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Structures and physical properties of rigid polyurethane foams with water as the sole blowing agent

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Science china Chemistry 2006年第4期49卷 363-370页

作者： LI Xiaobin1,2. CAO Hongbin1 & ZHANG Yi1 1. institute of Process Engineering, chinese academy of sciences, Beijing 100080,{2. 2. Graduate School of the chinese academy of sciences, Beijing 100039,{2. 1. institute of Process Engineering Chinese Academy of Sciences Beijing 100080 China 2. Graduate School of the chinese academy of sciences Beijing 100039 China

Rigid polyurethane foams blown by varying water level were prepared in this study. The structures and physical properties of rigid polyurethane foams blown by water were measured with FT-IR, universal testing machine (Instron3365), scanning electron microscope (SEM) and differential scanning calorimeter (DSC). The results show that polyurea and polybiuret were the typical charac- teristics, and the cream time and gel time were shorter for the fully water blown rigid foams than that for the fully cyclopentane blown foams. The density of foam samples decreased from 45.0 kg/m3 to 2..4 kg/m3 with the increase of water level from 3 pph to 7 pph. Compressive strength exhibited the similar behavior with density. The average cell size of foam samples ranged from 2.1 μm to 356 μm with the increase of water level from 3 pph to 7 pph, respectively. At the same time, poorer dimen- sional stability was encountered with the increase of average cell size due to fast diffusion rate of CO2.out of the foam. The results of thermal analysis show that the glass transition temperature (Tg) shifted to a higher temperature with the increase of isocyanate level when more water was used as chemical blowing agent.

关键词： polyether polyol, polyurethane rigid foam, compressive strength, dimensional stability, cell size, glass transition temperature.

Adjoint method for the optimum planning of industrial pollutant sources

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Science china Earth sciences 2005年第8期48卷 1270-1279页

作者： LIU Feng1,2. HU Fei2.& ZHU Jiang2.1. College of Environmental sciences, Peking University, Beijing 100871, china 2. LAPC, {2. of Atmospheric Physics, chinese academy of sciences, Beijing 10002., china 1. College of Environmental sciences Peking University 100871 Beijing China 2. LAPC Institute of Atmospheric Physics Chinese Academy of Sciences 100029 Beijing China

The optimum planning of industrial pollutant sources, which optimizes the economic object without violating environmental constraints, is an important and hard task to be conquered. In this paper, an adjoint method is developed to solve the problem. The penalty function is in-troduced to deal with the environmental inequality constraints, and Lagrange function is con-structed to derive the adjoint equation and the gradient of the object function. In this means, the gradient of the object function can be calculated by solving the adjoint equation, and the infor-mation from the gradient is used to make the object function descend and approach to an optimal solution after some iterations. A two-dimensional, simplified model is used for numerical experi-ments. The theoretical derivations are verified by the results of the experiments. Furthermore, the adjoint method is shown to be of excellent convergence and efficiency, which is adaptive to the fast development of air quality numerical models and super computers.

关键词： optimum planning, industrial pollutant sources, adjoint equation, penalty function, gradient.

Pattern phenomena in an rf discharge dusty plasma system

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Science china(Physics,Mechanics & Astronomy) 2006年第5期49卷 588-596页

作者： HUANG Feng1,2. YE Maofu2.& WANG Long2.1. College of Science, china Agricultural University, Beijing 100083, china 2. {2. of Physics, chinese academy of sciences, Beijing 100080, china 1. College of Science China Agricultural University Beijing 100083 China 2. institute of Physics Chinese Academy of Sciences Beijing 100080 China

Various dust patterns are observed in an rf discharge dusty plasma system. According to the dust growth process from small to large in size, the formation of different dust patterns can be divided into two stages: the small-particle stage (or dust cloud stage), and the large-particle stage (or dust crystal stage). The evolution relations between different dust patterns with gas pressure changing are investigated. Dust voids, dust acoustic waves and strong turbulence modes are presented at the small-particle stage. The self-organized dust lattices and dust clusters are investigated at the large-particle stage. The static structure of a dust lattice is characterized by means of the pair correlation function. Dust clusters formed by particles with different numbers and the regular evolution of the clusters with gas pressure are also investigated. The packing sequences of dust clusters are verified through two-dimensional confined molecular dynamics simulations.

关键词： dusty plasma dust patterns

Experimental investigation and numerical simulation on the effect of fissure water pressure in vertical sliding surface

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Science china(Technological sciences) 2005年第z1期48卷 53-64页

作者： ZHANG Lei1,2. LI Shihai1, LIAN Zhenzhong1,2.& WANG Yuannian1 1. institute of Mechanics, chinese academy of sciences, Beijing 100080,{2. 2. Graduate School, chinese academy of sciences, Beijing 100060,{2. 1. institute of Mechanics Chinese Academy of Sciences 100080 Beijing China 2. Graduate School Chinese Academy of Sciences 100060 Beijing China

This paper studies the effect of fissure water pressure in different fractures on the critical angle of landslide by laboratory investigation and numerical simulation in order to understand the mechanisms of fissure water pressure on landslide stability. Laboratory observations show that the effect of fissure water pressure on the critical angle of landslide is little when the distance between water-holding fracture and slope toe is three times greater than the depth of fissure water. These experimental results are also simulated by a three-dimensional face-to-face contact discrete element method. This method has included the fissure water pressure and can accurately calculate the critical angle of jointed slope when fissure water pressure in vertical sliding surface exists. Numerical results are in good agreement with experimental observations. It is revealed that the location of water-holding structural surface is important to landslide stability. The ratio of the distance between water-holding fissure and slope toe to the depth of fissure water is a key parameter to justify the effect of fissure water pressure on the critical angle of landslide.

关键词： jointed rock slope, discrete element method, fracture in vertical sliding surface, model experiment,fissure water pressure.

Wet-chemical synthesis and characteristics of Au nanoshell

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Science china Chemistry 2005年第5期48卷 431-435页

作者： LIU Zhongxin1,2. SONG Hongwei1, YU Lixin1,2. YANG Linmei1,2.& PAN Guohui1,2.1. Key Laboratory of Excited State Physics, Changchun institute of Optics, Fine Mechanics and Physics, chinese academy of sciences, Changchun 130033,{2. 2. Graduate School of the chinese academy of sciences, Beijing 100039,{2. 1. Key Laboratory of Excited State Physics Changchun Institute of Optics Fine Mechanics and Physics Chinese Academy of Sciences 130033 Changchun China 2. Graduate School of the chinese academy of sciences 100039 Beijing China

Gold nanoshells were prepared by an easy wet-chemical method, with Ag nanoparticles used as the templates. Transmission electron microscopy (TEM) indicated that the shells were sphere in shape, the size was homogenous, being about 2. nm, and no hard ag-glomerates were observed. The plasma resonance absorption of gold was tuned from visible to near-infrared (NIR) with the increased volume of HAuCl4. The temperature grads (?T) of the gold nanoshell hydrosol under the exposure of an 808-nm optical fiber laser with different power den-sities were measured. The highest ?T was 30℃ (5 W/cm2. irradiation area was 2.cm2.. This kind of gold nanoshell hydrosol is a promising material to be used in biomedicine such as photo-thermal cancer therapy, and its special photothermal convert property will photothermally trigger drug release.

关键词： wet-chemical synthesis, Au, nanoshell, NIR absorption, photothermal conversion.

Environmental characteristics of Mid-Holocene recorded by lacustrine sediments from Lake Daihai, north environment sensitive zone, china

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Science china Earth sciences 2006年第9期49卷 968-981页

作者： SUN Qianli1,2. ZHOU Jie1, SHEN Ji3, CHEN Peng1,2. WU Feng1,2.& XIE Xiuping1,2.1. State Key Lab of Loess and Quaternary Geology, institute of Earth Environment, chinese academy of sciences, Xi’an 710075,{2. 2. Graduate University of chinese academy of sciences, Beijing 100039,{2. 3. Nanjing institute of Geography and Limnology, chinese academy of sciences, Nanjing 2.0008,{2. 1. State Key Lab of Loess and Quaternary Geology Institute of Earth Environment Chinese Academy of Sciences Xi’an 710075 China 2. Graduate University of chinese academy of sciences Beijing 100039 China 3. Nanjing institute of Geography and Limnology Chinese Academy of Sciences Nanjing 210008 China

Climate proxies, such as total organic carbon and nitrogen (TOC, TN), carbonate content (CaCO3), grain-size and pollen of the sediment core retrieved from enclosed Lake Daihai which lies in the north china environment sensitive zone are analyzed to reconstruct the environment evolution of the area based on high-resolution radiocarbon chronology. The results reveal that the TOC and TN contents of the sediments correlate well with pollen percentage and pollen flux variations during the Holocene, and both reach their peak values simultaneously at 6.7―3.5 ka BP (calendar age, 7.6―3.6 ka BP). Since 6.7 ka BP, both the CaCO3 and organic matter contents of the core have simultaneous variations, and their high values also occur during 6.7―3.5 ka BP. While during 9.0―6.7 ka BP (calendar age, 10―7.6 ka BP) relatively lower level of organic matter content and pollen flux corre- spond to the higher level of carbonate content. The above relations suggest that during 6.7―3.5 ka BP, the productivity and effective precipitation were greatly improved in the lake drainage area, and this would probably strengthen the hydrodynamic conditions, enhancing organic matter, pollen and carbonate inputs from terrestrial sources. Such processes would account for the enrichment of both organic matter and carbonate in the sediments. While during 9.0―6.7 ka BP, the lower level of or- ganic matter, pollen flux but high carbonate content show depressed productivity and declined vege- tation coverage. The higher carbonate content at this stage would have probably resulted from the higher evaporation ratio of the lake water under relatively drier climate conditions. Therefore, it is in- ferred that during 6.7―3.5 ka BP, the climate was more humid with abundant rainfalls and vegetation was more flourishing in the Lake Daihai area. This can be seen as Holocene Climate Optimum (HCO). As a result, this has evident discrepancies with the traditional notion that the HCO occurs at Early Holocene or early Mid

关键词： Lake Daihai, Mid-Holocene, lacustrine sediments, environmental characteristics.

Variation properties of ionospheric eclipse factor and ionospheric influence factor

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Progress in Natural Science:Materials International 2005年第6期15卷 573-576页

作者： ZHAO Chunmei 1,2.*, YUAN Yunbin1, OU Jikun1 and CHEN Jinping3(1. institute of geodesy and Geophysics,{2., wuhan 43.077, china 2. Graduate School of{2., Beijing 100039, china 3. Department of Precision Instrument and Mechanology, Tsinghua University, Beijing 100084, china) institute of geodesy and Geophysics Chinese Academy of Sciences Wuhan 430077 China Graduate School of chinese academy of sciences Beijing 100039 China Department of Precision Instrument and Mechanology Tsinghua University Beijing 100084 China

The concepts and calculation methods of ionospheric eclipse factor (IEF) and ionospheric influence factor (IFF) are further illustrated. The temporal and spacial variation properties of IEF and IFF are studied, which shows that the properties are influenced by the geographic position and season. The possibility of improving the precision of using GPS data to determine ionospheric delay based on the above variation properties is also analysed.

关键词： GPS ionospheric eclipse factor ionospheric influence factor

Sea level variations in the South china Sea inferred from satellite gravity,altimetry,and oceanographic data

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Science china Earth sciences 2012年第10期55卷 1696-1701页

作者： FENG Wei 1,2.ZHONG Min 1,3 & XU HouZe 1,3 1 State Key Laboratory of geodesy and Earth’s Dynamics,institute of geodesy and Geophysics,chinese academy of sciences,wuhan 43.077,china 2.Graduate University of chinese academy of sciences,Beijing 100049,china 3 institute of Geophysics,Huazhong University of Science and Technology,wuhan 430074,china 1. State Key Laboratory of geodesy and Earth’s Dynamics Institute of Geodesy and Geophysics Chinese Academy of Sciences Wuhan 430077 China2. Graduate University of Chinese Academy of Sciences Beijing 100049 China3. Institute of Geophysics Huazhong University of Science and Technology Wuhan 430074 China

Sea level variations(SLVs) can be divided into two major components:the steric SLV and the mass-induced *** two components of SLV in the South china Sea(SCS) are studied by using satellite altimetry,GRACE(Gravity Recovery and Climate Experiment) satellite gravity,and oceanographic data on annual and inter-annual *** the annual timescale,the geographic distribution of mass-induced SLV's amplitude jointly estimated from altimetry and the ECCO(Estimation of the Circulation and Climate of the Ocean) model agrees very well with that from *** observes obvious seasonal mass-induced SLV in the SCS with annual amplitude of 2.7±0.4 cm,which is consistent with the annual amplitude of 2.7±0.3 cm estimated from the steric-corrected *** the inter-annual timescales,the mean SLV in the SCS shows a large oscillation,which is mainly caused by the steric *** trend of mean SLV inferred from altimetry in the SCS is 5.5±0.7 mm/yr for the period of 1993-2.09,which is significantly higher than the global sea level rise rate of 3.3±0.4 mm/yr in the same *** is no obvious trend signal in the mass-induced SLV detected from GRACE that indicates the water exchange between the SCS and its adjacent seas and land is in balance within the study period.

关键词： altimetry GRACE ECCO the South china Sea sea level variation

The deep thermal characteristic of continental margin of the northern South china Sea

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chinese Science Bulletin 2000年第18期45卷 1717-1722页

作者： ZHANG Jian & WANG Jiyang1. Graduate School, University of Science and Technology of china, chinese academy of sciences, Beijing 100039, china 2. institute of Geology, chinese academy of sciences, Beijing 10002., china Graduate School University of Science and Technology of China Chinese Academy of Sciences Beijing China institute of Geology Chinese Academy of Sciences Beijing China

Heat flow plays an important role in the study ot thermal structure and thermal evolutionof continental margin of the northern South china Sea. The analysis of heat flow value shows that margin heat flow in the northern South china Sea is relatively high setting, but the percentage of crustal heat flow is lower than 35% in terrestrial heat flow. The terrestrial heat flow exhibited a current of rise from the Northern Continental Margin to the Southern Central Basin. However, the proportion of crustal heat flow in terrestrial heat flow slowly dropped down in the same direction. It is suggested that the main factor causing high heat flow setting is the moving up of hot material from asthenosphere.

关键词： margin of northern South china Sea terrestrial heat flow thermal structures.