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Interfacial behaviors of PMMA-PEO block copolymers at the air/water interface

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Science China Chemistry 2005年第6期48卷 567-573页

作者： CHENG Caixia1, JIAO Tifeng2. TANG Rupei1, LIU Minghua2.& XI Fu1 1. State Key Laboratory of Polymer Physics and Chemistry, Joint Laboratory of Polymer Science and Materials, institute of Chemistry, chinese academy of sciences,{2. 100080, China 2. CAS Key Laboratory of Colloid and Interface Science, institute of Chemistry, chinese academy of sciences,{2. 100080, China State Key Laboratory of Polymer Physics and Chemistry Joint Laboratory of Polymer Science and Materials Institute of Chemistry Chinese Academy of Sciences Beijing China CAS Key Laboratory of Colloid and Interface Science Institute of Chemistry Chinese Academy of Sciences Beijing China

Diblock copolymer of PMMA2.1-b-PEO114 and triblock copolymer of PMMA12.-b- PEO2.7-b-PMMA12. were synthesized and their interfacial properties at the air-water interface were investigated, where both blocks of polyethylene oxide (PEO) and poly(methyl methacrylate) (PMMA) are surface active but the former is soluble in water while the latter is not. Both the block copolymers could form monolayers with two obvious transition regions. The first transition point is around 10 mN/m, which could be assigned to the pancake-brush change of the PEO chains. The other is around 18 mN/m, which could be ascribed to the condensed packing of PMMA. The surface morphological changes during the compression of the Langmuir monolayers are inves-tigated by using the AFM and SEM methods for the films deposited at different surface pressure or molecular areas. At a lower surface pressure, a typical morphology of PEO-con- taining lipopolymers is observed. Upon compression, sphere-dominant morphologies were observed. While the diblock copolymer is easy to folding, the triblock copolymer is in favor of formation of circular domains through vesiculation.

关键词： PMMA-PEO, block copolymers, monolayer, Langmuir-Blodgett films, AFM.

Modeling and verifying Web services driven by requirements:An ontology-based approach

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Science in China(Series F) 2006年第6期49卷 792-820页

作者： HOU Lishan1,3,JIN ZHi1,2.& WU Budan1,4 1. academy of Mathematics and Systems Science, chinese academy of sciences,{2. 100080, China 2. institute of Computing Technology, chinese academy of sciences,{2. 100080, China 3. institute of Software, chinese academy of sciences,{2. 100080, China 4. Graduate University of chinese academy of sciences,{2. 100049, China academy of Mathematics and Systems Science Chinese Academy of Sciences Beijing China institute of Software Chinese Academy of Sciences Beijing China institute of Computing Technology Chinese Academy of Sciences Bejing China Graduate University of chinese academy of sciences Beijing China

Automatic discovery and composition of Web services is an important research area in Web service technology, in which the specification of Web services is a key issue. This paper presents a Web service capability description framework based on the environment ontology. This framework depicts Web services capability in two aspects： the operable environment and the environment changes resulting from behaviors of the Web service. On the basis of the framework, a requirement-driven Web service composition model has been constructed. This paper brings forward the formalization of Web service interactions with π calculus. And an automatic mechanism converting conceptual capability description to the formal process expression has been built. This kind of formal specification assists in verifying whether the composite Web service model matches the requirement.

关键词： Web service environment ontology automatic composition π calculus formal verification.

Estimation on dynamic release of phosphorus from wind-induced suspended particulate matter in Lake Taihu

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Science China Earth sciences 2004年第8期47卷 710-719页

作者： FAN Chengxin1, ZHANG Lu1,2. QIN Boqiang1, WANG Sumin1, HU Weiping1 & ZHANG Chen1 1. Taihu Lake Laboratory for Ecosystem Research, Nanjing institute of Geography & Limnology, chinese academy of sciences, Nanjing 2.0008, China 2. Graduate School of chinese academy of sciences, beijing 100039, China Taihu Lake Lab. for Ecosystem Res. Nanjing Inst. of Geography/Limnology Chinese Academy of Sciences Nanjing 210008 China Grad. Sch. of chinese Acad. of Sci. Beijing 100039 China

Through man-made disturbance experiments, the corresponding relationships be-tween suspended particulate matter (SPM) and wind speed in different lake areas were simu-lated, the physicochemical formal transformation and biological mineralizing and decaying processes of phosphorus in SPM were studied, the contribution of phosphorus transformation to phosphorus loading of the water of Lake Taihu was quantitatively estimated. The results show that about 0.44 t·a-1 loading in Lake Taihu mainly comes from phosphorus-releasing action of SPM in physicochemical transformed to soluble reactive phosphorus (SRP), and the contribution mainly from biological mineralizing and decaying was about 42..8 t·a-1, which is equal to 15.0% of the total external loading of Lake Taihu, namely 4.7—7.5 times as much as SRP loading en-tering the lake by the rivers; thus it is the important source in dynamical internal loading of the lake. The determining factors for dynamical internal loading in lakes are organic phosphorus content in suspended solid and its biological transition availability.

关键词： phosphorus release,wind wave disturbance,particulate decaying,dynamical loading,Lake Taihu.

Uncertainty in magnetic activity indices

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Science China(Technological sciences) 2008年第10期51卷 1659-1664页

作者： XU WenYao institute of geology and Geophysics,{2., beijing 10002., China institute of geology and Geophysics Chinese Academy of Sciences Beijing China

Magnetic activity indices are widely used in theoretical studies of solar-terrestrial coupling and space weather prediction. However, the indices suffer from various uncertainties, which limit their application and even mislead to incorrect conclu-sion. In this paper we analyze three most popular indices, Kp, AE and Dst. Three categories of uncertainties in magnetic indices are discussed: "data uncertainty" originating from inadequate data processing, "station uncertainty" caused by in-complete station covering, and "physical uncertainty" stemming from unclear physical mechanism. A comparison between magnetic disturbances and related indices indicate that the residual Sq will cause an uncertainty of 1―2.in K meas-urement, the uncertainty in saturated AE is as much as 50%, and the uncertainty in Dst index caused by the partial ring currents is about a half of the partial ring cur-rent.

关键词： magnetic activity indices Kp AE Dst solar-terrestrial coupling space weather

Effect of rock mass structure and block size on the slope stability——Physical modeling and discrete element simulation

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Science China(Technological sciences) 2005年第Z1期48卷 1-17页

作者： LI Shihai1, LIAN Zhenzhong1,2.& J. G. Wang3 1. institute of Mechanics, chinese academy of sciences,{2. 100080, China 2. Graduate School, chinese academy of sciences,{2. 100060, China 3. Tropical Marine Science institute, National University of Singapore, Singapore 1192.0 institute of Mechanics Chinese Academy of Sciences Beijing 100080 China Graduate School Chinese Academy of Sciences Beijing 100060 China Tropical Marine Science institute National University of Singapore Singapore 119260 Singapore

This paper studies the stability of jointed rock slopes by using our improved three-dimensional discrete element methods (DEM) and physical modeling. Results show that the DEM can simulate all failure modes of rock slopes with different joint configurations. The stress in each rock block is not homogeneous and blocks rotate in failure development. Failure modes depend on the configuration of joints. Toppling failure is observed for the slope with straight joints and sliding failure is observed for the slope with staged joints. The DEM results are also compared with those of limit equilibrium method (LEM). Without considering the joints in rock masses, the LEM predicts much higher factor of safety than physical modeling and DEM. The failure mode and factor of safety predicted by the DEM are in good agreement with laboratory tests for any jointed rock slope.

关键词： rock masses, slope stability, DEM simulation, block size effect, joints configuration effect, limit equilibrium method.

Geometry of Broad Line Regions of Active Galactic Nuclei

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chinese Journal of Astronomy and Astrophysics 2008年第1期8卷 50-62页

作者： Xiao-Rong Lü1 Key Laboratory for Particle Astrophysics, institute of High Energy Physics, chinese academy of sciences,{2. 100049 2.Graduate School of chinese academy of sciences,{2. 100049 Key Laboratory for Particle Astrophysics Institute of High Energy Physics Chinese Academy of Sciences Beijing 100049 Graduate School of chinese academy of sciences Beijing 100049

It has long remained an open question as to the geometry of the broad line region （BLR） in active galactic nuclei （AGNs）. The reverberation mapping technique which measures the response of the broad emission lines to the ionizing continuum, when combined with multiwavelength continuum fitted by sophisticated accretion disks, provides a way of probing the BLR geometry. We analyze a sample of 35 AGNs, which have been monitored by the reverberation mapping campaign. In view of energy budget, the reverberation-based BH masses are found to be in agreement with those obtained by accretion disk models in two thirds of the present sample while the reverberation mapping methods underestimate the BH masses in about one third of objects, as also suggested by CoUin et al. in a recent work. We point out that there are obviously two kinds of BLR geometry, which are strongly dependent on the Eddington ratio, and separated by the value LBol/LEdd - 0.1. These results prefer a scenario of the disk and wind configuration of the BLR and identify the Eddington ratio as the physical driver regulating the wind in the BLR.

关键词： accretion, accretion disks - galaxies active - galaxies Seyfert - quasars general

Vermiform trace fossils from the Precambrian Ruyang Group, western Henan

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chinese Science Bulletin 1997年第3期42卷 251-254页

作者： HU Jianmin, MENG Qingren and LI Wenhou1 Xi’ an College of geology, Xi’an 710054, China 2. institute of Geophysics,{2., beijing 100101, China 3 Department of geology, Northwest University, Xi’an 710069, China Xi’an College of geology Xi’an China institute of Geophysics Chinese Academy of Sciences Beijing China Department of geology Northwest University Xi’an China

THE origin and evolution of Precambrian lives has been a long-standing controversial problem. It is now generally accepted by most paleontologists that the origin of metazoa can be traced back to more than 1000 Ma, because the Ediacara and latest pre-Ediacara fauna, such as the Huainan fauna, are featured by their diversification of forms, complicated structures

关键词： Precambrian trace fossil Ruyang Group.

Study of the circulation theory of the cooling system in vertical evaporative cooling generator

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Science China(Technological sciences) 2006年第3期49卷 358-364页

作者： YU Shunzhou1, CAI Jing2. GUO Chaohong1 & GU Guobiao1 1. institute of Electrical Engineering, chinese academy of sciences,{2. 100080, China 2.{2. Changcheng institute of Metrology and Measurement,{2. 100095, China institute of Electrical Engineering Chinese Academy of Sciences Beijing China beijing Changcheng institute of Metrology and Measurement Beijing China

The article briefly states the current development of evaporative cooling generator; its advantages comparing with generators of traditional cooling. Vertical evaporative cooling generator, which adopts Close-Loop-Self-Cycle with no-pump; free convection boil in the hollow stator bar, is one of the great developments in generator design. This article emphasizes the importance of cooling system in generator; expatiates the circulation theory in two aspects, energy; flow;; analyzes the essential reason, motivity; stability of Close-Loop-Self-Cycle. The article points out that the motivity of the circulation is the heat absorbed by coolant. After absorbing heat the coolant will have the ability of doing work because of the phase change. In another words, it is the buoyancy causing by density difference leads to the Close-Loop-Self-Cycle. This conclusion is validated by experimental data.

关键词： vertical evaporative cooling generator, cooling system, circulation theory.

Variations of δ^(18)O in precipitation from the Muztagata Glacier, East Pamirs

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Science China Earth sciences 2006年第1期49卷 36-42页

作者： LI Zhen1, YAO Tandong1,2. TIAN Lide1,2. XU Baiqing1,2.& Wu Guangjian2.1. Key Laboratory of Cryosphere and Environment, Jointly Established by Cold and Arid Regions Environmental and Engi-neering Research institute and institute of Tibetan Plateau Research,{2. and chinese academy of Meteorological sciences, China Meteorological Administration, CAS, Lanzhou 730000, China 2. Laboratory of Environment and Process on Tibetan Plateau, institute of Tibetan Plateau Research,{2., beijing 100085, China Key Laboratory of Cryosphere and Environment Jointly Established by Cold and Arid Regions Environmental and Engineering Research Institute and Institute of Tibetan Plateau Research Chinese Academy of Sciences and Chinese Academy of Meteorological Sciences China Meteorological Administration Lanzhou China Laboratory of Environment and Process on Tibetan Plateau Institute of Tibetan Plateau Research Chinese Academy of Sciences Beijing China

Expeditions to Muztagata (in the eastern Pamirs) during the summer seasons of2.02.and 2.03 collected precipitation samples and measured their oxygen isotopes. The δ^(18)O inprecipitation displays a wide range, varying from -17.40per thousand to +1.33per thousand inJune—September 2.02.and from -2..31per thousand to +4.59per thousand in May—August 2.03. Theδ^(18)O in precipitation correlates with the initial temperature of precipitation during theobserving periods. The positive correlation between δ^(18)O and temperature suggests that δ^(18)Ocan be used as an indicator of temperature in this region. The δ^(18)O values in fresh-snow samplescollected from two snow events at different elevations on the Muztagata Glacier show a strong''altitude effect'', with a ratio of nearly -0.40per thousand per 100 m from 5500 m to 7450 m.

关键词： Muztagata, δ18O, temperature, altitude effect.