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Size-dependent hydroxyl radicals generation induced by SiO_2 ultra-fine particles: The role of surface iron

Science china Chemistry 2009年第7期52卷 1033-1041页

作者： SHANG Yu1, ZHU Tong1, LI Yi1,2 & ZHAO JinCai3 1 College of Environmental sciences and Engineering, Peking University, beijing 100871, china 2 chinese academy of meteorological sciences, beijing 100871, china 3 Institute of Chemistry, chinese academy of sciences, beijing 100871, china College of Environmental sciences and Engineering Peking University Beijing China chinese academy of meteorological sciences Beijing China Institute of Chemistry Chinese Academy of Sciences Beijing China

Oxidative stress and hydroxyl radicals (·OH) play important roles in adverse health effects caused by inhalable ambient air particles (PM10). The ultra-fine fraction of PM10 has been hypothesized as one of the critical contributors to ·OH generation. Both in vivo and in vitro studies have shown that ultra-fine particles (UFPs) or nano-particles generate more ·OH than larger particles with identical mass and composition. Both the surface area and surface-adsorbed redox-active metals have been suggested as factors to determine the oxidative capacity of UFPs. In this study, the ·OH-generating capability of dif-ferent sizes of SiO2 particles was investigated in order to determine which factor influences particle-induced ·OH generation. The amount of ·OH generated in both acellular and cellular systems was quantified using a capillary electrophoresis method following exposure to SiO2 particles with diameters of 14, 100, and 500 nm. The amount of ·OH was strongly dependent on particle size, and a significant enhancement was observed only with 14 nm particles. Further studies indicated a close association between ·OH and iron ion concentration (R2 = 0.812, p2 particles is presented as a possible mechanism of UPFs-induced ·OH generation. The SiO2 acted as an inert substrate, and the surface of ultra-fine SiO2 particles acted as a carrier for iron.

关键词： ultra-fine particles nano-particles ·OH oxidative stress size-effect

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Role of atmospheric heat source/sink over the Qinghai-Xizang Plateau in quasi-4-year oscillation of atmosphere-land-ocean interaction

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chinese Science Bulletin 2001年第3期46卷 241-245页

作者： ZHAO Ping & CHEN LongxunDepartment of Geophysics, Peking University, beijing 100871, china chinese academy of meteorological sciences, beijing 100081, china Department of Geophysics Peking University Beijing China chinese academy of meteorological sciences Beijing China

Using 1961-1995 monthly atmospheric apparent heat source/sink over the Qinghai-Xizang Plateau (QXP)and reanalysis data of NCEP/NCAR, and 1961 ?1994 monthly SST of UK/GISST2, the statistical study is undertaken on the QXP heat source/sink in relation to both atmospheric circulation in Asia and El Nino/La Nina events. It is discovered that there exists noticeable interaction in aquasi-4-year period among the of the QXP, low-levelmeridional winds east of the QXP, low-level zonal winds in the equatorial Pacific, SST in the equatorial eastern Pacific, and the circulation at mid and high latitudes north of the QXP. They have difference in phase. The cold source intensity of the QXP in winter favours a low-level meridional wind anomaly to prevail in the mainland of china and its coast east of the QXP and to last until the subsequent autumn. The wind anomaly can induce a low-level zonal wind anomaly of the tropic Pacific that finally affects an El Nino/La Nina event in the autumn and subsequent winter.

关键词： Qinghai-Xizang Plateau thermal effect interannual variation atmosphere-land-ocean interaction.

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ON THE CENTRAL RELAXING SCHEME Ⅱ: SYSTEMS OF HYPERBOLIC CONSERVATION LAWS

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Journal of Computational Mathematics 2001年第6期19卷 571-582页

作者： Hua-zhong Tang (School of Mathematical sciences, Peking University, beijing 100871, china) (LSEC,ICMSEC academy of Mathematics and Systems sciences, chinese academy of sciences, beijing 100080, china) School of Mathematical sciences Peking University Beijing 100871 China

This paper continues to study the central relaxing schemes for system of hyperbolic conservation laws, based on the local relaxation approximation. Two classes of relaxing systems with stiff source term are introduced to approximate system of conservation laws in curvilinear coordinates. Based on them, the semi-implicit relaxing schemes are con- structed as in [6, 12] without using any linear or nonlinear Riemann solvers. Numerical experiments for one-dimensional and two-dimensional problems are presented to demon- strate the performance and resolution of the current schemes.

关键词： Hyperbolic conservation laws The relaxing system The central relaxing schemes The Euler equations.

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Teleconnection between the Indian summer monsoon onset and the Meiyu over the Yangtze River Valley

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Science china Earth sciences 2008年第7期51卷 1021-1035页

作者： LIU YunYun1,2,3 & DING YiHui2 1 chinese academy of meteorological sciences, beijing 100081, china 2 National Climate Center, beijing 100081, china 3 Graduate University of chinese academy of sciences, beijing 100049, china chinese academy of meteorological sciences Beijing China National Climate Center Beijing China Graduate University of chinese academy of sciences Beijing China

Based on the Indian and chinese precipitation data and the NCEP-NCAR reanalysis circulation data, the relationship between the Indian summer monsoon (ISM) onset and the Meiyu over the Yangtze River Valley has been discussed by the methods of correlation analysis and composite analysis. The results show that the date of ISM onset over Kerala in the southwestern coast of the Indian Peninsula is about two weeks earlier than the beginning of the Meiyu over the Yangtze River Valley. After the outbreak of ISM, the teleconnection mode sets up from the western coast of India via the Bay of Bengal (BOB) to the Yangtze River Valley and southern Japan. It is different both in time and space from the telecon- nection mode which is from the northwest of India via the Tibetan Plateau to northern china. The for- mer mode is defined as the "south" teleconnection of the Asian summer monsoon, forming in the pe- riod of ISM onset; while the latter mode is called the "north" teleconnection, mainly occurring in the Asian monsoon culminant period. During the process of the "south" teleconnection’s formation, the Asian monsoon circulation has experienced a series of important changes: ISM onset, the northward movement of the south Asia high (SAH), the onset vortex occurrence, the eastward extension of the stronger tropical westerly belt, and the northeastward jump of the western Pacific subtropical high (WPSH), etc. Consequently, since ISM sets up over Kerala, the whole Asian continent is covered by the upper SAH after about two weeks, while in the mid- and lower troposphere, a strong wind belt forms from the Arabian Sea via the southern India, BOB and the South china Sea (SCS), then along the western flank of WPSH, to the Yangtze River Valley and southern Japan. With the northward moving of the subtropical jet streams, the upper westerly jet stream and the low level jet have been coupled ver- tically over east Asia, while the Yangtze River Valley happens to locate in the ascending motion

关键词： Indian summer monsoon (ISM) the Meiyu over the Yangtze River Valley teleconnection mode

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CONVERGENCE OF VORTEX METHODS FOR 3-D EULER EQUATIONS

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Journal of Computational Mathematics 2000年第3期18卷 239-250页

作者： Jia-fu Lin (Institute of System Science, academy of Mathematics and System sciences, chinese academy of sciences, beijing, 100080, china School of Mathematical sciences, Peking University, beijing 100871, china) 中科院系统科学所北京 100080

Presents a study on the convergence of vortex methods for the three-dimensional Euler equations in bounded domains. Related studies on the convergence of vortex methods; Formulation of vortex methods; Convergence for ... 详细信息

关键词： Euler equations vortex methods convergence initial-boundary value problem

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An integrated decision method for prediction of tropical cyclone movement by using genetic algorithm

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Science china Earth sciences 2005年第3期48卷 429-440页

作者： YANG Yuanqin1 & WANG Jizhi2 1. National meteorological Center, beijing 100081,china 2. chinese academy of meteorological sciences, beijing 100081, china National meteorological Center Beijing China chinese academy of meteorological sciences Beijing China

In this study an integrated decision method for the multi-prediction results of tropical cyclone movements by using genetic algorithm (GA) has been adopted. A genetic learning artifi- cial neural network (GLANN) as a learning mechanism for track prediction was developed through training with the huge samples of typhoon tracks from 1884 to 2002. The prediction of typhoon motion is to consider how to suit the dynamic change of environment, where typhoon passed through. The neural network structure is described by GA. A fitness function for choice of GA is given to approach the maximum of fitness (the minimum of the errors). Parallel comparing analyses for prediction abilities of unusual typhoon tracks in recent years by GLANN with multi-forecast methods were conducted. More types of cases were employed in the comparing analyses, which consist of the typhoon, Winnie, No.11, in 1997, characterized by a long life over the ocean and in the mainland with severe effect on china, the 10 unusual typhoon tracks in the 1990s, the tracks with landfall and affected action in 1998 and the typhoons born in the Northwestern Pacific and the South china Sea in 2000, including the 24—48 h forecast, etc. The results indicated that for prediction ability of typhoon tracks, specially for unusual typhoons, GA decision-making developed in this study is superior to the others.

关键词： genetic algorithm, integrated decision, prediction of tropical cyclone.

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GM-CSF-induced Ca_(2+) -activated non-voltage-dependent inwardly rectifying K_+ channel in murine peritoneal exudate macrophages

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chinese Science Bulletin 1997年第11期42卷 947-952页

作者： ZHANG Xiaofeng, FENG Meifu, WU Caihong and ZHOU Pei’aiState Key Laboratory of Biomembrane and Membrane Biotechnology, chinese academy of sciences, beijing 100080, china 1 . In-stitute of Zoology, chinese academy of sciences, beijing 100080, china 2 College of Life sciences, Peking University, beijing 100871, china State Key Laboratory of Biomembrane and Membrane Biotechnology Chinese Academy of Sciences Beijing 100080 China

GRANULOCYTE-MACROPHAGE colony-stimulating factor(GM-CSF),a member in the family ofglycoprotein cytokines,can not only act to stimulate proliferation of immature progenitors,butalso enhance differentiated functions of mature effector *** has two kinds of biologicaleffects on mature effector cells,*** effect and indirect *** latter is also

关键词： K+ channel patch clamp GM-CSF macrophage.

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Interannual variation of annual precipitation and urban effect on precipitation in the beijing region

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Progress in Natural Science:Materials International 2007年第9期17卷 1042-1050页

作者： Yu Shuqiu(State Key Laboratory on Severe Weather,chinese academy of meteorological sciences,beijing 100081,china) State Key Laboratory on Severe Weather Chinese Academy of Meteorological Sciences Beijing 100081 China

The large scale character of the interannual variation of precipitation and the urban effect on local annual precipitation anomaly are investigated in this paper based on the 1960-2000 annual precipitation observations at 20 stations in the beijing *** results show that:the annual precipitation in the beijing region possesses the large scale variation character with the linear trend of-1.197/10 yr,which corresponds to a total reduction of 27.82 mm in annual precipitation in the 41 years;the local annual precipitation anomalies(percent of the normal 1960-2000)show a positive center near the urban area,*** precipitation island(UPI),whose intensity increases with the linear trend of 0.6621%/10 yr,opposite to the interannual trend of large scale precipitation over the beijing region;changes in the UPI are also associated with the intensity of synoptic processes of precipitation,and when the synoptic processes are strong(wet years),the intensity of UPI strengthens,while the synoptic processes are weak(dry years),and the UPI disappears in the beijing region.

关键词： urban precipitation island effect interannual climate variation precipitation beijing atmospheric science

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An integrative estimation model of summer rainfall-band patterns in china

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Progress in Natural Science:Materials International 2007年第3期17卷 280-288页

作者： WEI Fengying (State Key Laboratory of Severe Weather, chinese academy of meteorological sciences, beijing 100081, china) State Key Laboratory of Severe Weather Chinese Academy of Meteorological Sciences Beijing 100081 China

Three variation indices are defined to objectively and quantitatively represent fluctuations of three rainfall-band patterns in summers in china for the period from 1951 to 2005, and the variation features of these indices are analyzed on both of interdecadal and interannual scales. A new method is proposed to establish an integrative estimation model based on the analysis of rainfall-band indices, and the model is applied to air, ocean factors to estimate their roles on variations of three rainfall-band patterns on different time-scales. The tests of estimation effects show that the fluctuations of three rainfall-band patterns are composed of variations on both significant inter-decadal and interannual scales, of which the interannual variation is mainly influenced by the Elnino/Lanina events, the East Asia monsoon and the ridge locations of subtropical high pressures in western pacific, while the interdecadal variation is mainly controlled by the Pacific decadal oscillation and interdecadal oscillations of the Arctic oscillation, ENSO, Nino3 sea surface temperature and summer monsoon. The estimated results from the integrative estimation model of rainfall-band patterns suggest that the way of estimation first according to each time scale of both the interdecadal and interannual scales, then estimating with an integration, which is proposed in this paper, has an obvious improvement on that without separation of time scales.

关键词： rainfall-band pattern interannual variation interdecadal variation integration estimation model.

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Infrared Galaxies in the Nearby Universe

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chinese Journal of Astronomy and Astrophysics 2008年第6期8卷 643-652页

作者： Jian-Ling Wang 1 National Astronomical Observatories,chinese academy of sciences,beijing 100012,china 2 Graduate School of chinese academy of sciences,beijing 100049,china National Astronomical Observatories Chinese Academy of Science

We used the Sloan Digital Sky Survey （SDSS） Data Release 5 （DR5） to study the morphological properties of 1137 nearby infrared （IR） galaxies, most of which are brighter than 15.9 mag in r-band. This sample was drawn from a cross-correlation of the Infra-Red Astronomical Satellite （IRAS） point source catalog redshift survey with DR5 at z ≤ 0.08. Based on this IR galaxy sample, we constructed five volume-limited sub-samples with IR luminosity ranging from 10^9.5 L⊙ to 10^12L⊙. By deriving the IR luminosity functions （LF） for different morphological types, we found that normal spiral galaxies are the dominant population below LIR ~ 8 ~ 10^10 L⊙; while the fraction of barred spiral galaxies increases with increasing IR luminosity and becomes dominant in spiral galaxies beyond LIR ≈ 5 × 10^10L⊙. As the IR luminosity decreases, the IR galaxies become more compact and have lower stellar masses. The analysis also shows that normal spiral galaxies give the dominant contribution to the total comoving IR energy density in the nearby universe, while, in contrast, the contribution from peculiar galaxies is only 39%.

关键词： galaxies evolution galaxies interactions galaxies starburst infrared galaxies galaxies luminosity function

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