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Towards advanced zinc anodes by interfacial modification strategies for efficient aqueous zinc metal batteries

Journal of Energy Chemistry 2024年第6期93卷 79-110,I0003页

作者： changchun Fan Weijia Meng Jiaye Ye Key Laboratory of Bio-Inspired Smart Interfacial science and Technology Ministry of EducationSchool of ChemistryBeihang UniversityBeijing 100191China Shaanxi Key Laboratory of New Transportation Energy and Automotive Energy Saving School of Energy and Electrical EngineeringChang’an UniversityXi’an 710061ShaanxiChina school of Chemistry and Physics Faculty of ScienceQueensland University of TechnologyBrisbaneQLD 4001Australia Centre for Materials science Queensland University of TechnologyBrisbaneQLD 4001Australia

Developing sustainable and clean energy sources(e.g.,solar,wind,and tide energy)is essential to achieve the goal of carbon *** to the discontinuous and inco nsistent nature of common clean energy sources,high-performance energy storage technologies are a critical part of achieving this *** zinc metal batteries(AZMBs)with inherent safety,low cost,and competitive performance are regarded as one of the promising candidates for grid-scale energy ***,zinc metal anodes(ZMAs)with irreversible problems of dendrite growth,hydrogen evolution reaction,self-corrosio n,and other side reactions have seriously hindered the development and commercialization of *** increasing number of researchers are focusing on the stability of ZMAs,so assessing the effectiveness of existing research strategies is critical to the development of *** review aims to provide a comprehensive overview of the fundamentals and challenges of *** rch strategies for interfacial modification of ZMAs are systematically *** features of artificial interfacial coating and in-situ interfacial coating of ZMAs are compared and discussed in detail,as well as the effect of modified interfacial ZMA on the full-battery ***,perspectives are provided on the problems and challenges of *** review is expected to offer a constructive reference for the further development and commercialization of AZMBs.

关键词： Aqueous zinc metal batteries Zinc metal anode Interfacial modification Artificial interfacial coating In-situ interfacial coating

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Quantifying quantum entanglement via machine learning models

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Communications in Theoretical Physics 2024年第7期76卷 52-56页

作者： changchun Feng Lin Chen LMIB(Beihang university) Ministry of EducationBeijing 100191China school of Mathematical sciences Beihang UniversityBeijing 100191China International Research Institute for Multidisciplinary science Beihang UniversityBeijing 00191China

Quantifying entanglement measures for quantum states with unknown density matrices is a challenging *** learning offers a new perspective to address this *** training machine learning models using experimentally measurable data,we can predict the target entanglement *** this study,we compare various machine learning models and find that the linear regression and stack models perform better than *** investigate the model's impact on quantum states across different dimensions and find that higher-dimensional quantum states yield better ***,we investigate which measurable data has better predictive power for target entanglement *** correlation analysis and principal component analysis,we demonstrate that quantum moments exhibit a stronger correlation with coherent information among these data features.

关键词： quantum information entanglement predict machine learning coherence

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Portable fluorescence instrument for detecting membrane integrity in membrane bioreactor (MBR)

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Frontiers of Environmental science & Engineering 2024年第2期18卷 121-131页

作者： Yang Yu changchun Xin Yuxiang Liu Fei Gao Lei Zhang Hui Jia Jie Wang State Key Laboratory of Separation Membranes and Membrane Processes Tiangong UniversityTianjin 300387China school of Environmental science and Engineering Tiangong UniversityTianjin 300387China school of Environmental science and Engineering Tianjin UniversityTianjin 300072China Shenyang Academy of Environmental sciences Shenyang 110167China Cangzhou Institute of Tiangong university Tiangong UniversityCangzhou 061000China

This study proposed the design, fabrication, and assembly of membrane integrity detection instruments in membrane bioreactors (MBR) based on fluorescence spectroscopy. Based on the PARAFAC model, we found that the peak at 280/3.5 nm strengthened after membrane breakage. The peak at 3.0/43. nm reflected the sludge concentration in the MBR and reduced the influence of internal filtration effects on detection. Therefore, we determined that the dual-LED light source excitation detection system can detect tryptophan-like substances at 280 nm (T-peak) and humic acid at 3.0 nm (C-peak). T-peak was identified as the core index indicating membrane integrity. Moreover, the C-peak is the reference indicator factor for a sensitive response to changes in the sludge concentration. The portable fluorescence instrument exhibited high sensitivity and good feedback accuracy compared to particle counting and turbidity detection, where the log reduction value was greater than 3.5. This overcomes the disadvantage of false alarms in particle counters and is not affected by the position of the pump system. This portable instrument provides a flexible and highly sensitive method for the assessment of industrial membrane integrity.

关键词： Membrane integrity Fluorescence spectrum Portable instrument Membrane bioreactor

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Recent progress on the structure of Ser/Thr protein phosphatases

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science China(life sciences) 2008年第6期51卷 487-494页

作者： WANG BaiJing1,2, ZHANG Peng1 & WEI Qun1 1 Department of Biochemistry and Molecular Biology, Beijing normal university, Beijing Key Laboratory, Beijing 100875, China 2 school of life science,{3., changchun 13.03., China 1. Department of Biochemistry and Molecular Biology Beijing Normal University Beijing Key Laboratory Beijing 100875 China 2. school of life science Changchun Normal University Changchun 130032 China

PP1, PP2A and PP2B, belonging to the PPP family of Ser/Thr protein phosphatases, participate in regulating many important physiological processes, such as cell cycle control, regulation of cell growth and division regulation, etc. The sequence homology between them is relatively high, and ter- tiary structure is conserved. Because of the complexity of the structure of PP2A and the diversity of its regulatory subunits, its structure is less well known than those of PP1 and PP2B. The PP2A holoen- zyme consists of a heterodimeric core enzyme, comprising a scaffolding subunit and a catalytic sub- unit, as well as a variable regulatory subunit. In this study, the subunit compositions, similarities and differences between the Ser/Thr protein phsphatases structures are summarized.

关键词： Ser/Thr phosphatases subunit composition similarities and differences crystal structure

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Anisotropism of the Non-Smooth Surface of Butterfly Wing

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Journal of Bionic Engineering 2009年第1期6卷 71-76页

作者： Gang Sun~(1,2), Yan Fang~(1,2), Qian Cong~1, Lu-quan Ren~11. Key Laboratory of Terrain-Machine Bionics Engineering (Ministry of Education, China), Jilin university,changchun 13.022, P. R. China2. school of {3. science, changchun normal university, changchun 13.03., P. R. China [a]Key Laboratory of Terrain-Machine Bionics Engineering (Ministry of Education China) Jilin University Changchun 130022 P. R. China [b]School of Life Science Changchun Normal University Changchun 130032 P. R. China

Twenty-nine species of butterflies were collected for observation and determination of the wing surfaces using a Scanning Electron Microscope(SEM).Butterfly wing surface displays structural anisotropism in micro-,submicro- and *** scales on butterfly wing surface arrange like overlapping roof *** are submicrometric vertical gibbosities,horizontal links,and nano-protuberances on the ***-incline-then-drip method and first-drip-then-incline method were used to measure the Sliding Angle(SA)of droplet on butterfly wing surface by an optical Contact Angle(CA)measuring system. Relatively smaller sliding angles indicate that the butterfly wing surface has fine self-cleaning *** different SAs in various directions indicate the anisotropic self-cleaning property of butterfly wing *** SAs on the butterfly wing surface without scales are remarkably larger than those with scales,which proves the crucial role of scales in determining the self-cleaning *** wing surface is a template for design and fabrication ofbiomimetic materials and self-cleaning *** work may offer insights into how to design directional self-cleaning coatings and anisotropic wetting surface.

关键词： micro-/nano-structure anisotropism self-cleaning super-hydrophobicity sliding angle

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Alterations in DNA methylation and genome structure in two rice mutant lines induced by high pressure

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science China(life sciences) 2006年第2期49卷 97-104页

作者： SHEN Sile1,3. WANG Zhenwei3. SHAN Xiaohui2, WANG Hua3. LI Ling3. LIN Xuyun2, LONG Likun2, WENG Kenan4, LIU Bao2 & ZOU Guangtian1 1. National Laboratory of Superhard Materials, Jilin university, changchun 13.012, China 2. Institute of Genetics and Cytology, Northeast normal university, changchun 13.024, China 3. College of life science, Jilin university, changchun 13.012, China 4. Guangzhou Institute of Geochemistry, Chinese Academy of sciences, Guangzhou 510640, China 1. National Laboratory of Superhard Materials Jilin University Changchun 130012 China 3. College of life science Jilin University Changchun 130012 China 2. Institute of Genetics and Cytology Northeast Normal University Changchun 130024 China 4. Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China

By using high-pressure treatment, two mutant lines were obtained from agenetically stable japonica rice cultivar Bijing3.. Genomic DNA of the mutant lines, together withthe original line (Bijing3.), was either undigested or digested by Hpa ⅡIMspⅠ, and then subjectedto molecular analysis using two markers, ISSR and RAPD. Results indicated that changes in the PCRamplification profiles of both markers are apparent in the two mutant lines compared with theoriginal rice cultivar, suggesting that there had been both sequence changes and DNA methylationmodifications in the mutant lines. Southern blot analysis using diverse sequences, including twocellular genes (S2 and S3., a set of retrotransposons (Osr7, Osr3., Tos19 and more), and a MITEtransposon family (mPing and Pong), confirmed the results, and indicated that changes in DNAmethylation pattern, genomic structure, and possible activation of some transposons indeed occurredin the mutant lines. Moreover, these changes are stably maintained through selfed generations and indifferent organs. Thus, our results indicate that it is possible to obtain stable mutants in riceby high pressure treatments, and the molecular basis of the mutants may include both genetic andepigenetic changes. Therefore, high hydrostatic pressure seems a promising approach for plantmutagenesis.

关键词： DNA methylation, genomic changes, high pressure, mutagenesis, rice.

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A PSTAIRE CDK-like protein localizes in nuclei and cytoplasm of Physarum polycephalum and functions in the mitosis

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Cell Research 2004年第2期14卷 169-175页

作者： Gui Ying LI~(1,2), Miao XING~(1,*), Bo HU~(1,3. ~1College of life science, Shenzhen Key Laboratory of Microbial Gene Engineering, Shenzhen university, Shenzhen 518060, China. ~2Department of Immunology, {3. of Basic Medical sciences, Jilin university, changchun 13.021, China ~3.nstitute of Genetics and Cytology, Northeast normal university, changchun 13.024, China. College of life science Shenzhen Key Laboratory of Microbial Gene Engineering Shenzhen University Shenzhen 518060 China.

CDKs play key roles in controlling cell cycle progression in all eukaryotes. In plants, multiple CDKs are present, among which the best characterized CDKs are PSTAIRE CDKs. In this study, we carried out Western blot, immunoelectron microscopy and antibody treatment with an anti-PSTAIRE monoclonal antibody to explore the subcellular localization and functions of PSTAIRE CDKs in Physarum polycephalum. The results of Western blot and immunoelectron microscopy showed that in P. polycephalum, a PSTAIRE CDK-like protein was 3. kD in molecular weight and located in both nuclei and cytoplasm. In nuclei, the protein was mainly associated with chromosomes and nucleoli. The expression of the PSTAIRE CDK-like protein in both the plasmodia and nuclei showed little fluctuation through the whole cell cycle. When treated with an anti-PSTAIRE monoclonal antibody at early S phase, the cells were arrested in S phase, and the mitotic onset of P. polycephalum was blocked for about 1 h when treated at early G2 phase. Our dat

关键词： PSTAIRE CDK-like protein Physarum polycephalum mitosis immunoelectron microscopy.

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Measurement of the linear electro-optic coefficient of a minute cBN sample

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science China(Technological sciences) 2005年第2期48卷 233-340页

作者： DOU Qingping1, , MA Haitao1, JIA Gang1, CHEN Zhanguo1 2 & ZHANG Tiechen3.1. College of Electronic science and Engineering, State Key Laboratory on Integrated Optoelectronics, Jilin university, changchun 13.023. China 2. Mudanjiang {3. Institute, Mudanjiang 157012, China 3. State Key Laboratory of Superhard Materials, Jilin university, changchun 13.012, China 1. College of Electronic science and Engineering State Key Laboratory on Integrated Optoelectronics Jilin University 130023 Changchun China 2. Mudanjiang normal Institute 157012 Mudanjiang China 3. State Key Laboratory of Superhard Materials Jilin University 130012 Changchun China

Cubic boron nitride (cBN) is a kind of artificial (synthetic) crystal. Transverse electro-optic modulation in a minute cBN sample was carried out. Basing on the practical form of the crystal, we established the theoretical and experimental method according to the sample. For the first time, the linear electro-optic effect was observed in cBN, and half-wave voltage of the cBN sample was measured successfully. Furthermore, its linear electro-optic coefficient was calculated at 1.17×10?14 m/V.

关键词： cBN crystal, linear electro-optic effect, half-wave voltage, linear electro-optic coefficient.

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pH-Dependent Stability of EGX, A Multi-functional Cellulase from Mollusca, Ampullaria crossean

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Acta Biochimica et Biophysica Sinica 2004年第9期36卷 603-608页

作者： Wen-Ying LI2, Ji WANG1, Yan-Hong LI1, Ming DING1, Gen-Jun XU1,3. Lan-Ying LIU2, and Fu-Kun ZHAO1,3. 1Key Laboratory of Proteomics, Institute of Biochemistry and Cell Biology, Shanghai Institutes for Biological sciences, the Chinese Academy of sciences,Graduate school of the Chinese Academy of sciences, Shanghai 20003., China 2College of life science, Jilin university, changchun 13.023. China College of life science, Zhejiang university of science and Technology, Hangzhou 3.0018, China Key Laboratory ofProteomics Institute of Biochemistry and Cell BiologyShanghai Institutes for Biological Sciencesthe Chinese Academy of SciencesGraduate School of the Chinese Academy of SciencesShanghai 200031China

The cellulase activity and stability of EGX, a multi-functional cellulase previously purified from the mollusca Ampullaria crossean, was systematically studied under different pH. The pH induced con- formation and stability change of EGX have been investigated by using the intrinsic fluorescence, ANS fluorescence and CD spectrum. It has been found that the conformation and activity of this cellulase were strongly dependent on the pH. EGX was stable for both the enzyme activity and the conformation from pH 5.6 to pH 7.4. As shown by intrinsic and ANS fluorescence, no red shift of emission maximum occurred and a negligible intensity change was observed at pH 5.6–7.4. The activity of EGX remained about 80% in pH 5.6–7.4 and obviously decreased out of side the pH range. Urea-induced changes in EGX at pH 5.4 and pH 8.0 were measured by intrinsic fluorescence and CD spectrum. At pH 5.4, a significantly red shift of emission maximum occurred when the concentration of urea was 5 M compared to the concentration was 3.M at pH 8.0. The α-helix at pH 5.4 was 40.51% in the absence of urea and 3..04% in the presence of 4 M urea. At pH 8.0 the α-helix was 7.23. in the presence of 4 M urea. The data indicated that EGX was much susceptible to urea-induced unfolding at pH 8.0 and much stable at pH 5.4. The greater pH dependent stability of EGX may allow the enzyme to adequately catalyze the hydrolysis of cellulosic materials under natural or industrial extreme conditions.

关键词： multi-functional cellulase stability Ampullaria crossean fluorescence spectroscopy pH-dependent structural change CD spectrum

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PDMS prism-glass optical coupling for surface plasmon resonance sensors based on MEMS technology

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science China(Information sciences) 2010年第10期53卷 2144-2158页

作者： GENG ZhaoXin 1,2 , LI Qing 3., WANG Wei 1 & LI ZhiHong 1 1 Institute of Microelectronics, Peking university, Beijing 100871, China 2 school of Information engineering, Minzu university of China, Beijing 100081, China 3.school of sciences, changchun university of science and Technology, changchun 13.000, China 1. Institute of Microelectronics Peking University Beijing 100871 China2. School of Information engineering Minzu University of China Beijing 100081 China3. School of Sciences Changchun University of Science and Technology Changchun 130000 China

A miniaturized surface plasmon resonance (SPR) chip has been developed for biomedical and chem-ical analysis with low cost and high performance. The techniques of bulk silicon micromachining and polymer replication were used to fabricate the Kretschmann SPR sensor composed of a Polydimethylsiloxane (PDMS) prism, a coupling glass and microchannels. The plasmon properties of thin metal films were investigated theoret-ically based on Fresnel analysis, with optical boundary conditions pertaining to the surface plasmon resonance at the gold/water and gold/air interfaces. The theoretical results show that difference in the refractive index (RI) between the PDMS prism and the coupling glass layer affect the precision of the SPR angle and the SPR curve. Meanwhile, the period of the interference fringe attaching on the SPR curve increases with an increase in wavelength and a decrease in the refractive index of the coupling glass layer. The gold thickness of 50 nm is required while employing a fixed incident wavelength of 650 nm, to achieve optimum SPR excitation conditions and the sensor sensitivity. The characteristics of this SPR sensor were evaluated in the angular interrogation mode of employing the incident wavelength of 650 nm in air and water media, respectively. The obtained SPR angles were approximately consistent with the theoretical ones.

关键词： surface plasmon resolance polymer microfluidic PDMS

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