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Accurate studies on the full vibrational energy spectra and molecular dissociation energies for some electronic states of N_(2)molecule

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Science China(physics,Mechanics & Astronomy) 2005年第4期48卷 385-398页

作者： REN Weiyi1,2, SUN Weiguo1, HOU Shilin3.& FENG Hao4.1. Institute of physics, College of Chemical Engineering, Sichuan university, Chengdu 610065, China 2. Institute of Theoretical physics, Xihua Normal university, Nanchong 63.002, China {4., China oceanography university, qingdao 2.6003, China 4. College of physics, Sichuan university, Chengdu 610065, China 1. Institute of physics College of Chemical Engineering Sichuan University 610065 Chengdu China 2. Institute of Theoretical physics Xihua Normal University 637002 Nanchong China 3. department of physics China Oceanography University 266003 Qingdao China 4. College of physics Sichuan University 610065 Chengdu China

It is usually very difficult to directly obtain molecular dissociation energy De and all accurate high-lying vibrational energies for most diatomic electronic states using modern experimental techniques or quantum theories, and it is also very difficult to give accurate analytical expression for diatomic molecular dissociation energy. This study proposes a new analytical formula for obtaining accurate molecular dissociation energy based on the LeRoy and Bernstein’s energy expression in dissociation limit. A set of full vibrational energy spectra for some electronic states of N2 molecule are studied using the algebraic method (AM) suggested recently, and the corresponding accurate molecular dissociation energies are evaluated using the proposed new formula and high-lying AM vibrational energies. The results show that the AM spectra and the new theoretical dissociation energies agree excellently with experimental data, and thereby providing a new physical approach to generating accurate dissociation energies for electronic states of diatomic molecules.

关键词： vibrational energy, dissociation energy, nitrogen molecule, algebraic method.

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X-ray spectra induced in highly charged 4.Ar^q+ interacting with Au surface

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Science China(physics,Mechanics & Astronomy) 2006年第2期49卷 203-212页

作者： ZHANG Xiao’an1,2, XIAO Guoqing1, YANG Zhihu1, CHEN Ximeng3. ZHAO Yongtao1, LI Fuli4. ZHANG Yinping1, CUI Ying3. ZHANG Hongqiang3. XU Xu3. SHAO Jianxiong3.& ZHAN Wenlong11. Institute of Modern physics, Chinese Academy of Sciences, Lanzhou 73.000, China 2. department of physics, Xianyang Normal {3., Xianyang 712000, China 3. department of Modern physics, Lanzhou {3., Lanzhou 73.000, China 4. department of Applied physics, Xi’an Jiaotong {3., Xi’an 71004., China 1. Institute of Modern physics Chinese Academy of Sciences Lanzhou 730000 China 2. department of physics Xianyang Normal University Xianyang 712000 China 3. department of Modern physics Lanzhou University Lanzhou 730000 China 4. department of Applied physics Xi’an Jiaotong University Xi’an 710049 China

By use of optical spectrum technology, the spectra of X-ray induced by highly charged 4.Arq+ ions interacting with Au surface have been studied. The results show that the argon Kα X-ray were emitted from the hollow atoms formed below the surface. There is a process of multi-electron exciting in neutralization of the Ar16+ion, with electronic con-figuration 1s2 in its ground state below the solid surface. The yield of the projectile Kα X-ray is related to its initial electronic configuration, and the yield of the target X-ray is related to the projectile kinetic energy.

关键词： highly charged ion hollow multi-electron excitation X- ray.

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Study on the two and three-parameter working stability regions of 3.-TZP suspension

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Science China(Technological Sciences) 2006年第5期49卷 547-568页

作者： CHEN Youqiang1, 2, ZHANG Xinni3. CHEN Sha’ou3.& QI Ping3.1. department of Chemistry, {4. university, {4. 266071, China 2. department of Chemistry, Tsinghua university, Beijing 100084. China 3. department of physics, {4. university, {4. 266071, China 1. department of Chemistry Qingdao University Qingdao 266071 China 2. department of Chemistry Tsinghua University Beijing 100084 China 3. department of physics Qingdao University Qingdao 266071 China

We determined the variation tendency of viscosity (η) at various solids load- ing (α) for 3.-TZP suspension as a function of dispersant concentration (Cw) using vis- cosity measurement, measured the diameter of particles as a function of Cw in very dilute suspension using light scattering method, and obtained the surface features of the sedi- ment of suspension with different Cw using SEM. We also discussed the influence of the microstructure of adsorbed polymer layers on particles and their interactions in the dis- persing medium on the stability of suspension. Then two different stable states and two different unstable states for 3.-TZP suspension were given. Accordingly, the (Cw, η), (Cw, α), and (α, η) two-parameter, and (Cw, α, η) three-parameter stability maps were con- structed. Based on the DLVO theory calculations, the dispersant concentration, particle distance (r), and interparticle potential energy (VT) maps with various solids loading for 3.-TZP aqueous suspension were also constructed. In (Cw, r) two-parameter coordinate system, the stable motion region map for particles was established. The Cw, α, and VT,max (the highest potential energy) surface of the potential barrier map was obtained through calculation and simulation on the basis of the surfaces of Cw, r, VT maps introduced above. The (Cw, α) two-parameter stability map was then obtained from the Cw, α, VT,max map. The results showed that this theoretical map can qualitatively prove the experimentally obtained results—the existence of different dispersed states of particles in suspension system and the variation tendency of suspension stability with changing each parame- ter—were reasonable.

关键词： 3.-TZP, suspension, stability, DLVO theory, interparticle potential energy.

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β-delayed proton decays near the proton drip line

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Science China(physics,Mechanics & Astronomy) 2005年第3期48卷 257-267页

作者： XU Shuwei 1 , LI Zhankui 1 , XIE Yuanxiang 1 , HUANG Wenxue 1 , SHU Nengchuan 2 , CHEN Yongshou 2 , XU Furong 3., WANG Kun 4., PAN Qiangyan 1 , WANG Xudong 1 , YU Yong 1 & XING Yebing 1 1. Institute of Modern physics, Chinese Academy of Sciences, Lanzhou 73.000, China 2. Nuclear physics {4., China Institute of Atomic Energy, Beijing 1024.3. China 3. {4. of Technical physics, Peking university, Beijing 100871, China 4. Shanghai Institute for Nuclear Research, Shanghai 201800, China 1. Institute of Modern physics Chinese Academy of Sciences 730000 Lanzhou China 2. Nuclear physics department China Institute of Atomic Energy 102413 Beijing China 3. department of Technical physics Peking University 100871 Beijing China 4. Shanghai Institute for Nuclear Research 201800 Shanghai China

We briefly reviewed the experimental study on a-delayed proton decays near the proton drip line published by our group during the period of 1996―2004. namely the first observation of the a-delayed proton decays of 9 new nuclides in the rare-earth region and the new measurements of a-delayed proton decays of 5 nuclides in the mass ～90 region near the N = Z line with the aid of the “p-?” coincidence in combination with a He-jet tape transport system. In the meantime some important experimental technique details were supplemented. The experimental results, including the half -lives, spins, parities, deformations and production reaction cross sections for the 14.nuclei were summarized and compared with the current nuclear-model predictions, and then the following points were represented. (1) The experimental half-lives for 85Mo and 92Rh as well as the predicted “waiting point” nuclei 89Ru and 93.d are 5―10 times longer than the theoretical predictions given by M?ller et al. using a macroscopic-microscopic model. It considerably influences the predictions of the abundances of the nuclides produced in the rp-process. (2) The current-model predictions are not consistent with the experimental assignments of the spins and parities for the proton drip-line nuclei 14.Ho and 128Pm. However, the nuclear potential energy surface (PES) calculated by using a Woods- Saxon-Strutinsky method reproduced the experimental results. (3. The Alice code overestimated the production reaction cross sections of the studied 9 rare-earth nuclei by one order of magnitude or two, while HIVAP code overestimated them by one order of magnitude approximately.

关键词： proton drip line, β-delayed proton decay, He-jet tape transport system, "p-γ" coincidence, spin, parity, deformation, production reaction cross section.

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Entropy product measure for multipartite pure states

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Science China(physics,Mechanics & Astronomy) 2006年第5期49卷 606-615页

作者： CAO Wancang1,2, LIU Dan2, PAN Feng3.& LONG Guilu2,4.1. department of physics, Chifeng College, Chifeng 024.01, China 2. Key Laboratory for Quantum Information and Measurements, department of physics, Tsinghua {4., Beijing 100084. China 3. department of physics, Liaoning Normal {4., Dalian 116029, China 4. Key Laboratory for Atomic and Molecular Nano-Sciences, Tsinghua {4., Beijing 100084. China Correspondence should be addressed to Long Guilu department of physics Chifeng College Chifeng 024001 China Key Laboratory for Quantum Information Measurements Department of Physics Tsinghua University Beijing 100084 China department of physics Liaoning Normal University Dalian 116029 China Key Laboratory for Atomic Molecular Nano-Sciences Tsinghua University Beijing 100084 China

An entanglement measure for multipartite pure states is formulated using the product of the von Neumann entropy of the reduced density matrices of the constituents. Based on this new measure, all possible ways of the maximal entanglement of the triqubit pure states are studied in detail and all types of the maximal entanglement have been compared with the result of ‘the average entropy’. The new measure can be used to calculate the degree of entanglement, and an improvement is given in the area near the zero entropy.

关键词： multipartite pure state von Neumann entropy entanglement measure

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Proton induced X-ray emission (PIXE) analysis of sources of porcelain body of Ru Guan and Jun Guan porcelains

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Science China(physics,Mechanics & Astronomy) 2006年第4期49卷 411-420页

作者： LI Guoxia1, ZHAO Weijuan1, LI Rongwu2, SUN Hongwei1, GUO Min1, WANG Yanfang1, LIU Hui1, ZHAO Qingyun3. SUN Xinmin3. ZHAO Wenjun3.& CHENG Huansheng4.1. Faculty of Physical Engineering, Zhengzhou university, Zhengzhou 4.0052, China 2. {4. of physics, Beijing Normal university, Beijing 100875, China 3. Institute of Cultural Relic and Archaeology of Henan Province, Zhengzhou 4.0000, China 4. Institute of Modern physics, Fudan university, Shanghai 2004.0}, China Faculty of Physical Engineering Zhengzhou University Zhengzhou 450052 China department of physics Beijing Normal University Beijing 100875 China Institute of Cultural Relic Archaeology of Henan Province Zhengzhou 450000 China Institute of Modern physics Fudan University Shanghai 200433 China

3. samples of Ru Guan porcelain body and 50 samples of Jun Guan porcelain body (both kinds being in different body colors) were selected with the purpose of finding out the source of raw materials and their classification relationship so as to search for ways of non-destructive discrimination. Proton induced X-ray emission (PIXE) has been applied to these samples to determine their chemical elements. The data of seven major chemical elements collected from these samples were further studied through fuzzy cluster analysis. Results indicate that the origin of raw materials of Jun Guan porcelain body samples is comparatively more concentrated in certain places, while that of Ru Guan porcelain body samples is scattered about. The places of origin of raw materials of the majority of Ru Guan and Jun Guan porcelain body samples have something in common, but some differences still exist. It might be an important way for non-destructive discrimination among Ru Guan and Jun Guan porcelains by combining PIXE with fuzzy cluster analysis.

关键词： Ru Guan and Jun Guan porcelain, source of porcelain body, PIXE, fuzzy cluster analysis, non-destructive discrimination.

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Estimating surface evapotranspiration using combined MODIS and CBERS-02 data

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Science China(Technological Sciences) 2005年第S2期48卷 145-160页

作者： XIN Xiaozhou1,2, LIU Qinhuo1, TANG Yong1,3. TIAN Guoliang1, GU Xingfa1, LI Xiaowen1,2, ZHENG Hongsheng4.& CHEN Jiayi4.1. State Key Laboratory of Remote Sensing Science, Institute of Remote Sensing Applications, Chinese Academy of Sciences, Beijing 100101, China 2. Research Center for Remote Sensing and GIS, department of Geography, Beijing Normal university, Beijing 100875, China 3. Graduate university of Chinese Academy of Sciences, Beijing 10003., China 4. department of Atmospheric {4., Peking university, Beijing 100871, China 1. State Key Laboratory of Remote Sensing Science Institute of Remote Sensing Applications Chinese Academy of Sciences 100101 Beijing China2. Research Center for Remote Sensing and GIS Department of Geography Beijing Normal University 100875 Beijing China3. Graduate University of Chinese Academy of Sciences 100039 Beijing China4. Department of Atmospheric Physics Peking University 100871 Beijing China

Spatial scale error is one of the most serious problems in the estimates of land surface heat fluxes of sensible and latent from satellite-borne data such as MODIS 1km resolution reflectance and emissive data. One of the feasible and economic ways to decrease the spatial scale error is to use high resolution land use class data together with the MODIS data. CBERS-02 data were used to produce land use class of Baiyangdian area, Hebei Province, China in the autumn of 2004. The area ratio of each class in MODIS pixel was calculated, and used to derive the heat fluxes of the mixed pixel. The results showed that the estimated heat fluxes of soil, sensible and latent have been changed remarkably after using the high resolution land class data. It could be concluded from the comparison between simulated and ground-measured fluxes as well as the theoretical analysis that high resolution land class data are useful to diminishing the scale error of heat fluxes estimated from low resolution satellite data.

关键词： surface evapotranspiration spatial scale error MODIS CBERS land class.

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Virtualities of quark and gluon in QCD vacuum

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Science China(physics,Mechanics & Astronomy) 2008年第10期51卷 1439-1447页

作者： ZHOU LiJuan1, QIN SongMei2, WU Qing3.& MA WeiXing4.1 Collaboration Group of Hadron physics and Non-perturbative QCD Study, Guangxi university of Tech- nology, Liuzhou 54.006, China 2 department of physics, Guangxi university, Nanning 54.003. China 3.department of physics, qingdao university, qingdao 266071, China 4.Institute of High Energy physics, Chinese Academy of Sciences, Beijing 10004., China 1. Collaboration Group of Hadron physics and Non-perturbative QCD Study Guangxi University of Technology Liuzhou 545006 China 2. department of physics Guangxi University Nanning 540003 China 3. department of physics Qingdao University Qingdao 266071 China 4. Institute of High Energy physics Chinese Academy of Sciences Beijing 100049 China

The non-local vacuum condensates of quantum chromodynamics (QCD) describe the distributions of quarks and gluons in the non-perturbative QCD vacuum state. Physically, this means that vacuum quarks and gluons have a nonzero mean-squared momentum in the vacuum, called virtuality. The quark virtuality is given by the ratio of the local quark-gluon mixed vacuum condensate to the quark local vacuum condensate. The gluon virtuality is expressed by gluon vacuum condensates and four-quark vacuum condensates. We study the two virtualities by solving Dyson-Schwinger Equations and calculating quark and gluon vacuum condensates. Our theoretical results for quark virtuality are in good agreement with many other theoretical model predictions such as QCD sum rules and lattice QCD calculations. Our calculation on gluon virtuality is initial and the results are quite interesting.

关键词： quark gluon virtuality QCD vacuum condensate non-perturbative QCD

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PIXE and INAA studies on ancient potteries from Guangfulin relics in Shanghai

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Progress in Natural Science:Materials International 2007年第11期17卷 1348-1356页

作者： Lin Jiawei1, Cheng Huansheng1, Zhang Zhengquan1, Zhang Bin1, Feng Songlin2, Song Jian3. Gao Menghe4.and Zhu Dan1(1. Applied Ion Beam physics Laboratory, Key Laboratory of the Ministry of Education, Institute of Modern physics, Fudan university, Shanghai 2004.0}, China 2. Key Laboratory of Nuclear Analytical Techniques, Institute of High Energy physics, Beijing 10003., China 3. Shanghai Museum, Shanghai 200003. China 4. {4. of Cultural Heritage and Museology, Fudan university, Shanghai 2004.0}, China) Applied Ion Beam physics Laboratory Key Laboratory of the Ministry of Education Institute of Modern Physics Fudan University Shanghai 200433 China Key Laboratory of Nuclear Analytical Techniques Institute of High Energy Physics Beijing 100039 China Shanghai Museum Shanghai 200003 China department of Cultural Heritage and Museology Fudan University Shanghai 200433 China

This paper reports the study of ancient potteries unearthed from the Guangfulin site in Shanghai. From the external features of these potteries, archeologists can classify them into two different cultural types: Liangzhu culture (local culture) and a new culture which might be derived elsewhere, but they can not recognize whether they were produced in the same place. Proton induced X-ray emission (PIXE) and instrumental neutron activation analysis (INAA) were used to measure the chemical compositions of the samples and the results were analyzed using multivariate statistics. We found that the two methods can complement each other and their database can be mutually referenced in the study of ancient potteries. Experimental results show that the compositions of the potteries from the two cultural types are different, which means that the materials for ancient potteries of new culture originate from elsewhere. This supports the archaeologists’ speculation that a group of ancient people migrated to Shanghai from some other places 4.00 years ago.

关键词： PIXE INAA factor analysis Guangfulin ancient pottery

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Implementation of a multiple round quantum dense coding using nuclear magnetic resonance

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Science China(physics,Mechanics & Astronomy) 2005年第6期48卷 706-715页

作者： ZHANG Jingfu1, XIE Jingyi2, WANG Chuan1, DENG Zhiwei3. LU Zhiheng4. & LONG Guilu1,5 1. Key Laboratory For Quantum Information and Measurements of MOE, department of physics, Tsinghua university, Beijing 100084.China 2. department of Materials Science and Engineering, Beijing Normal university, Beijing 100875, China 3. Testing and Analytical Center, Beijing Normal university, Beijing 100875,China 4. department of physics, Beijing Normal university, Beijing 100875, China 5. Key Laboratory For atomic and Molecular Nanosciences, Tsinghua university, Beijing 100084.China 1. Key Laboratory For Quantum Information and Measurements of MOE Department of Physics Tsinghua University 100084 Beijing China 2. department of Materials science and Engineering Beijing Normal University 100875 Beijing China 3. Testing and Analytical Center Beijing Normal University 100875 Beijing China 4. department of physics Beijing Normal University 100875 Beijing China 5. Key Laboratory For Atomic and Molecular Nanosciences Tsinghua University 100084 Beijing China

A multiple round quantum dense coding scheme based on the quantum phase estimation algorithm is proposed and implemented in a three qubit nuclear magnetic resonance (NMR) quantum computer. Using an m + 1 qubit system, Bob can transmit one of 2m+1 messages to Alice, through manipulating only one qubit and exchanging it between Alice and Bob for m rounds. The information capacity is enhanced to m + 1 bits as compared to m bits in a classical scheme. The scheme has been demonstrated in NMR system, and the experimental results show a good agreement between theory and experiment.

关键词： quantum dense coding, multiple round, nuclear magnetic resorance

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