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Gas formation mechanism of marine carbonate source rocks in china

Science china Earth Sciences 2005年第4期48卷 441-453页

作者： ZHAO Wenzhi1, WANG Zhaoyun1, HE Haiqing2. ZHANG Mingjie3, WANG Hongjun1, WANG Yunpeng4 & QIN Yong5 1. research Institute of petroleum {2. & development, petrochina, beijing 100083. china 2. petrochina {2. & Production, beijing 100011, china 3. Department of Geology, Lanzhou University, Lanzhou 730000, china 4. Guangzhou Geochemical Institute, Chinese Academy of Sciences, Guangzhou 510640, china 5. china University of Mining and Technology, Xuzhou 2.1000, china 1. research Institute of petroleum {2. & development 100083 PetroChinaBeijin China 2. petrochina exploration & Production 100011 Beijing China 3. Department of Geology Lanzhou University 730000 Lanzhou China 4. Guangzhou Geochemical Institute Chinese Academy of Sciences 510640 Guangzhou China 5. china University of Mining and Technology 221000 Xuzhou China

By breaking through the conventional ideology on the study of gas-formation mechanism of source rocks which focused on merely the characteristics of source rocks them- selves, and based on the development and distribution characteristics of marine carbonate source rocks in the medium-to-bottom parts of the Chinese superimposed sedimentary basins as well as various processes in the course of gas generation and reservoir forming, the complex hydrocarbon-generating model of carbonates is established. Such a model concerns not only the “three-stage” gas formation characteristics of carbonates, but also the gas generation process due to a thermal cracking of oil and the re-generation process of gas from heated secondary organic matters during the gas-generation and reservoir-forming course. The high-quality hy- drocarbon generating matter of marine carbonate source rocks determined a high gas-oil ratio and tended to form paleo-oil-reservoirs, representing an enrichment process of organic matters. The thermal cracking of oil in palaeo-oil-reservoirs is an important means for the effective forma- tion of gas reservoirs. The secondary organic matters in carbonate reservoirs may regenerate gas after a secondary deep burial, thus becoming an effective gas source.

关键词： carbonate, three-stage hydrocarbon generation, inhibitive effect of maturity, oil-cracking gas, second-ary asphalt gas.

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CHARACTERISTICS　OF　COAL－FORMED　GAS　ACCUMULATION　BELTS　IN　THE　EAST　PART　OF　THE　CENTRAL－ASIA　COAL－FORMED　GAS　ACCUMULATION　DOMAIN　──SERIES　STUDY　Ⅲ　ON　THE　CENTRAL－ASIA　COAL－FORMED　GAS　ACCUMULATION　DOMAIN

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石油勘探与开发 1995年第5期22卷 87-95页

作者： Dai Jin-xing Li Xian-qi(research Institute of petroleum {2. and development, CNPC. beijing, 100083. P. R. china)

ＣＨＡＲＡＣＴＥＲＩＳＴＩＣＳＯＦＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＢＥＬＴＳＩＮＴＨＥＥＡＳＴＰＡＲＴＯＦＴＨＥＣＥＮＴＲＡＬ－ＡＳＩＡＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＤＯＭＡ... 详细信息

ＣＨＡＲＡＣＴＥＲＩＳＴＩＣＳＯＦＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＢＥＬＴＳＩＮＴＨＥＥＡＳＴＰＡＲＴＯＦＴＨＥＣＥＮＴＲＡＬ－ＡＳＩＡＣＯＡＬ－ＦＯＲＭＥＤＧＡＳＡＣＣＵＭＵＬＡＴＩＯＮＤＯＭＡＩＮ──ＳＥＲＩＥＳＳＴＵＤＹⅢＯ...

关键词： GAS FORMED COAL ACCUMULATION BELTS ASIA EAST

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AN APPROACH TO CUTTINGS FLUOROLOGGING USING HEXANE AS A SUBSTITUTE

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石油勘探与开发 1997年第4期24卷 92-96页

作者： Zhao Juying(research Institute of petroleum {2. and Devempment, CNPC, beijing, 100083.

It is discovered that carbon tetrachloride is a fluorescence quencher in crude oil detedion with cottings fluorologging. Hexane, which has many advantages as a substitute for carbon tetrachloride, is proposed. In this paper, four typical comparison results of fluorescence spectra of crude oil samples and some of field cores and cuttings are *** sensitivity of fluorescence analysis is increased by 10 to 35 times when we substitute hexane for carbon tetrachloride as the solvent of crude oil. We also find that the lighter the crude oil,the more Obvious the increase in analysis sensitivity. lt challenges the old concopt that coal-derived oil, condensate and some light oils do not emit fluorescence. The merit of hexane system in eliminating or reducing the fluorescent interference of modified asphalts in drilling fluids for cuttings fluorologging has also been discussed.

关键词： Cuttings logging Fluorescence analysis Hexane Carbon tetrachloride Crude oil (Fluorescence quench)

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Primary migration and secondary alteration of the Upper Paleozoic gas reservoir in Ordos Basin,china―Application of fluid inclusion gases

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Science china Earth Sciences 2008年第S1期51卷 165-173页

作者： GONG Se 1,2.,PENG PingAn 1 ,SHUAI YanHua 3 ,DAI JinXing 3 &ZHANG WenZheng 4 1 Guangzhou Institute of Geochemistry,the Chinese Academy of Sciences,Guangzhou 510640,china 2.Common Wealth Scientific and research Organization,{2. Resources,PO Box 136,North Ryde,New South Wales,1670,Australia 3 research Institute of {2. exploration and development,petrochina,beijing 100083.china 4 research Institute of exploration and development,Changqing {2. Corporation,Xi’an 71002.,china Guangzhou Institute of Geochemistry the Chinese Academy of Sciences Guangzhou 510640 China Common Wealth Scientific and research Organization Petroleum Resources PO Box 136 North Ryde New South Wales 1670 Australia research Institute

The composition of fluid inclusions(FI)often represents the initial geochemical characteristics of palaeo-fluid in reservoir *** on composition and carbon isotopic composition of gas during primary migration,reservoir-forming and subsequent secondary alterations are discussed through comparing fluid inclusion gas with coal-formed gas and natural gas in present gas reservoirs in the Ordos *** results show that primary migration of gas has significant effect on the molecular but not on the carbon isotopic composition of *** and diffusion fractionation took place during the secondary migration of gas in Upper Paleozoic gas reservoir according to carbon isotopic composition of methane in *** and carbon isotopic composition of natural gas were nearly unchanged after the gas reservoir forming through comparing the FI gases with the natural gas in present gas reservoir.

关键词： secondary alteration fluid inclusion carbon isotope Ordos Basin

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Genetic types and distribution of shallow-buried natural gases

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petroleum Science 2010年第3期7卷 347-354页

作者： Gao Yang Jin Qiang Zhu Guangyou College of Geo-resources and Information China University of Petroleum Dongying Shandong 257061 China petroleum exploration and {2. Institute PetroChina Beijing 100083 China

Great volumes of shallow-buried （〈2.000 m） natural gases which are mainly composed of biogases and low-mature gases have been found in the Mesozoic-Cenozoic sedimentary basins in china. Many shallow gas reservoirs in china are characterized by coexistence of biogas and low-mature gas, so identifying the genetic types of shallow gases is important for {2. and development in sedimentary basins. In this paper, we study the gas geochemistry characteristics and distribution in different basins, and classify the shallow gas into two genetic types, biogas and low-mature gas. The biogases are subdivided further into two subtypes by their sources, the source rock-derived biogas and hydrocarbon-derived biogas. Based on the burial history of the source rocks, the source rock-derived biogases are divided into primary and secondary biogas. The former is generated from the source rocks in the primary burial stage, and the latter is from uplifted source rocks or those in a secondary burial stage. In addition, the identifying parameters of each type of shallow gas are given. Based on the analysis above, the distributions of each type of shallow gas are studied. The primary biogases generated from source rocks are mostly distributed in Quaternary basins or modem deltas. Most of them migrate in watersoluble or diffused mode, and their migration distance is short. Reservoir and caprock assemblages play an important role in primary biogas accumulation. The secondary biogases are distributed in a basin with secondary burial history. The oil-degraded biogases are distributed near heavy oil pools. The low-mature gases are widely distributed in shallow-buried reservoirs in the Meso-Cenozoic basins.

关键词： Primary biogas secondary biogas oil-degraded biogas low-mature gas genetic type gas identification gas accumulation distribution

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THE CHARACTERISTICS OF REMOTE SENSING TECTONICS IN QIANGTANG-CHANGDU MASSIF, QINGHAI-TIBET PLATEAU

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地学前缘 2000年第S1期7卷 435-437页

作者： Zhao Zhengzhang 1,Ye Hefei 2.Li Yongtie 2.1 china National petroleum Corporation, {2. 10072.,china 2.research Institute of petroleum exploration and development, CNPC, {2. 100083.china)

The northern Tibet plateau is the core of generalized Qinghai—Tibet plateau. The main part of Qiangtang—Changdu massif, which is 45×10 4km 2.and more than 5000m in altitude, conforms to the northern Tibet plateau in area.1 The shape features and boundary conditions of Qiangtang—Changdu massif\;(1) Qiangtang—Changdu massif shows huge flat\|lying “S” area In MSS7 mosaic image, Qiangtang—Changdu massif extends in west and east, and appears a long\|elliptic huge block composed of feathered and dendritic textures.. Noticeably, there are two similar texture “tails" in the west and east ends of the massif. The western tail turns and constringes to the north, and eastern tail to the south. Thereby, the massif shows huge “S" area. According to the regional analysis, the eastern tail locates between Shaluli Mt.\|Taniantaweng Mt. and Mujiang River, and western part through Bangong\|Co connects with Pamirs along Karakoram Mt. In regional tectonics, the massif locates between Lazhulong\|Xijinwulan\|Co\|Jinshajiang River and Bangong\|Co\|Dongqiao\|Nujiang River fault belts.

关键词： Qiangtang—Changdu massif remote sensing boundary condition circular structure deformin g features mechanic characteristic dynamics

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Micro-mechanisms of residual oil mobilization by viscoelastic fluids

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petroleum Science 2008年第1期5卷 56-61页

作者： Zhang Lijuan Yue Xiang＇an Guo Fenqiao Key Laboratory of petroleum Engineering Ministry of Education China University of Petroleum Beijing 102249 China development Department Sinopec Exploration and Production Research Institute Beijing 100083 China

Four typical types of residual oil, residual oil trapped in dead ends, oil ganglia in pore throats, oil at pore corners and oil film adhered to pore walls, were studied. According to main pore structure characteristics and the fundamental morphological features of residual oil, four displacement models for residual oil were proposed, in which pore-scale flow behavior of viscoelastic fluid was analyzed by a numerical method and micro-mechanisms for mobilization of residual oil were discussed. Calculated results indicate that the viscoelastic effect enhances micro displacement efficiency and increases swept volume. For residual oil trapped in dead ends, the flow field of viscoelastic fluid is developed in dead ends more deeply, resulting in more contact with oil by the displacing fluid, and consequently increasing swept volume. In addition, intense viscoelastic vortex has great stress, under which residual oil becomes small oil ganglia, and finally be carried into main channels. For residual oil at pore throats, its displacement mechanisms are similar to the oil trapped in dead ends. Vortices are developed in the depths of the throats and oil ganglia become smaller. Besides, viscoelastic fluid causes higher pressure drop on oil ganglia, as a driving force, which can overcome capillary force, consequently, flow direction can be changed and the displacing fluid enter smaller throats. For oil at pore corners, viscoelastic fluid can enhance displacement efficiency as a result of greater velocity and stress near the corners. For residual oil adhered to pore wall, viscoelastic fluid can provide a greater displacing force on the interface between viscoelastic fluid and oil, thus, making it easier to exceed the minimum interfacial tension for mobilizing the oil film.

关键词： Viscoelastic chemical flooding displacement mechanism residual oil swept volume

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Stratigraphic thermohistory and its implications for regional geoevolution in the Tarim Basin,NW china

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Science china Earth Sciences 2010年第10期53卷 1495-1505页

作者： WANG TieGuan1,DAI ShiFeng2.LI MeiJun1,ZHANG WeiBiao1,3,Qiu NanSheng1 & WANG GuangLi1 1 State Key Laboratory of petroleum Resources and Prospecting,china University of petroleum,beijing 102.49,china 2.State Key Laboratory of Coal Resources & Safe Mining,china University of Mining & Technology,beijing 100083.china 3 exploration research Center,exploration & {12. Institute,china Petrochemical Corporation,beijing 100083.china 1. State Key Laboratory of petroleum Resources and Prospecting China University of Petroleum Beijing 102249 China2. State Key Laboratory of Coal Resources & Safe Mining China University of Mining & Technology Beijing 100083 China3. Exploration Research Center Exploration & Development Institute China Petrochemical Corporation Beijing 100083 China

Fourteen vitrinite reflectance profiles from the Tarim Basin,NW china,show that the vitrinite reflectance profiles of individual wells follow a faulted and dislocated dual-stage pattern in the eastern section of the Tazhong Uplift and in the Tabei *** reflectance values in these profiles change sharply at the unconformity beneath the Lower Carboniferous Bachu or Upper Devonian Donghetang Formations,where the overlying Triassic to Carboniferous strata are still in a mature phase within the "liquid oil window".However,the underlying Lower Paleozoic reached the overmature phase beyond the "liquid oil window" towards the end of the Silurian,or in the Early Devonian at the *** the vitrinite reflectance profiles are attributed to a continuous,single-stage pattern in the western section of the Tazhong Uplift,in which the Lower Paleozoic is also in an overmature phase,their overmaturity would have been achieved relatively late in geological *** stratigraphic thermohistory has the following implications to regional geoevolution:(1) The overmature Lower Ordovician to Cambrian strata in the eastern section of the Tazhong Uplift and in the Tabei Uplift,as well as in the Manjiaer Depression,could not have acted as the source kitchen for normal oil(so-called black oil);(2. The dissimilarity in vitrinite reflectance profiles between the eastern and western sections of the Tazhong Uplift reveals Early Paleozoic paleotectonic features,i.e.,lower at the east and higher at the west,whereas recent tectonic features formed since the Late Paleozoic are in reverse,i.e.,higher in the east and lower at the west;(3) Reconstruction of the denuded thickness of sediments overlying the Lower Ordovician strata suggests reconsideration on the paleotectonic features in the Tarim Basin;(4) Based on the sustained duration of the "liquid oil window" for overmature source beds,it is predicted that the Suntuoguole Lower Uplift between the Awati and Manjiaer Depressions is a

关键词： vitrinite reflectance profile faulted and dislocated dual-stage pattern paleotectonic features sustained "liquid oil window" period source kitchen

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Application of C5-C13 light hydrocarbons in depositional environment diagnosis

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Progress in Natural Science:Materials International 2008年第9期18卷 1129-1137页

作者： Peirong Wanga,b,, Guanjun Xu a,c, Tingrong Xiaoc, Dajiang Zhanga,c, Bin Zhanga,c a Key Laboratory of petroleum Geochemistry, china National petroleum Corporation, beijing 100083. china b Department of Organic Geochemistry, Yangtze University, Jingzhou 43402., china c Central Laboratory of petroleum Geology, research Institute of petroleum exploration and development, petrochina, beijing 100083. china Key Laboratory of petroleum Geochemistry China National Petroleum Corporation Beijing 100083 China Department of Organic Geochemistry Yangtze University Jingzhou 434023 China Central Laboratory of petroleum Geology Research Institute of Petroleum Exploration and Development PetroChina Beijing 100083 China

Based on the geological background and Gammacerane/C31H(S + R) ratios, source rock depositional environments of the studied oil samples (194) from 13 oilfields were classified into three groups according to salinity:saline-lacustrine facies, fresh to brackish lacustrine facies (including limnetic facies), and semi-saline to saline facies (including marine facies of the Tarim Basin).C5-C13 compound groups in the crude oils were separated by GC, and about 2.6 compounds were qualitatively *** geochemical application of the C6-C13 compound groups and their ratios between each group with individual carbon number was *** studies show that (1) C6-C13 compound groups and their ratios in the crude oils could serve as new reliable parameters for oil-oil correlation because the C6-C13 light fractions are the major oil component, especially in light oil or condensate, in which they account for almost 90% of the whole oil;(2. the compound groups of C7 light hydrocarbons in oils derived from difierent depositional environments with difierent salinity have difierent characteristics;(3) C6-C13 compound groups and ratios may be afiected by other factors such as maturity, but they are mainly controlled by salinity of depositional waters.

关键词： Light hydrocarbons Crude oil Depositional environment Salinity

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TTHE METHODOLOGY OF petroleum development GEOLOGY(Ⅲ)

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石油勘探与开发 1996年第4期 78-82页

作者： Qiu Yinan (research Institute of petroleum {2. and development, CNPC, beijing, 100083. P.R.china)

ＴＨＥ　ＭＥＴＨＯＤＯＬＯＧＹ　ＯＦ　ＰＥＴＲＯＬＥＵＭ　ＤＥＶＥＬＯＰＭＥＮＴ　ＧＥＯＬＯＧＹ（Ⅲ）ＴＨＥＭＥＴＨＯＤＯＬＯＧＹＯＦＰＥＴＲＯＬＥＵＭＤＥＶＥＬＯＰＭＥＮＴＧＥＯＬＯＧＹ（Ⅲ）￥ＱｉｕＹｉｎａｎ（Ｒ...

ＴＨＥ　ＭＥＴＨＯＤＯＬＯＧＹ　ＯＦ　ＰＥＴＲＯＬＥＵＭ　ＤＥＶＥＬＯＰＭＥＮＴ　ＧＥＯＬＯＧＹ（Ⅲ）ＴＨＥＭＥＴＨＯＤＯＬＯＧＹＯＦＰＥＴＲＯＬＥＵＭＤＥＶＥＬＯＰＭＥＮＴＧＥＯＬＯＧＹ（Ⅲ）￥ＱｉｕＹｉｎａｎ（ＲｅｓｅａｒｃｈＩｎｓｔｉｔｕｔｅｏ...

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