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Effect of concentration on surfactant micelle shapes——A molecular dynamics study

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Science china Chemistry 2005年第5期48卷 470-475页

作者： GAO Jian1,2. GE Wei1 & LI Jinghai1 1. Multiphase Reaction Laboratory, Institute of Process Engineering, chinese academy of sciences, beijing 100080,{2. 2. Graduate School of The chinese academy of sciences, beijing 100085,{2. 1. Multiphase Reaction Laboratory Institute of Process Engineering Chinese Academy of Sciences 100080 Beijing China 2. Graduate School of The chinese academy of sciences 100085 Beijing China

Many aspects of the behavior of surfactants have not been well understood due to the coupling of many different mechanisms. Computer simulation is, therefore, attractive in the sense that it can explore the effect of different mechanisms separately. In this paper, the shapes, structures and sizes of sodium dodecylbenzenesulfonate (SDBS) micelles under different con-centrations in an oil/water mixture were studied via molecular dynamics (MD) simulations using a simplified atomistic model which basically maintains the hydrophile and lipophile properties of the surfactant molecules. Above the critical micellar concentration (cmc), surfactant molecules ag-gregate spontaneously to form a wide variety of assemblies, from spherical to rodlike, wormlike and bilayer micelles. Changes in their ratios of the principle moments of inertia (g1/g3, g2.g3) in-dicated the transition of micelle shapes at different concentrations. The aggregation number of micelle is found to have a power-law dependence on surfactant concentration.

关键词： surfactant, MD simulation, sodium dodecylbenzenesulfonate, micelle shape.

The age of the plant fossil assemblage in the Liuqu Conglomerate of southern Tibet and its tectonic significance

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Progress in Natural Science:Materials International 2006年第1期16卷 55-64页

作者： FANG Aimin1, YAN Zhen1, LIU Xiaohan2. PAN Yusheng1, LI Jiliang1, YU Liangjun1, HUANG Feixing2.and TAO Junrong3 (1.Laboratory of Lithosphere Tectonic Evolution, Institute of Geology and Geophysics, chinese academy of sciences, beijing 10002.,{2. 2. Institute of Tibet Plateau research, chinese academy of sciences, beijing 100085,{2. 3. Institute of Botany, chinese A cademy of sciences, beijing 100093,{2.) Laboratory of Lithosphere Tectonic Evolution Institute of Geology and Geophysics Chinese Academy of Sciences Beijing 100029 China Institute of Tibet Plateau research Chinese Academy of Sciences Beijing 100085 China Institute of Botany Chinese A-cademy of Sciences Beijing 100093 China

The Liuqu Conglomerate, situated to the south of Yarlung Tsangbo Suture Zone (YTSZ), is a suit of molasse formed in a foreland basin of the Himalayan orogenic belt after the collision between the two plates of the Indian and Eurasion, It is of great significance in constraining the younger limit time of the collision of the two plates and providing stratigraphic evidence to reveal the post-colli sional tectonic evolution and uplifting history of the Tibet plateau. However, the age of this molasse suit and its correlation to other synchronous strata distributed in southern Tibet have been in great disputes for a long time. Especially in recent years, argues on its ages are growing violently with the recognition of the great sedimentary tectonic significances of this molasse. During the field work carried out recently on this molasse suit, a lot of plant fossils were found preserved in fairly good conditions in the upper part of this strata, which is of great help in determining its age. By identification, the assemblage of the plant fossils belongs to a tropic to subtropic flora developed in the southern margin of the Northern Hemisphere supercontinent during the Middle to Later Eocene, which can provide good constraint on its formation age. This paper is to give a brief introduction of the plant assemblage and its age, and to discuss their tectonic significances.

关键词： Liuqu conglomerate plant fossils age Eocene Tectonic implications.

Estimation on dynamic release of phosphorus from wind-induced suspended particulate matter in Lake Taihu

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Science china Earth sciences 2004年第8期47卷 710-719页

作者： FAN Chengxin1, ZHANG Lu1,2. QIN Boqiang1, WANG Sumin1, HU Weiping1 & ZHANG Chen1 1. Taihu Lake Laboratory for Ecosystem research, Nanjing Institute of Geography & Limnology, chinese academy of sciences, Nanjing 2.0008,{2. 2. Graduate School of chinese academy of sciences, beijing 100039,{2. 1. Taihu Lake Laboratory for Ecosystem research Nanjing Institute of Geography & Limnology Chinese Academy of Sciences 210008 Nanjing China 2. Graduate School of chinese academy of sciences 100039 Beijing China

Through man-made disturbance experiments, the corresponding relationships be-tween suspended particulate matter (SPM) and wind speed in different lake areas were simu-lated, the physicochemical formal transformation and biological mineralizing and decaying processes of phosphorus in SPM were studied, the contribution of phosphorus transformation to phosphorus loading of the water of Lake Taihu was quantitatively estimated. The results show that about 0.44 t·a-1 loading in Lake Taihu mainly comes from phosphorus-releasing action of SPM in physicochemical transformed to soluble reactive phosphorus (SRP), and the contribution mainly from biological mineralizing and decaying was about 42..8 t·a-1, which is equal to 15.0% of the total external loading of Lake Taihu, namely 4.7—7.5 times as much as SRP loading en-tering the lake by the rivers; thus it is the important source in dynamical internal loading of the lake. The determining factors for dynamical internal loading in lakes are organic phosphorus content in suspended solid and its biological transition availability.

关键词： phosphorus release,wind wave disturbance,particulate decaying,dynamical loading,Lake Taihu.

Ionization state of cosmic hydrogen by early stars and quasars

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research in Astronomy and Astrophysics 2009年第6期9卷 665-681页

作者： Xiao-Chun Mao1,2.1 National Astronomical Observatories, chinese academy of sciences, beijing 100012.{2. 2.Graduate University of chinese academy of sciences, beijing 100049,{2. National Astronomical Observatories Chinese Academy of Sciences Beijing 100012 China Graduate University of chinese academy of sciences Beijing 100049 China

Cosmic hydrogen is reionized and maintained in its highly ionized state by the ultraviolet emission attributed to an early generation of stars and quasars. The Lyα opacity observed in absorption spectra of high-redshift quasars permits more stringent constraints on the ionization state of cosmic hydrogen. Based on density perturbation and structure formation theory, we develop an analytic model to trace the evolution of the ionization state in the post-overlap epoch of reionization, in which the bias factor is taken into account. For quasars, we represent an improved luminosity function by utilizing a hybrid approach for the halo formation rate that is in reasonable agreement with the published measurements at 2.≤ z ≤ 6. Comparison with the classic Press-Schechter mass function of dark matter halos, we demonstrate that the biased mass distribution indeed enhances star formation efficiency in the overdense environment by more than 2. per cent following the overlap of ionized bubbles. In addition, an alternative way is introduced to derive robust estimates of the mean free path for ionizing photons. In our model, star-forming galaxies are likely to dominate the ionizing background radiation beyond z = 3, and quasars contribute equally above a redshift of z ～ 2.5. From 5 ≤ z ≤ 6, the lack of evolution in photoionization rate can thus be explained by the relatively flat evolution in star formation efficiency, although the mean free path of ionizing photons increases rapidly. Moreover, in the redshift interval z ～ 2.- 6, the expected mean free path and Gunn-Peterson optical depth obviously evolve by a factor of ～ 500 and ～50 respectively. We find that the relative values of critical overdensities for hydrogen ionization and collapse could be 430% at z ≈2.and 2. at z ≈6, suggesting a rapid overlap process in the overdense regions around instant quasars following reionization. We further illustrate that the absolute estimates of the fraction of neutral hydrogen computed fr

关键词： cosmology theory -- formation galaxies -- quasars general -- diffuse radiation -- intergalactic medium

Spatial and environmental effects on plant communities in the Yellow River Delta,Eastern china

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Journal of Forestry research 2009年第2期20卷 117-122页

作者： SONG Chuang-ye1, 2. LIU Gao-huan1, LIU Qing-sheng1 1 Institute of geographic sciences and Nature {2. research, chinese academy of sciences, beijing 100101, china 2.Graduated School of chinese academy of sciences, beijing 100039, china Institute of geographic sciences and Nature {2. research Chinese Academy of Sciences Beijing 100101 China Graduated School of chinese academy of sciences Beijing 100039 China

Types and structure of plant communities in the Yellow River Delta were investigated by using detrended canonical correspon-dence analyses(DCCAs) and a two-way indicator species analysis(TWINSPAN).The distribution pattern and influential factors of the plant communities were also analyzed by testing elevation, slope, soil characteristics, longitude and latitude of 134 vegetation samples collected by representative plot sampling *** showed that all the 134 vegetation samples could be divided into seven vegetation groups, separately dominated by Robinia pseucdoacacia, Imperata cylindrical, Miscanthus saccharifleus, Suaeda salsa, Aeluropus sinensis, Phragmites australis and Tamarix *** vegetation distribution pattern was mainly related to elevation, ground water depth and soil characteristics such as salinity and soluble *** the factors affecting distribution pattern of the plant communities, the species matrix explained by non-spatial environmental variation accounts for 45.2. of total *** variation and spatial-structured environmental variation explain 11.8%, and 2.2., *** 40.8% of undetermined variation is attributed to biological and stochastic factors.

关键词： detrended canonical correspondence analyses environmental factors plant communities spatial factors Yellow River Delta two-way indicator species analysis

Continuous wavelet transform and discrete multi-resolution analysis of surface fluxes and atmospheric stability

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Progress in Natural Science:Materials International 2006年第4期16卷 403-409页

作者： JIANG Zhaoyang, YU Qiang, WANG Tianduo, SUN Xiaomin and ZHANG Renhua Shanghai Institute of Plant Physiology and Ecology, chinese academy of sciences, Shanghai 2.0032. china Institute of {2. sciences and Natural resources research, chinese academy of sciences, beijing 100101, china [a]Shanghai Institute of Plant Physiology and Ecology Chinese Academy of Sciences Shanghai China [b]Institute of Geograhpic sciences and Natural resources {2. Chinese Academy of Sciences Beijing China

Variations of land surface fluxes of sensible heat (H), latent heat (LE), and CO2.F-CO2. obtained from the eddy-co-variance measurements above a winter wheat field from March 30 to April 2., 2.01 have been studied at scales ranging from 10 minutes to days. Wavelet transform is used in the analysis of land surface fluxes and atmospheric stability (ξ) calculated from the measurements to reveal the changes in land surface fluxes in hours to days scales. The main results are: (1) Concise and compact information about the fluxes, net radiation (Rn), temperature ( T) and ξ in the scale-time domain are extracted from the data by continuous wavelet analysis, and 1 day, 0.5 day and short-period (shorter than 0.5 day) components are revealed. Continuous wavelet coefficients can be used to characterize periodic components of changes in fluxes and ξ. (2. Discrete-time multi-resolution analysis can be used to concentrate total energy variance of time series of the measurements to a small number of coefficients, plotting the relative energy distribution to get several meaningful characteristics of the data. (3) Under neutral atmospheric conditions, the relative energy distributions of the Haar multi-resolution analysis of the three non-dimensional coefficients ( T/T* , q/q * and c/c * ) display clear similarities.

关键词： atmospheric stability flux continuous wavelet transform multi-resolution wavelet analysis.

A new principle of synthetic cascade utilization of chemical energy and physical energy

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Science china(Technological sciences) 2005年第2期48卷 163-179页

作者： JIN Hongguang1, HONG Hui1,2. WANG Baoqun1,2. HAN Wei1,2.& LIN Rumou1,2.1. Institute of Engineering Thermophysics, chinese academy of sciences, beijing 100080,{2. 2. Graduate School of the chinese academy of sciences, beijing 100039,{2. 1. Institute of Engineering Thermophysics Chinese Academy of Sciences 100080 Beijing China 2. Graduate School of the chinese academy of sciences 100039 Beijing China

We propose a new principle of the cascade utilization of both chemical energy and physical energy in energy systems with the integration of chemical processes and thermal cycles. Particularly, a general equation of energy levels of substance, Gibbs free energy of chemical reaction and physical energy is explicitly founded. On the basis of this equation, a chemical-looping combustion and an indirect combustion are investigated. Furthermore, a mechanism of energy release, with the combination of decreasing the energy level of Gibbs free energy and upgrading the energy level of low or middle- temperature thermal energy, is clarified. The promising results obtained here establish a theoretical basis for the further investigation of multi-function systems in which energy and the environment are compatible, and create a new approach to improve the performance of traditional thermal cycles.

关键词： chemical energy, cascade utilization, exergy, energy conversion.

“Double dawn”eclipse and the rotational variation of the earth

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chinese Science Bulletin 2000年第11期45卷 988-991页

作者： ZHANG Peiyu & HAN Yanben1. Purple Mountain Observatory, chinese academy of sciences, Nanjing 2.0008, china 2. {2. Astronomical Observatory, chinese academy of sciences, {2. 100012. National Astronomical Observatory, chinese academy of sciences, {2. 100012. china Purple Mountain Observatory Chinese Academy of Sciences Nanjing China beijing Astronomical Observatory Chinese Academy of Sciences Beijing National Astronomical Observatory Chinese Academy of Sciences Beijing China

A record of 'double dawn' at State Zheng in the first year of the reign of King Yi in Western Zhou Dynasty in the chronicle 'Bamboo Annals' (Zhushu Jinian) is discussed. We think that it may be a record of an annular solar eclipse happening in 899 BC. The record and the AT, which describes the secular variation of the earth’s rotation, are analyzed and discussed.

关键词： solar eclipse earth’s rotation.

Modified conceptual model for predicting the tendency of alluvial channel adjustment induced by human activities

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chinese Science Bulletin 2001年第S1期46卷 51-57页

作者： XU JiongxinInstitute of geographical sciences and Natural {2. research, chinese academy of sciences, beijing 100101, china (e-mail: xujxin?***) 1. Institute of geographical sciences and Natural {2. research Chinese Academy of Sciences 100101 Beijing China

After a discussion about some limitations of Schumm’s conceptual model for prediction of river metamorphosis, this study introduces the channel boundary material as an independent variable, and thereby establishes a conceptual model that can be used to predict the direction of channel adjustment induced by human activities. This model has been tested by data from natural rivers and a laboratory model river, and can be used to explain the complex behavior of channel adjustment after reservoir construction.

关键词： human influence on channels channel boundary condi- tions feedback in channel system prediction of channel adjustment.