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Trace element characteristics and origin of intergranular components in mantle peridotites

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Chinese Science Bulletin 2000年第7期45卷 643-649页

作者： XU Yigangguangzhou institute of geochemistry, Chinese {3. of{4., guangzhou 51064., China guangzhou institute of geochemistry Chinese Academy of Sciences Guangzhou China

Leaching experiment has been carried out on mantle xenoliths with different petrographic features in order to directly characterize the nature of intergranular components. ICP-MS analyses of leachates show that they are characterized by high LREE concentrations with strong depletion of Ta. The total REE contents and whether the negative Rb, Ba and Nb anomalies are present or not in intergranular components are largely dependent upon the nature of mantle metasomatism experienced by its host rock. It is proposed that intergranular components may represent residues of small volume metasomatic melts.

关键词： peridotite xenoliths intergranular components trace elements upper mantle.

Superlarge ore deposits and development of China's mineral resources

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Chinese Science Bulletin 1999年第15期44卷 1436-1440页

作者： ZHAO Zhenhuaguangzhou institute of geochemistry , Chinese {3. of{4. , guangzhou 51064., China Guangzhau institute of geochemistry Chinese Academy of Sciences Guangzhou China

The ever increasing demand of mineral resources in China was assessed and it is suggested that the development of superlarge ore deposits was the best way to meet such demand. Research and exploitation of superlarge ore deposits can bring great economic and social benefits to the society. It is also the best way to a better integration of resource industry development and environmental protection and therefore provides a basis of sustainable development of China. China has made important advancements in the research of superlarge ore deposits and especially in classification, selectivity and confinement of deposit types and temporal and spatial distributions. It is suggested that the metallodynamics and the interaction between the crust and the mantle and the core should be studied. At the same time, a new concept of resources should be established in order to build a new integrated system for research, and resource development and environmental proiection.

关键词： superlarge ore deposit metallodynamics resource-environmental integration.

Discovery of seep carbonate nodules as new evidence for gas venting on the northern continental slope of South China Sea

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Chinese Science Bulletin 2006年第10期51卷 1228-1237页

作者： CHEN Zhong1,2,3. YAN Wen1,2,3. CHEN Muhong1,3. WANG Shuhong1,2,3. LU Jun1,3. ZHANG Fan1,3. XIANG Rong1,3. XIAO Shangbin1,3. YAN Pin1,2,3.& GU Senchang1,2,3.1. South China Sea institute of Oceanology, Chinese academy of Sci-ences, guangzhou 5103.1, China 2. guangzhou Center for Gas Hydrate Research, Chinese academy of sciences, guangzhou 5103.1, China 3. Key Laboratory of Marginal Sea Geology, South China Sea institute of Oceanology and guangzhou institute of geochemistry, Chinese academy of sciences, guangzhou 5103.1, China South China Sea institute of Oceanology Chinese Academy of Science Guangzhou China guangzhou Center for Gas Hydrate Research Chinese Academy of Sciences Guanzhou China Key Laboratory of Marginal Sea Geology South China Sea Institute of Oceanology and Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou China

Seep carbonate nodules were firstlycollected from the southwestern Dongsha area onnorthern continental slope of South China Sea formineralogical and geochemical studies. The resultsof X-ray diffraction show that carbonate nodules arecomposed of Fe-rich domolite,siderite and a few cal-cite and aragonite, as well as a small quantity ofnon-carbonate minerals such as goethite, quartz andclay minerals. Fe-rich dolomite and siderite charac-terized by euhedral microcrystalline structure weredirectly precipitated at cold seeps. The δ 13. valuesfor Fe-rich dolomite and siderite in the bulk nodulesvary from ?18.24. to ?3..07‰, and the δ 18O valuesrange from 0.4. to 2.76‰. Their moderate depleted13. reflects that carbon origin is possibly thermoge- netic gas or mixed gas, which is evidence of gasventings in the seafloor. Moreover, massive wormtube fossils related to cold seeps were found on thesurfaces of carbonate nodules, and the conduitsand/or channels in semi-solidified nodules whichwere not filled by carbonate or sediment were alsoobserved. A preliminary conclusion is that activemicro gas venting with a conduit/channel diameterrange from 200 μm to 600 μm possibly exists inmodern seafloor of the carbonate nodule area.

关键词：渗出碳酸盐节碳氧同位素甲烷渗漏天然气水化物

Eclogites in the interior of the Tibetan Plateau and their geodynamic implications

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Chinese Science Bulletin 2009年第15期54卷 2556-2567页

作者： ZHANG KaiJun1,2 & TANG XianChun2,3.1 Department of Earth sciences, Nanjing University, Nanjing 210093. China 2 guangzhou institute of geochemistry, Chinese {4. of sciences, guangzhou 51064., China 3.Graduate University of Chinese {4. of sciences, Beijing 10004., China Department of Earth sciences Nanjing University Nanjing 210093 China guangzhou institute of geochemistry Chinese Academy of Sciences Guangzhou 510640 China Graduate University of Chinese academy of sciences Beijing 100049 China

Eclogites have been recently reported in the interior of the Tibetan Plateau, including in the central Qiangtang metamorphic belt, in the Basu metamorphic massif of the eastern Bangong-Nujiang suture zone, and at Songdo and Pengco in the eastern Lhasa terrane. Some typical ultrahigh-pressure (UHP) metamorphic phenomena, e.g., garnet exsolution from clinopyroxene, were documented in the Basu and Pengco eclogites. The UHP metamorphism in the interior of the Tibetan Plateau marked by these eclogites generally took place in the Early Mesozoic. Along with exhumation of these eclogites, (post-) collision-related magmatism extensively occurred around the central Qiangtang belt, the eastern Ban-gong-Nujiang suture zone, and the eastern Lhasa terrane. The occurrence of these Early Mesozoic ec-logites manifests an out-of-sequence evolution of the Tethys, and they could be a product of diachro-nous collision between the eastern Qiangtang terrane and the irregular continental margin of the united western Qiangtang-Lhasa plate, along the linked eastern Bangong-Nujiang-central Qiangtang zone. The collision-related magmatic rocks could have been originated from lithospheric thickening, melting, or detachment due to the collision. The presence of UHP metamorphic rocks in central Qiangtang and Basu implies likely continental deep-subduction, and the denudation of these two metamorphic zones could have served as the source of the Triassic turbidites in the Songpan-Garzê complex and the Ju-rassic turbidites in the western Bangong-Nujiang zone, respectively. However, studies of the eclogites in the interior of the Tibetan Plateau just began, and many principal aspects still remain to be explored, such as their distributions, typical lithologies and minerals, temperature-pressure conditions, timing of formation and exhumation, protoliths and tectonic setting, and relationship with the evolution of the Tethys and large-scale basins in Tibet.

关键词：地球动力学意义青藏高原榴辉岩

Alterations in DNA methylation and genome structure in two rice mutant lines induced by high pressure

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Science China(Life sciences) 2006年第2期49卷 97-104页

作者： SHEN Sile1,3. WANG Zhenwei3. SHAN Xiaohui2, WANG Hua3. LI Ling3. LIN Xuyun2, LONG Likun2, WENG Kenan4. LIU Bao2 & ZOU Guangtian1 1. National Laboratory of Superhard Materials, Jilin University, Changchun 13.012, China 2. institute of Genetics and Cytology, Northeast Normal University, Changchun 13.024. China 3. College of Life Science, Jilin University, Changchun 13.012, China 4. guangzhou institute of {3., Chinese {4. of sciences,{14., China 1. National Laboratory of Superhard Materials Jilin University Changchun 130012 China 3. College of Life Science Jilin University Changchun 130012 China 2. institute of Genetics and Cytology Northeast Normal University Changchun 130024 China 4. guangzhou institute of geochemistry Chinese Academy of Sciences Guangzhou 510640 China

By using high-pressure treatment, two mutant lines were obtained from agenetically stable japonica rice cultivar Bijing3.. Genomic DNA of the mutant lines, together withthe original line (Bijing3.), was either undigested or digested by Hpa ⅡIMspⅠ, and then subjectedto molecular analysis using two markers, ISSR and RAPD. Results indicated that changes in the PCRamplification profiles of both markers are apparent in the two mutant lines compared with theoriginal rice cultivar, suggesting that there had been both sequence changes and DNA methylationmodifications in the mutant lines. Southern blot analysis using diverse sequences, including twocellular genes (S2 and S3., a set of retrotransposons (Osr7, Osr3., Tos19 and more), and a MITEtransposon family (mPing and Pong), confirmed the results, and indicated that changes in DNAmethylation pattern, genomic structure, and possible activation of some transposons indeed occurredin the mutant lines. Moreover, these changes are stably maintained through selfed generations and indifferent organs. Thus, our results indicate that it is possible to obtain stable mutants in riceby high pressure treatments, and the molecular basis of the mutants may include both genetic andepigenetic changes. Therefore, high hydrostatic pressure seems a promising approach for plantmutagenesis.

关键词： DNA methylation, genomic changes, high pressure, mutagenesis, rice.

Advances in the study of current-use non-PBDE brominated flame retardants and dechlorane plus in the environment and humans

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Science China Chemistry 2010年第5期53卷 961-973页

作者： LUO XiaoJun,CHEN SheJun,MAI BiXian & FU JiaMo State Key Laboratory of Organic geochemistry guangzhou institute of geochemistry,Chinese{4. of sciences,guangzhou 51064.,China 1. State Key Laboratory of Organic geochemistry Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China

The fate of the high production volume,currently in use,and not regulated non-polybrominated diphenyl ether(PBDE) flame retardants,such as tetrabromobisphenol A(TBBPA) ,hexabromocyclododecane(HBCD) and dechlorane plus(DP),and the alternative flame retardants of PBDE,such as BTBPE and DBDPE,in the environment has attracted increasing attention and aroused concern due to the increasing regulation and phasing-out of *** paper reviews the distribution,bioaccumulation,human exposure and environmental behavior of those non-PBDE flame retardants in various environmental *** data gaps and needs for future research are discussed.

关键词： TBBPA HBCD BTBPE DBDPE DP

Research on the dynamics of the South China Sea opening:Evidence from analogue modeling

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Science China Earth sciences 2006年第10期49卷 1053-1069页

作者： SUN Zhen1,2, ZHOU Di1, ZHONG Zhihong3. XIA Bin2, QIU Xuelin1, ZENG Zuoxun4.& JIANG Jianqun5 1. CAS Key Laboratory of Marginal Sea Geology, South China Sea institute of Oceanology, Chinese academy of sciences, {3. 5103.1, China 2. CAS Key Laboratory of Marginal Sea Geology, {3. institute of geochemistry, Chinese academy of sciences, guangzhou 51064., China 3. Department of Technology, Shenzhen Branch of CNOOC, {3. 51024., China 4. Faculty of Earth sciences, China University of Geosciences, Wuhan 4.0}074. China 5. Hainan Oil & Gas Exploration Company, Liaohe Oilfield PetroChina, Panjin 124.10, China 1. CAS Key Laboratory of Marginal Sea Geology South China Sea Institute of Oceanology Chinese Academy of Sciences Guangzhou 510301 China 2. CAS Key Laboratory of Marginal Sea Geology Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China 3. Department of Technology Shenzhen Branch of CNOOC Guangzhou 510240 China 4. Faculty of Earth sciences China University of Geosciences Wuhan 430074 China 5. Hainan Oil & Gas Exploration Company Liaohe Oilfield PetroChina Panjin 124010 China

Independent of Indochina extrusion, the South China Sea experienced a process from passive continental rifting to marginal sea drifting. According to the fault patterns in the Beibu Gulf basin and the Pearl River Mouth basin, the continental rifting and early spreading stage from 3. to 26 Ma were controlled by extensional stress field, which shifted clockwise from southeastward to south southeastward. From 24.Ma on, the sea spread in NW-SE direction and ceased spreading at around 15.5 Ma. Integrated geological information with the assumption that the South China Sea developed along a pre-Cenozoic weakness zone, we did analogue experiments on the South China Sea evolu- tion. Experiments revealed that the pre-existing weakness zone goes roughly along the uplift zone between the present Zhu-1 and Zhu-2 depression. The pre-existing weakness zone is composed of three segments trending NNE, roughly EW and NEE, respectively. The early opening of the South China Sea is accompanied with roughly 15° clockwise rotation, while the SE sub-sea basin opened with SE extension. Tinjar fault was the western boundary of the Nansha block (Dangerous Ground), while Lupar fault was the eastern boundary of the Indochina, NW-trending rift belt known as Zengmu basin developed between above two faults due to block divergent of Indochina from Nansha. In the experiment, transtensional flower structures along NW-trending faults are seen, and slight inversion occurs along some NE-dipping faults. The existence of rigid massifs changed the orientations of some faults and rift belt, and also led to deformation concentrate around the massifs. The rifting and drifting of the South China Sea might be caused by slab pull from the proto South China Sea subducting toward Borneo and/or mantle flow caused by India-Asia collision.

关键词： South China Sea, rifting and drifting, clockwise rotation, analogue modeling, rigid massifs.

geochemistry of high-Mg andesites from the early Cretaceous Yixian Formation, western Liaoning: Implications for lower crustal delamination and Sr/Y variations

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Science China Earth sciences 2006年第9期49卷 904-914页

作者： WANG Xiaorui1, GAO Shan1,2, LIU Xiaoming1, YUAN Honglin1, HU Zhaochu1, ZHANG Hong1,3.& WANG Xuance4.1. State Key Laboratory of Continental Dynamics, Department of Geology, Northwest University, Xi`an 710069, China 2. State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 4.0}074. China 3. Shenyang {4. of Geology and Mineral Resources, Shenyang 11003., China 4. guangzhou {4. of {4., Chinese academy of sciences, guangzhou 51064., China 1. State Key Laboratory of Continental Dynamics Department of Geology Northwest University Xi’an 710069 China 2. State Key Laboratory of Geological Processes and Mineral Resources China University of Geosciences Wuhan 430074 China 3. Shenyang institute of Geology and Mineral Resources Shenyang 110032 China 4. guangzhou institute of geochemistry Chinese Academy of Sciences Guangzhou 510640 China

85 volcanic rocks of the Yixian Formation from the Sihetun type section werecollected and analyzed for geochemical and isotopic compositions. Major element compositionsindicate that the Sihetun volcanic rocks are high magnesium andesites with some basalts occurring atthe bottom of section. The Sihetun high magnesium andesites (SiO_2 = 52.82-59.3. wt%, Al_2O_3.14.15-16.3.wt%) show many characteristics of adakites such as depletion in heavy rare-earth elements(HREE; Yb = 1.03.1.88 μg/g) and Y(12-20 μg/g) and high Sr (620-13.3.μg/g) and Sr/Y(3.-88), withhigh La_N/Yb_N ratio (10-25). They share similar major and trace element characteristics to volcanicrocks from the Xinglonggou Formation except their lower Nd isotope ratios (^(14.0}Nd/^(14.)Nd(13.Ma) = 0.5118-0.5119, ε_(Nd) (13.Ma) = -11.6-13.8, ^(87)Sr/^(86)Sr (13. Ma) = *** were interpreted in a way that eclogite that formed at the base of thickened Archean lowercrust of the North China craton foundered into the convecting mantle and subsequently melted andinteracted with peridotite. However, compared to the Xinglonggou volcanic rocks, the source of theSihetun magma contained more ancient continental crustal material in order to explain its evolved Ndisotopes. The age of the Sihetun Formation was 120 to 13. Ma, and this indicates that delaminationlasted to the early Cretaceous period. The Sr contents and Sr/Y ratios of the Sihetun high-Mgandesites show significant negative correlations with SiO_2 for samples with SiO_2 > 56%. Thesesuggest that the Sr and Sr/Y values were reduced due to fractional crystallization of ***, the effect of crystallization on volcanic Sr and Sr/Y ratio has to be taken intoaccount.

关键词： High-Mg andesite, Adakite, Yixian Formation, North China Craton, delamination.

Total alkyl dibenzothiophenes content tracing the filling pathway of condensate reservoir in the Fushan Depression,South China Sea

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Science China Earth sciences 2008年第S2期51卷 138-145页

作者： LI MeiJun1,WANG TieGuan1,LIU Ju2,ZHANG MeiZhu2,LU Hong3.MA QinLin2 & GAO LiHui2 1 State Key Laboratory of Petroleum Resources and Prospecting,Earth sciences and Geoinformatics School,China University of Petroleum,Beijing 10224.,China 2 Southern Oil Exploration and Development Company,PetroChina,guangzhou 51064.,China 3.guangzhou {4. of geochemistry,Chinese academy of sciences,guangzhou 51024.,China China Univ Petr Earth Sci & Geoinformat Sch State Key Lab Petr Resources & Prospecting Beijing 102249 Peoples R China PetroChina So Oil Explorat & Dev Co Guangzhou 510640 Peoples R China Chinese Acad Sci Guangzhou Inst Geochem Guangzhou 510240 Guangdong Peoples R China

The condensates are generally characterized by high maturity,low concentration of steranes and ter-panes biomarkers and low content of non-hydrocarbon fraction. In this case commonly used steranes,terpanes and carbazoles parameters cannot be effectively applied in the reservoir-filling tracing. The hydrogen bond formed by sulfur atom in the dibenzothiophenes (DBTs) results in molecule adsorption and fractionation during oil migration in reservoir. Like carbazoles,total DBTs content decreases with the increasing of oil migration distance. Therefore,a new parameter——total DBTs content is proposed to be used to trace the oil migration orientation and filling pathway. In present study,total DBTs con-tents of condensates and light oils are obtained by adding internal standard——eight deuterium atoms substituted DBT during Gas Chromatography-Mass Spectrometry analysis of aromatic fraction. Except for a few samples with much lower content of non-hydrocarbon fraction,the total DBTs content shows a fine positive correlation with that of carbazoles. Large errors can be caused in the process of pyrrolic nitrogen compounds separation. The application of this new parameter in the Fushan Depression of Beibu Gulf Basin,South China Sea indicates that this parameter is a reliable one to trace filling pathway in condensate reservoirs. Combined with other DBTs-related parameters,such as 4./1-methydibenzo-thiophene and 2,4./1,4.dimethyldibenzothiophene,oil migration orientation and filling pathway of the Fushan Depression was determined. The accumulations of Huachang oil field in the Fushan Depres-sion are mainly migrated and charged from northeast to southeast along the Huachang uplift. It can be predicated that the light oil and condensates in the Huachang oil field should be sourced from the source kitchen at the Bailian Sag. It shows that total DBTs content is an effective parameter to tracing oil migration orientation and filling pathway.

关键词： dibenzothiophene alkyl dibenzothiophene condensate reservoir filling pathway molecular markers the Fushan Depression