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Local and non-local sources of airborne particulate pollution at beijing——The ratio of Mg/Al as an element tracer for estimating the contributions of mineral aerosols from outside beijing

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Science china Chemistry 2005年第3期48卷 253-264页

作者： HAN Lihui1, ZHUANG Guoshun1,2,3. SUN Yele1 & WANG Zifa3.1. The Center for atmospheric Environmental Study, Department of Chemistry, beijing Normal University, beijing 100875,{3. 2. Center for atmospheric Chemistry Study, Department of Environmental Science & Engineering, Fudan University, Shanghai 20043.,{3. 3. lapc/nzc, institute of atmospheric Physics, cas, beijing 10002.,{3. 1. The Center for atmospheric Environmental Study Department of Chemistry Beijing Normal University 100875 Beijing China 2. Center for atmospheric Chemistry Study Department of Environmental Science & Engineering Fudan University 200433 Shanghai China 3. institute of atmospheric Physics CAS LAPC/NZC 100029 Beijing China

A new element tracer technique has firstly been established to estimate the contri-butions of mineral aerosols from both inside and outside beijing. The ratio of Mg/Al in aerosol is a feasible element tracer to distinguish between the sources of inside and outside beijing. Mineral aerosol, inorganic pollution aerosol mainly as sulfate and nitrate, and organic aerosol are the major components of airborne particulates in beijing, of which mineral aerosol accounted for 3.%―67% of total suspended particles （TSP）, 10%―70% of fine particles （PM2.5）, and as high as 74% and 90% of TSP and PM2.5, respectively, in dust storm. The sources from outside beijing contributed 62% （3.%―86%） of the total mineral aerosols in TSP, 69% （52%―90%） in PM10, and 76% （59%―93.） in PM2.5 in spring, and 69% （52%―83.）, 79% （52%―93.）, and 45% （7%―79%） in TSP, PM10, and PM2.5, respectively, in winter, while only20% in summer and autumn. The sources from outside beijing contributed as high as 97% during dust storm and were the dominant source of airborne particulates in beijing. The contributions from outside Bei-jing in spring and winter are higher than those in summer, indicating clearly that it was related to the various meteorological factors.

关键词： mineral aerosol local sources non-local sources dust storm re-suspended dust element tracer technique.

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Speciation of the elements and compositions on the surfaces of dust storm particles:The evidence for the coupling of iron with sulfur in aerosol during the long-range transport

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Chinese Science Bulletin 2005年第8期50卷 738-744页

作者： ZHANG Xingying1,2, ZHUANG Guoshun1,2,3. CHEN Jianmin2 & XUE Huaxin2 1. Center for atmospheric Environment Study, Department of Chemistry, beijing Normal University, beijing 100875,{3. 2. Center for atmospheric Chemistry Study, Department of Environ- mental Science and Engineering, Fudan University, Shanghai 20043.,{3. 3. lapc/nzc, institute of atmospheric Physics, nzc/lapc, Chinese Academy of Sciences, beijing 10002.,{3. Center for atmospheric Environment Study Department of Chemistry Beijing Normal University Beijing 100875 China Center for atmospheric Chemistry Study Department of Environmental Science and Engineering Fudan University Shanghai 200433 China lapc/nzc Institute of Atmospheric Physics NZC/LAPC Chinese Academy of Sciences Beijing 100029 China

The speciation of the elements on the surface of the particles collected during dust storm and non-dust storm in beijing and Inner Mongolia was studied by XPS. The ma- jor species of iron on the surface were oxides, sulfate, silicate, FeOOH and minor part sorbed on SiO2/Al2O3. Sulfate is the dominant species of sulfur on the surface. SiO2 and Al2O3.are the main components of Si and Al on the surface respectively. One of the most important findings was that the Fe(II) (FeS and FeSO4) produced could account for up to 44.3. and 45.6% of the total Fe on the surface in the aerosol sample collected at that night and next day of the “peak” time of the dust storm occurring on March 20, 2002, while Fe2(SO4)3. one of the Fe(III) species on the surface decreased from 67.1% to 49.5% and 48.0% respectively. Both S and Fe en- riched on the surface of aerosol particles. Fe(II) accounted for 1.3.?5.3. of total Fe in bulk aerosol samples during dust storm. These results provided strong evidence to sup- port the hypothesis of the coupling between iron and sulfur in aerosols during the long-range transport, which would have important impact on the global biogeochemical cycle.

关键词：物种形成原理 XPS 大气悬浮物 Fe-S结合粒子集合

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Three-dimensional decomposition method of global atmospheric circulation

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Science china Earth Sciences 2008年第3期51卷 386-402页

作者： LIU HaiTao1,2,3. HU ShuJuan4, XU Ming5 & CHOU JiFan6,7 1 State Key Laboratory of Numerical Modeling for atmospheric Sciences and Geophysical Fluid Dynamics, institute of atmospheric Physics, Chinese Academy of Sciences,{3., china 2 Graduate University of Chinese Academy of Sciences, beijing 100049, china 3.beijing Climate Center, beijing 100089, china 4 Department of Mathematics, Lanzhou University, Lanzhou 73.000, china 5 Shanghai Typhoon institute, Shanghai 20003., china 6 Department of atmospheric Sciences, Lanzhou University, Lanzhou 73.000, china 7 china Meteorological Administration Training Center, beijing 100089, china 1. State Key Laboratory of Numerical Modeling for atmospheric Sciences and Geophysical Fluid Dynamics Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China 2. Graduate University of Chinese Academy of Sciences Beijing 100049 China 3. beijing Climate Center Beijing 100089 China 4. Department of Mathematics Lanzhou University Lanzhou 730000 China 5. Shanghai Typhoon institute Shanghai 200030 China 6. Department of atmospheric Sciences Lanzhou University Lanzhou 730000 China 7. china Meteorological Administration Training Center Beijing 100089 China

By adopting the idea of three-dimensional Walker, Hadley and Rossby stream functions, the global atmospheric circulation can be considered as the sum of three stream functions from a global perspective. Therefore, a m... 详细信息

关键词： three-dimensional decomposition of the global atmospheric circulation generalized Walker Hadley and Rossby stream functions existence and uniqueness vertical motion

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Interannual variability of Antarctic Oscillation and its influence on East Asian climate during boreal winter and spring

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Science china Earth Sciences 2006年第5期49卷 554-560页

作者： FAN Ke1,2,3.& WANG Huijun2 1. Nansen-Zhu International Research Center, institute of atmospheric Physics, Chinese Academy of Sciences, beijing 10002.,{3. 2. Department of atmospheric Science, Yunnan University, Kunming 650091,{3. 3. Graduate University of the Chinese Academy of Sciences, beijing 100049,{3. 1. Nansen-Zhu International Research Center Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China 2. Department of atmospheric Science Yunnan University Kunming 650091 China 3. Graduate University of the Chinese Academy of Sciences Beijing 100049 China

The interannual variability of Antarctic Oscillation (AAO) and its influence on East Asian climate during both boreal winter and spring are addressed. The results show that the positive AAO anomaly decreases the cold activity over East Asia during both boreal winter and spring. AAO-related barotropic meridional teleconnection from Antarctic to Arctic is found through analysis of mean me- ridional circulations. This meridional teleconnection is remarkable over Eurasia during boreal winter and over the Pacific Ocean during boreal spring. The results also show that zonal mean zonal wind at high latitudes in Southern Hemisphere has well positive correlation with that of Eurasia during boreal winter and has negative correlation with Pacific North American teleconnection (PNA) during boreal spring, which again display the meridional teleconnection. Thus, local meridional teleconnection is a possible linkage for interaction of circulations at mid-high latitudes between both hemispheres.

关键词： Antarctic Oscillation, Eurasian west wind, meridional teleconnection, mean meridional circulation.

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Hierarchical structures in climate and atmospheric turbulence

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Progress in Natural Science:Materials International 2002年第10期 29-34页

作者： SHE Zhensu, FU Zuntao, CHEN Jiong, LIANG Shuang and LIU Shida(1. State Key Laboratory for Studies of Turbulence and Complex Systems, Department of Mechanics and Engineering Sciences, Peking University, beijing 100871, china 2. School of Physics, Peking University, beijing 100871, china 3. lapc, institute of atmospheric Physics, Chinese Academy of Sciences, beijing 10002., china) State Key Laboratory for Studies of Turbulence and Complex Systems，Department of Mechanics and Engineering Sciences，Peking University，beijing 100871，china lapc，institute of atmospheric Physics，Chinese Academy of Sciences，{3. 10002.，china School of Physics，Peking University，beijing 100871，china State Key Laboratory for Studies of Turbulence and Complex Systems，Department of Mechanics and Engineering Sciences，Peking University，beijing 100871，china School of Physics，Peking University，beijing 100871，china

The climatic time series encompass many time scales, forming multi-scale climatic variations and hierarchies. The periods and magnitudes of cooling or warming, especially for extreme climatic events, vary with the time scales. On the other hand, high-frequency atmospheric turbulent motions, which are certainly related to the climatic changes, are also typical multi-scale phenomena. In this paper, certain properties of the fluctuations are examined that are invariant with the change of the time scales. Specifically, the existence of a statistical similarity law is demonstrated in climatic time series and in atmospheric turbulent motions. This is the hierarchical similarity law. Further analyses show that the hierarchical similarity law is a general property of multi-scale fluctuation systems. Therefore, the study on the hierarchical similarity law is important for understanding the inherent universal physical mechanism of complex systems in the atmospheric motions.

关键词： climate multi-scale hierarchical structure atmospheric turbulence.

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Global analysis theory of climate system and its applications

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Chinese Science Bulletin 2003年第10期48卷 1034-1039页

作者： LI Jianping1,2 & CHOU Jifan2,3.1. LASG, institute of atmospheric Physics, Chinese Academy of Sciences, beijing 10002.,{3. 2. Department of atmospheric Sciences, Lanzhou University, Lanzhou 73.000,{3. 3. Training Center for{3. Meteorological Administration, beijing 100081,{3. Department of atmospheric Sciences Lanzhou University Lanzhou 730000 China LASG Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China

The idea and main theoretical results of the global analysis theory of climate system are briefly summarized in this paper. A theorem on the global behavior of climate system is given, i.e. there exists a global attractor in the dynamical equations of climate, any state of climate system will be evolved into the global attractor as time increases, indicating the nonlinear adjustment process of climate system to external forcing. The different effects of external forcing, dissipation and nonlinearity on the long-term behavior of solutions are pointed out, and some main applications of the global analysis theory are also introduced. Especially, three applications, the adjustment and evolution processes of climate, the principle of numerical model design and the optimally numerical integration, are discussed.

关键词：整体分析理论气侯体系应用不定性计算法则气侯科学数字模型

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Computational stability of the forced dissipative nonlinear atmospheric equations

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Chinese Science Bulletin 1999年第10期44卷 949-952页

作者： LI Jianping and CHOU Jifan LASG , institute of atmospheric Physics , Chinese Academy of Sciences , beijing 100080,{3. Department of atmospheric Sciences , Lanzhou University , Lanzhou 73.000,{3. beijing Meteorological College, beijing 100081,{3. LASG Institute of Atmospheric Physics Chinese Academy of Sciences Beijing China Department of atmospheric Sciences Lanzhou University Lanzhou China beijing Meteorological College Beijing China

A new concept of computational quasi-stability (CQS) is introduced to study the computational stability (CS) of the forced dissipative nonlinear (FDN) evolution equations. Based on the concept, the CQS criterion of difference scheme of FDN atmospheric equations is obtained. So it provides the theoretical basis for designing the computational stable difference scheme of FDN atmospheric equations.

关键词： computational stability (CS) computational quasi-stability (CQS) operator equation difference scheme forced dissipative nonlinear (FDN) equations.

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Two possible mechanisms for vortex self-organization

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Science china Earth Sciences 2006年第2期49卷 202-211页

作者： LUO Zhexian2, ZHOU Xiuji1 & GAO Shouting3.1. Chinese Academy of Meteorological Sciences, beijing 100081, china 2. Department of Space Information Science, Nanjing University of Information Science and Technology, Nanjing 210044, china 3. {3. of atmospheric Physics, Chinese Academy of Sciences, beijing 10002., china 2. Department of Environmental Science Nanjing University of Information Science and Technology Nanjing 210044 China 1. Chinese Academy of Meteorological Sciences Beijing 100081 China 3. institute of atmospheric Physics Chinese Academy of Sciences Beijing 100029 China

The vortex self-organization is investigated in this paper by four groups of numerical experiments within the framework of quasi-geostrophic model, and based on the experimental results two types of possible mechanisms for vortex self-organization are suggested. The meso-scale to-pography may enable separated vortices to merge into a larger scale vortex; and the interaction of meso-γ and meso-β scale systems may make separated vortices to self organize a typhoon-like vor-tex circulation.

关键词： vortex, self-organization, meso-scale topography, interaction of different scales.

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2002:The extra-strong warm winter event in North Asia and its accompanying anomalous atmospheric circulation

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Chinese Science Bulletin 2003年第10期48卷 1031-1033页

作者： WANG Huijun LASG, institute of atmospheric Physics, Chinese Academy of Sciences, beijing 10002.,{3. LASG Institute of Atmospheric Physics Chinese Academy of Science China

Features of an extra-strong warm winter event in North Asia in 2002 and its accompanying anomalous atmospheric circulation were studied through diagnosis on the atmospheric reanalysis data set. Results show that the winter of 2002 is of the warmest in the recent 54 years in North Asia, which was caused by both decadal scale and interannual scale variability. The interannual variability is proved to be as the main cause for the event, and it is related to the global scale atmospheric circulation anomalies, with the strongest of them in the Eastern Hemisphere and in the middle and high latitude region of the Southern Hemisphere.

关键词：大气环流亚洲北部高强度暖冬现象天气资料

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Inertial theory of the mean Hadley circulation under the condition of nonstatic equilibrium

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Science china Earth Sciences 2006年第5期49卷 546-553页

作者： CHAO Jiping1 & LIU Fei2,3.1. National Marine Environmental Forecasting Center, beijing 100081, china 2. Key Laboratory Regional Climate-Environment for Temperate East Asia, {3. of atmospheric Physics, Chinese Academy of Sciences, beijing 10002., china 3. Graduate University of Chinese Academy of Sciences, beijing 100049, china 1. National Marine Environmental Forecasting Center Beijing 100081 China 2. Key Laboratory Regional Climate-Environment for Temperate East Asia Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China 3. Graduate University of Chinese Academy of Sciences Beijing 100049 China

Tropical atmosphere is divided into two layers, the layer near the ground is the planet boundary layer, where the motion is linear, if the radiation equilibrium temperature is given at the top of the boundary layer, the vertical motion there can be obtained. It is the non-viscous ideal atmos- pheric layer above the boundary one, where the motion is nonlinear. After getting the conservation laws of angular momentum, potential temperature and potential vortex, the inertial theory of the Hadley circulation driven by the vertical motion of the boundary layer is established, followed by sev- eral examples of its application.

关键词： Hadley circulation, inertial theory, conservation laws of angular momentum, potential temperature and potential vortex.

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