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Adjoint method for the optimum planning of industrial pollutant sources

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Science china Earth Sciences 2005年第8期48卷 1270-1279页

作者： LIU Feng1,2. HU Fei2.& ZHU Jiang2.1. College of Environmental Sciences, Peking University, beijing 100871, china 2. LAPC, {2. of Atmospheric physics, Chinese Academy of Sciences, beijing 10002., china College of Environmental Sciences Peking University Beijing China LAPC Institute of Atmospheric Physics Chinese Academy of Sciences Beijing China

The optimum planning of industrial pollutant sources, which optimizes the economic object without violating environmental constraints, is an important and hard task to be conquered. In this paper, an adjoint method is developed to solve the problem. The penalty function is in-troduced to deal with the environmental inequality constraints, and Lagrange function is con-structed to derive the adjoint equation and the gradient of the object function. In this means, the gradient of the object function can be calculated by solving the adjoint equation, and the infor-mation from the gradient is used to make the object function descend and approach to an optimal solution after some iterations. A two-dimensional, simplified model is used for numerical experi-ments. The theoretical derivations are verified by the results of the experiments. Furthermore, the adjoint method is shown to be of excellent convergence and efficiency, which is adaptive to the fast development of air quality numerical models and super computers.

关键词： optimum planning, industrial pollutant sources, adjoint equation, penalty function, gradient.

Magnetron sputtering synthesis of large area well-ordered boron nanowire arrays

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Science china(physics,Mechanics & Astronomy) 2004年第4期47卷 403-415页

作者： CAO Limin1,2. ZHANG Ze2.& WANG Wenkui1,2.1. Key Laboratory of Metastable Materials Science and Technology and College of Materials Science and Engineering, Yanshan University, Qinhuangdao 066004, china 2. institute of physics, Chinese Academy of Sciences,{2., china Key Laboratory of Metastable Materials Science and Technology and College of Materials Science and Engineering Yanshan University Qinhuangdao China institute of physics Chinese Academy of Sciences Beijing China

One-dimensionally nanostructured materials, such as nanowires and nanotubes, are the smallest dimensional structures for efficient transport of electrons and excitons, and are therefore critical building blocks for nanoscale electronic and mechanical devices. In this paper, boron nanowires with uniform diameters from 2. to 80 nm were synthesized by radio-frequency magnetron sputtering of pure boron powder and B2.3 powder mixtures in argon atmosphere. The boron nanowires produced stand vertically on the substrate surface to form well-ordered arrays over large areas with self- organized arrangements without involvement of any template and patterned catalyst. The high-density boron nanowires are parallel to each other and well distributed, forming highly ordered and uniform arrays. A more interesting and unique feature of the boron nanowires is that most of their tips are flat rather than hemispherical in morphologies. Detailed studies on its structure and composition indicate that boron nanowires are amorphous. Boron nanowire appears as a new member in the family of one-dimensional nanostructures. Considering the unique properties of boron-rich solids and other nanostructures, it is reasonable to expect that the boron nanowires will display some exceptional and interesting properties. A vapor-cluster-solid (VCS) mechanism was proposed to explain the growth of boron nanowires based on our experimental observations.

关键词： boron nanowires, magnetron sputtering, arrays, self-assembly.

Interfacial behaviors of PMMA-PEO block copolymers at the air/water interface

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Science china Chemistry 2005年第6期48卷 567-573页

作者： CHENG Caixia1, JIAO Tifeng2. TANG Rupei1, LIU Minghua2.& XI Fu1 1. State Key Laboratory of Polymer physics and Chemistry, Joint Laboratory of Polymer Science and Materials, institute of Chemistry, Chinese Academy of Sciences,{2., china 2. CAS Key Laboratory of Colloid and Interface Science, institute of Chemistry, Chinese Academy of Sciences,{2., china State Key Laboratory of Polymer physics and Chemistry Joint Laboratory of Polymer Science and Materials Institute of Chemistry Chinese Academy of Sciences Beijing China CAS Key Laboratory of Colloid and Interface Science Institute of Chemistry Chinese Academy of Sciences Beijing China

Diblock copolymer of PMMA2.1-b-PEO114 and triblock copolymer of PMMA12.-b- PEO2.7-b-PMMA12. were synthesized and their interfacial properties at the air-water interface were investigated, where both blocks of polyethylene oxide (PEO) and poly(methyl methacrylate) (PMMA) are surface active but the former is soluble in water while the latter is not. Both the block copolymers could form monolayers with two obvious transition regions. The first transition point is around 10 mN/m, which could be assigned to the pancake-brush change of the PEO chains. The other is around 18 mN/m, which could be ascribed to the condensed packing of PMMA. The surface morphological changes during the compression of the Langmuir monolayers are inves-tigated by using the AFM and SEM methods for the films deposited at different surface pressure or molecular areas. At a lower surface pressure, a typical morphology of PEO-con- taining lipopolymers is observed. Upon compression, sphere-dominant morphologies were observed. While the diblock copolymer is easy to folding, the triblock copolymer is in favor of formation of circular domains through vesiculation.

关键词： PMMA-PEO, block copolymers, monolayer, Langmuir-Blodgett films, AFM.

Experimental study of electron capture excitation in collisions between Li-like N^(4+) ions and Na atoms

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Chinese Science Bulletin 1997年第5期42卷 368-371页

作者： LIU Zhanwen, ZHOU Sixin, ZHANG Wen, ZHANG Xuezhen GUOXiaohong, WANG Youde, MA Xinwen, YANGZhihu, LIU Huiping, ZHAO Mengchun, YANG Feng, PAN Guangyan and LI Dawan1. institute of Modern physics, Chinese Academy of Sciences, Lanzhou 730000,{2. 2. institute of physics, Chinese Academy of Sciences, beijing 100080,{2. institute of Modern physics Chinese Academy of Sciences Lamhou China institute of Physia Chinese Academy of Sciences Beijing China

WITH the rapid development of the technique of ionized atoms, the charge states of atoms that can be obtained now are so high that the H-like U91+ ions and naked U92. ions

关键词： single electron capture double electron capture emission cross section excited states.

Synthesis of Ag_2. nano-sized clusters and their chemical sensitizations in AgCl cubic and {100} tabular microcrystal imaging systems

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Science china Chemistry 2005年第6期48卷 516-522页

作者： LI Zhi1, ZHENG Tong1, CHEN Lijuan1, PENG Bixian1 & YANG Li2.1. Technical institute of physics and Chemistry, Chinese Academy of Sciences, {2. 100101, china 2. {2. Satellite Manufacturing Factory, beijing 100080, china Technical institute of physics and Chemistry Chinese Academy of Sciences Beijing 100101 China

In recent years much attention has been devoted to AgCl emulsion owing to its se-rial advantages and inimitable potential. But in the research of this emulsion a thorny problem remains unsolved till now, which is the improvement in sensitivity is always accompanied with high fog density. In this work 5 nm Ag2. particles were prepared and used as novel sensitizers in AgCl cubic and {100} tabular microcrystal emulsions. The novel sensitizer shows an effective sensitizing ability for silver chloride emulsion, and it is superior to the traditional Na2.2.3 sensi-tizer because by using it comparatively high sensitivity can be obtained with lower fog density. So the above sensitizing problem is going to be effectively solved. To discover the evolution mechanism of the sensitizer clusters and explain their excellent sensitizing properties, diffuse reflectance spectroscopy (DRS) was used as a probe on the AgCl microcrystal surface.

关键词： silver sulfide, nano-sized, silver chloride {100} tabular microcrystal, chemical sensitization.

Numerical simulation of Meiyu front and the diagnosis of moist vorticity vector

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Progress in Natural Science:Materials International 2007年第11期17卷 1341-1347页

作者： Ping Fan1,2.and Luo Zhexian2.1. institute of Atmospheric physics, Chinese Academy of Sciences, {2. 10002., china 2. Nanjing University of Information Sciences & Technology, Nanjing 2.0044, china) institute of Atmospheric physics Chinese Academy of Sciences Beijing 100029 Chin

Moist vorticity vector is introduced to study the development and evolution of mesoscale convective vortex (MCV) in the Meiyu front precipitation with the Advanced Regional Predication System (ARPS). In this study, the heavy rainfall is simulated to investigate the genesis, development and dissipation of middle scale convective vortex, which occurred from 0000 UTC 3 July to 12.0 UTC 5 July over the Jianghuai River valley. Moist vorticity vector (MVV) has zonal, radial and vertical components in its 3D spatial distribution. The simulation shows that the vertical component of moist vorticity vector well demonstrates the spatial distribution characteristics of middle scale convective vortex, especially in the process of Meiyu front precipitation. Diagnosis upon zonal, radial averaged and mass-integrated quantities of MVV shows that its vertical component and the surface precipitating ratio are in phase with a correlation coefficient of 0.68, indicating that the vertical component of MVV is closely associated with the Meiyu front precipitation. In addition, the tendency of the vertical component of MVV is mainly determined by the interaction between the vorticity and the zonal and radial gradient of condensational or depositional heating.

关键词： moist vorticity vector mesoscale convective vortex Meiyu front precipitation

Strengthening of the boreal winter Hadley circulation and its connection with ENSO

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Progress in Natural Science:Materials International 2007年第11期17卷 1327-1333页

作者： Ma Jie1,2.and Li Jianping2.1. College of Atmospheric Sciences, Lanzhou University, Lanzhou 730000, china 2. LASG, institute of Atmospheric {2., Chinese Academy of Sciences, beijing 10002., china) College of Atmospheric Sciences Lanzhou University Lanzhou 730000 China

Empirical orthogonal function (EOF) analysis is carried out for the year-to-year variability of the boreal winter (DJF) mass stream function of the mean meridional circulation (MMC) during the period 1948—2.05. The results demonstrate that it is dominated by the equatorially asymmetric and symmetric modes. Further analysis shows that the former mode is linked with the boreal winter Hadley cell mainly on the decadal time-scale, and the latter on the interannual time-scale. The asymmetric mode index (AMI) with a clear upward trend contributes to the decadal strengthening of the boreal Hadley circulation, and is closely correlated with the tropical SST warming, especially in the region of Indo-west Pacific warm pool (INWP). Furthermore, the AMI also contributes to the abrupt change of the correlation coefficient between the boreal Hadley circulation and ENSO after 1976. The symmetric mode index (SMI) with robust and stable linkage with ENSO shows a significant interannual variability, suggesting that the variability of the Hadley circulation is mainly associated with ENSO on the interannual time-scale.

关键词： the Hadley circulation interannual time-scale decadal time-scale

Role of gallium wetting layer in high-quality ZnO growth on sapphire (0001) substrates

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Science china(physics,Mechanics & Astronomy) 2004年第5期47卷 612-620页

作者： ZENG Zhaoquan1,3, WANG Yong2. DU Xiaolong1, MEI Zengxia1, KONG Xianghe3, JIA Jinfeng1, XUE Qikun1 & ZHANG Ze2. 4 1. State Key Laboratory for Surface physics, institute of physics, Chinese Academy of Sciences, beijing 100080, china 2. Laboratory of Electron Microscopy, institute of physics, Chinese Academy of Sciences, beijing 100080, china 3. College of physics and Engineering, Qufu Normal University, Qufu 2.3165, china 4. beijing University of Technology, beijing 10002., china State Key Laboratory for Surface physics Institute of Physics Chinese Academy of Sciences Beijing China College of physics and Engineering Qufu Normal University Qufu China Laboratory of Electron Microscopy Institute of Physics Chinese Academy of Sciences Beijing China beijing University of Technology Beijing China

A Ga wetting layer was used to modify the surface structure of sapphire (0001) substrate to prepare high-quality ZnO film by radio frequency plasma-assisted molecule beam epitaxy. We found that this Ga layer plays a crucial role in eliminating 30 rotation domains, controlling polarity and decreasing defect density in ZnO epilayers, as demonstrated by in situ reflection high energy electron diffraction, ex situ high resolution X-ray diffraction and high resolution cross-sectional transmission electron microscopy. Zn-polar film of ZnO was determined by convergent beam electron diffraction. A Ga bilayer model is proposed to understand the effects of the Ga wetting layer on high-quality ZnO growth.

关键词： Ga wetting layer, sapphire, polarity, defect density, zinc oxide, rf-MBE, RHEED, HRXRD, TEM, CBED.

Gasdynamic characteristics of toroidal shock and detonation wave converging

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Science china(physics,Mechanics & Astronomy) 2005年第6期48卷 739-749页

作者： TENG Honghui1,2.& JIANG Zonglin2.1. Key Laboratory of High Temperature Gas Dynamics, institute of Mechanics, Chinese Academy of Sci- ences, beijing 100080,{2. 2. Graduate University of Chinese Academy of Sciences, beijing 100039,{2. Key Laboratory of High Temperature Gas Dynamics Institute of Mechanics Chinese Academy of Sciences Beijing China Graduate University of Chinese Academy of Sciences Beijing China

The modified CCW relation is applied to analyzing the shock, detonation wave converging and the role of chemical reactions in the process. Results indicate that the shock wave is strengthened faster than the detonation wave in the converging at the same initial Mach number. Euler equations implemented with a detailed chemical reaction model are solved to simulate toroidal shock and detonation wave converging. Gasdynamic characteristics of the converging are investigated, including wave interaction patterns, observable discrepancies and physical phenomena behind them. By comparing wave diffractions, converging processes and pressure evolutions in the focusing area, the different effects of chemical reactions on diffracting and converging processes are discussed and the analytic conclusion is demonstrated through the observation of numerical simulations.

关键词： converging, CCW relation, shock wave, detonation wave.