Craton

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chinese Science Bulletin 1999年第24期44卷 2267-2269页

作者： LIU Jianzhong, ZHANG Fuqin, LI Chunlai and WANG Shijie institute of Geochemistry , chinese academy of sciences , {3. 550002., china institute of Geophysics , chinese academy of sciences , Beijing 100101 , china institute of Geochemistry Chinese Academy of Sciences Guiyang China institute of Geophysics Chinese Academy of Sciences Beijing China

The oxygen isotopic data for amphibolites from Archaean continental nucleus, North china Craton indicate that ( i ) the evolving lines structured by the data are parallel to the geoselenic evolving line, which means that the parent materials of these continental nucleus o-riginated from solar matter; ( ii ) different intercepts for these evolving lines manifest that oxy-

关键词： North china Craton oxygen isotope (I7O-18O ) heterogeneity.