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Diagenesis and Restructuring Mechanism of Oil and Gas Reservoir in the Marine Carbonate Formation,Northeastern Sichuan:A Case Study of the Puguang Gas Reservoir

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Acta Geologica Sinica(English Edition) 2009年第6期83卷 1173-1181页

作者： DU Chunguo1, 2. WANG Jianjun1, ZOU Huayao2. ZHU Yangming3 and WANG Cunwu4 1 research Institute of petroleum {2. and development, Beijing 100034, china 2.petroleum University of china, Beijing 102.49, china 3 Department of Earth Science, Zhejiang University, Hangzhou 31002., china 4 Faculty of Earth Resources, china University of Geosciences, Wuhan 430074, china Faculty of Earth Resources China University of Geosciences Wuhan 430074 China

Based on the technology of balanced cross-section and physical simulation experiments associated with natural gas geochemical characteristic analyses, core and thin section observations, it has been proven that the Puguang gas reservoir has experienced two periods of diagenesis and restructuring since the Late Indo-Chinese epoch. One is the fluid transfer controlled by the tectonic movement and the other is geochemical reconstruction controlled by thermochemical sulfate reduction (TSR). The middle Yanshan epoch was the main period that the Puguang gas reservoir experienced the geochemical reaction of TSR. TSR can recreate the fluid in the gas reservoir, which makes the gas drying index higher and carbon isotope heavier because C2. (ethane and heavy hydrocarbon) and 12. (carbon 12.isotope) is first consumed relative to CH4 and 13C (carbon 13 isotope). However, the reciprocity between fluid regarding TSR (hydrocarbon, sulfureted hydrogen (H2.) , and water) and reservoir rock results in reservoir rock erosion and anhydrite alteration, which increases porosity in reservoir, thereby improving the petrophysical properties. Superimposed by later tectonic movement, the fluid in Puguang reservoir has twice experienced adjustment, one in the late Yanshan epoch to the early Himalayan epoch and the other time in late Himalayan epoch, after which Puguang gas reservoir is finally developed.

关键词： diagenesis and restructuring mechanism marine carbonate formation thermochemical sulfate reduction Puguang gas reservoir

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Mechanism of catalytic hydropyrolysis of sedimentary organic matter with MoS_2

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petroleum Science 2011年第2期8卷 134-142页

作者： He Kun Zhang Shuichang Mi Jingkui Chen Jianping Cheng Lei petroleum Geology research and Central Laboratory Research Institute of Petroleum Exploration and Development （RIPED） PetroChina Beijing 100083 China CNPC Key Laboratories for petroleum Geochemistry Beijing 100083 China

MoS2.was used as an efficient catalyst for hydropyrolysis （Hypy） of three samples of sedimentary organic matter with different maturities. Through comparison with Soxhlet extraction （SE）, it was found that MoS2.catalytic Hypy can remarkably promote the yields of total chloroform extracts, saturates, aromatics, hopanes and steranes. In addition, the difference of biomarker parameters indicated that isomerization of covalently-bound biomarkers is much more difficult than their free counterparts. Meanwhile, the high conversion of total organic carbon （TOC） in MoS2.catalytic Hypy of organic matter proved that the presence of dispersed molybdenum sulfide accelerated the breaking of C-C bonds and the release of hydrocarbons. To address the catalytic mechanism, a series of control experiments based on free Hypy and catalytic Hypy were conducted. The results showed that the calculated atomic ratio of carbon conversion/hydrogen conversion for catalytic Hypy was much larger than the presumed value of 1/2. indicating that intensive hydrogenation took place and significantly influenced the distribution of liquid products. Analysis of stable hydrogen isotope data, infrared spectra and m/z 83 ion chromatograph of the saturate fraction further confirmed this hypothesis. The difference of S content changing （AS） between catalyst-free Hypy and catalytic Hypy, and the thermal characteristics of the catalyst, indicated that active H2. was definitely generated and it probably initiated free radical reactions in the early stage of hydropyrolysis of organic matter.

关键词： Catalytic hydropyrolysis molybdenum disulfide kerogen coal Soxhlet extraction,biomarkers

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Numerical simulation and application of three-dimensional oil resources migration-accumulation of fluid dynamics in porous media

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Science china(Physics,Mechanics & Astronomy) 2008年第8期51卷 1144-1163页

作者： YUAN YiRang1 & HAN YuJi2.1 Institute of Mathematics,Shandong University,Ji’nan 2.0100,china 2.Physical exploration Institute of Shengli {2. Administration,Dongying 2.702.,china Institute of Mathematics Shandong University Ji’nan 250100 China Physical exploration Institute of Shengli petroleum Administration Dongying 257022 China

Numerical simulation of oil migration and accumulation is to describe the history of oil migration and accumulation in basin evolution. It is of great value in evaluation of oil resources and determination of the location and amount of oil deposits. Based on such actual conditions as the effects of fluid mechanics in porous media and 3-dimensional geology characteristics,a kind of modified method of second order upwind finite difference fractional steps implicit interactive scheme was put forward. As for the actual problem of Dongying hollow,Huimin hollow,Tanhai region and Yangxin hollow in Shengli petroleum Oil Field,a numerical simulation test was carried out,and the result is basically coincident with the actual conditions. For the model problem,optimal order estimates were derived. Thus the well-known problem on oil resources was solved.

关键词： nonlinear mechanics of immiscible flow 3-dimensional migration-accumulation of oil resources upwind fractional steps numerical simulation numerical analysis

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Prediction of petroleum exploration risk and subterranean spatial distribution of hydrocarbon accumulations

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petroleum Science 2011年第1期8卷 17-23页

作者： Xie Hongbing Guo Qiulin Li Feng Li Jianzhong Wu Na Hu Suyun Liang Kun School of Energy Resources China University of GeosciencesBeijing 100083China research Institute of petroleum {2. ＆ development PetroChinaBeijing 100083China Science ＆ Technology Management Department China National Petroleum CorporationBeijing 100007China

Investigation of spatial distribution of oil and gas resource and accurate prediction of the geographic location of its undiscovered resource is significant for reducing exploration risk and improving exploration benefit.A new method for predicting spatial distribution of oil resource is discussed in this *** consists of prediction of risk probability in {2. exploration and simulation of hydrocarbon abundance. exploration risk probability is predicted by multivariate statistics,fuzzy mathematics and information processing techniques.A spatial attribute database for sample wells was set up and the Mahalanobis distance and Fuzzy value of given samples were ***,the Bayesian formula was used to calculate the hydrocarbon-bearing probability at the area of exploration ***,a hydrocarbon probability template is formed and used to forecast the probability of the unknown area. The hydrocarbon abundance is simulated based on Fourier integrals,frequency spectrum synthesis and fractal ***,the fast Fourier transformation（FFT） is used to transform the known hydrocarbon abundance from the spatial domain to the frequency domain,then,frequency spectrum synthesis is used to produce the fractal frequency spectrum,and FFT is applied to get the phase information of hydrocarbon-bearing ***,the frequency spectrum simulation is used to calculate the renewed hydrocarbon abundance in the play. This method is used to predict the abundance and possible locations of the undiscovered {2. accumulations in the Nanpu Sag of the Bohai Bay Basin,*** prediction results for the well-explored onshore area of the northern Nanpu Sag agree well with the actual *** the less-explored offshore areas in the southern Nanpu Sag,the prediction results suggest high hydrocarbon abundance in Nanpu-1 and Nanpu-2.providing a useful guiding for future exploration.

关键词： Hydrocarbon resources abundance risk forecast Nanpu sag frequency spectrum simulation fractal theory

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Natural gas origins of large and medium-scale gas fields in china sedimentary basins

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Science china Earth Sciences 2008年第S1期51卷 1-13页

作者： ZHANG ShuiChang &ZHU GuangYou research Center of research Institutes of {2.china exploration and development,Beijing 100083,china research Center of research Institutes of {2.china exploration and development Beijing 100083 China

china sedimentary basins present abundant natural gas resource thanks to its unique geological *** highly-matured hydrocarbon source rocks,widespread coal-measure strata and low temperature Quaternary saline strata,etc.,indicate the wide foreground of china natural gas resources. Up to now,most of the {2.liferous basins have been discovered to have wholesale natural gas accumulation from Precambrian,Paleozoic,Mesozoic to Cenozoic in the east,the central,the west and the coast of *** large and medium-scale gas reservoirs are mainly composed of hydrocarbon gas with big dry coefficient,tiny non-hydrocarbon,wide carbon isotope distribution and varying origin types,the hydrocarbon gas includes coal-formed gas,oil-formed gas,biogenic gas and inorganic gas, ***-formed gas is the main type of china natural gas resources,in particular several explored large-scale gas fields(>100 billion cubic meter)of Kela 2.Sulige and Daniudi,etc.,they all belong to coal-formed gas fields or the gas fields consisting mostly of coal-formed ***-formed gas is also abundant in china marine basins,for example marine natural gas of Sichuan Basin generated from crude oil cracking *** and secondary biogenic gas fields were discovered respectively in the Qaidam Basin and Western Slope of Songliao *** addition,inorganic gases are mainly distributed in the eastern china,in particular the Songliao Basin with abundant carbon dioxide accumulation,indicating that the eastern china present large exploration potential of inorganic gas.

关键词： natural gas origin sedimentary basin large and medium-scale gas field

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ESTABLISHMENT OF THE GEOLOGICAL MODEL OF FRACTURED RESERVOIRS

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石油勘探与开发 1995年第6期22卷 90-97页

作者： Mu Long-xin (research Institute of petroleum {2. and development, CNPC)

ＥＳＴＡＢＬＩＳＨＭＥＮＴＯＦＴＨＥＧＥＯＬＯＧＩＣＡＬＭＯＤＥＬＯＦＦＲＡＣＴＵＲＥＤＲＥＳＥＲＶＯＩＲＳ￥ＭｕＬｏｎｇ－ｘｉｎ（ＲｅｓｅａｒｃｈＩｎｓｔｉｔｕｔｅｏｆＰｅｔｒｏｌｅｕｍＥｘｐｌｏｒａｔｉｏｎａｎｄ... 详细信息

ＥＳＴＡＢＬＩＳＨＭＥＮＴＯＦＴＨＥＧＥＯＬＯＧＩＣＡＬＭＯＤＥＬＯＦＦＲＡＣＴＵＲＥＤＲＥＳＥＲＶＯＩＲＳ￥ＭｕＬｏｎｇ－ｘｉｎ（ＲｅｓｅａｒｃｈＩｎｓｔｉｔｕｔｅｏｆＰｅｔｒｏｌｅｕｍＥｘｐｌｏｒａｔｉｏｎａｎｄＤｅｖｅｌｏｐｍｅｎｔ，ＣＮＰＣ）...

关键词： Fracture Geological model Low permeability sandstone oil field

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Complex petroleum accumulating process and accumulation series in the buried-hill trend in the rift basin:An example of Xinglongtai structure trend,Liaohe subbasin

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Science china Earth Sciences 2008年第S2期51卷 108-116页

作者： GAO XianZhi1,PANG XiongQi1,LI XiaoGuang2.CHEN ZhenYan2.SHAN JunFeng2.LIU Feng1,ZOU ZhiWen1 & Li WeiLian1 1 Faculty of Resources and Information Technology,china University of petroleum,Beijing 102.49,china 2.exploration and development Institute of Liaohe Oilfield,petrochina Liaohe Oil Company,Panjin 12.010,china china Univ Petr Fac Resources & Informat Technol Beijing 102249 Peoples R China petrochina Liaohe Oil Co Explorat & Dev Inst Liaohe Oilfield Panjin 124010 Peoples R China

The buried-hill trend is a typical style of the petroliferous structure in the faulted basin of eastern china. The Xinglongtai structure trend in the Liaohe subbasin,Bohai Bay Basin is a buried faulted-hill trend resulting from the periodic faulting of the Tai’an-Dawa faults. The structure was cut by various faults,which are interlinked and constitute the conduits for {2. migration. {2. accumulated in the Tertiary sandstones and pre-Tertiary basement of metamorphosed rocks through the migration pathways of the fault system. {2. in the structure was derived from different hydrocarbon kitchens to form a hybrid field complex. {2. charged the structure from different directions and accumulated in various reservoirs through different pathways in different times. The accumulations in the buried hill trend of Xingongtai are composed of two types of traps in the two stratigraphic systems: traps in the Tertiary sandstones were formed by the fault blocks and by the pinchout of the sandstone,and traps in the pre-Tertiary basement of metamorphosed rocks were formed by fissures in the inner part of the buried hills and by the unconformity near the surface of the buried hills.

关键词： faulted basin petroleum migration and accumulation petroleum occurrence buried hills Achaean basement Liaohe subbasin Bohai Bay basin

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Genetic types and distribution of shallow-buried natural gases

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petroleum Science 2010年第3期7卷 347-354页

作者： Gao Yang Jin Qiang Zhu Guangyou College of Geo-resources and Information China University of Petroleum Dongying Shandong 257061 China petroleum exploration and {2. Institute PetroChina Beijing 100083 China

Great volumes of shallow-buried （〈2.000 m） natural gases which are mainly composed of biogases and low-mature gases have been found in the Mesozoic-Cenozoic sedimentary basins in china. Many shallow gas reservoirs in china are characterized by coexistence of biogas and low-mature gas, so identifying the genetic types of shallow gases is important for {2. and development in sedimentary basins. In this paper, we study the gas geochemistry characteristics and distribution in different basins, and classify the shallow gas into two genetic types, biogas and low-mature gas. The biogases are subdivided further into two subtypes by their sources, the source rock-derived biogas and hydrocarbon-derived biogas. Based on the burial history of the source rocks, the source rock-derived biogases are divided into primary and secondary biogas. The former is generated from the source rocks in the primary burial stage, and the latter is from uplifted source rocks or those in a secondary burial stage. In addition, the identifying parameters of each type of shallow gas are given. Based on the analysis above, the distributions of each type of shallow gas are studied. The primary biogases generated from source rocks are mostly distributed in Quaternary basins or modem deltas. Most of them migrate in watersoluble or diffused mode, and their migration distance is short. Reservoir and caprock assemblages play an important role in primary biogas accumulation. The secondary biogases are distributed in a basin with secondary burial history. The oil-degraded biogases are distributed near heavy oil pools. The low-mature gases are widely distributed in shallow-buried reservoirs in the Meso-Cenozoic basins.

关键词： Primary biogas secondary biogas oil-degraded biogas low-mature gas genetic type gas identification gas accumulation distribution

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Wide/narrow azimuth acquisition footprints and their effects on seismic imaging

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petroleum Science 2008年第4期5卷 308-313页

作者： Di Bangrang Xu Xiucang Wei Jianxin Key Laboratory of CNPC Geophysical exploration China University of Petroleum Beijing 102249 China State Key Laboratory of petroleum Resource and Prospecting China University of Petroleum Beijing 102249 China Key Laboratory of Earth Prospecting and Information Technology China University of Petroleum Beijing 102249 China

Acquisition footprint is a new concept to describe the seismic noise in three-dimensional seismic exploration and it is closely related to geometry and observation shuttering. At present, the study on acquisition footprints has become a hot spot. In partnership with the Dagang Oilfield, we used the channel sand body seismic physical model to study the characteristics of wide/narrow azimuth acquisition footprints and analyzed and compared the two types of footprints and their effects on target imaging. In addition, the footprints caused by data processing of the normal moveout offset （NMO） stretching aberration were discussed. These footprints are located only in the shallow or middle layer in the time slice, and possibly affect the imaging of shallow target layers, and have no influence on deep target imaging. Seismic physical modeling has its advantages in the study of acquisition footprints.

关键词： Wide/narrow azimuth geometry acquisition footprint stretching aberration time slice seismic imaging

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Potential risks of spectrum whitening deconvolution——compared with well-driven deconvolution

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petroleum Science 2009年第2期6卷 146-152页

作者： Li Guofa Zhou Hui Zhao Chao State Key Laboratory of petroleum Resource and Prospecting China University of Petroleum Beijing 102249 China Key Laboratory of CNPC Geophysical exploration China University of Petroleum Beijing 102249 China

Deconvolution is widely used to increase the resolution of seismic data. To compare the resolution ability of conventional spectrum whitening deconvolution to thin layers with that of welldriven deconvolution, a complex sedimentary geological model was designed, and then the simulated seismic data were processed respectively by each of the two methods. The amplitude spectrum of seismic data was almost white after spectrum whitening, but the wavelet resolution was low. The amplitude spectrum after well-driven deconvolution deviated from white spectrum, but the wavelet resolution was high. Further analysis showed that if an actual reflectivity series could not well satisfy the hypothesis of white spectrum, spectrum whitening deconvolution had a potential risk of wavelet distortion, which might lead to a pitfall in high resolution seismic data interpretation. On the other hand, the wavelet after well- driven deconvolution had higher resolution both in the time and frequency domains. It is favorable for high resolution seismic interpretation and reservoir prediction.

关键词： Well-driven high resolution spectrum whitening deconvolution seismic wavelet

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