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Chinese Science Bulletin 2000年第S1期45卷 26-34页

作者： WANG Yunpengguangzhou institute of {2., Chinese Academy of Sciences, guangzhou 51064., china Chinese Acad Sci Guangzhou Inst Geochem Guangzhou 510640 Peoples R China

This paper presents the contents of 17 kinds of trace elements in plant leaf samples collected from 4 sections in the North Jiangsu oil field, and the dada on their visible-near infrared spectra. By comparing the results of the inner and outer oil-gas remote-sensing anomaly areas, the plant trace element composition, and the enrichment characteristics and their influence on the plant spectral properties are described. The results indicated that the plant leaves had very strong enrichment ability toward some elements such as Mg, Ca, K, Na, Fe, Al, Mn, V, Zn and Cr. The plant leaves from the oil-gas abnormal areas were enriched in trace elements of the Fe-series, but depleted in alkali and alkali-earth metal elements. The plant trace elements had a strong influence on the 'blue-shift' strength and the reflectance of visible bands. And the ratios between Fe, Co and K, Na, Cd, Cu, Ba are the effective remote-sensing oil-indicating factors of plant trace elements. plant trace element, geochemistry, remote

关键词： plant trace element geochemistry remote sensing spectra North Jiangsu oil fleld.

geochemistry of high-Mg andesites from the early Cretaceous Yixian Formation, western Liaoning: Implications for lower crustal delamination and Sr/Y variations

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Science china Earth Sciences 2006年第9期49卷 904-914页

作者： WANG Xiaorui1, GAO Shan1,2. LIU Xiaoming1, YUAN Honglin1, HU Zhaochu1, ZHANG Hong1,3 & WANG Xuance4 1. State Key Laboratory of Continental Dynamics, Department of Geology, Northwest University, Xi`an 710069, china 2. State Key Laboratory of Geological Processes and Mineral Resources, china University of Geosciences, Wuhan 430074, china 3. Shenyang institute of Geology and Mineral Resources, Shenyang 110032. china 4. guangzhou institute of geochemistry, Chinese Academy of Sciences, guangzhou 51064., china 1. State Key Laboratory of Continental Dynamics Department of Geology Northwest University Xi’an 710069 China 2. State Key Laboratory of Geological Processes and Mineral Resources China University of Geosciences Wuhan 430074 China 3. Shenyang institute of Geology and Mineral Resources Shenyang 110032 China 4. guangzhou institute of {2. Chinese Academy of Sciences Guangzhou 510640 China

85 volcanic rocks of the Yixian Formation from the Sihetun type section werecollected and analyzed for geochemical and isotopic compositions. Major element compositionsindicate that the Sihetun volcanic rocks are high magnesium andesites with some basalts occurring atthe bottom of section. The Sihetun high magnesium andesites (SiO_2.= 52.82.59.31 wt%, Al_2._3=14.15-16.35wt%) show many characteristics of adakites such as depletion in heavy rare-earth elements(HREE; Yb = 1.03-1.88 μg/g) and Y(12.2. μg/g) and high Sr (62.-132. μg/g) and Sr/Y(32.88), withhigh La_N/Yb_N ratio (10-2.). They share similar major and trace element characteristics to volcanicrocks from the Xinglonggou Formation except their lower Nd isotope ratios (^(143)Nd/^(144)Nd(130Ma) = 0.5118-0.5119, ε_(Nd) (130Ma) = -11.6-13.8, ^(87)Sr/^(86)Sr (130 Ma) = *** were interpreted in a way that eclogite that formed at the base of thickened Archean lowercrust of the North china craton foundered into the convecting mantle and subsequently melted andinteracted with peridotite. However, compared to the Xinglonggou volcanic rocks, the source of theSihetun magma contained more ancient continental crustal material in order to explain its evolved Ndisotopes. The age of the Sihetun Formation was 12. to 130 Ma, and this indicates that delaminationlasted to the early Cretaceous period. The Sr contents and Sr/Y ratios of the Sihetun high-Mgandesites show significant negative correlations with SiO_2.for samples with SiO_2.> 56%. Thesesuggest that the Sr and Sr/Y values were reduced due to fractional crystallization of ***, the effect of crystallization on volcanic Sr and Sr/Y ratio has to be taken intoaccount.

关键词： High-Mg andesite, Adakite, Yixian Formation, North china Craton, delamination.

The role of reservoir mediums in natural oil cracking:Preliminary experimental results in a confined system

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Chinese Science Bulletin 2010年第33期55卷 3787-3793页

作者： XIAO QiLin1,2.SUN YongGe1,3 & ZHANG YongDong1,2.1 State Key Laboratory of Organic geochemistry,guangzhou {2. of geochemistry,Chinese Academy of Sciences,guangzhou 51064.,china 2.Graduate Schools,Chinese Academy of Sciences,Beijing 100049,china 3 {2. of Environmental and Biogeochemistry(eBig),Zhejiang University,Hangzhou 31002.,china State Key Laboratory of Organic geochemistry Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China Graduate Schools Chinese Academy of Sciences Beijing 100049 China institute of Environmental and Biogeochemistry (eBig) Zhejiang University Hangzhou 310027 China

Large amounts of data regarding the influence of temperature and pressure on the thermal stability of crude oil have been pub-lished;however,the role of reservoir mediums has received little *** involving oil cracking in the presence of montmorillonite,illite,calcite,quartz and water were conducted in closed gold tubes to investigate the effects of these reservoir mediums on oil *** was done by screening variations in the chemical and stable carbon isotopic components of nC10+ and gasoline-range hydrocarbons(nC8-)present in various *** indicated that reservoir mediums have an active role in oil cracking under experimental *** concentrations of nC10+ in the cracked residues progressively decreased in systems containing oil+water+illite,oil+water+montmorillonite,oil+water,oil+water+quartz and oil+water+*** comparison with the system containing oil+water,our results indicated a retardation effect for oil cracking in systems in the presence of illite and montmorillonite,and an acceleration effect on oil destruction in systems in the presence of calcite and ***10+ became increasingly depleted in 13C in systems with oil+water+illite,oil+water+calcite,oil+water+montmorillonite,oil+water+ quartz and oil+*** obvious correlation was observed between concentrations and stable carbon isotopic components of nC6-nC8 and nC10+ in the individual *** discrepancies in chemical and stable carbon isotopic components of nC6-nC8 and nC10+ in the pyrolyzed residues highlighted the important role of reservoir mediums to control carbon-carbon cleavage of nC10+ and then the isomerization,cyclolization and aromatization reactions;as well as governing the occurrence and thermal destruction of nC6-nC8 under experimental *** research may have critical implications in reconstructing chemical kinetic models for natural oil cracking.

关键词：裂解作用实验条件密闭系统原油裂解水库介质天然同位素组成

Research on the dynamics of the South china Sea opening:Evidence from analogue modeling

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Science china Earth Sciences 2006年第10期49卷 1053-1069页

作者： SUN Zhen1,2. ZHOU Di1, ZHONG Zhihong3, XIA Bin2. QIU Xuelin1, ZENG Zuoxun4 & JIANG Jianqun5 1. CAS Key Laboratory of Marginal Sea Geology, South china Sea institute of Oceanology, Chinese Academy of Sciences, {2. 510301, china 2. CAS Key Laboratory of Marginal Sea Geology, {2. institute of geochemistry, Chinese Academy of Sciences, guangzhou 51064., china 3. Department of Technology, Shenzhen Branch of CNOOC, {2. 5102.0, china 4. Faculty of Earth Sciences, china University of Geosciences, Wuhan 430074, china 5. Hainan Oil & Gas Exploration Company, Liaohe Oilfield Petrochina, Panjin 12.010, china 1. CAS Key Laboratory of Marginal Sea Geology South China Sea Institute of Oceanology Chinese Academy of Sciences Guangzhou 510301 China 2. CAS Key Laboratory of Marginal Sea Geology Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China 3. Department of Technology Shenzhen Branch of CNOOC Guangzhou 510240 China 4. Faculty of Earth Sciences China University of Geosciences Wuhan 430074 China 5. Hainan Oil & Gas Exploration Company Liaohe Oilfield PetroChina Panjin 124010 China

Independent of Indochina extrusion, the South china Sea experienced a process from passive continental rifting to marginal sea drifting. According to the fault patterns in the Beibu Gulf basin and the Pearl River Mouth basin, the continental rifting and early spreading stage from 32.to 2. Ma were controlled by extensional stress field, which shifted clockwise from southeastward to south southeastward. From 2. Ma on, the sea spread in NW-SE direction and ceased spreading at around 15.5 Ma. Integrated geological information with the assumption that the South china Sea developed along a pre-Cenozoic weakness zone, we did analogue experiments on the South china Sea evolu- tion. Experiments revealed that the pre-existing weakness zone goes roughly along the uplift zone between the present Zhu-1 and Zhu-2.depression. The pre-existing weakness zone is composed of three segments trending NNE, roughly EW and NEE, respectively. The early opening of the South china Sea is accompanied with roughly 15° clockwise rotation, while the SE sub-sea basin opened with SE extension. Tinjar fault was the western boundary of the Nansha block (Dangerous Ground), while Lupar fault was the eastern boundary of the Indochina, NW-trending rift belt known as Zengmu basin developed between above two faults due to block divergent of Indochina from Nansha. In the experiment, transtensional flower structures along NW-trending faults are seen, and slight inversion occurs along some NE-dipping faults. The existence of rigid massifs changed the orientations of some faults and rift belt, and also led to deformation concentrate around the massifs. The rifting and drifting of the South china Sea might be caused by slab pull from the proto South china Sea subducting toward Borneo and/or mantle flow caused by India-Asia collision.

关键词： South china Sea, rifting and drifting, clockwise rotation, analogue modeling, rigid massifs.

Trace element characteristics and origin of intergranular components in mantle peridotites

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Chinese Science Bulletin 2000年第7期45卷 643-649页

作者： XU Yigangguangzhou institute of {2., Chinese Academy of Sciences, guangzhou 51064., china guangzhou institute of {2. Chinese Academy of Sciences Guangzhou China

Leaching experiment has been carried out on mantle xenoliths with different petrographic features in order to directly characterize the nature of intergranular components. ICP-MS analyses of leachates show that they are characterized by high LREE concentrations with strong depletion of Ta. The total REE contents and whether the negative Rb, Ba and Nb anomalies are present or not in intergranular components are largely dependent upon the nature of mantle metasomatism experienced by its host rock. It is proposed that intergranular components may represent residues of small volume metasomatic melts.

关键词： peridotite xenoliths intergranular components trace elements upper mantle.

Glacial atmospheric CO_(2. decline in association with decrease of marine sedimentary phosphorus

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Science china Earth Sciences 2006年第3期49卷 322-330页

作者： WENG Huanxin1, ZHANG Xingmao1, WU Nengyou2. WANG Ying1, CHEN Lihong1, ZHONG Hexian2.& QIN Yachao1 1. institute of Environment & Biogeochemistry, Zhejiang University, Hangzhou 31002.,{2. 2. guangzhou Marine Geological Survey, CGS, MLR, guangzhou 510760,{2. 1. institute of Environment & Biogeochemistry Zhejiang University Hangzhou 310027 China 2. guangzhou Marine Geological Survey CGS MLR Guangzhou 510760 China

The environmental and biogeochemical information extracted from the sediments col- lected from the northern shelf of the South china Sea shows that terrigenous inputs of phosphorus into the sea remained relatively constant, and the variation of phosphorus contents at different depths was caused by climatic and environmental changes. The findings also suggest that the vertical varia- tion of phosphorus content was opposite to those of calcium carbonate and cadmium, and the func- tional correlation between CO2.and PO43? in seawater was given by calculating the chemical equilib- rium, indicating that the accumulation of marine sedimentary phosphorus may have something to do with the variation of atmospheric CO2. The decreased phosphorus accumulation as well as the cor- respondingly-increased calcium carbonate content might be one of key factors causing glacial at- mospheric CO2.decline.

关键词： sedimentary phosphorus, calcium carbonate, atmospheric CO2. northern shelf of the South china Sea, biogeochemistry.

Eclogites in the interior of the Tibetan Plateau and their geodynamic implications

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Chinese Science Bulletin 2009年第15期54卷 2556-2567页

作者： ZHANG KaiJun1,2.& TANG XianChun2.3 1 Department of Earth Sciences, Nanjing University, Nanjing 2.0093, china 2.guangzhou {2. of geochemistry, Chinese Academy of Sciences, guangzhou 51064., china 3 Graduate University of Chinese Academy of Sciences, Beijing 100049, china Department of Earth Sciences Nanjing University Nanjing 210093 China guangzhou institute of {2. Chinese Academy of Sciences Guangzhou 510640 China Graduate University of Chinese Academy of Sciences Beijing 100049 China

Eclogites have been recently reported in the interior of the Tibetan Plateau, including in the central Qiangtang metamorphic belt, in the Basu metamorphic massif of the eastern Bangong-Nujiang suture zone, and at Songdo and Pengco in the eastern Lhasa terrane. Some typical ultrahigh-pressure (UHP) metamorphic phenomena, e.g., garnet exsolution from clinopyroxene, were documented in the Basu and Pengco eclogites. The UHP metamorphism in the interior of the Tibetan Plateau marked by these eclogites generally took place in the Early Mesozoic. Along with exhumation of these eclogites, (post-) collision-related magmatism extensively occurred around the central Qiangtang belt, the eastern Ban-gong-Nujiang suture zone, and the eastern Lhasa terrane. The occurrence of these Early Mesozoic ec-logites manifests an out-of-sequence evolution of the Tethys, and they could be a product of diachro-nous collision between the eastern Qiangtang terrane and the irregular continental margin of the united western Qiangtang-Lhasa plate, along the linked eastern Bangong-Nujiang-central Qiangtang zone. The collision-related magmatic rocks could have been originated from lithospheric thickening, melting, or detachment due to the collision. The presence of UHP metamorphic rocks in central Qiangtang and Basu implies likely continental deep-subduction, and the denudation of these two metamorphic zones could have served as the source of the Triassic turbidites in the Songpan-Garzê complex and the Ju-rassic turbidites in the western Bangong-Nujiang zone, respectively. However, studies of the eclogites in the interior of the Tibetan Plateau just began, and many principal aspects still remain to be explored, such as their distributions, typical lithologies and minerals, temperature-pressure conditions, timing of formation and exhumation, protoliths and tectonic setting, and relationship with the evolution of the Tethys and large-scale basins in Tibet.

关键词：地球动力学意义青藏高原榴辉岩

Advances in the study of current-use non-PBDE brominated flame retardants and dechlorane plus in the environment and humans

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Science china Chemistry 2010年第5期53卷 961-973页

作者： LUO XiaoJun,CHEN SheJun,MAI BiXian & FU JiaMo State Key Laboratory of Organic geochemistry guangzhou {2. of geochemistry,Chinese Academy of Sciences,guangzhou 51064.,china 1. State Key Laboratory of Organic geochemistry Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China

The fate of the high production volume,currently in use,and not regulated non-polybrominated diphenyl ether(PBDE) flame retardants,such as tetrabromobisphenol A(TBBPA) ,hexabromocyclododecane(HBCD) and dechlorane plus(DP),and the alternative flame retardants of PBDE,such as BTBPE and DBDPE,in the environment has attracted increasing attention and aroused concern due to the increasing regulation and phasing-out of *** paper reviews the distribution,bioaccumulation,human exposure and environmental behavior of those non-PBDE flame retardants in various environmental *** data gaps and needs for future research are discussed.

关键词： TBBPA HBCD BTBPE DBDPE DP

Geochemical behavior of elements at fossil sea floor water/sediment interface

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Chinese Science Bulletin 1999年第S2期44卷 232-233页

作者： ZHANG Haihua~1, XIA Yu~1, WANG Zuwei~2.and ZHOU Yongzhang~3 1. guangzhou institute of {2., Chinese Academy of Science, guangzhou 51064., china 2. Department of Geography, Tianjin Normal University, Tianjin 300071, china 3. Department of Earth Sciences, Zhongshan University, guangzhou 5102.5, china guangzhou institute of {2. Chinese Academy of Science Guangzhou 510640 China Department of Geography Tianjin Normal University Tianjin 300071 China Department of Earth Sciences Zhongshan University Guangzhou 510275 China

THIS note deals with the geochemical behavior of elements near the water/sediment interface of a fossil seafloor. The Nandan-Hechi basin, located in northwest Guangxi, Southern china, is selected for exemplified study. It is an elongated basin, and developed on a Caledonian basement. Its Devonian strata hosthydrtothermally sedimentary formations, and are typical of the intra-platformal basin facies sediments oversouthern china. A steady sedimentary sequence may be observed, commonly going from carboniferouspelite at bottom, upward through bedded chert, thickly banded argillaceous limestone, thinly bandedsiliceous limestone and small lensiod argillaceous limestone in the middle, to coarse lensoid siliceousand/or argillaceous limestone at the top. The chert and some argillaceous limestone are related to hydrothermally sedimentary origin. The present study focuses on the lensoid argillaceous limestone formation. This formation contains the following characteristic sedimentary structures: small lensoid structure,vermiform structure, wave-shaped banded structure, massive structure, white framboid structure, andcage netting structure.

关键词： water/sediment interface sedimentation periodicity sedimentary geochemistry basin.

Superlarge ore deposits and development of china's mineral resources

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Chinese Science Bulletin 1999年第15期44卷 1436-1440页

作者： ZHAO Zhenhuaguangzhou institute of {2. , Chinese Academy of Sciences , guangzhou 51064., china Guangzhau institute of geochemistry Chinese Academy of Sciences Guangzhou China

The ever increasing demand of mineral resources in china was assessed and it is suggested that the development of superlarge ore deposits was the best way to meet such demand. Research and exploitation of superlarge ore deposits can bring great economic and social benefits to the society. It is also the best way to a better integration of resource industry development and environmental protection and therefore provides a basis of sustainable development of china. china has made important advancements in the research of superlarge ore deposits and especially in classification, selectivity and confinement of deposit types and temporal and spatial distributions. It is suggested that the metallodynamics and the interaction between the crust and the mantle and the core should be studied. At the same time, a new concept of resources should be established in order to build a new integrated system for research, and resource development and environmental proiection.

关键词： superlarge ore deposit metallodynamics resource-environmental integration.