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Estimation methods of eco-environmental water requirements: Case study

Science china Earth Sciences 2005年第8期48卷 1280-1292页

作者： YANG Zhifeng1,2. CUI Baoshan1 & LIU Jingling 1. School of Environment, beijing Normal University, beijing 100875,{2. 2. state key joint laboratory of environmental simulation and pollution control, beijing 100875,{2. 1. School of Environment Beijing Normal University 100875 Beijing China 2. state key joint laboratory of environmental simulation and pollution control 100875 Beijing China

Supplying water to the ecological environment with certain quantity and quality is significant for the protection of diversity and the realization of sustainable development. The conception and connotation of eco-environmental water requirements, including the definition of the conception, the composition and characteristics of eco-environmental water requirements, are evaluated in this paper. The classification and estimation methods of eco-environmental water requirements are then proposed. On the basis of the study on the Huang-Huai-Hai Area, the present water use, the minimum and suitable water requirement are estimated and the cor-responding water shortage is also calculated. According to the interrelated programs, the eco-environmental water requirements in the coming years (2.10, 2.30, 2.50) are estimated. The result indicates that the minimum and suitable eco-environmental water requirements fluc-tuate with the differences of function setting and the referential standard of water resources, and so as the water shortage. Moreover, the study indicates that the minimum eco-environmental water requirement of the study area ranges from 2.84×1010m3 to 1.02.1011m3, the suitable water requirement ranges from 6.45×1010m3 to 1.78×1011m3, the water shortage ranges from 9.1×109m3 to 2.16×1010m3 under the minimum water requirement, and it is from 3.07×1010m3 to 7.53×1010m3 under the suitable water requirement. According to the different values of the water shortage, the water priority can be allocated. The ranges of the eco-environmental water re-quirements in the three coming years (2.10, 2.30, 2.50) are 4.49×1010m3?1.73×1011m3, 5.99×10m3?2.09×1011m3, and 7.44×1010m3?2.52.1011m3, respectively.

关键词： eco-environmental water requirements, assessment methods, Huang-Huai-Hai area.

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Biogenic Isoprene Emission Mechanism from ^(13)CO_2.Exposure Experiments

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Chinese Chemical Letters 2002年第9期13卷 897-900页

作者： Min SHAO state joint {2. laboratory of environmental simulation and pollution control, Center for environmental Sciences, Peking University, beijing 100871 state joint {2. laboratory of environmental simulation and pollution control Center for Environmental Sciences Peking University Beijing 100871 China

Biogenic isoprene emissions have been believed to be from only photosynthesis processes in plant. However nocturnal isoprene emission from pine is detected. And by feeding 13CO2.to plants, it is found that both photos... 详细信息

关键词： Emissions volatile organic compounds (VOCs) 13C labeling isoprene.

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Influence of fuel quality on vehicular NOx emissions

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Journal of environmental Sciences 2001年第3期13卷 265-271页

作者： WANG Shao xia, SHAO Min, ZHANG Yuan hang (state joint {2. laboratory of environmental simulation and pollution control, Center for environmental Sciences, Peking University, beijing 100871, china. state joint {2. laboratory of environmental simulation and pollution control Center for Environmental Sciences Peking University Beijing 100871 China.

The quality of gasoline and diesel fuel affects pollutant emissions from vehicles. By applying the COMPLEX model, developed by the US EPA and industry to relate fuel composition to vehicle emissions, this paper estimates the influence of improvements in gasoline quality to lower vehicular NOx emissions. A case study is performed for Guangzhou City that has NOx concentrations significantly above the national ambient air quality standards (NAAQS). The paper discusses the potential for reducing NOx in Guangzhou by improving the quality of gasoline.

关键词： Air quality Automotive fuels Gasoline

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A HIGH-ORDER-ACCURATE DIFFERENCE SCHEME WITH UNCONDITIONAL STABILITY FOR THE DIFFUSION EQUATION ON NONUNIFORM GRIDS

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Journal of Hydrodynamics 2001年第1期13卷 92-98页

作者： Wang Xuan, Yang Zhi-feng state key {2. of Environment simulation and pollution control, Institute of environmental Sciences, beijing Normal University, beijing 100875, china[WT5”HZ] beijing Normal Univ. Beijing 100875 China

WT5”BZ]A high-order-accurate difference scheme with unconditional stability is developed for the diffusion equation on nonuniform grids. The theoretical analysis shows that the accuracy of this scheme is between third order and fourth order, and fourth-order accuracy is achieved in the case of the same grid steps being used within the computational domain. Two numerical examples are given to demonst ate the advantages of the proposed scheme. Compared with the conventional difference scheme, more accurate numerical solution can be obtained by using the proposed scheme even with relatively larger grid sizes. It is also pointed out that the appropriate structure of the nonuniform grid can not only make the proposed scheme more practical, but lead to a solution superior to that for a uniform grid structure. [WT5”HZ]

关键词： ]finite difference scheme diffusion equation nonuniform grid high accuracy computational fluid dynamics

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Heterogeneous reactions of gaseous methanesulfonic acid with calcium carbonate and kaolinite particles

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Science china Chemistry 2010年第12期53卷 2657-2662页

作者： TANG MingJin,LI MengQiu & ZHU Tong state key {2. laboratory of environmental simulation and pollution control College of environmental Sciences and Engineering,Peking University,beijing 100871,china 1. state key {2. laboratory of environmental simulation and pollution control College of environmental Sciences and Engineering Peking University Beijing 100871 China

Heterogeneous reactions of gaseous methanesulfonic acid (MSA) with calcium carbonate (CaCO3) and kaolinite particles at room temperature were investigated using diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) and ion chromatography (IC).Methanesulfonate (MS-) was identified as the product in the condensed phase,in accordance with the product of the reaction of gaseous MSA with NaCl and sea salt *** the concentration of gaseous MSA was 1.34 × 10-13 molecules cm-3,the uptake coefficient was (1.2. ± 0.06) × 10-8 (1) for the reaction of gaseous MSA with CaCO3 and (4.10 ± 0.65) × 10 10 (1) for the reaction with *** uptake coefficients were significantly smaller than those of the reactions of gaseous MSA with NaCl and sea salt particles.

关键词： gaseous MSA heterogeneous reaction calcium carbonate kaolinite

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Heterogeneous reaction of SO_2.on TiO_2.particles

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Science china Chemistry 2010年第12期53卷 2637-2643页

作者： SHANG Jing,LI Jia & ZHU Tong state key {2. laboratory of environmental simulation and pollution control College of environmental Sciences and Engineering,Peking University,beijing 100871,china 1. state key {2. laboratory of environmental simulation and pollution control College of environmental Sciences and Engineering Peking University Beijing 100871 China

The heterogeneous reaction of SO2.on TiO2.particles was studied using in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS).The influences of the oxygen concentration,relative humidity (RH),and ultraviolet (UV) light illumination (λ=365 nm) intensity on the reaction were *** main product of the heterogeneous reaction of SO2.on TiO2.particles was sulfate with UV illumination and sulfite without *** production of sulfate was promoted significantly with UV illumination or water,and there was a synergistic effect when both were *** the dry system without UV,the heterogeneous reaction of SO2.on TiO2.particles was found to be second-order for SO2.and the initial uptake coefficient,BET,was determined to be 1.94 × *** UV and RH=40%,the reaction order was first-order and the initial uptake coefficient was 1.35 × 10-5.

关键词： SO2 TiO2 DRIFTS heterogeneous oxidation

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Biodegradation of polycyclic aromatic hydrocarbons in sediments from the Daliao River watershed, china

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Journal of environmental Sciences 2009年第7期21卷 865-871页

作者： QUAN Xiangchun, TANG Qian, HE Mengchang, YANG Zhifeng, LIN Chunye, GUO Wei state key {2. laboratory of environmental simulation and pollution control, School of Environment, beijing Normal University, beijing 100875, china. [a]state key {2. laboratory of environmental simulation and pollution control School of Environment Beijing Normal University Beijing 100875 China

The Daliao River, as an important water system in Northeast china, was reported to be heavily polluted by polycyclic aromatic hydrocarbons （PAHs）. Aerobic biodegradations of four selected PAHs （naphthalene, phenanthrene, fluorene and anthracene） alone or in their mixture in river sediments from the Daliao River water systems were studied in microcosm systems. Effects of additional carbon source, inorganic nitrogen and phosphorus, temperature variation on PAHs degradation were also investigated. Results showed that the degradation of phenanthrene in water alone system was faster than that in water-sediment combined system. Degradation of phenanthrene in sediment was enhanced by adding yeast extract and ammonium, but retarded by adding sodium acetate and not significantly influenced by adding phosphate. Although PAHs could also be biodegraded in sediment under low temperature （5~C）, much lower degradation rate was observed. Sediments from the three main streams of the Daliao River water system （the Hun River, the Taizi River and the Daliao River） demonstrated different degradation capacities and patterns to four PAHs. Average removal rates （15 or 19 d） of naphthalene, phenanthrene, fluorene and anthracene by sediment were in the range of 0.062.0.087, 0.005-0.066, 0.008- 0.016 and 0-0.059 mg/（L.d）, respectively. As a result, naphthalene was most easily degraded compound, anthracene was the hardest one. In multiple PAHs systems, the interactions between PAHs influenced each PAH biodegradation.

关键词： biodegradation the Daliao River microcosm polycyclic aromatic hydrocarbon sediment

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Effect of CH3OOH on the atmospheric concentration of OH radicals

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Progress in Natural Science:Materials International 2006年第11期16卷 1141-1149页

作者： WANG Caixia and CHEN Zhongming**(The state key {2. of environmental simulation and pollution control, College of environmental Sciences, Peking University, beijing 100871, china) [a]The state key {2. of environmental simulation and pollution control College of Environmental Sciences Peking University Beijing China

Methyl hydroperoxide （CH3OOH, MHP） is known to be a significant sink and reservoir of HOx and ROx radicals in the atmosphere. In order to investigate the impact of MHP on the concentration of atmospheric OH radicals, two key gas-phase reactions of MHP, i.e. the reactions with OH radicals and with UV photolysis, have been simulated at temperature of 2.3±2.K and total pressure of 1.01×105 Pa, using the long path Fourier transform infrared （LP-FTIR） spectrometry. OH radicals are generated by the photolysis of O3 in the presence of water vapor. Combined with the relative rate method, the reaction rate constant of MHP with OH radicals is determined to be （3.99±0.15）×10 -12.cm3·molecule -1 ·s -1 , and thus the atmospheric lifetime of MHP is estimated at 2.9 days. Furthermore, from detailed analysis of the UV photolysis of MHP, the yield of OH radicals is obtained to be 0.91±0.04. Based on the MHP atmospheric lifetime and the yield of OH radicals, it is concluded that MHP plays an essential role in the redistribution of OH radicals in the troposphere.

关键词： OH radicals methyl hydroperoxide rate coefficient UV photolysis gas-phase reaction LP-FTIR.

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Reinvestigation of the Henry's law constant for hydrogen peroxide with temperature and acidity variation

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Journal of environmental Sciences 2010年第4期22卷 570-574页

作者： Daoming Huang,Zhongming Chen The state key {2. of environmental simulation and pollution control,College of environmental Sciences and Engineering,Peking University,beijing 100871,china. [a] The state key {2. of environmental simulation pollution control College of Environmental Sciences Engineering Peking University Beijing 100871 China

Hydrogen peroxide is not only an important oxidant in itself; it also serves as both sink and temporary reservoir for other important oxidants including HOx （OH and HO2. radicals and O3 in the atmosphere. Its partitioning between gas and aqueous phases in the atmosphere, usually described by its Henry＇s law constant （KH）, significantly influences its role in atmospheric processes. Large discrepancies between the KH values reported in previous work, however, have created uncertainty for atmospheric modelers. Based on our newly developed online instrumentation, we have re-determined the temperature and acidity dependence of KH for hydrogen peroxide at an air pressure of （0.960 ± 0.013） atm （1 atm = 1.0132. × 10^5 Pa）. The results indicated that the temperature dependence of KH for hydrogen peroxide fits to the Van＇t Hoff equation form, expressed as lnKH = a/T - b, and a = -△H/R, where KH is in M/atm （M is mol/L）, T is in degrees Kelvin, R is the ideal gas constant, and AH is the standard heat of solution. For acidity dependence, results demonstrated that the KH value of hydrogen peroxide appeared to have no obvious dependence on decreasing pH level （from pH 7 to pH 1）. Combining the dependence of both temperature and acidity, the obtained a and b were 702. ± 138 and 11.97 ± 0.48, respectively, AH was （58.40 ± 1.15） kJ/（***）, and the uncertainties represent σ. Our determined KH values for hydrogen peroxide will therefore be of great use in atmospheric models.

关键词： hydrogen peroxide Henry's law constant atmosphere acidity

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A HIGH-ORDER FINITE DIFFERENCE METHOD FOR UNSTEADY CONVECTION-DIFFUSION PROBLEMS WITH SOURCE TERM

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Journal of Hydrodynamics 1999年第2期11卷 97-102页

作者： Yang Zhi-feng Wang Xuan(state key {2. of Environment simulation and pollution control, Institute of environmental Sciences, beijing Normal University, beijing 100875, P. R. china.) beijing Normal Univ Beijing China

The convection and diffusion are the basic processes in fluid flow and heat& mass transfer. The upwind and evolution functions for the convection term are introduced to give a comprehensive transformation to one-dimensional unsteady convection-diffusion equation involving source term. The corresponding compact fourth-order finite difference methed is developed. With the trans formation, the authors overcome the difficultyin dealing with the convection term, and the high-order expression for the convection-diffusion term can be conveniently obtained. The proposed difference scheme with thefourth-order accuracy and unconditional stability can fully reflect the upwind and evolutioneffects of the convection. The calculated results show that the errors of the referencescheme are 600 or 6000 times those of the proposed scheme for the same computationalgrid. With the one time decrease of the space grid, the errors of the proposed scheme andthe reference scheme reduce about 2. times and 2.times respectively. It is evident that theaccuracy of the proposed scheme is remarkably higher than that of the reference scheme.

关键词： convection-diffusion compact difference method comprehensive transformation unsteady computational fluid dynamics

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