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Geochemical characteristics of abiogenic alkane gases

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petroleum Science 2009年第4期6卷 327-338页

作者： Yunyan Ni Jinxing Dai Petrochina Res Inst Petr Explorat & Dev Beijing 100083 Peoples R China

Recently abiogenic alkanes have been found in various locations in the world and other celestial bodies. The chemical composition of abiogenic alkane gases varies widely. The content of methane is low and nearly no C2. is found in the abiogenic alkane gases from fluid inclusions in volcanic rocks or hot springs in china. In the unsedimented submarine hydrothermal vent system C1/C2. ratios are much greater than those for the thermogenic gases, mostly >800 and in some cases up to 8,000. In the Songliao Basin, china, C1/C2. of some abiogenic gases are often less than 150. Abiogenic alkane gases which have been found in nature often have carbon isotopic reversal among C1–C4 alkanes (δ13C1>δ13C2.δ13C3>δ13C4), whereas both regular and reversed hydrogen isotope distribution pattern among C1–C4 alkanes have been reported. The δ13C of abiogenic methane is mainly greater than ?30‰ though laboratory synthesized methane can have δ13C as low as ?57‰, and its δD1 values vary widely and overlap with biogenic gases. High 3He/4He ratios often indicate the addition of mantle-derived helium and are related to abiogenic gases. However, some biogenic gases can also have high 3He/4He ratios up to 8. The CH4/3He end-member is often lower than 106 for abiogenic alkane gases while greater than 1013 for biogenic gases, and the values between these two end-members often reflect the mixing of biogenic and abiogenic gases.

关键词： Abiogenic origin alkane gas carbon isotopic reversal trend geochemical characteristics

Geochemical characteristics of pyrolysis gas from epimetamorphic rocks in the northern basement of Songliao Basin,Northeast china

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Science china Earth Sciences 2008年第S1期51卷 140-147页

作者： YANG Chun 1 ,LUO Xia 2.,LI Jian 2.,LI ZhiSheng 2.,LIU QuanYou 3 &Wang YuLin 4 1 Department of Earth Sciences,Zhejiang University,Hangzhou 31002.,china 2.research {2. of petroleum exploration and Development(Langfang Branch),Langfang 065007,china 3 research {2. of petroleum exploration and Development,beijing 100083,china 4 Department of Source and Environment,Liaoning Technical University,Fuxin 12.000,china Department of Earth Sciences Zhejiang University Hangzhou China research institute of {2. exploration and Development (Langfang Branch) Langfang China research institute of {2. exploration and Development Beijing China Department of Source and Environment Liaoning Technical University Fuxin China

The Xushen gas field,located in the north of Songliao Basin,is a potential giant gas area for china in the *** proved reserves have exceeded 1000×10 8 m 3 by the end of ***,the origin of natural gases from the deep strata is still in *** rocks as a potential gas source are widely spreading in the northern basement of Songliao *** to pyrolysis experiments for these rocks in the semi-confined system,gas production and geochemistry of alkane gases are discussed in this *** Carboniferous-Permian epimetamorphic rocks were heated from 300℃to 550℃,with temperature interval of 50℃.The gas production was quantified and measured for chemical and carbon isotopic *** show thatδ13C 1 is less than?2.‰,carbon isotope trend of alkane gas isδ13C 1 2.2.>δ13C 3 ,these features suggest that the gas would be coal-type gas at high-over maturity,not be inorganic gas with reversal trend of gaseous alkanes (δ13C 1 >δ13C 2.>δ13C 3 ).These characteristics of carbon isotopes are similar with the natural gas from the basin basement,but disagree with gas from the Xingcheng ***,the mixing gases from the pyrolysis gas with coal-typed gases at high-over maturity or oil-typed gases do not cause the reversal trend of carbon *** gas generation intensity for epimetamorphic rocks is 3.0×10 8 ―2..8×10 8 m 3 /km 2.,corresponding to Ro from 2.0%to 3.5%for organic matter.

关键词： Northern Songliao Basin epimetamorphic rock pyrolysis experiment gas generation potential carbon isotope

Geological evolution of the Dongsha Uplift and its surrounding depressions in the South china Sea

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Acta Oceanologica Sinica 1989年第4期8卷 559-564页

作者： Li Desheng and Jiang Renqi research institute of {2. exploration and Development , P. O. Box 910. beijing 100083, china Res Inst petroleum exploration & Dev PO Vox 910 Beijing 100083 China

-The tectonic types of the Zhujiang (Pearl) River Mouth Basin in the South china Sea are epicontinental rift-depression basins. Prior to Early Cretaceous time, the Dongsha Uplift arid its surrounding depressions had been combined with the Eurasia Plate in a single unit. Many ENE-trending narrow rifted basins were formed in the third episode of Yanshan orogeny (Late Laramide). The rifted basins in the Paleocene and Eocene were stretched and extended, forming Zhu 1, Zhu 2.and Zhu 3 depressions. The Dongsha Uplift is located between Zhu 1 and Zhu 2.depressions . covering an area of 2. 000 Km2. Its geologic evolution can be divided into four stages:(1) Late Cretaceous - Paleocene block-faulting stage.(2. Eocene -Oligocene uplifting and eroding stage.(3) Late Oligocene - Early Miocene sustained subsiding stage.(4) Middle Miocene -Recent noncompensated subsiding *** Dongsha Uplift is a structural zone favourable for oil-gas accumulation.

关键词： Geological evolution of the Dongsha Uplift and its surrounding depressions in the South china Sea

GENETIC　CLASSIFICATION　AND　DISTRIBUTION　CHARACTERISTICS　OF　CONTINENTAL　petroleum　SYSTEMS　IN　china

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石油勘探与开发 1996年第1期23卷 92-98页

作者： Don Lirong Li Wei Fang Xiang(Pesearch institute of petroleum {2. and Development, CNPC, beijing 100083, P. R. china)

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关键词： petroleum province petroleum supersystem petroleum system Continental sedimentary basin china

Stratigraphic thermohistory and its implications for regional geoevolution in the Tarim Basin,NW china

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Science china Earth Sciences 2010年第10期53卷 1495-1505页

作者： WANG TieGuan1,DAI ShiFeng2.LI MeiJun1,ZHANG WeiBiao1,3,Qiu NanSheng1 & WANG GuangLi1 1 State Key Laboratory of petroleum Resources and Prospecting,china University of petroleum,beijing 102.49,china 2.State Key Laboratory of Coal Resources & Safe Mining,china University of Mining & Technology,beijing 100083,china 3 exploration research Center,exploration & Development {12.,china Petrochemical Corporation,beijing 100083,china State Key Laboratory of petroleum Resources and Prospecting China University of Petroleum Beijing China State Key Laboratory of Coal Resources & Safe Mining China University of Mining & Technology Beijing China exploration research Center Exploration & Development Institute China Petrochemical Corporation Beijing China

Fourteen vitrinite reflectance profiles from the Tarim Basin,NW china,show that the vitrinite reflectance profiles of individual wells follow a faulted and dislocated dual-stage pattern in the eastern section of the Tazhong Uplift and in the Tabei *** reflectance values in these profiles change sharply at the unconformity beneath the Lower Carboniferous Bachu or Upper Devonian Donghetang Formations,where the overlying Triassic to Carboniferous strata are still in a mature phase within the "liquid oil window".However,the underlying Lower Paleozoic reached the overmature phase beyond the "liquid oil window" towards the end of the Silurian,or in the Early Devonian at the *** the vitrinite reflectance profiles are attributed to a continuous,single-stage pattern in the western section of the Tazhong Uplift,in which the Lower Paleozoic is also in an overmature phase,their overmaturity would have been achieved relatively late in geological *** stratigraphic thermohistory has the following implications to regional geoevolution:(1) The overmature Lower Ordovician to Cambrian strata in the eastern section of the Tazhong Uplift and in the Tabei Uplift,as well as in the Manjiaer Depression,could not have acted as the source kitchen for normal oil(so-called black oil);(2. The dissimilarity in vitrinite reflectance profiles between the eastern and western sections of the Tazhong Uplift reveals Early Paleozoic paleotectonic features,i.e.,lower at the east and higher at the west,whereas recent tectonic features formed since the Late Paleozoic are in reverse,i.e.,higher in the east and lower at the west;(3) Reconstruction of the denuded thickness of sediments overlying the Lower Ordovician strata suggests reconsideration on the paleotectonic features in the Tarim Basin;(4) Based on the sustained duration of the "liquid oil window" for overmature source beds,it is predicted that the Suntuoguole Lower Uplift between the Awati and Manjiaer Depressions is a

关键词： vitrinite reflectance profile faulted and dislocated dual-stage pattern paleotectonic features sustained "liquid oil window" period source kitchen

The special sealing mechanism of caprock for Quaternary biogenetic gas in Sanhu area,Qaidam Basin,china

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Science china Earth Sciences 2008年第S1期51卷 45-52页

作者： LI Jian 1 ,YAN QiTuan 1 ,ZHANG Ying 1 ,LIU GuangDi 2.&WANG XiaoBo 1 1 research institute of {2. exploration and Development-Langfang,Langfang 065007,china 2.University of {2.,beijing 102.49,china research institute of {2. exploration and Development-Langfang Langfang China University of petroleum Beijing China

The Quaternary biogenetic gas reservoirs in the east of Qaidam Basin have many characteristics such as late forming time,shallow burial depth,low diagenetic grade,high porosity and high permeability and so *** cannot be considered as caprock according to the traditional evaluation ***, the large scale and high efficient biogenetic gas reservoirs of the Qaidam Basin are really formed under these kinds of caprocks,so it does have some specialty in its sealing *** at the special sealing mechanism,some simulating experiments have been *** research results show that the sealing ability of biogenetic gas caprock is related with water saturation,the caprock that is saturated with salt water can effectively block seepage and ***,the multiple reservoir-caprock groups have accumulated sealing effect,causing the formation of big gas *** evaluation method with traditional caprock parameters cannot be adopted in evaluating the study area.

关键词： Qaidam Basin biogenetic gas caprock sealing mechanism diffusion water saturation accumulated sealing

A method of identifying effective source rocks and its application in the Bozhong Depression,Bohai Sea,china

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petroleum Science 2010年第4期7卷 458-465页

作者： Jiang Fujie Pang Xiongqi Meng Qingyang Zhou Xiaohui Basin and Reservoir research Center China University of Petroleum Beijing 102249 China State Key Laboratory of petroleum Resource and Prospecting Beijing 102249 China research institute of {2. exploration and Development PetroChina Beijing 100083 China

research on effective source rocks directly affects the accuracy of identifying hydrocarbon resources, and indirectly affects the exploration decisions in petroliferous basins. Although the previous evaluation methods of effective source rocks vary relatively widely, a complete quantitative evaluation approach has not yet been developed. For that reason, we redefined the concept of effective source rocks based on the existing research results. Surrounding this definition, and guided by the hydrocarbon expulsion theory, the quantitative model called ＂two stages and three steps＂ method is established to predict effective source rocks. Its application in the Bozhong Depression indicates that among the four sets source rocks in the Bozhong Depression, the Member 3 of the Shahejie Formation （Es 3 ） has the largest effective source rock thickness, and the Member 1 Member 2.of the Shahejie Formation （Es 1＋2.） is the second largest .The effective part of dark mudstone is only 30%-80% of the total volume and with the increase of buried depth and improvement of quality, the effective part increases. Comprehensive analysis indicates that the ＂two stages and three steps＂ method is a practical technique for effective source rock prediction.

关键词： Source rock effectiveness hydrocarbon expulsion threshold Bozhong Depression Bohai Sea

Two conceptual models of displacement transfer and examples

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Science china Earth Sciences 2005年第7期48卷 900-911页

作者： GUAN Shuwei1,2. WANG Xin2. YANG Shufeng2. HE Dengfa1 & ZHAO Weidong3 1. research institute of {2. exploration and Development, beijing 100083, china 2. Department of Geosciences, Zhejiang University, Hangzhou 31002., china 3. Tarim Oilfield Company, Korla 841000, china research institute of {2. exploration and Development Beijing 100083 China Department of Geosciences Zhejiang University Hangzhou 310027 China Tarim Oilfield Company Korla 841000 China

This paper presents two conceptual models of displacement transfer, reverse sym- metry model and infinitely equal division model, based on the fault-bend folding theory. If the fault shape is held constant in the trend, then the distribution of slip magnitude, geometry of imbricate structures and its axial surface map all display reverse symmetry on the process of displacement transfer, as called reverse symmetry model in this paper. However, if the ramp height of thrust fault decreases gradually along its strike, the displacement is postulated to be equally and infinitely divided to every thrust that is formed subsequently, this kinematic process is described using infinitely equal division model. In both models, displacement transfer is characterized by the regular changes of imbricate thrusting in the trend. Geometric analysis indicates that the displacement transfer grads can be estimated using the tangent of deflective angle of hinterland structures. Displacement transfer is often responsible for the distortion and branching of the surface anticlines, especially in the region where the multi-level detachment structures is developed. We also present some examples from the frontal structures of the Southern Tianshan fold-and-thrust belt, Xinjiang, china. Displacement transfer between deep imbricate thrusts in the middle segment of Qiulitag anticline zone causes the Kuqatawu and Southern Qiulitag deep an- ticlines left-lateral echelon. The region, where these two deep anticlines overlap, is characterized by duplex structures, and extends about 18 km. The shallow anticline is migrated southward displaying obvious “S” form in this area.

关键词： displacement transfer fault-bend folding reverse symmetry model infinitely equal division model Qiulitag zone.

Application of C5-C13 light hydrocarbons in depositional environment diagnosis

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Progress in Natural Science:Materials International 2008年第9期18卷 1129-1137页

作者： Peirong Wanga,b,, Guanjun Xu a,c, Tingrong Xiaoc, Dajiang Zhanga,c, Bin Zhanga,c a Key Laboratory of petroleum Geochemistry, china National petroleum Corporation, beijing 100083, china b Department of Organic Geochemistry, Yangtze University, Jingzhou 43402., china c Central Laboratory of petroleum Geology, research institute of petroleum exploration and Development, Petrochina, beijing 100083, china Key Laboratory of petroleum Geochemistry China National Petroleum Corporation Beijing 100083 China Department of Organic Geochemistry Yangtze University Jingzhou 434023 China Central Laboratory of petroleum Geology Research Institute of Petroleum Exploration and Development PetroChina Beijing 100083 China

Based on the geological background and Gammacerane/C31H(S + R) ratios, source rock depositional environments of the studied oil samples (194) from 13 oilfields were classified into three groups according to salinity:saline-lacustrine facies, fresh to brackish lacustrine facies (including limnetic facies), and semi-saline to saline facies (including marine facies of the Tarim Basin).C5-C13 compound groups in the crude oils were separated by GC, and about 2.6 compounds were qualitatively *** geochemical application of the C6-C13 compound groups and their ratios between each group with individual carbon number was *** studies show that (1) C6-C13 compound groups and their ratios in the crude oils could serve as new reliable parameters for oil-oil correlation because the C6-C13 light fractions are the major oil component, especially in light oil or condensate, in which they account for almost 90% of the whole oil;(2. the compound groups of C7 light hydrocarbons in oils derived from difierent depositional environments with difierent salinity have difierent characteristics;(3) C6-C13 compound groups and ratios may be afiected by other factors such as maturity, but they are mainly controlled by salinity of depositional waters.

关键词： Light hydrocarbons Crude oil Depositional environment Salinity