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Mechanism for calcite dissolution and its contribution to development of reservoir porosity and permeability in the Kela 2 gas field,Tarim Basin,China

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Science China Earth Sciences 2008年第4期51卷 567-578页

作者： YU BingSong1,3, DONG HailLiang2,3 & RUAN Zhuang1,3 1 State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Beijing 100083, China 2 department of geology, miami University,oxford, oh 4.056,{4. 3 Geomicrobiology Laboratory, China University of Geosciences, Beijing, 100083, China State Key Laboratory of Geological Processes and Mineral Resources China University of Geosciences Beijing 100083 China department of geology Miami University Oxford OH 45056 USA Geomicrobiology Laboratory China University of Geoscien

This study is undertaken to understand how calcite precipitation and dissolution contributes to depth-related changes in porosity and permeability of gas-bearing sandstone reservoirs in the Kela 2 gas field of the Tarim Basin, Northwestern China. Sandstone samples and pore water samples are col-lected from well KL201 in the Tarim Basin. Vertical profiles of porosity, permeability, pore water chem-istry, and the relative volume abundance of calcite/dolomite are constructed from 3600 to 4.00 m below the ground surface within major oil and gas reservoir rocks. Porosity and permeability values are in-versely correlated with the calcite abundance, indicating that calcite dissolution and precipitation may be controlling porosity and permeability of the reservoir rocks. Pore water chemistry exhibits a sys-tematic variation from the Na2SO4.type at the shallow depth (3600-3630 m), to the NaHCO3 type at the intermediate depth (3630―3695 m),and to the CaCl2 type at the greater depth (3728―3938 m). The geochemical factors that control the calcite solubility include pH, temperature, pressure, Ca2+ concen-tration, the total inorganic carbon concentration (ΣCO2), and the type of pore water. Thermodynamic phase equilibrium and mass conservation laws are applied to calculate the calcite saturation state as a function of a few key parameters. The model calculation illustrates that the calcite solubility is strongly dependent on the chemical composition of pore water, mainly the concentration difference between the total dissolved inorganic carbon and dissolved calcium concentration (i.e., [ΣCO2] -[Ca2+]). In the Na2SO4.water at the shallow depth, this index is close to 0, pore water is near the calcite solubility. Calcite does not dissolve or precipitate in significant quantities. In the NaHCO3 water at the intermedi-ate depth, this index is greater than 0, and pore water is supersaturated with respect to calcite. Massive calcite precipitation was observed at this depth interval and

关键词： calcite dissolution porosity thermodynamic Tarim Basin

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A restudy of Oryctocephalus indicus (Reed,1910)

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Progress in Natural Science:Materials International 2006年第11期16卷 1177-1182页

作者： ZHAO Yuanlong~1**, YUAN Jinliang~2, PENG Shanchi~ 2,3 , YANG Xinglian~1, PENG Jin~1, LIN Jihpai~4. and GUO Qingjun~5(1. College of Resource and Environment of Guizhou University, Guiyang 550003, China 2. Nanjing Institute of geology and Palaeontology, Chinese Academy of Sciences, Nanjing 210008, China 3. State Key Laboratory of Papaeobiology and Stratigraphy, Nanjing Institute of geology and Palaeontology, Nanjing 210008, China 4. department of Geological Science, ohio State University, Columbus, oh 4.210, usa 5. Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550002, China) College of Resource and Environment of Guizhou University Guiyang 550003 China Nanjing Institute of geology and Palaeontology Chinese Academy of Sciences Nanjing 210008 China State Key Laboratory of Papaeobiology and Stratigraphy Nanjing Institute of Geology and Palaeontology Nanjing 210008 China department of Geological Science Ohio State University Columbus OH 43210 United States Institute of Geochemistry Chinese Academy of Sciences Guiyang 550002 China

Restudy on morphology of Oryctocephalus indicus (Reed, 1910), based on specimens from Guizhou, China and Nevada usa, suggests that the subspecies regarded previously as Oryctocephalus indicus indicus (Reed, 1910), O. indicus latus Zhao et Yuan 2002, and O. indicus kobayashi Saito, 1934. are synonymous, and Oryctocephalus americanus Sundberg et McCollum, 2003 is a similar form of O. indicus. Oryctocephalus indicus is rediagnosed as having a glabella that is subconical in outline and tapering forward slightly; a thorax that comprises 12 segments, and a small pygidium that bears 2—3 axial rings with a terminal piece and a postaxial ridge. Oryctocephalus indicus is widely distributed in eastern Guizhou and ranges through a great interval of Kaili Formation. Its first appearance is almost identical with these events of trilobite extinction-recovery occurring at the end of the Early Cambrian, the alternation of acritach assemblages, the change of trace elements (REE) and stable isotopes (carbon) at the Wuliu-Zengjiaya section. As one of the key forms for defining the traditional Lower-Middle Cambrian boundary (the base of Cambrian Series 3 and Stage 5 in the new Cambrian chronstratigraphic standard), O. indicus has received detailed study and has more advantages than other species such as Ovatoryctocara granulata Tchernysheva, 1962 or Arthricocephalus chauveaui Bergeron, 1899.

关键词： Oryctocephalus indicus restudy Kaili Formation Cambrian Guizhou China.

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On interpolation for Hormander’s algebras

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Science China Mathematics 2010年第3期53卷 763-770页

作者： LI Bao Qin department of Mathematics, Florida International University, miami, FL 33199, usa 1. department of Mathematics Florida International University Miami FL 33199 USA

We discuss some recent results on interpolation problems for weighted Hrmander’s algebras of holomorphic functions in several complex variables, and also give a sharp estimate on counting functions of interpolating... 详细信息

关键词： weight pseudoconvex set Hrmander’s algebra interpolating variety plurisubharmonic function holomorphic function entire function

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Sorption behavior of U(VI), ^(234.U(VI) and ^(238)U(VI) onto fracture-filling clays in Beishan granite, Gansu: Application to selecting the site of high-level radwaste repository in China

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Science China Earth Sciences 2005年第10期48卷 1649-1655页

作者： MIN Maozhong1,2, LUO Xingzhang3, WANG Ju4. JIN Yuanxin4.& WANG Rucheng1 1. department of Earth Sciences, State Key Laboratory of Mineral Deposit Research, Nanjing University, Nanjing 210093, China 2. Center of Materials Analysis, Nanjing University, Nanjing 210093, China 3. department of Environmental Science and Engineering, Nanjing University, Nanjing 210093, China 4. Beijing geology Institute, Nuclear Industry, Beijing 100029, China department of Earth Sciences State Key Laboratory of Mineral Deposit Research Nanjing University Nanjing China Center of Materials Analysis Nanjing University Nanjing China department of Environmental Science and Engineering Nanjing University Nanjing China Beijing geology Institute Nuclear Industry Beijing China

The first results of sorption experiments of U(VI), 234.(VI) and 238U(VI) onto original (unpurified) fracture-filling clays from No.1 monzonitic granite intrusion, Beishan area, Gansu Province, China are reported. The monzonitic granite intrusion is a potential location for a high-level radwaste (HLW) repository in China. The present experimental results show that the maximum U(VI) sorption reached 92% at near-neutral pH and the distribution coefficient (Kd) was 1226 mL/g. A high sorption capacity of the fracture-filling clays in host rock on radioactive ele-ments is necessary for HLW deep geological disposal repository. No preferential sorption of 234. onto the clays was found. Finally, the sorption of U(VI) onto the clays was also modeled using a surface complexation model.

关键词： HLW geological disposal repository, granite, uranium, radionuclide, clay, sorption.

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Relationships between bacterial-algal proliferating and mass extinction in the Late Devonian Frasnian-Famennian transition:Enlightening from carbon isotopes and molecular fossils

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Science China Earth Sciences 2005年第10期48卷 1656-1665页

作者： GONG Yiming1,2, XU Ran1, TANG Zhongdao1, SI Yuanlan3 & LI Baohua4.1. Faculty of Earth Science and State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 4.0074. China 2. Institute of Resources & Environments, Henan Polytechnic University, Jiaozuo 4.4.03, China 3. department of Computer Science, South-Central University for Nationalities, Wuhan 4.0074. China 4. Laboratory of Marine geology, Tongji University, Shanghai 200092, China Faculty of Earth Science and State Key Laboratory of Geological Processes and Mineral Resources China University of Geosciences Wuhan China Institute of Resources & Environments Henan Polytechnic University Jiaozuo China department of Computer Science South-Central University for Nationalities Wuhan China Laboratory of Marine geology Tongji University Shanghai China

Studies show positive shifts of inorganic and organic carbon isotope values (δ 13Ccarb and δ 13Ckerogen) from +0.4. (‰ V-PDB) to +3.54.(‰ V-PDB) and from ?29.38 (‰ V-PDB) to ?24.14.(‰ V-PDB), respectively, B* (Ba* = Ba/ (Al2O3 X 15%)) values from 0.015 to 0.14., TOC values from 0.02% to 0.21%, V/Cr values from 0.3 to 2.0, Sr/Ba values from 3.20 to 4..50 in the Late Devonian Frasnian Upper rhenana zone to the top linguiformis zone of the Yangdi sec-tion deposited in carbonate slope facies of Guilin, Guangxi, South China, which indicates that biomass, productivity, organic carbon burial and salinity increase and that oxygenation near the boundary between sediments and waters decreases from the Late Devonian Frasnian Upper rhenana zone to the top linguiformis zone. Abundance of molecular fossils increases and normal alkanes, isoprenoid hydrocarbon, terpanes and steranes are dominated from the Late Devonian Frasnian to the bottom of Famennian, which shows that the predecessors of molecular fossils of the Frasnian-Famennian (F-F) transition are dominated by marine phytoplankton, zooplankton and benthic bacteria with no photosynthesis. Therefore, it is considered that the F-F transitional mass extinction with a multistage, selection and global synchronizing was caused by bacte-rial-algal proliferating, continuing deterioration of the shallow marine ecoenvironment of the mid-dle-lower latitudes. A simple cause and effect chain can be expressed as: appearance of seed plants and multi-storied forests → enhanced chemical and biochemical weathering and pe-dogenesis → wide development of soils → increasing riverine nutrient fluxes in epicontinental sea → from superoligotrophic to eutrophic in epicontinental sea → proliferating of marine phyto-plankton and zooplankton → frequent red tide and anoxia → mass extinction of shallow marine organisms in the middle-lower latitudes. It is worth notice that the factor drawdown of atmos-pheric Pco2, climatic cooling and sea level falling c

关键词： mass extinction, bacteria-algae, carbon isotopes, molecular fossils, biodiversity, Late Devonian, Guangxi, South China.

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Geomorphologic evidence of phased uplift of the northeastern Qinghai-Tibet Plateau since 14.million years ago

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Science China Earth Sciences 2004年第9期47卷 822-833页

作者： LU Huayu1, WANG Xiaoyong1, AN Zhisheng1, MIAO Xiaodong1, ZHU Rixiang3, MA Haizhou2, LI Zhen4. TAN Hongbing2 & WANG Xianyan1 1. State Key Laboratory of Loess and Quaternary geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710075 China 2. Qinghai Institute of Salt Lakes, Chinese Academy of Sciences. Xining 810008, China 3. Institute of geology and Geophysics, Chinese Academy of Sciences, Beijing 100029, China 4. department of Geography, Qinghai Normal University, Xining 810008, China Chinese Acad Sci Inst Earth Environm State Key Lab Loess & Quaternary Geol Xian 710075 Peoples R China Chinese Acad Sci Qinghai Inst Salt Lakes Xining 810008 Peoples R China Chinese Acad Sci Inst Geol & Geophys Beijing 100029 Peoples R China Qinghai Normal Univ Dept Geog Xining 810008 Peoples R China

A typical sequence of fluvial terraces and aeolian deposits overlying these ter- races were multidisciplinary investigated. New evidences for uplift process of the northeastern Qinghai-Tibetan Plateau in the past 14.million years were obtained. At least 11 river terraces along Huangshui, the first-class tributary of Yellow River, at the Xining-Huzhu region are identi- fied. While the first one (T1) is classified as an accumulation terrace, the others are all basement river terraces, which consist of the Tertiary sandstone and siltstone bedrock, fluvial gravel and pebbles and the overlying aeolian loess-Red Clay deposit. Samples from the aeolian deposits were examined for paleomagnetic stratigraphic reconstruction (1030 samples), luminescence dating (16 samples), magnetic susceptibility and grain-size distribution (more than 4.00 sam- ples). The luminescence dating and stratigraphic correlation suggest that terraces of Tll, T10, T8, T7, T3, T2, T1 were formed at 14. 11.3, 1.55, 1.2, 0.15, 0.07 and 0.01 million years ago, re- spectively. Sedimentological analysis and geomorphological observation indicate that formation and evolution of these terraces were mainly driven by tectonic uplift. Therefore, the terrace se- quence provides an ideal geological record, of the uplift process of the northeastern during the past 14.million years, and the timings of the terraces formation are regarded as the timings of tectonic uplift. The significant uplifting events took place at 14. 11.3, 1.2 and 0.15 mil- lion years ago, respectively. The fluvial incision at the Xining-Huzhu region is less than 100 m during a period of ~12 million years in the Miocene era (between the Tll and T9), while the Huangshui River had incised 4.2 m during the past 1.2 million years (from T7 to the present floodplain). The river incision process clearly demonstrates that accelerated rising of the north- eastern Qinghai-Tibet Plateau during the late Cenozoic, and provides new evidence of previous thoughts

关键词： river terrace, tectonic uplift, loess-Red Clay, the past 14 million years, northeastern Qinghai-Tibet Plateau.

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Paleotemperature changes over the past 3000 years in eastern Beijing, China: A reconstraction based on Mg/Sr records in a stalagmite

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Chinese Science Bulletin 2003年第4期48卷 395-400页

作者： MA Zhibang1, LI Hongchun2, XIA Ming1, KU Tehlung2, PENG Zicheng3, CHEN Yushu4.& ZHANG Zhaofeng3 1. Institute of geology and Geophysics, Chinese Academy of Sciences, Beijing 100029, China 2. department of Earth Sciences, University of Southern California, Los Angeles, CA90089-074., usa 3. department of Earth and Space Science, University of Science and Technology of China, Hefei 230026, China 4. Beijing Foshan Tourist Service Centre, Beijing 101201, China Institute of geology and Geophysics. Chinese Academy of Sciences Beijing 100029 China

The Mg/Sr ratio in a stalagmite, which is di-rectly proportional to DMg/Ca, the solid-liquid distribution coefficient of Mg, is proposed as a geochemical thermometer to estimate paleotemperature changes. The paleotempera-ture change in eastern Beijing over the past 3000 years has been reconstructed by using this thermometer in the stalag-mite ZFFS-1 from Jingdong Cave. The records can be di-vided into two periods: 3000—2000 aBP, cool and wet, the air temperature averaging 9.8℃; and 2000 aBP—present, hot and dry, the air temperature being 1℃ higher than the mean value (11.7℃) of the past 3000 years. During 500—200 aBP, the air temperature was about 1.2℃ lower than that of the present, corresponding to the Little Ice Age in Europe. Like d 18O and d 13C, Mg/Sr (or DMg/Ca) reflects an obviously warming trend of the past 200 years. These results are sup-ported by historic records.

关键词：北京京东溶洞石笋 Mg/Sr记录古气温测年 3000年

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Phylogeography of regional fauna on the Tibetan Plateau: A review

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Progress in Natural Science:Materials International 2009年第7期19卷 789-799页

作者： Shujuan Yanga, Hailiang Dongb,c, Fumin Lei d a State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Beijing 100083, China b Geomicrobiology Laboratory, China University of Geosciences, Beijing 100083, China c department of geology, miami University, oxford,{4., usa d Institute of Zoology, Chinese Academy of Sciences, Beijing 100101, China [a]State Key Laboratory of Geological Processes and Mineral Resources China University of Geosciences Beijing 100083 China [b]Geomicrobiology Laboratory China University of Geosciences Beijing 100083 China [c]Department of Geology Miami University Oxford OH 45056 USA [d]Institute of Zoology Chinese Academy of Sciences Beijing 100101 China

The studies of uplift and glaciations of the Tibetan Plateau are summarized, and a series of recent case studies of the endemic species based on DNA sequences are detailed. In general, these molecular data show that all the organisms originated from Early Pliocene to Late Miocene, and then multi-stages of divergence/speciation occurred within each taxa following their original occupation on the plateau, mainly as a result of periodic glacial cycles and geographic isolation. The regional fauna may have undergone several range contractions and expansions during the Pleistocene glaciations. However, the population expansion and refugia may vary in space, time, and extent. The regional fauna of the Tibetan Plateau may be combinations of ancient movement from adjacent zoogeographical regions, speciation in situ, and postglacial colonization from adjacent areas. Geomorphic and climatic changes on the plateau definitely have a remarkable influence on the regional and adjacent biogeographic patterns, and the mechanism is very complex.

关键词： Divergence Refugia Postglacial colonization Phylogeography Regional fauna Tibetan Plateau

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Application of backflush and micro-flow techniques to the analysis of C5—C13 hydrocarbons in crude oils and its geochemical significance

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Progress in Natural Science:Materials International 2007年第11期17卷 1382-1387页

作者： Wang Peirong1,2, Zhao Hong2,3, Xu Guanjun1,4. Zhu Cuishan2,3, Xiao Tingrong4. Zhang Min2,3 and Zhang Bin1,4.1. Key Laboratory of Petroleum Geochemistry, China National Petroleum Corporation, Beijing 100083, China 2. Geochemistry department of Yangtze University, Jingzhou 4.4.23, China 3. Key Laboratory of Exploration Technologies for Oil and Gas Resources, Ministry of Education, Yangtze University, Jingzhou 4.4.23, China 4. Petroleum geology Central Laboratory, Research Institute of Petroleum Exploration and Development, PetroChina, Beijing 100083, China) Key Laboratory of Petroleum Geochemistry China National Petroleum Corporation Beijing 100083 China Geochemistry department of Yangtze University Jingzhou 434023 China Key Laboratory of Exploration Technologies for Oil and Gas Resources Ministry of Education Yangtze University Jingzhou 434023 China Petroleum geology Central Laboratory Research Institute of Petroleum Exploration and Development PetroChina Beijing 100083 China

An Agilent 6890N GC equipped with both FID and Agilent 5975 MSD analyzer has been employed to analyze C5—C13 hydrocarbon fractions of crude oils. A technical combination of program temperature volatilizer injection, backflush and micro-flow controller afforded a fine separation of C5—C13 compounds on a PONA column with the heavy part of crude oils being cut off before entering the analytical column. Both GC-FID chromatogram and GC-MS mass chromatograms (MID and full scan) could be obtained at the same time. The retension time differences of nC6—nC13 alkanes between GC and TIC were in the range of 0.02—0.58 minutes. Totally 286 peaks have been assigned group compositions. Results on 8 typical oil samples from CNPC Key Laboratory Crude Oil Library showed that the characteristics of C6—C13 hydrocarbon group composition could be used in oil-oil correlation studies.

关键词： GC analysis GC/MS analysis backflush micro-flow controller light fraction in crude oil

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Distributions of fatty acids in a stalagmite related to paleoclimate change at Qingjiang in Hubei,southern China

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Science China Earth Sciences 2005年第9期48卷 1463-1469页

作者： XIE Shucheng1,HUANG Junhua1,WANG Hongmei2,YI Yi1,HU Chaoyong1, CAI Yanjun3 & CHENG Hai4.1. Faculty of Earth Science,China University of Geosciences,Wuhan 4.0074.China 2. School of Environmental Studies,China University of Geosciences,Wuhan 4.0074.China 3. SKLLQG,Institute of Earth Environment,Chinese Academy of Sciences,Xi’an 710075,China 4. department of geology and Geophysics,University of Minnesota,MN554.5,usa 1. Faculty of Earth Science China University of Geosciences 430074 Wuhan China 2. School of Environmental Studies China University of Geosciences 430074 Wuhan China 3. SKLLQG Institute of Earth Environment Chinese Academy of Sciences 710075 Xi’an China 4. department of geology and Geophysics University of Minnesota 55455 MN USA

Fatty acids extracted from a subtropical stalagmite at Qingjiang in Southern China’s Hubei Province were analysed using gas chromatography-mass spectrometry. These n-alkanoic acids range from C14.to C26 in carbon number, maximizing at C16, with a second dominance at C22. In contrast to the stalagmite analysed, the overlying soils are characterized by the dominance of heavy-molecular-weight homologues (>C20). The n-fatty acids in the stalagmite were proposed to be contributed by both the soil ecosystems and the microbes harboring in the percolating water and the cave. The ratios of unsaturated to saturated n-fatty acids (C16:1i/C16:0, C18:1/C18:0) appear to show trends comparable with the oxygen isotope records of the stalagmite carbonate, with enhanced values associated with the cold episode such as Heinrich event 1. This paleoclimate-dependent record of the n-fatty acids might reflect microbial changes in physiology and activity in response to the temperature. This record shows somewhat difference from the previous paleoclimate signal extracted from n-alkanols and n-alkan-2-ones of the same stalagmite. The acid record fails to document the well-known Younger Dryas event which was effectively shown by the latter two biomarkers derived from soil ecosystems. This discrepancy might result from the changing biogeochemical impact on different lipid fractions as well as the varied organism populations in different ecosystems.

关键词： biomarker, ecosystem, microbe, speleothem, paleoclimate, Quaternary.

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