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AFM study on the adsorption and aggregation behavior of dissolved humic substances on mica

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Science China Chemistry 2006年第3期49卷 256-266页

作者： GE Xiaopeng1, ZHOU Yanmei2. Lü Chunhua1 & TANG Hongxiao1 1. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental sciences, chinese {2. of sciences, beijing 100085, China 2. school of Civil Engineering & Architecture, beijing Jiaotong University, beijing 100044, China 1. State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 China 2. school of Civil Engineering & Architecture Beijing Jiaotong University Beijing 100044 China

Humic substances constitute the major organic fractions of soils, sediments and natural waters, and play a dominant role in the binding, mobilization, transport and ultimate fate of organic contaminants in subsurface systems. In this paper, two humic acid samples, Guanting and Tianjin, with different origin and chemical compositions have been investigated with AFM imaging for their adsorption and aggregation behaviors on mica. While the Tianjin humic sample is found to form small spheres with 2.0 to 330 nm in diameter at lower concentrations, irregular loop-chain assemblies of hundreds of nanometer in diameter with the chain width of about 40 nm are dominant for the Guanting humic sample, which may attribute to the more polar aliphatic fractions in the chemical composition in the latter. The heterogeneous and polydisperse nature of humic substances with multiple structural features, such as sponge-like structures, perforated sheets, aggregate of spheres, branches and chain-like assemblies etc., is apparent at higher concentrations for both humic samples, showing morphologically new evidence for the dominant view of the humic dual-mode sorption model. With naphthalene introduced, the assemblies of Guanting humic substances clearly become more compact with significantly narrowed branches and less porous the perforated sheet-like structures. It is indica- tive of that smaller nanometer scale rings present along the perforated assemblies could potentially represent hydrophobic domains, which may facilitate the adsorption and aggregation of naphthalene onto the natural particle surfaces and therefore lead to an important role of dissolved humic sub- stances in the sorption of environmental pollutants.

关键词： atomic force microscopy (AFM) dissolved humic substances morphology aggregation adsorption

Formal analysis and design of multi-party fair exchange protocols

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Science in China(Series F) 2006年第2期49卷 155-174页

作者： QING Sihan1,2.3 & LI Gaicheng1,3 1. Engineering Research Center for Information Security Technology, Institute of Software, chinese academy of {2., beijing 100080, China 2. beijing Zhongke Ansheng Corporation of Information Technology, beijing 100080, China 3. graduate school of the chinese academy of {2., beijing 1.0039, China 1. Engineering Research Center for Information Security Technology Institute of Software Chinese Academy of Sciences Beijing 100080 China 2. beijing Zhongke Ansheng Corporation of Information Technology Beijing 100080 China 3. graduate school of the {2. academy of sciences Beijing 100039 China

Based on the origin of message items and channel combination between transacting parties, and events and relations among events, this paper presents a concise, precise, and hierarchical model for general fair exchange protocols, formally specifies various security requirements which are able to reflect inherent requirements for fair exchange protocols more rigorously, and partition these security requirements with fine granularity. This work helps analyze, debug, and design multi-party fair exchange protocols more effectively and elaborately,

关键词： fair exchange logical protocol formal model security requirement.

Possible Energy Network with polygeneration system and CCS for China

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中国科学：技术科学英文版 2010年第1期53卷 33-39页

作者： GAO Lin1,LI Sheng1,2.JIN HongGuang1 & LIN Hu1 1 Institute of Engineering Thermophysics,chinese academy of {2.,beijing 100190,China 2.graduate school of chinese academy of {2.,beijing 1.0039,China 1. Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing 100190 China2. Graduate School of Chinese Academy of Sciences Beijing 100039 China

On basis of adopting polygeneration systems for power and alternative fuels,capturing CO2.with near zero energy penalties,and storing CO2.on sites,a new kind of Energy Network can integrate energy utilization,CO2.capture,transportation and storage ***-economic analysis of this solution focusing on Inner Mongolia and the Yangtze River Delta districts had been carried with comparison to the chain method for energy utilization and CO2.*** solution can save 2..5% of energy,and reduce 35% of total *** adoption of advanced polygeneration systems contributes 52.2. of the total saved costs,and the integration of energy utilization and CO2.sequestration in the Energy Network contributes 47.8%.From the aspect of CCS,the CO2.sequestration cost in the Energy Network can be as low as 12.$/t due to the lower energy penalties of capture in polygeneration systems and the combination of CO2.source and *** Energy Network exhibits attractive performance on energy saving,costs reduction for CCS,which may be a promising solution for sustainable development of China.

关键词： CO2 capture and storage Energy Network polygeneration system

Effects of various solar indices on accuracy of Earth’s thermospheric neutral density models

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Science China(Physics,Mechanics & Astronomy) 2009年第7期52卷 1120-1128页

作者： WANG HongBo1,2.& ZHAO ChangYin1 1 Purple Mountain Observatory, chinese academy of {2., Nanjing 2.0008, China 2.graduate University of chinese academy of {2., beijing 100049, China Purple Mountain Observatory Chinese Academy of Sciences Nanjing 210008 China graduate University of chinese {2. of sciences Beijing 100049 China

Four kinds of solar indices F10.7, E10.7, S10, Mg10 and four thermospheric neutral density models, i.e., CIRA72. DTM94, NRLMSISE00 and JB2.06, are discussed. The CHAMP accelerometer data are used to calculate thermospheric total mass density. Based on the comparison of the model densities with CHAMP observations, the effects of various indices on the model accuracy are detected. It is found that under quiet and moderate solar conditions (F10.72.0) the error’s standard deviation using E10.7 increases quickly and causes the models’ accuracy to fall down. With regard to S10, Mg10, their effects under quiet solar conditions are inconspicuous. If under active solar conditions, they can reduce the model error’s standard deviation by 5%-10%, implying that S10, Mg10 make the model error more stable. The JB2.06 model, which was constructed by multi-solar-index (F10.7, S10, Mg10), is compared with DTM94 and NRLMSISE00 based on single-solar-index. It is found that JB2.06’s accuracy is better than DTM94’s, and is close to NRLMSISE00 under the quiet solar condition. During the solar burst occurring on October 2., 2.03, JB2.06 has been in best agreement with CHAMP observations. All in all, the new indices may improve thermospheric density models’ accuracy under some special conditions. Concretely, E10.7 may reduce the average error of models and S10, Mg10 may prevent the error’s divergence.

关键词： solar radiation index CHAMP accelerometer data neutrals density model

Sequence analysis of mRNA polyadenylation signals of rice genes

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chinese Science Bulletin 2006年第9期51卷 1069-1077页

作者： LU Ying1, 2. GAO Chenxi1,2.3 & HAN Bin1,3,41. National Center for Gene Research, Shanghai Institutes for Biological sciences, chinese {2. of sciences, Shanghai 2.02.3, China 2. graduate school of the chinese academy of sciences, beijing 1.0039, China 3. Institute of Plant Physiology and Ecology, Shanghai Institutes for Biological sciences, chinese {2. of sciences, Shanghai 2.0032. China National Center for Gene Research Shanghai Institutes for Biological Sciences Chinese Academy of Sciences Shanghai 200233 China graduate school of the {2. academy of sciences Beijing 100039 China Institute of Plant Physiology and Ecology Shanghai Institutes for Biological Sciences Chinese Academy of Sciences Shanghai 200032 China

The formation of eukaryotic mRNAs involves the cleavage and polyadenylation of pre- mRNAs. To investigate the sequence requirement of putative polyadenylation signals (PASs), poly(A) sites and downstream elements (DUEs) in 3′-end-pro- cessing in rice, we compared expressed sequences tags (ESTs) with poly(A) extremity to full-length cDNA sequences and constructed a database of 12.69 pre- mRNA sequences in ?40―+40 nt surrounding the poly(A) sites, which were from 9953 genes. The al- ternative poly(A) sites were revealed in approxi- mately 2.% of mRNAs. Nearly 80% of pre-mRNAs showed stringent requirement of the YA (CA or UA) at poly (A) sites for polyadenylation. About 7.9% had the AAUAAA signals on ?40―?1 nt upstream of the poly(A) sites. Over 60% of mRNAs probably used the one- or two-base variants of AAUAAA hexamers as their PASs in 3′ fragments. The single-base variants of AAUGAA revealed the high frequency in 11.5% of 3′ fragments. The DUEs were detected in 90% of pre- mRNAs, especially more than half of the pre-mRNAs with multi-base variants of AAUAAA had the DUEs surrounding the poly(A) site. The location of DUE is also important for defining the cleavage site. Al- though most of the rice pre-mRNAs did not contain AAUAAA signal, the existence of downstream ele- ments ensured the efficiency of cleavage-polyade-

关键词：多聚腺苷酸序列分析 mRNA 水稻基因工程

Study on the atmospheric photochemical reaction of CF_3 radicals using ultraviolet photoelectron and photoionization mass spectrometer

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Science China Chemistry 2008年第4期51卷 316-321页

作者： YAO Li1,2. DU Lin1,2. YIN Shi1,2.& GE MaoFa1 1 beijing National Laboratory for Molecular sciences (BNLMS), State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, {2. academy of sciences, beijing 100080, China 2.graduate University of {2. academy of sciences, beijing 100080, China 1. beijing National Laboratory for Molecular sciences (BNLMS) State Key Laboratory for Structural Chemistry of Unstable and Stable Species Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China 2. graduate University of chinese {2. of sciences Beijing 100080 China

A study of the atmospheric photochemical reaction of CF3 radical with CO and O2.was performed by using a homemade ultraviolet photoelectron spectrometer-photoionization mass spectrometer (PES- PIMS). The electronic structures and mechanism of ionization and dissociation of CF3OC(O)OOC(O)- OCF3 were investigated. It was indicated that the two bands on the photoelectron spectrum of CF3OC(O)OOC(O)OCF3 are the result of ionization of an electron from a lone pair of oxygen and a fluo- rine lone pair of CF3 group. The outermost electrons reside in the oxygen lone pair. The experimental and theoretical first vertical ionization energy is 13.2. and 13.178 eV, respectively, with the PES and OVGF method. They are in good agreement. The photo ionization and dissociation processes were discussed with the help of theoretical calculations and PES-PIMS experiment. After ionization, the parent ions prefer the dissociation of the C-O bond and giving the fragments CF3OCO+ and CF3+. It demonstrated that the ultraviolet photoelectron and photoionization mass spectrometer could be ap- plied widely in the study of atmospheric photochemical reaction.

关键词： photochemical reaction CF3 radical ultraviolet photoelectron and photoionization mass spectroscopy transient species

A new class of symmetric periodic solutions of the spatial elliptic restricted three-body problem

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Science China(Physics,Mechanics & Astronomy) 2009年第9期52卷 1404-1413页

作者： XU XingBo1,2.& FU YanNing1 1 Purple Mountain Observatory, chinese academy of {2., Nanjing 2.0008, China 2.graduate University of chinese academy of {2., beijing 1.0039, China 1. Purple Mountain Observatory Chinese Academy of Sciences Nanjing 210008 China 2. graduate University of chinese {2. of sciences Beijing 100039 China

We show that there exists a new class of symmetric periodic solutions of the spatial elliptic restricted three-body problem. In such a solution, the infinitesimal body is confined to the vicinity of a primary and moves on a nearly circular orbit. This orbit is almost perpendicular to the orbital plane of the primaries, where the line of symmetry of the orbit lies. The existence is shown by applying a corollary of Arenstorf's fixed point theorem to a periodicity equation system of the problem. And this existence doesn't require any restriction on the mass ratio of the primaries, nor on the eccentricity of their relative elliptic orbit. Potential relevance of this new class of periodic solutions to real celestial body systems and the follow-up studies in this respect are also discussed.

关键词： periodic orbits spatial restricted three-body problem symmetric orbits averaging

Effects of diatoms on reproduction and growth of marine copepods

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Progress in Natural Science:Materials International 2004年第10期14卷 1-7页

作者： ZHANG Guangtao 1,2. and SUN Song 1 (1.Key Laboratory of Marine Ecology&Environment sciences,Institute of Oceanology,chinese {2. of sciences,Qingdao2.6071,China 2.graduate school,chinese {2. of sciences,beijing1.0039,China) chinese Acad Sci Inst Oceanol Key Lab Marine Ecol & Environm Sci Qingdao 266071 Peoples R China chinese Acad Sci Grad Sch Beijing 100039 Peoples R China

Two hot spots in marine ecology,deleterious effects of diatoms and feeding selectivity of copepods,as well as new progress on these two issues achieved in the recent ten years,are *** two issues are considered correlated *** and their metabolites can induce deleterious effects on growth,reproduction and development of copepods,including increase of mortality and decrease of egg production,hatching and growth *** negative effects,resulting from either chemical toxin or nutritional defi-ciency,can be conquered in natural environments by diverse *** is therefore concluded that deleterious effects of diatoms observed in laboratory or during blooming period are only a special case that accommodation of feeding strategy of copepods is *** under-stand their feeding strategy in natural environments is a prerequisite to explaining the mechanisms of deleterious effects caused by diatoms,and makes it possible to re-evaluate the energy flow in marine ecosystems.

关键词： diatoms copepod feeding strategy reproduction deleterious effects

Exploration of combined adjustment laws about IGV,stator and rotational speed in off-design conditions in an axial compressor

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中国科学：技术科学英文版 2010年第4期53卷 969-975页

作者： HU YanMing1,2.& NIE ChaoQun1 1 Key Laboratory of Advanced Energy and Power Technology,Institute of Engineeting Thermophysics,chinese academy of Science,{2. 100190,China 2.graduate school of chinese academy of sciences,{2. 100190,China 1. Key Laboratory of Advanced Energy and Power Technology Institute of Engineeting Thermophysics Chinese Academy of Science Beijing 100190 China2. Graduate School of Chinese Academy of Sciences Beijing 100190 China

Experimental investigations are performed in a three-stage low-speed axial compressor with variable inlet guide vanes(IGV) and adjustable *** characteristics of the compressor,especially the efficiency and stall margin,are analyzed in design and off-design operation conditions by adjusting stagger angles of IGV and stators as well as changing the rotational *** experimental results show that the off-design performance of the multistage axial compressor is improved by restaggering of IGV and stators related to rotational *** the background of engineering applications,digital signal processing(DSP) technique is used to realize online adjustment of stagger angles according to the corresponding relations between incidence angles of rotor and rotational speed.

关键词： axial compressor IGV surge DSP techniques off-design