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Total alkyl dibenzothiophenes content tracing the filling pathway of condensate reservoir in the Fushan Depression,South china Sea

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Science china Earth Sciences 2008年第S2期51卷 138-145页

作者： LI MeiJun1,WANG TieGuan1,LIU Ju2.ZHANG MeiZhu2.LU Hong3,MA QinLin2.& GAO LiHui2.1 State Key Laboratory of Petroleum Resources and Prospecting,Earth Sciences and Geoinformatics School,china University of Petroleum,Beijing 102.49,china 2.Southern Oil {2. and development Company,petrochina,Guangzhou 510640,china 3 Guangzhou institute of Geochemistry,Chinese Academy of Sciences,Guangzhou 5102.0,china china Univ Petr Earth Sci & Geoinformat Sch State Key Lab Petr Resources & Prospecting Beijing 102249 Peoples R China petrochina So Oil Explorat & Dev Co Guangzhou 510640 Peoples R China Chinese Acad Sci Guangzhou Inst Geochem Guangzhou 510240 Guangdong Peoples R China

The condensates are generally characterized by high maturity,low concentration of steranes and ter-panes biomarkers and low content of non-hydrocarbon fraction. In this case commonly used steranes,terpanes and carbazoles parameters cannot be effectively applied in the reservoir-filling tracing. The hydrogen bond formed by sulfur atom in the dibenzothiophenes (DBTs) results in molecule adsorption and fractionation during oil migration in reservoir. Like carbazoles,total DBTs content decreases with the increasing of oil migration distance. Therefore,a new parameter——total DBTs content is proposed to be used to trace the oil migration orientation and filling pathway. In present study,total DBTs con-tents of condensates and light oils are obtained by adding internal standard——eight deuterium atoms substituted DBT during Gas Chromatography-Mass Spectrometry analysis of aromatic fraction. Except for a few samples with much lower content of non-hydrocarbon fraction,the total DBTs content shows a fine positive correlation with that of carbazoles. Large errors can be caused in the process of pyrrolic nitrogen compounds separation. The application of this new parameter in the Fushan Depression of Beibu Gulf Basin,South china Sea indicates that this parameter is a reliable one to trace filling pathway in condensate reservoirs. Combined with other DBTs-related parameters,such as 4-/1-methydibenzo-thiophene and 2.4-/1,4-dimethyldibenzothiophene,oil migration orientation and filling pathway of the Fushan Depression was determined. The accumulations of Huachang oil field in the Fushan Depres-sion are mainly migrated and charged from northeast to southeast along the Huachang uplift. It can be predicated that the light oil and condensates in the Huachang oil field should be sourced from the source kitchen at the Bailian Sag. It shows that total DBTs content is an effective parameter to tracing oil migration orientation and filling pathway.

关键词： dibenzothiophene alkyl dibenzothiophene condensate reservoir filling pathway molecular markers the Fushan Depression

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Genetic types and distribution of shallow-buried natural gases

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Petroleum Science 2010年第3期7卷 347-354页

作者： Gao Yang Jin Qiang Zhu Guangyou College of Geo-resources and Information China University of Petroleum Dongying Shandong 257061 China Petroleum exploration and development {2. PetroChina Beijing 100083 China

Great volumes of shallow-buried （〈2.000 m） natural gases which are mainly composed of biogases and low-mature gases have been found in the Mesozoic-Cenozoic sedimentary basins in china. Many shallow gas reservoirs in china are characterized by coexistence of biogas and low-mature gas, so identifying the genetic types of shallow gases is important for {2. and development in sedimentary basins. In this paper, we study the gas geochemistry characteristics and distribution in different basins, and classify the shallow gas into two genetic types, biogas and low-mature gas. The biogases are subdivided further into two subtypes by their sources, the source rock-derived biogas and hydrocarbon-derived biogas. Based on the burial history of the source rocks, the source rock-derived biogases are divided into primary and secondary biogas. The former is generated from the source rocks in the primary burial stage, and the latter is from uplifted source rocks or those in a secondary burial stage. In addition, the identifying parameters of each type of shallow gas are given. Based on the analysis above, the distributions of each type of shallow gas are studied. The primary biogases generated from source rocks are mostly distributed in Quaternary basins or modem deltas. Most of them migrate in watersoluble or diffused mode, and their migration distance is short. Reservoir and caprock assemblages play an important role in primary biogas accumulation. The secondary biogases are distributed in a basin with secondary burial history. The oil-degraded biogases are distributed near heavy oil pools. The low-mature gases are widely distributed in shallow-buried reservoirs in the Meso-Cenozoic basins.

关键词： Primary biogas secondary biogas oil-degraded biogas low-mature gas genetic type gas identification gas accumulation distribution

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Isotopic compositions of small shelly fossil Anabarites from Lower Cambrian in Yangtze Platform of South china: Implications for palaeocean temperature

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Progress in Natural Science:Materials International 2007年第10期17卷 1185-1191页

作者： Chen Yongquan1,2. Jiang Shaoyong1, Ling Hongfei1, Yang Jinghong1 and Wan Defan3(1. State Key Laboatory for Mineral Deposits research and Center for Marine Geochemistry research, Department of Earth Sciences, Nanjing University, Nanjing 2.0093, {2. 2. Tarim Oilfield Company exploration & development research institute, Ku’erle 841000, {2. 3. institute of Mineral Resources, Chinese Academy of Geological Sciences, Beijing 100037, {2.) State Key Laboatory for Mineral Deposits research and Center for Marine Geochemistry research Department of Earth Sciences Nanjing University Nanjing 210093 China arim Oilfield Company exploration & development {2. institute Ku’erle 841000 China institute of Mineral Resources Chinese Academy of Geological Sciences Beijing 100037 China

Anabarites belong to small shelly fossils (SSF), which occur widely in the Lower Cambrian strata of Yangtze Platform in South china. They are phosphate shell in composition and represent the earliest stage of the Cambrian bioradiation of Bilateria, the so-called "Cambrian Explosion". In this study, we attempted to separate Anabarites fossils from Lower Cambrian dolostones, and we obtained samples of both the fossils (SSF) and the granular phosphates (GP). Isotopic analyses were performed on samples of SSF, GP, and matrix dolostone (DH-2.). The results showed that the δ30Si values of the quartz filling in fossils celoms, and the siliceous materials in granular phosphates are -0.6‰ and -0.7‰, which is different from normal sedimentary siliceous rocks from the Lower Cambrian strata (0—0.7‰) as reported by Li et al., but is consistent with the data for siliceous rocks and cherts of submarine hydrothermal origin. It is likely that a later hydrothermal replacement could have taken place in the SSF-bearing sedimentary rocks. The oxygen isotope values of the phosphate of SSF and GP are 16.8‰ and 17.0‰, respectively. These are significantly higher than the Neoproterozoic phosphate ores (10.9‰—13.9‰) as reported by Ling et al., hence, late diagenesis and hydrothermal replacement may not have caused a significant change in the oxygen isotope compositions of the small shelly fossils, and the calculated temperatures (2..4—2..3℃) for palaeo-seawater using a SSF phosphate oxygen isotope thermometer are therefore considered here as the upper limit of seawater temperature in the Early Cambrian ocean of the Yangtze Platform.

关键词： Anabarites oxygen isotope silicon isotope paleo-temperature.

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CHARACTERISTICS　OF　COAL－FORMED　GAS　ACCUMULATION　BELTS　IN　THE　EAST　PART　OF　THE　CENTRAL－ASIA　COAL－FORMED　GAS　ACCUMULATION　DOMAIN　──SERIES　STUDY　Ⅲ　ON　THE　CENTRAL－ASIA　COAL－FORMED　GAS　ACCUMULATION　DOMAIN

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石油勘探与开发 1995年第5期22卷 87-95页

作者： Dai Jin-xing Li Xian-qi(research institute of Petroleum {2. and development, CNPC. Beijing, 100083, P. R. china)

ＣＨＡＲＡＣＴＥＲＩＳＴＩＣＳＯＦＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＢＥＬＴＳＩＮＴＨＥＥＡＳＴＰＡＲＴＯＦＴＨＥＣＥＮＴＲＡＬ－ＡＳＩＡＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＤＯＭＡ... 详细信息

ＣＨＡＲＡＣＴＥＲＩＳＴＩＣＳＯＦＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＢＥＬＴＳＩＮＴＨＥＥＡＳＴＰＡＲＴＯＦＴＨＥＣＥＮＴＲＡＬ－ＡＳＩＡＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＤＯＭＡＩＮ──ＳＥＲＩＥＳＳＴＵＤＹⅢＯ...

关键词： GAS FORMED COAL ACCUMULATION BELTS ASIA EAST

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Hydrocarbon test in lower-layer atmosphere to predict deep-sea petroleum or hydrate in the Okinawa Trough: an example

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Acta Oceanologica Sinica 2003年第4期22卷 569-576页

作者： Gong Jianming1, Chen Jianwen 1, 2. Li Gang1, Zhang Xunhua1, Li Jipeng3, Huang Fulin1 1. Qingdao institute of Marine Geology, Qingdao 2.6071, china. 2. Ocean University of china, Qingdao 2.6003, china 3. Hefei institute of Petroleum Chemical exploration, china Petroleum exploration and development research institute, Hefei 2.002.,china Qingdao Inst Marine Geol Qingdao 266071 Peoples R China Ocean Univ china Qingdao 266003 Peoples R China china Petr Explorat & Dev Res Inst Hefei Inst Petr Chem Explorat Hefei 230022 Peoples R China

Light hydrocarbon (methane, ethane, propane, butane and CO2. test and C isotopic analysis of CO are conducted for over 100 lower-layer atmospheric samples from the East china Sea slope and the Okinawa Trough. The results show that the lower-layer atmosphere mainly consists of CO2.and then of CH4, and the CO2.concentrations are calculated to have a high average value of 0.87 omega/10(-2. about three times that of the regional background (0-3 omega/10(-2.). The result also shows that the average value of C isotope - 2..8 x 10(-3) is given to the CO2. inferring that it is inorganic gas. Thus, for the future 's work in the Okinawa Trough, special attention should be paid to CO2.hydrate, which is very possibly an important hydrate type.

关键词： lower-layer atmosphere hydrocarbon test C isotopic analysis deep-sea petroleum gas hydrate

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A hydrocarbon enrichment model and prediction of favorable accumulation areas in complicated superimposed basins in china

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Petroleum Science 2010年第1期7卷 10-19页

作者： Pang Xiongqi Meng Qingyang Jiang Zhenxue Liu Luofu Lu Xiuxiang State Key Laboratory of Petroleum Resources and Prospecting China University of Petroleum Beijing 102249 China Basin and Reservoir research Center China University of Petroleum Beijing 102249 China research institute of Petroleum {2. and development PetroChina Beijing 100083 China

The geologic conditions of superimposed basins in china are very complicated. This is mainly shown by multi-phase structural evolution, multiple sets of source-reservoir-cap rock combinations, multiple stages of hydrocarbon generation and expulsion from source rocks, multi-cycle hydrocarbon enrichment and accumulation, and multi-phase reservoir adjustment and reconstruction. The enrichment, accumulation and distribution of hydrocarbon is mainly controlled by the source rock kitchen, paleo- anticline, regional cap rock and intensity of tectonic movement. In this paper, the T-BCMS model has been developed to predict favorable areas of hydrocarbon accumulation in complicated superimposed basins according to time and spatial relationships among five key factors. The five factors include unconformity surface representing tectonic balancing （B）, regional cap rock representing hydrocarbon protection （C）, paleo-anticline representing hydrocarbon migration and accumulation （M）, source rock kitchen representing hydrocarbon generation and expulsion （S） and geological time （T）. There are three necessary conditions to form favorable areas of hydrocarbon accumulation. First, four key factors BCMS should be strictly in the order of BCMS from top to bottom. Second, superimposition of four key factors BCMS in the same area is the most favorable for hydrocarbon accumulation. Third, vertically ordered combination and superimposition in the same area of BCMS should occur at the same geological time. The model has been used to predict the most favorable exploration areas in Ordovician in the Tarim Basin in the main hydrocarbon accumulation periods. The result shows that 95% of the discovered Ordovician hydrocarbon reservoirs are located in the predicted areas, which indicates the feasibility and reliability of the key factor matching T-BCMS model for hydrocarbon accumulation and enrichment.

关键词： Complicated superimposed basin key factor matching T-BCMS model favorable area for hydrocarbon accumulation hydrocarbon distribution prediction

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THE CHARACTERISTICS OF REMOTE SENSING TECTONICS IN QIANGTANG-CHANGDU MASSIF, QINGHAI-TIBET PLATEAU

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地学前缘 2000年第S1期7卷 435-437页

作者： Zhao Zhengzhang 1,Ye Hefei 2.Li Yongtie 2.1 china National Petroleum Corporation, Beijing 10072.,china {2. institute of Petroleum exploration and development, CNPC, Beijing 100083,china)

The northern Tibet plateau is the core of generalized Qinghai—Tibet plateau. The main part of Qiangtang—Changdu massif, which is 45×10 4km 2.and more than 5000m in altitude, conforms to the northern Tibet plateau in area.1 The shape features and boundary conditions of Qiangtang—Changdu massif\;(1) Qiangtang—Changdu massif shows huge flat\|lying “S” area In MSS7 mosaic image, Qiangtang—Changdu massif extends in west and east, and appears a long\|elliptic huge block composed of feathered and dendritic textures.. Noticeably, there are two similar texture “tails" in the west and east ends of the massif. The western tail turns and constringes to the north, and eastern tail to the south. Thereby, the massif shows huge “S" area. According to the regional analysis, the eastern tail locates between Shaluli Mt.\|Taniantaweng Mt. and Mujiang River, and western part through Bangong\|Co connects with Pamirs along Karakoram Mt. In regional tectonics, the massif locates between Lazhulong\|Xijinwulan\|Co\|Jinshajiang River and Bangong\|Co\|Dongqiao\|Nujiang River fault belts.

关键词： Qiangtang—Changdu massif remote sensing boundary condition circular structure deformin g features mechanic characteristic dynamics

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Formation mechanism and geochemical characteristics of shallow natural gas in heavy oil province,china

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Science china Earth Sciences 2008年第S1期51卷 96-106页

作者： ZHU GuangYou,ZHANG ShuiChang,ZHAO WenZhi,WANG ZhengJun,LIANG YingBo, ZHAO XueFeng&ZHANG JingYan petrochina Oil Geologic Lab Center,research {2.s of petrochina exploration and development,Beijing 100083,china petrochina Oil Geol Lab Ctr Res Inst PetroChina Explorat & Dev Beijing 100083 Peoples R China

Shallow gas reservoirs are distributed widely in Chinese heavy oil-bearing *** present,shallow gas resources have opened up giant *** previous researches indicate the intimate genetic relationship between shallow gas and heavy *** gas resources are generated from crude oil degraded by anaerobic microscopic organism,it belongs to biogenic gas family of secondary genesis, namely heavy oil degraded *** gas resources are usually distributed in the upward position or the vicinity of heavy oil *** are mainly of dry gas,which are composed of methane and only tiny C2.+ heavy hydrocarbon and relatively higher contents of nitrogen ***,methane isotopes are light,whose values are between biogenic gas and thermal cracking *** isotopes are heavy,which mixed possibly with thermogenic *** dioxide bear the characteristics of very heavy carbon isotope,so carbon isotopic fractionation effects are very obvious on the process of microscopic organism degradation crude *** heavy oil degraded gas formation,a very complex geological,geochemical and microbiological geochemical process,is the result of a series of reactions of organic matter-microbes and water-hydrocarbon,which is controlled by many factors.

关键词： heavy oil degraded gas shallow gas heavy oil biogenic gas anaerobic degradation

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TTHE METHODOLOGY OF PETROLEUM development GEOLOGY(Ⅲ)

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石油勘探与开发 1996年第4期 78-82页

作者： Qiu Yinan (research institute of Petroleum {2. and development, CNPC, Beijing, 100083, P.R.china)

ＴＨＥ　ＭＥＴＨＯＤＯＬＯＧＹ　ＯＦ　ＰＥＴＲＯＬＥＵＭ　ＤＥＶＥＬＯＰＭＥＮＴ　ＧＥＯＬＯＧＹ（Ⅲ）ＴＨＥＭＥＴＨＯＤＯＬＯＧＹＯＦＰＥＴＲＯＬＥＵＭＤＥＶＥＬＯＰＭＥＮＴＧＥＯＬＯＧＹ（Ⅲ）￥ＱｉｕＹｉｎａｎ（Ｒ...

ＴＨＥ　ＭＥＴＨＯＤＯＬＯＧＹ　ＯＦ　ＰＥＴＲＯＬＥＵＭ　ＤＥＶＥＬＯＰＭＥＮＴ　ＧＥＯＬＯＧＹ（Ⅲ）ＴＨＥＭＥＴＨＯＤＯＬＯＧＹＯＦＰＥＴＲＯＬＥＵＭＤＥＶＥＬＯＰＭＥＮＴＧＥＯＬＯＧＹ（Ⅲ）￥ＱｉｕＹｉｎａｎ（ＲｅｓｅａｒｃｈＩｎｓｔｉｔｕｔｅｏ...

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Stratigraphic thermohistory and its implications for regional geoevolution in the Tarim Basin,NW china

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Science china Earth Sciences 2010年第10期53卷 1495-1505页

作者： WANG TieGuan1,DAI ShiFeng2.LI MeiJun1,ZHANG WeiBiao1,3,Qiu NanSheng1 & WANG GuangLi1 1 State Key Laboratory of Petroleum Resources and Prospecting,china University of Petroleum,Beijing 102.49,china 2.State Key Laboratory of Coal Resources & Safe Mining,china University of Mining & Technology,Beijing 100083,china 3 exploration research Center,exploration & development institute,china Petrochemical Corporation,Beijing 100083,china 1. State Key Laboratory of Petroleum Resources and Prospecting China University of Petroleum Beijing 102249 China2. State Key Laboratory of Coal Resources & Safe Mining China University of Mining & Technology Beijing 100083 China3. Exploration Research Center Exploration & Development Institute China Petrochemical Corporation Beijing 100083 China

Fourteen vitrinite reflectance profiles from the Tarim Basin,NW china,show that the vitrinite reflectance profiles of individual wells follow a faulted and dislocated dual-stage pattern in the eastern section of the Tazhong Uplift and in the Tabei *** reflectance values in these profiles change sharply at the unconformity beneath the Lower Carboniferous Bachu or Upper Devonian Donghetang Formations,where the overlying Triassic to Carboniferous strata are still in a mature phase within the "liquid oil window".However,the underlying Lower Paleozoic reached the overmature phase beyond the "liquid oil window" towards the end of the Silurian,or in the Early Devonian at the *** the vitrinite reflectance profiles are attributed to a continuous,single-stage pattern in the western section of the Tazhong Uplift,in which the Lower Paleozoic is also in an overmature phase,their overmaturity would have been achieved relatively late in geological *** stratigraphic thermohistory has the following implications to regional geoevolution:(1) The overmature Lower Ordovician to Cambrian strata in the eastern section of the Tazhong Uplift and in the Tabei Uplift,as well as in the Manjiaer Depression,could not have acted as the source kitchen for normal oil(so-called black oil);(2. The dissimilarity in vitrinite reflectance profiles between the eastern and western sections of the Tazhong Uplift reveals Early Paleozoic paleotectonic features,i.e.,lower at the east and higher at the west,whereas recent tectonic features formed since the Late Paleozoic are in reverse,i.e.,higher in the east and lower at the west;(3) Reconstruction of the denuded thickness of sediments overlying the Lower Ordovician strata suggests reconsideration on the paleotectonic features in the Tarim Basin;(4) Based on the sustained duration of the "liquid oil window" for overmature source beds,it is predicted that the Suntuoguole Lower Uplift between the Awati and Manjiaer Depressions is a

关键词： vitrinite reflectance profile faulted and dislocated dual-stage pattern paleotectonic features sustained "liquid oil window" period source kitchen

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