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Compression behavior of Zr_(41)Ti_(14)Cu_(12.5)Ni_(10)Be_(22.5) bulk metallic glass up to 24 GPa

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Science China(physics,Mechanics & Astronomy) 2005年第3期48卷 319-324页

作者： LI Gong 1, 2 , ZHAN Zaiji 2 , LIU Jing 3., YUN Jinku 1 , SUN Liling 2 , LIU Riping 1 , ZHANG Jun 2 & WANG Wenkui 1, 2 1. Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004, China 2. center for condensed Matter physics, Institute of physics, Chinese Academy of Sciences, Beijing 100080, China 3. BSRF, Institute of High Energy physics, Chinese Academy of Sciences, Beijing 10003., China 1. Key Laboratory of Metastable Materials Science and Technology Yanshan University 066004 Qinhuangdao China 2. center for condensed Matter physics Institute of Physics Chinese Academy of Sciences 100080 Beijing China 3. BSRF Institute of High Energy Physics Chinese Academy of Sciences 100039 Beijing China

The compression of a Zr41Ti14Cu12.5Ni10Be22.5 bulk metallic glass (BMG) is investigated at room temperature up to 24 GPa using in-situ high pressure energy dispersive X-ray diffraction with a synchrotron radiation source. The pressure-induced structural relaxation is exhibited. It is found that below about 8 GPa, the existence of excess free volume contributes to the rapid structural relaxation, which gives rise to the rapid volumetric change, and the structural relaxation results in the structural stiffness under higher pressure.

关键词： bulk metallic glass, high pressure, structural relaxation, synchrotron radiation.

Approaches to improving critical current density of YBCO superconducting thick films deposited by electrophoresis

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Science China(physics,Mechanics & Astronomy) 2004年第2期47卷 165-172页

作者： ZHU Yabin1,2, ZHOU Yueliang2, LIU Zhen2, WANG Shufang2, CHEN Zhenghao2, L?Huibin2, YANG Guozhen2, XIAO Ling3. REN Hongtao3. JIAO Yulei3.& ZHENG Minghui3.1. Department of physics, College of Science, Beijing Jiaotong University, Beijing 100044, China 2. Laboratory of Optical physics, Institute of physics and {3. for condensed Matter physics, Chinese Academy of Sciences, Beijing 100080, China 3. General Research Institute for Nonferrous Metals, Beijing 100088, China Correspondence should be addressed to Zhu Yabin (email: ybzhu@***) 1. Department of physics College of Science Beijing Jiaotong University 100044 Beijing China 2. Laboratory of Optical physics Institute of physics and center for {3. Matter physics Chinese Academy of Sciences 100080 Beijing China 3. General Research Institute for Nonferrous Metals 100088 Beijing China

Fabrication of YBCO superconducting thick films by electrophoresis has been widely reported. However, the value of critical current density (J c) is far from what the practical application requires. The superconducting thick films are obtained using top-seeded melt growth method with different proportional Y2BaCuO5 (Y211) addition. High-pressure oxygen has been used in the annealing process to improve the uniformity of the oxygen content in the superconducting thick films. When 40mol% Y211 powder is added to the YBa2Cu3.7–5 (Y123. powder,J c for the superconducting thick film by approaches described above reaches 7.008×103.A/cm2 (77 K, 0 T), which is greater than the value ever reported.

关键词： YBCO thick films, electrophoretic deposition, melt-textured.

An Explicit Function Expression for dc Bias and Temperature Dependence of Magnetoresistances in Magnetic Tunnel Junctions

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Journal of Materials Science & Technology 2002年第6期18卷 497-501页

作者： Xiufeng HANState Key Laboratory of Magnetism, Institute of physics and center of condensed Matter physics, Chinese Academy of Sciences, Beijing 100080, China Chinese Acad Sci Inst Phys State Key Lab Magnetism Beijing 100080 Peoples R China Chinese Acad Sci Ctr Condensed Matter Phys Beijing 100080 Peoples R China

An explicit function expression for the bias voltage or/and temperature dependences of tunnel magnetoresistance ratio and resistances were obtained with a unique set of intrinsic parameters. Two of these intrinsic parameters are the Curie temperature TC and the density of state (DOS) for itinerant majority and minority electrons ξ(ρM/ρm), which are the eigen parameters of ferromagnetic electrodes. Others are the spin-dependent matrix-element ratio (i.e., |Td|2/|TJ|2 ) and the anisotropic-wavelength-cutoff energy ECγ of spin-wave spectrum in magnetic tunnel junction (MTJ), which are the structure parameters of an MTJ. These intrinsic parameters can be predetermined using the experimental measurement or, in principle, using the first-principle calculation method for an MTJ with the three key layers of FM/I/FM. Furthermore, a series of experimental data for an MTJ, for example, a spin-valve-type MTJ of Ta (5 nm)/Ni79Fe21(25 nm)/lr22Mn78(12 nm)/Co75Fe25(4 nm)/AI(0.8 nm)-oxide/Co75Fe25(4 nm)/Ni79Fe21(20 nm)/Ta (5 nm) in this work, can be self-consistently evaluated and explained using such concise explicit function formulations.

关键词： Magnetic tunnel junction TMR Spin-electron transport Magnon excitation Spin-polarization Magnetotransport

Collision dynamics of He@C_(60)+He@C_(60) at low energies

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Science China(physics,Mechanics & Astronomy) 2008年第7期51卷 765-772页

作者： ZHAO Qiang1,2, ZHANG FengShou1,2,3.& ZHOU HongYu1,2 1 Key Laboratory of Beam Technology and Material Modification of Ministry of Education, Institute of Low Energy Nuclear physics, Beijing Normal University, Beijing 100875, China 2 Beijing radiation center, Beijing 100875, China 3.center of Theoretical Nuclear physics, National Laboratory of Heavy Ion Accelerator of Lanzhou, Lanzhou 73.000, China 1. Key Laboratory of Beam Technology and Material Modification of Ministry of Education Institute of Low Energy Nuclear Physics Beijing Normal University Beijing 100875 China 2. Beijing radiation center Beijing 100875 China 3. center of Theoretical Nuclear physics National Laboratory of Heavy Ion Accelerator of Lanzhou Lanzhou 730000 China

A semi-empirical molecular dynamics model is developed. The central collisions of C60+C60 and He@C60+He@C60 at different incident energies are investigated based on this model. It is found that the dimer structures have been produced at proper incident energies and these fullerene dimers could be formed by a self-assembly of C60 fullerene and He@C60. The He atom has a significant effect at higher incident energy and this embedded He atom can enhance the stability of the dimer structure.

关键词： C60 He@C60 collision molecular dynamics

The size effect on transport properties of colossal magnetoresistance materials La_(0.67)Ca_(0.3.)MnO_3

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Science China(physics,Mechanics & Astronomy) 2008年第3期51卷 251-257页

作者： LI PeiGang1,2,LEI Ming1,2,GUO YanFeng2,GUO Xi2,CHEN LeiMing2, TANG WeiHua1,2,SONG PengYun3.& CHEN JinPing3.1 Department of physics,center for Optoelectronics Materials and Devices,Zhejiang Sci-Tech University,Hangzhou 3.0018,China 2 National Laboratory for condensed Matter physics,Institute of physics,Chinese Academy of Sciences,Beijing 100080,China 3.Department of physics,Peking University,Beijing 100875,China 1. Department of physics Center for Optoelectronics Materials and Devices Zhejiang Sci-Tech University Hangzhou 310018 China 2. National Laboratory for condensed Matter physics Institute of Physics Chinese Academy of Sciences Beijing 100080 China 3. Department of physics Peking University Beijing 100875 China

High quality La0.67Ca0.3.MnO3.(LCMO) film was deposited via a novel pulsed electron deposition technique on SrTiO3.100) single crystal substrate. The micro-bridge with different widths was fabricated by using electron beam lithography (EBL) technique and their transport properties were studied. For the micro-bridges with width of 2 and 1.5 μm,the insulator-to-metal transition temperature (TP) keeps un-changed compared with the film. For the micro-bridges with width of 1 μm,the TP shifts towards the lower temperature by 50 K. When the width decreases down to 500 nm,the insulator-to-metal transition disappears. The magnetoresistance be-havior of these micro-bridges was studied,and the results show that the low field magnetoresistance (LFMR) decreases and the high field magnetoresistances (HFMR) keep almost unchanged as the width of micro-bridge is reduced.

关键词： colossal magnetoresistance pulsed electron deposition electron beam lithography electrical transport properties

Fluorescence dynamics of interactions between polyamide PyPyPyβDp and DNA

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Science China Chemistry 2006年第1期49卷 75-80页

作者： ZHANG Huijuan1,2, WANG Jin3. WU Yishi1, YUAN Gu3. AI Xicheng1, WANG Li4 & ZHANG Jianping1 1. State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, China 2. School of Life Science and Technology, Beijing Institute of Technology, Beijing 100081, China 3. College of Chemistry and Molecular Engineering, Peking University, Beijing 100080, China 4. center for condensed Matter physics, Institute of physics, Chinese Academy of Sciences, Beijing 100080, China Correspondence should be addressed to Ai Xicheng and Zhang Jianping 1. State Key Laboratory for Structural Chemistry of Unstable and Stable Species Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China 2. School of Life Science and Technology Beijing Institute of Technology Beijing 100081 China 3. College of Chemistry and Molecular Engineering Peking University Beijing 100080 China 4. center for condensed Matter physics Institute of Physics Chinese Academy of Sciences Beijing 100080 China

The photophysical properties of the polyamide PyPyPyβDp (PPP) were investigated by means of steady-state absorption and fluorescence spectroscopies, as well as time-resolved fluo-rescence spectroscopy. It was found that the excited-state properties of PPP are very sensitive to solvents. In TKMC buffer PPP exhibited weak fluorescence with a decay time constant of 16 ps, while with the decrease of the solvent polarity PPP showed the blue-shifted peak position, increased inten-sity and lengthened life-time for its fluorescence behavior. In the presence of calf thymus DNA, it was observed that the fluorescence intensity was enhanced and the fluorescence lifetime increased from 16 to 3. ps for PPP, which verified that PPP bound into the minor groove of DNA duplex.

关键词： polyamide (PPP), calf thymus DNA (ctDNA), time-resolved fluorescence spectroscopy, recognition dynamics.

Colossal magnetoresistive p-n junctions of perovskite oxide La_(0.9)Sr_(0.1)MnO_3.SrNb_(0.01)Ti_(0.99)O_3

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Chinese Science Bulletin 2003年第13期48卷 1328-1330页

作者： L Huibin, DAI Souyu, CHEN Zhenghao, YAN Lei, ZHOU Yueliang & YANG Guozhen Laboratory of Optical physics, Institute of physics & center for {3. Matter physics, Chinese Academy of Sciences, 100080 Beijing, China Laboratory of Optical physics Center for Condensed Matter Physics Chinese Academy of Sciences 100080 Beijing China

We have successfully fabricated the colossal magnetoresistive (CMR) p-n junctions of perovskite oxide La0.9Sr0.1MnO3.SrNb0.01Ti0.99O3.(LSMO/SNTO) with laser molecular beam epitaxy. The I-V characteristics of the LSMO/SNTO p-n junctions as a function of applied magnetic field (05 T) were studied between 100 and 3.0 K. We found that the p-n junction exhibited the CMR behavior. The CMR ratio rR/R0 (rR = RH - R0) is positive in magnetic fields below 0.13.T and at high temperature, while it displays a negative CMR near 100 K and in magnetic fields over 0.13.T. The CMR ratio values are 8% at 0.1 T and 13. at 5 T and 3.0 K, 40% at 0.1 T and 150 K, 10% at 0.13.T and 60% at 5 T and 100 K. The CMR behavior of the p-n junction is different from those of the LaMnO3.compound family.

关键词：巨磁电阻钙钛矿氧化物 LSMO/SNTO CMR 激光分子束外延超导体

Dye-sensitized solar cells: Atomic scale investigation of interface structure and dynamics

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Chinese physics B 2014年第8期23卷 2-12页

作者：马薇张帆孟胜 Beijing National Laboratory for condensed Matter physics and Institute of physics Chinese Academy of Sciences Collaborative Innovation center of Quantum Matter

Recent progress in dye-sensitized solar cells （DSC） research is reviewed, focusing on atomic-scale investigations of the interface electronic structures and dynamical processes, including the structure of dye adsorption onto Ti02, ultrafast electron injection, hot-electron injection, multiple-exciton generation, and electron-hole recombination. Advanced exper- imental techniques and theoretical approaches are briefly summarized, and then progressive achievements in photovoltaic device optimization based on insights from atomic scale investigations are introduced. Finally, some challenges and oppor- tunities for further improvement of dye solar cells are presented.

关键词： dye-sensitized solar cells interface structure absorption electron injection multiple-exciton generation charge recombination

Exotic structure of the third excited state in^(21)Na

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Chinese Science Bulletin 2005年第23期50卷 2677-2680页

作者： LI Xihan1,2,3. LIANG Yujie1,2,3. DENG Fuguo1,2,3. LIU Zuhua1,4 & ZHOU Hongyu1,2,3.1. Key Laboratory of Beam Technology and Material Modification of Minister of Education, Beijing Normal University, Beijing 100875, China 2. Institute of Low Energy Nuclear physics, and Department of Material Science and Engineering, Beijing Normal University, Beijing 100875, China 3. Beijing radiation center, Beijing 100875, China 4. China Institute of Atomic Energy, Beijing 102413. China Key Laboratory of Beam Technology and Material Modification of Minister of Education Beijing Normal University Beijing 100875 China Institute of Low Energy Nuclear physics and Department of Material Science and Engineering Beijing Normal University Beijing 100875 China Beijing radiation center Beijing 100875 China China Institute of Atomic Energy Beijing 102413 China

The probability of the last proton being out of the binding potential, P and the root-mean-square (rms) ra- dius (1/2= of the third excited state in 21Na are calcu- lated by means of asymptotic normalization coefficient (ANC) method with the experimental date existing. The results are P=54.73. and 1/2=5.28 fm respectively. The P value and the contribution of the asymptotic part to the 1/2 are compared with those of several other low energy states in 21Na. It is found that the valence particle in the third excited state has an obvious larger P than those of other states. The density distribution of the valence proton in this state is also compared with the nucleons in the nuclear core 20Ne, and a far extended tail can be seen clearly. These results show that the third ex- cited state in 21Na is a proton halo state.

关键词：钠第三激发态外部结构有效半径密度分布渐近标准化系数