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Pollution characteristics of atmospheric fine particles and their secondary components in the atmosphere of Shenzhen in summer and in winter

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Science china Chemistry 2006年第5期49卷 466-474页

作者： NIU Yuwen1,2.HE Lingyan1,2.HU Min2.ZHANG Jing2.& ZHAO Yunliang2.1. Shenzhen graduate School of Peking university,Shenzhen 518055,{2. 2. State Joint Key Laboratory of Environmental Simulation and Pollution Control,College of Environmental Sciences,Peking university,beijing 100871,{2. 1. Shenzhen graduate School of Peking university Shenzhen 518055 China 2. State Joint Key Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences Peking University Beijing 100871 China

Two field measurements for atmospheric fine particles were conducted in Baoan district of Shenzhen during the summer and winter in 2.04. Totally 30 sets of 2. h samples were collected, and then the mass concentrations and chemical compositions were determined. The seasonal varia- tions and secondary pollution characteristics of fine particles during the sampling periods were dis-cussed with meteorological factors. The results show that seasonal variations of atmospheric particles are significant in Shenzhen. The average mass concentrations of PM2.5 and PM10 in summer were 35 μg·m-3 and 57 μg·m-3, respectively, and those in winter were 99 μg·m-3 and 135 μg·m-3, respec-tively. The concentrations of both PM2.5 and PM10 in winter increased 184% and 137%, respectively, compared to those in summer. PM2.5 accounted for 61% and 75% of PM10 in summer and in winter, respectively, indicating severe fine particle pollution in Shenzhen. During the summer and winter sampling periods, the mean OC/EC ratios were 3.4 and 1.6, respectively. The estimated secondary organic carbon (SOC) averagely accounted for 56% and 6% of the total OC in summer and in winter, respectively, which implies a major contribution of SOC to OC in summer. During the continuous high temperature period in summer, both the concentrations and fractions of secondary aerosol compo-nents in PM2.5 were highly elevated, suggesting severe secondary pollution again. The prevailing wind was from South china Sea in summer, and the air quality was good. The prevailing wind in winter was from china's Mainland to the north, and the polluted air mass led to poor air quality.

关键词： PM2.5, mass concentration, secondary pollution, seasonal variation, Shenzhen.

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Adjoint method for the optimum planning of industrial pollutant sources

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Science china Earth Sciences 2005年第8期48卷 1270-1279页

作者： LIU Feng1,2. HU Fei2.& ZHU Jiang2.1. College of Environmental Sciences, Peking university, beijing 100871,{2. 2. LAPC, Institute of Atmospheric Physics, Chinese Academy of Sciences, beijing 10002.,{2. 1. College of Environmental Sciences Peking University 100871 Beijing China 2. LAPC Institute of Atmospheric Physics Chinese Academy of Sciences 100029 Beijing China

The optimum planning of industrial pollutant sources, which optimizes the economic object without violating environmental constraints, is an important and hard task to be conquered. In this paper, an adjoint method is developed to solve the problem. The penalty function is in-troduced to deal with the environmental inequality constraints, and Lagrange function is con-structed to derive the adjoint equation and the gradient of the object function. In this means, the gradient of the object function can be calculated by solving the adjoint equation, and the infor-mation from the gradient is used to make the object function descend and approach to an optimal solution after some iterations. A two-dimensional, simplified model is used for numerical experi-ments. The theoretical derivations are verified by the results of the experiments. Furthermore, the adjoint method is shown to be of excellent convergence and efficiency, which is adaptive to the fast development of air quality numerical models and super computers.

关键词： optimum planning, industrial pollutant sources, adjoint equation, penalty function, gradient.

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The study of two-color excitation upconversion of Pr(0.5)Yb(3):ZBLAN

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Science china(Physics,Mechanics & Astronomy) 2006年第2期49卷 169-177页

作者： CHEN Xiaobo1 & SONG Zengfu2.1. Applied Optics beijing Area Major Laboratory, Analysis and testing center, beijing Normal {2., beijing 100875, china 2. Peking {2., Physics School, beijing 100871, china Applied Optics beijing Area Major Laboratory Analysis testing center Beijing Normal University Beijing 100875 China Physics School Peking University Beijing 100871 China

The excited state absorption upconversion of Pr(0.5)Yb(3):ZBLAN glass material, under two-color excitation of the 960 nm semiconductor laser and the Xe lamp light simultaneously, is reported in this article. It was found that the upconversion emission spectra of 480.1, 519.0, 601.9 and 631.8 nm coincide with the common emission spectra. Meanwhile, the upconversion-excitation spectrum has three obvious peaks under two-color excitation, and they respectively correspond to the 856.0 nm upconversion ex-citation transition [1G4(Pr3+)→1I6(Pr3+) and 1G4(Pr3+)→3P1(Pr3+)], the 789.0 nm upconver-sion excitation transition 1G4(Pr3+)→3P2.Pr3+), and the 803.7 nm upconversion excitation transition 3H6(Pr3+)→1D2.Pr3+). The upconversion excitation transition 1G4(Pr3+)→1I6(Pr3+) is strong because its oscillator strength f = 2..040×10?6 is large, which results in a large peak appearing in the upconversion excitation spectrum. That is just the new interesting two-color excitation upconversion luminescence phenomenon of Pr(0.5)Yb(3):ZBLAN induced by one laser and one continuous normal light simultaneously.

关键词： upconversion volumetric three-dimensional display two-color excitation.

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Explanation of the mechanism of carcinogenesis and syntheses of anticancer agents with high selectivity

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Science china Chemistry 2006年第1期49卷 44-62页

作者： DAI Qianhuan1,2.1. Center of Chemistry and Bioengineering of Cancer Research, beijing Polytechnic university (Now known as beijing Univer-sity of Technology), beijing 10002., china 2. Center of Environmental Sciences, Peking university, beijing 100871, china 1. Center of Chemistry and Bioengineering of Cancer Research Beijing Polytechnic University Beijing 100022 China 2. Center of Environmental Sciences Peking University Beijing 100871 China

In 1979, the mechanism of chemical carcinogenesis, a challenging anddifficult scientific problem pending for a number of years, was explained by Dai Qianhuan. Themechanism named di-region theory predicted that a carcinogen always metabolizes to form a specialbi-functional alky-lating agent. This agent induces cross-linkages between the complementary basepairs in DMA and switches on initial mutageneses in genomes including point and frameshiftmutations. This, in turn, induces further deep mutageneses including the production of variouschimeric chromosomes, deletions and other aberrations found in genomes. In the end this initiatescarcinogenesis of the whole cell through the reverse transcription mechanism after a lengthyincubation period. Recently, this laboratory has verified that physical carcinogenesis, includingthe oncogenesis induced by radiation and asbestos as well as the carcinogenesis induced byendogenous factors such as estrogen or diethyl-stilbestrol switch on carcinogenesis by inducing theformation of cross-linkages between the complementary base pairs in DNA. Di-region theory has nowbeen supported by many experimental observations such as mutational spectra of various *** potential for carcinogenesis, teratogenesis, sterility and mutagenesis lumped together asgenetic toxicity appears to originate almost uniformly from the cross-linking between complementarybases, i.e. malignant cross-linking, which is in accordance with di-region theory. Other forms ofcross-linking between non-complementary bases, benign cross-linkings, show bi-functional alkylationanticancer activity but lack genetic toxicity. The predictable design and synthesis of a highselectivity anticancer agent with high efficacy and low genetic toxicity, a goal long pursued incancer chemotherapy, have been realized for the first time in this laboratory by inhibitingmalignant and heightening benign cross-linking using the principles of di-region theory. A series ofpatented new anticanc

关键词： mechanism of carcinogenesis, di-region theory, minoplatin, selectivity of anticancer agent, cross-linking between DNA bases, anticancer platinum complexes, predictive design of anticancer agent, second generation anticancer agent.

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Inertial theory of the mean Hadley circulation under the condition of nonstatic equilibrium

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Science china Earth Sciences 2006年第5期49卷 546-553页

作者： CHAO Jiping1 & LIU Fei2.3 1. National Marine Environmental Forecasting Center, beijing 100081, china 2. Key Laboratory Regional Climate-Environment for Temperate East Asia, Institute of Atmospheric Physics, Chinese Academy of Sciences, beijing 10002., china 3. graduate university of Chinese Academy of Sciences, beijing 100049, china 1. National Marine Environmental Forecasting Center Beijing 100081 China 2. Key Laboratory Regional Climate-Environment for Temperate East Asia Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China 3. graduate university of Chinese Academy of Sciences Beijing 100049 China

Tropical atmosphere is divided into two layers, the layer near the ground is the planet boundary layer, where the motion is linear, if the radiation equilibrium temperature is given at the top of the boundary layer, the vertical motion there can be obtained. It is the non-viscous ideal atmos- pheric layer above the boundary one, where the motion is nonlinear. After getting the conservation laws of angular momentum, potential temperature and potential vortex, the inertial theory of the Hadley circulation driven by the vertical motion of the boundary layer is established, followed by sev- eral examples of its application.

关键词： Hadley circulation, inertial theory, conservation laws of angular momentum, potential temperature and potential vortex.

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Fluorescence fluctuation spectroscopy and its artifacts:simulations and tests

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Science china(Physics,Mechanics & Astronomy) 2005年第3期48卷 336-344页

作者： MENG Fanbo 1 , CHEN Bo 1 , LIU Guang 1 , DING Jianying 1 & MA Hui 2.1 1. Department of Physics and Key Laboratory of Atomic and Molecular Nano Sciences, Ministry of Educa- tion, Tsinghua university, beijing 100084,{2. 2. graduate School at Shenzhen, Tsinghua university, Shenzhen 518055,{2. 1. Department of Physics and Key Laboratory of Atomic and Molecular Nano Sciences Ministry of Education Tsinghua University 100084 Beijing China 2. graduate School at Shenzhen Tsinghua University 518055 Shenzhen China

Fluorescence fluctuation spectroscopy (FFS) technique is capable of monitoring changes in concentration, mass, size and structure of fluorescent-labeled bio-molecules in microscopic volume and is suitable for measuring biological interactions in living cells. FFS data may be affected by many experimental factors in complicated biological systems. Using a Monte Carlo approach, we generate fluorescence fluctuation data for different experimental systems. This approach helps to separate the contributions by different experimental factors in a complicated fluorescence fluctuation spectrum. It also helps to validate new theoretical models and new fitting formulations. We describe the algorithm of the simulation program and tests on its statistical performance. The program is then used successfully to study the effects of several experimental factors on FFS detection.

关键词： fluorescence fluctuation spectroscopy, fluorescence correlation spectroscopy, Monte Carlo simulation.

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Nonlinear interactions between gravity waves and background winds

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Progress in Natural Science:Materials International 2007年第6期17卷 639-644页

作者： Liu Xiao1,2.and Xu Jiyao1(1. State Key Laboratory for Space Weather, Center for Space Science and Applied Research, Chinese Academy of Sciences, beijing 100080, china 2. {2. university of Chinese Academy of Sciences, beijing 100039, china) [a]State Key Laboratory for Space Weather Center for Space Science and Applied Research Chinese Academy of Sciences Beijing China [b]graduate university of Chinese Academy of Sciences Beijing China

Using the nonlinear propagating gravity waves (GW) model in the two-dimensional compressible atmosphere and the linear GW theory, the process of GW propagation in different background winds, e.g. the direction of the background wind is opposite to (dead wind) or the same as (tail wind) the direction of the horizontal phase velocity of GW, is studied. The results show that the dead wind prolongs the vertical wavelength and accelerates GW propagation. Therefore, GW propagates up to a higher height becomes instable in a short time and eventually induces an inverse jet flow. Then, the vertical wavelength is becoming short due to the nonlinear interactions between GW and the inverse jet flow. The vertical wavelength and group velocity decrease after GW propagates into the tail wind. The initial instable time is delayed. Although most of GW is trapped in the instable region, some of GW propagates above the instable region. Compared with GW propagation in the tail wind, the nonlinear interactions between GW and the dead wind are also strong. In contrast, the linear GW theory predicts that GW can propagate freely in the dead wind. The vertical wavelength simulated by the nonlinear numerical model is different from that predicted by the linear theory greatly after GW propagates into the dead wind.

关键词： gravity waves background winds vertical group velocity vertical wavelength nonlinear interactions.

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Paleoceanographic evolution recorded in the northern South china Sea since 4 Ma

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Science china Earth Sciences 2005年第12期48卷 2166-2173页

作者： HUANG Baoqi1,2. JIAN Zhimin2.& WANG Pinxian2.1. School of Earth and Space Sciences, Peking university, beijing 100871,{2. 2. Laboratory of Marine Geology, Tongji university, Shanghai 2.0092.{2. 1. School of Earth and Space Sciences Peking University 100871 Beijing China 2. Laboratory of Marine Geology Tongji University 200092 Shanghai China

Upper water structure over the last 4 million years in the northern South china Sea (SCS) was reconstructed by sea surface temperature (SST) and primary productivity estimated by changes in the abundance of planktonic foraminifer, planktonic foraminifer transfer function, and the accumulation rate of benthic foraminifera. Results of SST and primary productivity show that SST gradually decreased since 4 Ma, but differential seasonal temperature and primary productivity increased in steps mainly at about 3.1, 2.7, 2.1, 1.6, 0.9 and 0.5 Ma. Comparison with tectonics and orbital variations indicates that phased rising of the Tibet since 3.6 Ma, closing of Panama and Indonesian seaways, and orbital changes were responsible for the changes of upper water structure in the SCS, respectively.

关键词： northern South china Sea, upper water structure, Late Pliocene, planktonic foraminifer, ODP 1146.

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Identification of high-lipid producers for biodiesel production from forty-three green algal isolates in china

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Progress in Natural Science:Materials International 2011年第4期21卷 269-276页

作者： An-yue LIU~(1,2.,Wei CHEN~1,Ling-ling ZHENG~1,Li-rong SONG~1 1.State Key Laboratory of Freshwater Ecology and Biotechnology,Institute of Hydrobiology, Chinese Academy of Sciences,Wuhan 430072.china 2.graduate School,Chinese Academy of Sciences,{2. 100049,china [a] State Key Laboratory of Freshwater Ecology and Biotechnology Institute of Hydrobiology Chinese Academy of Sciences Wuhan 430072 China [b] graduate School Chinese Academy of Sciences Beijing 100049 China

To identify some desirable algal strains for our future research and/or the production of algae-based biofuel,43 green algal strains were successfully isolated from Chinese freshwaters,and then incubated in the laboratory bioreactors for the growth and oil accumulation *** a 15 d incubation experiment,the accumulations of their biomass and total lipids,together with the lipid productivities for these green algal strains were systematically investigated and *** indicated that the accumulations of biomass for the 43 algal strains ranged from 0.53 g/L to 6.07 g/L during the experiments,with the highest biomass of 6.07 g/L for green algae Scenedesmus *** lipid content for the tested algal strains varied from 2.%to 51%of the dry biomass at the end of cultivation *** algae Chlorella pyrenoidosa was one of the best oil producers based on our investigations,with the total lipid content of 51%of dry *** the growth rates and the accumulations of intracellular lipids into the consideration,10 strains were considered to have significant potential for biofuel *** addition,the lipid productivities of the selected strains were further investigated.

关键词： biofuel microalgae lipid accumulation

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Strict constraints on 2. primitive pairs for engineering symbol recognition:Theory and application

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Science china(Information Sciences) 2012年第5期55卷 1032-1041页

作者： LI Ting 1,2.QIU XianJie 1,HUANG He 1 & WANG ZhaoQi 1 1 Virtual Reality Laboratory,Institute of Computing Technology Chinese Academy of Sciences,beijing 100190,china {2. university of Chinese Academy of Sciences,beijing 100049,china 1. Virtual Reality Laboratory Institute of Computing Technology Chinese Academy of Sciences Beijing 100190 China2. Graduate University of Chinese Academy of Sciences Beijing 100049 China

Geometric constraints on the line-line pair,line-arc pair and arcarc pair are *** con-straints are able to encode the geometric relations between lines,arcs and circles.A geometric proof is presented to demonstrate that the constraints are stable under translation,rotation,uniform scaling or reflection of the primitive *** on the constraints,an algorithm for recognizing symbols in drawings is ***-perimental results show that,compared with three other methods,our method can distinguish more primitive pairs and has higher accuracy in engineering symbol recognition.

关键词： coordinated multi-point transmission multicell cooperation capacity analysis MIMO-OFDM power allocation frequency selective MIMO channel

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