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Study on the two and three-parameter working stability regions of 3.-TZP suspension

Science china(Technological Sciences) 2006年第5期49卷 547-568页

作者： CHEN Youqiang1, 2, ZHANG Xinni3. CHEN Sha’ou3.& QI Ping3.1. Department of Chemistry, Qingdao University, Qingdao 266071, china 2. Department of Chemistry, Tsinghua University, Beijing 100084, china 3. Department of physics, Qingdao University, Qingdao 266071, china 1. Department of Chemistry Qingdao University Qingdao 266071 China 2. Department of Chemistry Tsinghua University Beijing 100084 China 3. Department of physics Qingdao University Qingdao 266071 China

We determined the variation tendency of viscosity (η) at various solids load- ing (α) for 3.-TZP suspension as a function of dispersant concentration (Cw) using vis- cosity measurement, measured the diameter of particles as a function of Cw in very dilute suspension using light scattering method, and obtained the surface features of the sedi- ment of suspension with different Cw using SEM. We also discussed the influence of the microstructure of adsorbed polymer layers on particles and their interactions in the dis- persing medium on the stability of suspension. Then two different stable states and two different unstable states for 3.-TZP suspension were given. Accordingly, the (Cw, η), (Cw, α), and (α, η) two-parameter, and (Cw, α, η) three-parameter stability maps were con- structed. Based on the DLVO theory calculations, the dispersant concentration, particle distance (r), and interparticle potential energy (VT) maps with various solids loading for 3.-TZP aqueous suspension were also constructed. In (Cw, r) two-parameter coordinate system, the stable motion region map for particles was established. The Cw, α, and VT,max (the highest potential energy) surface of the potential barrier map was obtained through calculation and simulation on the basis of the surfaces of Cw, r, VT maps introduced above. The (Cw, α) two-parameter stability map was then obtained from the Cw, α, VT,max map. The results showed that this theoretical map can qualitatively prove the experimentally obtained results—the existence of different dispersed states of particles in suspension system and the variation tendency of suspension stability with changing each parame- ter—were reasonable.

关键词： 3.-TZP, suspension, stability, DLVO theory, interparticle potential energy.

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Density functional theory study on the structural and electronic properties of Ag-adsorbed (MgO)_n clusters

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Science china(physics,Mechanics & Astronomy) 2009年第5期52卷 734-741页

作者： GE GuiXian1, JING Qun1 & LUO YouHua2,3.1 Key Laboratory of Ecophysics and Department of physics, Normal College, Shihezi University, Shihezi 83.003. china 2 School of Science, East china University of Science and Technology, Shanghai 20023., china 3.Institute for theoretical physics, henan University, kaifeng 475004, china Key Laboratory of Ecophysics and Department of physics Normal College Shihezi University Shihezi 832003 China School of Science East China University of Science and Technology Shanghai 200237 China Institute for theoretical physics Henan University Kaifeng 475004 China

Equilibrium geometries, charge distributions, stabilities and electronic properties of the Ag-adsorbed (MgO)n (n = 1-8) clusters have been investigated by density functional theory (DFT) with generalized gradient approximation (GGA) for exchange-correlation functional. The results show that hollow site is energetically preferred for n≥4, and the incoming Ag atoms tend to cluster on the existing Ag cluster. The Mulliken populations indicate that the interaction between the Ag atom and Magnesia clusters is mainly induced by a weak atomic polarization. The adsorbed Ag atom only causes charge redistributions of the atoms near itself. The effect of the adsorbed Ag atom on the bonding natures and structural features of Magnesia clusters is minor. Furthermore, the investigations on the first energy difference, fragmentation energies and electron affinities show that the Ag(MgO)4 and Ag(MgO)6 are the most stable among studied clusters.

关键词： Ag (MgO)_n clusters geometries electronic properties

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A computational investigation of boron-doped chromium and chromium clusters by density functional theory

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Science china(physics,Mechanics & Astronomy) 2010年第5期53卷 812-817页

作者： GE GuiXian1,JING Qun1 & LUO YouHua2,3.1 Key Laboratory of Ecophysics and Department of physics,Normal College,Shihezi University,Xinjiang 83.003.china 2 School of Science,East{3. University of Science and Technology,Shanghai 20023.,china 3.Institute of theoretical physics,School of physics and Information Optoelectronics,henan University,kaifeng 475004,china 1. Key Laboratory of Ecophysics and Department of physics Normal College Shihezi University Xinjiang 832003 China2. School of Science East China University of Science and Technology Shanghai 200237 China3. Institute of Theoretical Physics School of Physics and Information Optoelectronics Henan University Kaifeng 475004 China

The geometries,stabilities and electronic properties of Crn and CrnB(n=2-9) clusters have been systematically investigated by density functional *** results suggest that the lowest energy structures for CrnB clusters can be obtained by substituting one Cr atom in Crn+1 clusters with B *** geometries of CrnB clusters are similar to that of Crn+1 clusters except for local structural *** second-order difference and fragmentation energy show Cr4,Cr6,Cr8,Cr3.,Cr5B and Cr8B cluster are the most stable among these studied *** impurity B increases the stabilities of chromium *** B is doped on the Crn clusters,cluster geometry does dominate positive role in enhancing their *** doped B atom does not change the coupling way of the Cr site in Crn clusters,but breaks the symmetry and the Cr atoms are no longer *** doped B atom increases the total magnetic moments of Crn in most cases.

关键词： Crn and CrnB clusters geometries electronic properties

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The dynamical properties of Rydberg hydrogen atom near a metal surface

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Science china(physics,Mechanics & Astronomy) 2005年第6期48卷 667-675页

作者： GE Meihua1, ZHANG Yanhui1, WANG Dehua2, DU Mengli3.& LIN Shenglu1 1. College of physics and Electronics, Shandong Normal University, Jinan 250014, china 2. Department of Mathematics and physics, Shandong Institute of Architecture and Engineering, Jinan 250014, china 3. Institute of theoretical physics, Chinese Academy of Sciences, Beijing 100080, china 1. College of physics and Electronics Shandong Normal University 250014 Jinan China 2. Department of Mathematics and physics Shandong Institute of Architecture and Engineering 250014 Jinan China 3. Institute of theoretical physics Chinese Academy of Sciences 100080 Beijing China

The dynamical properties of Rydberg hydrogen atom near a metal surface are presented by using the methods of phase space analysis and closed orbit theory. Transforming the coordinates of the Hamiltonian, we find that the phase space of the system is divided into vibrational and rotational region. Both the Poincaré surface of section and the closed orbit theory verify the same conclusion clearly. In this paper we choose the atomic principal quantum number as n = 20. The dynamical character of the exited hydrogen atom depends sensitively on the atom-surface distance d. When d is sufficiently large, the atom-surface potential can be expressed by the traditional van der Waals force and the system is integrable. When d becomes smaller, there exists a critical value dc. For d > dc, the system is near-integrable and the motion is regular. While chaotic motion appears for d < dc, and the system tends to be non-integrable. The trajectories become unstable and the electron might be captured onto the metal surface.

关键词： Rydberg hydrogen atom, van der Waals interaction, Poincaré surface of section, closed orbit theory, chaos.

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Accurate studies on the full vibrational energy spectra and molecular dissociation energies for some electronic states of N_(2)molecule

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Science china(physics,Mechanics & Astronomy) 2005年第4期48卷 385-398页

作者： REN Weiyi1,2, SUN Weiguo1, HOU Shilin3.& FENG Hao4 1. Institute of physics, College of Chemical Engineering, Sichuan University, Chengdu 610065, china 2. Institute of theoretical physics, Xihua Normal University, Nanchong 63.002, china 3. Department of physics, china Oceanography University, Qingdao 266003. china 4. College of physics, Sichuan University, Chengdu 610065, china 1. Institute of physics College of Chemical Engineering Sichuan University 610065 Chengdu China 2. Institute of theoretical physics Xihua Normal University 637002 Nanchong China 3. Department of physics China Oceanography University 266003 Qingdao China 4. College of physics Sichuan University 610065 Chengdu China

It is usually very difficult to directly obtain molecular dissociation energy De and all accurate high-lying vibrational energies for most diatomic electronic states using modern experimental techniques or quantum theories, and it is also very difficult to give accurate analytical expression for diatomic molecular dissociation energy. This study proposes a new analytical formula for obtaining accurate molecular dissociation energy based on the LeRoy and Bernstein’s energy expression in dissociation limit. A set of full vibrational energy spectra for some electronic states of N2 molecule are studied using the algebraic method (AM) suggested recently, and the corresponding accurate molecular dissociation energies are evaluated using the proposed new formula and high-lying AM vibrational energies. The results show that the AM spectra and the new theoretical dissociation energies agree excellently with experimental data, and thereby providing a new physical approach to generating accurate dissociation energies for electronic states of diatomic molecules.

关键词： vibrational energy, dissociation energy, nitrogen molecule, algebraic method.

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Light A physics in the lepton-specific two-Higgs doublet model

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Science china(physics,Mechanics & Astronomy) 2010年第11期53卷 1981-1987页

作者： CAO JunJie 1,HENG ZhaoXia 2,3.& WAN PeiHua 1 1 College of physics & Information Engineering,henan Normal University,Xinxiang 453.07,china 2 Key Laboratory of Frontiers in {3. physics,Institute of {3. physics,Chinese Academy of Sciences,Beijing 100190,china 3.Kavli Institute for {3. physics china,Chinese Academy of Sciences,Beijing 100190,china 1. College of physics & Information Engineering Henan Normal University Xinxiang 453007 China2. Key Laboratory of Frontiers in Theoretical Physics Institute of Theoretical Physics Chinese Academy of Sciences Beijing 100190 China3. Kavli Institute for Theoretical Physics China Chinese Academy of Sciences Beijing 100190 China

We examine various direct and indirect constraints on the lepton-specific two-Higgs doublet model and discuss its phenomenology at colliders in the allowed parameter *** constraints we consider come from the precision electroweak data,the direct search for Higgs boson,the muon anomalous magnetic moment,as well as some theoretical consistency *** find that in the allowed parameter space the CP-odd Higgs boson A is rather light (m A 3. GeV with 95% possibility),which is composed dominantly by the leptonic Higgs and decays dominantly into τ + τ;while the SM-like Higgs boson h (responsible largely for electroweak symmetry breaking) decays dominantly in the mode h → AA → 4τ with a large decay width,which will make the Higgs discovery more difficult at the ***,this scenario predicts rare Z decays Z → AAA and Z →τ + τA with their branching ratios ranging from 10-8 to 10-and 10-5 to 10-4 respectively,which may be accessible at the GigaZ option of the ILC.

关键词： Lepton-specific two-Higgs doublt model light Higgs boson A Z decays

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Surface-induced interaction of colloidal particles in isotropic liquid crystals

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Communications in theoretical physics 2024年第7期76卷 114-122页

作者： Hualing Zhang kaifeng Weng Rui Ma Department of physics College of Physical Science and TechnologyXiamen UniversityXiamen 361005China Fujian Provincial Key Laboratory for Soft Functional Materials Research Research Institute for Biomimetics and Soft MatterXiamen UniversityXiamen 361005China

In this work,we study the interaction between two colloidal particles in a liquid crystal that is in the isotropic *** interaction is caused by surface-induced polarization of the liquid crystal molecules in the vicinity of the *** find that the interaction is short-ranged in both 2D and 3. *** symmetric homeotropic anchoring conditions,the interaction is *** under anti-symmetric homeotropic anchoring conditions,the interaction is repulsive at short distances but attractive at intermediate *** particle size has a strong impact on the effective interaction force.

关键词： surface-induced interaction colloidal particles liquid crystals

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Superconductivity of small metal grains

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Science china(physics,Mechanics & Astronomy) 2005年第4期48卷 431-441页

作者： ZHENG Renrong1 CHEN Zhiqian2 & ZHU Shunquan1,3.1. Department of physics, Shanghai Normal University, Shanghai 20023., china 2. Department of physics, Southwest Normal University, Chongqing 400715, china 3. Department of Computer and Electric Technology, Shanghai Business School, Shanghai 201400, china 1. Department of physics Shanghai Normal University 200234 Shanghai China 2. Department of physics Southwest Normal University 400715 Chongqing China 3. Department of Computer and Electric Technology Shanghai Business School 201400 Shanghai China

The formulas of the energy gap and superconducting critical temperature appropriate for systems with both odd and even number of electrons are derived; the bases of the derivations are BCS theory and energy level statistics. Numerical results qualitatively agree with the experimental phenomena. i.e., the superconductivity of small metallic grains will first enhance then decrease to zero when the grain are getting smaller and smaller. The calculations indicate that the above phenomena happen in the metallic grains belonging to Gaussian Orthogonal Ensemble (GOE) and Gaussian Unitary ensemble (GUE) with zero spin; The superconductivity of small metallic grains in Gaussian Symplectic Ensemble (GSE) will monotonically decrease to zero with the decreasing of the grain size. The analyses suggest that the superconductivity enhancements come from pairing and the balance of the strengths between spin-orbital coupling and external magnetic field. In order to take the latter into account, it is necessary to include the level statistics given by Random Matrix Theory (RMT) in describing small metallic grains.

关键词： size effect, superconductivity enhancements, small metallic grains.

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Isospin-dependent relativistic microscopic optical potential in the Dirac Brueckner-Hartree-Fock method

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Science china(physics,Mechanics & Astronomy) 2004年第2期47卷 189-198页

作者： RONG Jian1 & MA Zhongyu1,2,3.1. china Institute of Atomic Energy, Beijing 102413. china 2. Center of Nuclear theoretical {3., National Laboratory of Heavy Ion Accelerator of Lanzhou, Lan-zhou 73.000, china 3. Institute of theoretical {3., Chinese Academy of Sciences, Beijing 100080, china Correspondence should be addressed to Rong Jian (email: jrong@***) 1. china Institute of Atomic Energy 102413 Beijing China 2. Center of Nuclear theoretical physics National Laboratory of Heavy Ion Accelerator of Lanzhou 730000 Lanzhou China 3. Institute of theoretical physics Chinese Academy of Sciences 100080 Beijing China

The relativistic microscopic optical potential in the asymmetric nuclear matter is studied in the framework of the Dirac Brueckner-Hartree-Fock method. A new decomposition of the Dirac structure of the nuclear self-energy in nuclear matter is adopted. The self-energy of a nucleon with E > 0 in nuclear matter is calculated with the G matrix in the Hartree-Fock approach. The optical potential of a nucleon in the nuclear medium is identified with the nucleon self-energy. The energy and asymmetric parameter dependence of the relativistic optical potentials for proton and neutron are discussed. The resulting Schroedinger equivalent potentials have reasonable behaviors of the energy dependence. The asymmetric parameter dependence of relativistic optical potentials and Schroedinger potentials are emphasized.

关键词： Dirac Brueckner Hartree-Fock, relativistic microscopic optical potential, asymmetric nuclear matter, isospin-dependence.

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β-delayed proton decays near the proton drip line

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Science china(physics,Mechanics & Astronomy) 2005年第3期48卷 257-267页

作者： XU Shuwei 1 , LI Zhankui 1 , XIE Yuanxiang 1 , HUANG Wenxue 1 , SHU Nengchuan 2 , CHEN Yongshou 2 , XU Furong 3., WANG Kun 4 , PAN Qiangyan 1 , WANG Xudong 1 , YU Yong 1 & XING Yebing 1 1. Institute of Modern physics, Chinese Academy of Sciences, Lanzhou 73.000, china 2. Nuclear physics Department, china Institute of Atomic Energy, Beijing 102413. china 3. Department of Technical physics, Peking University, Beijing 100871, china 4. Shanghai Institute for Nuclear Research, Shanghai 201800, china 1. Institute of Modern physics Chinese Academy of Sciences 730000 Lanzhou China 2. Nuclear physics Department China Institute of Atomic Energy 102413 Beijing China 3. Department of Technical physics Peking University 100871 Beijing China 4. Shanghai Institute for Nuclear Research 201800 Shanghai China

We briefly reviewed the experimental study on a-delayed proton decays near the proton drip line published by our group during the period of 1996―2004, namely the first observation of the a-delayed proton decays of 9 new nuclides in the rare-earth region and the new measurements of a-delayed proton decays of 5 nuclides in the mass ～90 region near the N = Z line with the aid of the “p-?” coincidence in combination with a He-jet tape transport system. In the meantime some important experimental technique details were supplemented. The experimental results, including the half -lives, spins, parities, deformations and production reaction cross sections for the 14 nuclei were summarized and compared with the current nuclear-model predictions, and then the following points were represented. (1) The experimental half-lives for 85Mo and 92Rh as well as the predicted “waiting point” nuclei 89Ru and 93.d are 5―10 times longer than the theoretical predictions given by M?ller et al. using a macroscopic-microscopic model. It considerably influences the predictions of the abundances of the nuclides produced in the rp-process. (2) The current-model predictions are not consistent with the experimental assignments of the spins and parities for the proton drip-line nuclei 142Ho and 128Pm. However, the nuclear potential energy surface (PES) calculated by using a Woods- Saxon-Strutinsky method reproduced the experimental results. (3. The Alice code overestimated the production reaction cross sections of the studied 9 rare-earth nuclei by one order of magnitude or two, while HIVAP code overestimated them by one order of magnitude approximately.

关键词： proton drip line, β-delayed proton decay, He-jet tape transport system, "p-γ" coincidence, spin, parity, deformation, production reaction cross section.

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