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PREPARATION OF BISPHENOL A EPOXY RESIN WATERBORNE DISPERSIONS BY THE PHASE INVERSION EMULSIFICATION TECHNIQUE

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chinese Journal of Polymer Science 2000年第1期18卷 33-38页

作者： Zhen-zhong Yang De-lu Zhao Polymer physics laboratory, Institute of Chemistry, {2., {3., China 中科院化学所高分子物理及化学国家重点实验室北京

The phase inversion emulsification technique (PIET) is an effective physical method for preparing waterborne dispersions of polymer resins. Some results concerning the preparation of bisphenol A epoxy resin waterborne dispersions by PIET in our laboratory were summarized. Electrical properties, rheological behavior and morphological evolution during phase inversion progress were systematically characterized. The effects of the emulsifier concentration and emulsification temperature on phase inversion progress and the structural features of the waterborne particles were studied as well. The deformation and break up of water drops in a shear field were analyzed in terms of micro-theology, while the interaction and coalescence dynamics of water drops were discussed in terms of DLVO theory and Smoluchowski effective collision theory, respectively. Based on the experimental results and theoretical analysis, a physical model of phase inversion progress was suggested, by which the effects of the parameters on phase inversion progress and the structural features of the waterborne particles were interpreted and predicted.

关键词： phase inversion emulsification waterborne dispersions epoxy resin mechanism physical model

A new DNA algorithm to solve graph coloring problem

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Progress in Natural Science:Materials International 2007年第6期17卷 733-738页

作者： Jiang Xingpeng1, Li Yin2. Meng Ya3.and Meng Dazhi2.1. national {2. of Pattern Recognition,Institute of Automation, {2., {3., China 2. College of Applied sciences, beijing University of Technology, beijing 10002., China 3. School of Science, beijing Institute of Technology, beijing 100081, China) national laboratory of Pattern Recognition Institute of Automation Chinese Academy of Sciences Beijing 100080 China College of Applied sciences Beijing University of Technology Beijing 100022 China School of Science Beijing Institute of Technology Beijing 100081 China

Using a small quantity of DNA molecules and little experimental time to solve complex problems successfully is a goal of DNA computing. Some NP-hard problems have been solved by DNA computing with lower time complexity than conventional computing. However, this advantage often brings higher space complexity and needs a large number of DNA encoding molecules. One example is graph coloring problem. Current DNA algorithms need exponentially increasing DNA encoding strands with the growing of problem size. Here we propose a new DNA algorithm of graph coloring problem based on the proof of four-color theorem. This algorithm has good properties of needing a relatively small number of operations in polynomial time and needing a small number of DNA encoding molecules (we need only 6R DNA encoding molecules if the number of regions in a graph is R).

关键词： DNA computing NP-hard problem graph coloring problem.

Narrow line Seyfert 1 galaxies: where are the broad line regions?

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Science China(physics,Mechanics & Astronomy) 2010年第12期53卷 2307-2311,2339-2343页

作者： MAO WeiMing 1,2.3., HU Chen 2., WANG JianMin 2., BIAN WeiHao 4 , ZHANG Shu 2.& ZHAO Gang 1 1 Key laboratory of Optical Astronomy, {2. Astronomical Observatories, {2., {3. 100012. China 2.Key laboratory for Particle Astrophysics, Institute of High Energy physics, {2., {3. 100049, China 3.Graduate University of the {2., {3. 100049, China 4 Department of physics, Nanjing Normal University, Nanjing 2.0011, China Key laboratory of Optical Astronomy National Astronomical Observatories Chinese Academy of Sciences Beijing China Key laboratory for Particle Astrophysics Institute of High Energy Physics Chinese Academy of Sciences Beijing China Graduate University of the chinese academy of sciences Beijing China Department of physics Nanjing Normal University Nanjing China

A sample consisting of 2.1 narrow line Seyfert 1 galaxies (NLS1s) with high quality spectra from the Sloan Digital Sky Survey (SDSS) is selected to explore where broad line regions are in these objects. We find that the Hβ profile can be fitted well by three (narrow, intermediate and broad) Gaussian components, and the FWHM ratios of the broad to the intermediate components hold a constant of 3.0 roughly for the entire sample. If the broad components originate from the region scaled by the well-determined Hβ reverberation mapping relation, we find that the intermediate components originate from the inner edge of the torus, which is scaled by dust K-band reverberation. We find that the IC and the BC are strongly linked dynamically, but the relation of their covering factors is much more relaxed, implying that both regions are clumpy.

关键词： black hole physics galaxies: evolution quasars: general

Fluorescence dynamics of interactions between polyamide PyPyPyβDp and DNA

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Science China Chemistry 2006年第1期49卷 75-80页

作者： ZHANG Huijuan1,2. WANG Jin3. WU Yishi1, YUAN Gu3. AI Xicheng1, WANG Li4 & ZHANG Jianping1 1. State Key {2. for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, chinese academy of sciences, {2., China 2. School of Life Science and Technology, {3. Institute of Technology, {3. 100081, China 3. College of Chemistry and Molecular Engineering, Peking University, {2., China 4. Center for Condensed matter physics, Institute of physics, chinese academy of sciences, {2., China Correspondence should be addressed to Ai Xicheng and Zhang Jianping State Key laboratory for Structural Chemistry of Unstable and Stable Species Institute of Chemistry Chinese Academy of Sciences Beijing China School of Life Science and Technology Beijing Institute of Technology Beijing China College of Chemistry and Molecular Engineering Peking University Beijing China Center for Condensed matter physics Institute of Physics Chinese Academy of Sciences Beijing China

The photophysical properties of the polyamide PyPyPyβDp (PPP) were investigated by means of steady-state absorption and fluorescence spectroscopies, as well as time-resolved fluo-rescence spectroscopy. It was found that the excited-state properties of PPP are very sensitive to solvents. In TKMC buffer PPP exhibited weak fluorescence with a decay time constant of 16 ps, while with the decrease of the solvent polarity PPP showed the blue-shifted peak position, increased inten-sity and lengthened life-time for its fluorescence behavior. In the presence of calf thymus DNA, it was observed that the fluorescence intensity was enhanced and the fluorescence lifetime increased from 16 to 3. ps for PPP, which verified that PPP bound into the minor groove of DNA duplex.

关键词： polyamide (PPP), calf thymus DNA (ctDNA), time-resolved fluorescence spectroscopy, recognition dynamics.

Discovery of immune related factors in Fenneropenaeus chinensis by annotation of ESTs

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Progress in Natural Science:Materials International 2004年第1期14卷 48-55页

作者： SHEN Yaoqing 1,2. , XIANG Jianhai 1*, WANG Bing 1,2. , LI Fuhua 1 and TONG Wei 3.1. Experimental Marine Biology laboratory, Institute of Oceanology, {2., Qingdao 2.6071,China 2. Graduate School of the {2., {3. 10003., China 3. Genomics & Bioinformatics Institute, {2., {3. 1013.0, China) chinese Acad Sci Inst Oceanol Expt Marine Biol Lab Qingdao 266071 Peoples R China chinese Acad Sci Grad Sch Beijing 100039 Peoples R China chinese Acad Sci Geonom & Bioinformat Inst Beijing 101300 Peoples R China

A total of 10446 expressed sequence tags (ESTs) are obtained by a large scale sequencing of a cDNA library from cephalothorax of adult Fenneropenaeus chinensis . An EST analysis platform was built up based on local computers and bioinformatic techniques were used to annotate these ESTs in order to promptly find possible functional genes, especially for immune related factors. About 4% of the ESTs show similarity to the coding sequences of such factors, including lectin, serine protease, serpin, lysozyme, etc. These ESTs provide a partial profile of the immune system in F. chinensis and useful information for further study on these genes.

关键词： Fenneropenaeus chinensis bioinformatics ESTs immune factors

Application of the moist vorticity vector in the analysis of a heavy rainfall event in North China

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Progress in Natural Science:Materials International 2007年第12期17卷 1457-1465页

作者： Zhao Yu1,2.3. Wang Jianguo4 and Xue Deqiang2.1. laboratory of Cloud-Precipitation {2. and Severe Storms, Institute of Atmospheric {2., {3., beijing 10002., China 2. Shandong Provincial Meteorological Observatory, Jinan 2.003., China 3. Graduate University of {3., beijing 10003., China 4. Shandong Provincial Meteorological Bureau, Jinan 2.003., China) laboratory of Cloud-Precipitation physics and Severe Storms Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China Shandong Provincial Meteorological Observatory Jinan 250031 China Graduate University Chinese Academy of Sciences Beijing 100039 China Shandong Provincial Meteorological Bureau Jinan 250031 China

The moist vorticity vector (MVV), defined as (ζa×▽qv)/ρ introduced by Gao et al. is used to study a heavy rainfall event in North China. The MVV has zonal, meridional and vertical components in a three-dimensional framework. Analysis of domain-mean and mass-integrated quantities shows that the variation of the vertical component of the MVV closely follows the variation of the cloud hydrometeors, with a linear correlation coefficient of 0.95, indicating that the vertical component of the MVV is strongly associated with midlatitude convection. Further analysis shows that the vertical component of the MVV reflects the interaction between the horizontal vorticity and the horizontal specific humidity gradient, which can associate dynamic and thermodynamic processes with cloud microphysical processes. Thus, this study can help to understand how the interaction between circulations and clouds aids the development of convection, and the MVV can be used to trace the development and evolution of heavy rainfall.

关键词： moist vorticity vector heavy rainfall modeling study.

Interfacial behaviors of PMMA-PEO block copolymers at the air/water interface

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Science China Chemistry 2005年第6期48卷 567-573页

作者： CHENG Caixia1, JIAO Tifeng2. TANG Rupei1, LIU Minghua2.& XI Fu1 1. State Key laboratory of Polymer physics and Chemistry, Joint laboratory of Polymer Science and Materials, Institute of Chemistry, {3., beijing 100080, China 2. CAS Key laboratory of Colloid and Interface Science, Institute of Chemistry, {3., beijing 100080, China State Key laboratory of Polymer physics and Chemistry Joint Laboratory of Polymer Science and Materials Institute of Chemistry Chinese Academy of Sciences Beijing China CAS Key laboratory of Colloid and Interface Science Institute of Chemistry Chinese Academy of Sciences Beijing China

Diblock copolymer of PMMA2.1-b-PEO114 and triblock copolymer of PMMA12.-b- PEO2.7-b-PMMA12. were synthesized and their interfacial properties at the air-water interface were investigated, where both blocks of polyethylene oxide (PEO) and poly(methyl methacrylate) (PMMA) are surface active but the former is soluble in water while the latter is not. Both the block copolymers could form monolayers with two obvious transition regions. The first transition point is around 10 mN/m, which could be assigned to the pancake-brush change of the PEO chains. The other is around 18 mN/m, which could be ascribed to the condensed packing of PMMA. The surface morphological changes during the compression of the Langmuir monolayers are inves-tigated by using the AFM and SEM methods for the films deposited at different surface pressure or molecular areas. At a lower surface pressure, a typical morphology of PEO-con- taining lipopolymers is observed. Upon compression, sphere-dominant morphologies were observed. While the diblock copolymer is easy to folding, the triblock copolymer is in favor of formation of circular domains through vesiculation.

关键词： PMMA-PEO, block copolymers, monolayer, Langmuir-Blodgett films, AFM.

Geometry of Broad Line Regions of Active Galactic Nuclei

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chinese Journal of Astronomy and Astrophysics 2008年第1期8卷 50-62页

作者： Xiao-Rong Lü1 Key laboratory for Particle Astrophysics, Institute of High Energy physics, {3., beijing 100049 2.Graduate School of {3., beijing 100049 Key laboratory for Particle Astrophysics Institute of High Energy Physics Chinese Academy of Sciences Beijing 100049 Graduate School of chinese academy of sciences Beijing 100049

It has long remained an open question as to the geometry of the broad line region （BLR） in active galactic nuclei （AGNs）. The reverberation mapping technique which measures the response of the broad emission lines to the ionizing continuum, when combined with multiwavelength continuum fitted by sophisticated accretion disks, provides a way of probing the BLR geometry. We analyze a sample of 3. AGNs, which have been monitored by the reverberation mapping campaign. In view of energy budget, the reverberation-based BH masses are found to be in agreement with those obtained by accretion disk models in two thirds of the present sample while the reverberation mapping methods underestimate the BH masses in about one third of objects, as also suggested by CoUin et al. in a recent work. We point out that there are obviously two kinds of BLR geometry, which are strongly dependent on the Eddington ratio, and separated by the value LBol/LEdd - 0.1. These results prefer a scenario of the disk and wind configuration of the BLR and identify the Eddington ratio as the physical driver regulating the wind in the BLR.

关键词： accretion, accretion disks - galaxies active - galaxies Seyfert - quasars general

The gravity wave instability induced by photochemistry in summer polar mesopause region

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chinese Science Bulletin 2000年第3期45卷 267-272页

作者： Center for Space Science and Applied Research, chinese academy of sciences, beijing 100080, China {2. of Numeric Study of Heliospheric {3., chinese academy of sciences, beijing 100080, China Center for Space Science and Applied Research Chinese Academy of Sciences Beijing China laboratory of Numeric Study of Heliospheric physics Chinese Academy of Sciences Beijing China

The effect of diabatic process due to the photochemical heating and cooling on the gravity wave propagation in middle atmosphere is studied. A linear gravity wave model which considers the diabatic process is established. The unstable region and the growth rate of the gravity wave caused by photochemistry are calculated. And the comparison between the model and the adiabatic gravity wave theory of pure dynamics is made. The results indicate that the photochemical heating process can induce the instability of gravity wave at mesopause. The intensity of the instability becomes stronger as the temperature decreases. The temperature feature and the altitude characteristics of the instability are consistent with the observation. Therefore, the instability of the gravity wave induced by photochemistry may be an important mechanism in polar mesopause region in summer.

关键词： photochemistry instability gravity wave growth rate.