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Dual-symmetry-perturbed all-dielectric resonant metasurfaces for high-Q perfect light absorption

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Chinese Optics Letters 2024年第2期22卷 200-206页

作者：葛俊洋高一骁徐雷周宁沈祥 Laboratory of Infrared Materials and Devices Research Institute of Advanced TechnologiesNingbo UniversityNingbo 315211China Key Laboratory of Photoelectric Detection Materials and Devices of Zhejiang Province Ningbo 315211China Advanced Optics&Photonics Laboratory Department of EngineeringSchool of Science and TechnologyNottingham Trent UniversityNottingham NG118NSUK School of Physics and Optoelectronic Engineering Hangzhou Institute for Advanced StudyUniversity of Chinese Academy of SciencesHangzhou 310024China Ningbo Institute of Oceanography Ningbo 315832China

We demonstrate a high-Q perfect light absorber based on all-dielectric doubly-resonant *** bound states in the continuum(BICs)protected by different symmetries,we manage to independently manipulate the Q factors of the two degenerate quasi-BICs through dual-symmetry perturbations,achieving precise matching of the radiative and nonradiative Q factors for degenerate critical *** achieve a narrowband light absorption with a>600 Q factor and a>99%absorptance atλ_(0)=1550 nm on an asymmetric germanium metasurface with a 0.2λ_(0)*** work provides a new strategy for engineering multiresonant metasurfaces for narrowband light absorption and nonlinear applications.

关键词： resonant metasurface perfect light absorption bound states in the continuum

Electrocatalytic CO_(2) reduction to C_(2)H_(4): From lab to fab

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Journal of Energy Chemistry 2024年第3期90卷 540-564,I0012页

作者： Zeyu Guo Fabao Yang Xiaotong Li Huiwen Zhu Hainam Do Kam Loon Fow Jonathan D.Hirst Tao Wu Qiulin Ye Yaqi Peng Hao Bin Wu Angjian Wu Mengxia xu Department of Chemical and Environmental Engineering and New Materials InstituteUniversity of Nottingham Ningbo ChinaNingbo 315100ZhejiangChina Key Laboratory of Carbonaceous Waste Processing and Process Intensification of Zhejiang Province University of Nottingham Ningbo ChinaNingbo 315100ZhejiangChina Nottingham Ningbo China Beacons of Excellence Research and Innovation Institute University of Nottingham Ningbo ChinaNingbo 315100ZhejiangChina State Key Laboratory of Clean Energy Utilization Department of Energy EngineeringZhejiang UniversityHangzhou 310027ZhejiangChina Institute for Composites Science Innovation(InCSI)and State Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and EngineeringZhejiang UniversityHangzhou 310027ZhejiangChina School of Chemistry University of NottinghamUniversity ParkNottingham NG72RDUK Baima Lake Laboratory Hangzhou 310053ZhejiangChina

The global concerns of energy crisis and climate change,primarily caused by carbon dioxide(CO_(2)),are of utmost ***,the electrocatalytic CO_(2) reduction reaction(CO_(2)RR) to high value-added multi-carbon(C_(2+)) products driven by renewable electricity has emerged as a highly promising solution to alleviate energy shortages and achieve carbon *** these C_(2+) products,ethylene(C_(2)H_(4))holds particular importance in the petrochemical ***,this review aims to establish a connection between the fundamentals of electrocatalytic CO_(2) reduction reaction to ethylene(CO_(2)RRto-C_(2)H_(4)) in laboratory-scale research(lab) and its potential applications in industrial-level fabrication(fab).The review begins by summarizing the fundamental aspects,including the design strategies of high-performance Cu-based electrocatalysts and advanced electrolyzer ***,innovative and value-added techniques are presented to address the inherent challenges encountered during the implementations of CO_(2)RR-to-C_(2)H_(4) in industrial ***,case studies of the technoeconomic analysis of the CO_(2)RR-to-C_(2)H_(4) process are discussed,taking into factors such as costeffectiveness,scalability,and market *** review concludes by outlining the perspectives and challenges associated with scaling up the CO_(2)RR-to-C_(2)H_(4) *** insights presented in this review are expected to make a valuable contribution in advancing the CO_(2)RR-to-C_(2)H_(4) process from lab to fab.

关键词： CO_(2) electroreduction reaction Ethylene Gas diffusion electrode Machine learning Density functional theory Techno-economic analysis

失落的地理诗学:李劼人的中国革命时代的成都书写

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中国现代文学研究丛刊 2024年第5期 48-73页

作者：吴国坤() 胡安定(译) 香港浸会大学中国香港西南大学文学院 400715

李劼人作为一个地方性作家,在一系列小说中富有想象力地呈现了成都的微观历史,个中浓厚的地理历史兴趣和他的生活经历折射了成都独特的现代性转型,凸显了从清帝国到现代民族国家充满暴力和不确定性的转变历程。他通过对历史的微观“空... 详细信息

李劼人作为一个地方性作家,在一系列小说中富有想象力地呈现了成都的微观历史,个中浓厚的地理历史兴趣和他的生活经历折射了成都独特的现代性转型,凸显了从清帝国到现代民族国家充满暴力和不确定性的转变历程。他通过对历史的微观“空间化”来书写自己的家乡,这种微观的视角让作者将地方表述为拥有多元历史和当地日常生活片段之所在,从而挑战了“五四”以来进步的历史观,即单一、普遍的线性历史时间和目的。借助“大河小说”的广阔空间,他将晚清小说的多类代码重新改造为一种开放式的地方写作形式,完成了作为地方记忆载体的三部曲,从而形成了自己独特的风格。李劼人对地方主义和边缘之地的多重表述提供了一种超越精英和通俗二分的视角,从而管窥到地方性的诗学和小说写作的政治性以及地方、区域和国家层面的本土性与现代性之间的深层关联。

关键词：李劼人三部曲地理诗学地方性微观视角

生产性服务业与制造业融合发展的区域比较研究

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中国商论 2024年第13期33卷 130-133页

作者：刘玉丽 Vincent ng Kim Sheng 重庆第二师范学院旅游与服务管理学院重庆400065 SEGi University Malaysi

发展服务型制造、推动生产性服务和制造业融合是供给侧结构性改革的战略选择。从京津沪渝四个直辖市和粤鲁苏浙四个较为发达省份综合来看,制造业与生产性服务业之间存在着一定的关联效应和协同发展趋势,同时存在省市之间、行业之间的分... 详细信息

发展服务型制造、推动生产性服务和制造业融合是供给侧结构性改革的战略选择。从京津沪渝四个直辖市和粤鲁苏浙四个较为发达省份综合来看,制造业与生产性服务业之间存在着一定的关联效应和协同发展趋势,同时存在省市之间、行业之间的分异特征,且生产性服务业整体规模还与工业发展需求不相适应,表现在规模上其对工业的前向关联效应较弱。当然,近期呈现出生产性服务业在增长速度上与工业增速高度相关的发展态势。为更好实现生产性服务业与制造业融合协同发展,我国在服务业供给侧结构性改革进程中要转变制造业和服务业传统“二分法”思维,确立生产性服务业优先发展地位,着力推进研发性服务业高质量发展、坚守健康底线推进环保等高增长领域先行发展和坚持规模化导向推进商务服务业发展。

关键词：生产性服务业制造业融合发展灰色关联分析高质量发展

Experimental and numerical investigation of Weibullian behavior of grain crushing strength

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Geoscience Frontiers 2020年第2期11卷 401-411页

作者： Quanshui Huang Wei Zhou Gang Ma Tang-Tat ng Kun xu State Key Laboratory of Water Resources and Hydropower Engineering Science Wuhan UniversityWuhan 430072China Key Laboratory of Rock Mechanics in Hydraulic Structural Engineering Wuhan UniversityMinistry of EducationWuhan 430072China University of New Mexico AlbuquerqueNM87131USA

The Weibullian behavior of single grain crushing strength was investigated experimentally and numerically with the aim of enhancing the understanding of rock grain *** morphologies of pebble grains were obtained using white light 3D laser scanning and image processing.A grain shape library was constructed for grain shape analysis with different shape *** use of the shape library and grain stability analysis is discussed for a suggested procedure to rotate a grain to its most stable *** grain crushing tests were performed for 30 pebbles to obtain force-displacement curves and fracture *** grain was compressed diametrically between flat *** expected,the values of the stress at bulk fracture follow a Weibull distribution.A procedure for generating crushable agglomerates with realistic particle shapes was demonstrated,which was accomplished in the discrete element modeling(DEM)of the single grain crushing *** work presented here is novel in that both the heterogeneous micro-structures and randomly distributed flaws are *** DEM results demonstrate that the proposed modeling approach and calibrated parameters are reliable and can reflect the crushing behavior of rock ***,three parametric studies were presented evaluating the effects of micro-crack density,micro-crack disorder,and grain morphology on the Weibullian behavior of the crushing strength,none of which has previously been thoroughly *** three studies provide a deeper insight into the origin of the Weibullian behavior of single grain crushing strength.

关键词： Rock grain Grain crushing test Discrete element modeling 3D scanning technique Grain stability Weibullian behavior

基质辅助激光解吸电离-飞行时间质谱法快速测定米饭和乳制品中蜡样芽孢杆菌呕吐毒素Cereulide

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食品科学 2024年第1期45卷 232-238页

作者：曾羲王宇徐巨才黄穗东王涓徐振林华南农业大学食品学院广东省食品质量安全重点实验室广东广州510642 广州市食品检验所广东广州511400 五邑大学生物科技与大健康学院江门市大健康国际创新研究院广东江门529020

建立基质辅助激光解吸电离-飞行时间质谱(matrix-assisted laser desorption ionization time-of-flight mass spectrometry,MALDI-TOF MS)法分析蜡样芽孢杆菌呕吐毒素Cereulide的快速检测方法。分析了Cereulide标准物质的裂解规律,考察基质种类、点靶方式、基质溶剂和用量、激光强度等对Cereulide的质谱信号强度的影响,并进行方法学验证和实际样品检测。结果表明,选择以α-氰基-4-羟基肉桂酸为基质,均匀分散在50%乙腈-水(含0.1%三氟乙酸)中,采用先点基质再点样品的点样方式,反射线性正离子模式下选择激光强度70%进行食品中MALDI-TOF MS筛查时,可检测到Cereulide的[M+Na]^(+)和[M+K]^(+)目标离子峰,此质谱信号稳定、强度高、响应重复性好。方法学验证结果表明,Cereulide的[M+Na]^(+)和[M+K]^(+)目标离子峰在5~100 ng/mL范围内线性好,相关系数(r)>0.99;方法的检出限分别为3.0 ng/g和5.0 ng/g;对米饭和牛乳样品的加标回收率为73.3%~118.2%,相对标准偏差为0.3%~10.9%(n=6)。本方法分析速度快、准确性高、灵敏度好、抗干扰能力强、无需内标即可实现对米饭和乳制品中Cereulide的批量筛查和检测。

关键词：基质辅助激光解吸-电离飞行时间质谱蜡样芽孢杆菌呕吐毒素 α-氰基-4-羟基肉桂酸

Emergency medical services use and its association with acute ischaemic stroke evaluation and treatment in Singapore

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Stroke & Vascular Neurology 2020年第2期5卷 121-127页

作者： Hanzhang xu Ying Xian Fung Peng Woon Janet Prvu Bettger Daniel T Laskowitz Yih Yng ng Marcus Eng Hock ong David Bruce Matchar Deidre Anne De Silva Department of Family Medicine and Community Health Duke University School of MedicineDurhamNorth CarolinaUnited States Duke University School of Nursing DurhamNorth CarolinaUnited States Duke Clinical Research Institute DurhamNorth CarolinaUnited States Department of Neurology Duke University School of MedicineDurhamNorth CarolinaUnited States Department of Neurology National Neuroscience Institute-Singapore General Hospital CampusSingapore Department of Orthopaedic Surgery Duke University School of MedicineDurhamNorth CarolinaUnited States HomeTeam Government of Singapore Ministry of Home AffairsSingapore Department of Emergency Medicine Singapore General HospitalSingapore Program in Health Services and Systems Research Duke-NUS Graduate Medical SchoolSingapore Department of Medicine(General Internal Medicine) Duke University School of MedicineDurhamNorth CarolinaUnited States

Background Emergency medical services(EMS)is a critical link in the chain of stroke *** aimed to assess EMS use for stroke in Singapore,identify characteristics associated with EMS use and the association of EMS use with stroke evaluation and *** The Singapore Stroke Registry combines nationwide EMS and public hospital data for stroke cases in *** regressions with the generalised estimating equations were performed to examine the association between EMS use and timely stroke evaluation and *** Of 3555 acute ischaemic patients with symptom onset within 24 hours admitted to all five public hospitals between 2015 and 2016,68%arrived via *** who used EMS were older,were less likely to be female,had higher stroke severity by National Institute of Health Stroke Scale and had a higher prevalence of atrial fibrillation or peripheral arterial *** transported by EMS were more likely to receive rapid evaluation(door-to imaging time≤25 min 34.3%vs 11.1%,OR=2.74(95%CI 1.40 to 5.38))and were more likely to receive intravenous tissue plasminogen activator(tPA,22.8%vs 4.6%,OR=4.61(95%CI 3.52 to 6.03)).Among patients treated with tPA,patients who arrived via EMS were more likely to receive timely treatment than self-transported patients(door-to needle time≤60 min 52.6%vs 29.4%,OR=2.58(95%CI 1.35 to 4.92)).Conclusions EMS use is associated with timely stroke evaluation and treatment in *** EMS-Hospital stroke pathways and targeted public campaigns to advocate for appropriate EMS use have the potential to improve acute stroke care.

关键词： needle treatment likely

Federated Learning with Privacy-preserving and Model IP-right-protection

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Machine Intelligence Research 2023年第1期20卷 19-37页

作者： Qiang Yang Anbu Huang Lixin Fan Chee Seng Chan Jian Han Lim Kam Woh ng Ding Sheng ong Bowen Li WeBank Shenzhen 518057China Hong Kong University of Science and Technology Hong Kong 999077China University of Malaya Kuala Lumpur 50603Malaysia University of Surrey Guildford GU27XHUK University of Aberystwyth Wales SY233DDUK Shanghai Jiao Tong University Shanghai 200240China

In the past decades,artificial intelligence(AI)has achieved unprecedented success,where statistical models become the central entity in ***,the centralized training and inference paradigm for building and using these models is facing more and more privacy and legal *** bridge the gap between data privacy and the need for data fusion,an emerging AI paradigm feder-ated learning(FL)has emerged as an approach for solving data silos and data privacy *** on secure distributed AI,feder-ated learning emphasizes data security throughout the lifecycle,which includes the following steps:data preprocessing,training,evalu-ation,and *** keeps data security by using methods,such as secure multi-party computation(MPC),differential privacy,and hardware solutions,to build and use distributed multiple-party machine-learning systems and statistical models over different data *** data privacy concerns,we argue that the concept of“model”matters,when developing and deploying federated models,they are easy to expose to various kinds of risks including plagiarism,illegal copy,and *** address these issues,we introduce FedIPR,a novel ownership verification scheme,by embedding watermarks into FL models to verify the ownership of FL models and protect model intellectual property rights(IPR or IP-right for short).While security is at the core of FL,there are still many articles re-ferred to distributed machine learning with no security guarantee as“federated learning”,which are not satisfied with the FL definition supposed to *** this end,in this paper,we reiterate the concept of federated learning and propose secure federated learning(SFL),where the ultimate goal is to build trustworthy and safe AI with strong privacy-preserving and *** provide a com-prehensive overview of existing works,including threats,attacks,and defenses in each phase of SFL from the lifecycle perspective.

关键词： Federated learning privacy-preserving machine learning security decentralized learning intellectual property protection

Unravelling charge carrier dynamics in protonated g-C3N4 interfaced with carbon nanodots as co-catalysts toward enhanced photocatalytic CO2 reduction： A combined experimental and first-principles DFT study

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Nano Research 2017年第5期10卷 1673-1696页

作者： Wee-Jun ong Lutfi Kurnianditia Putri Yoong-Chuen Tan Lling-Lling Tan Neng Li Yun Hau ng Xiaoming Wen Siang-Piao Chai Institute of Materials Research and Engineering (IMRE) Agency for Science Technology and Research (A'STAR) 2 Fusionopolis Way Innovis Singapore 138534 Singapore Multidisciplinary Platform of Advanced Engineering Chemical Engineering Discipline School of Engineering Monash University Jalan Lagoon Selatan Bandar Sunway 47500 Selangor Malaysia Chemical Engineering School of Engineering and Physical Sciences Heriot-Watt University Jalan Venna PS/2 Precinct 5 62200 Putrajaya Malaysia State Key Laboratory of Silicate Materials for Architectures Wuhan University of Technology 122 Luoshi Road Wuhan 430070 China Particles and Catalysis Research Group (PARTCAT) School of Chemical Engineering The University of New South Wales Sydney New South Wales 2052 Australia Australian Centre for Advanced Photovoltaics School of Photovoltaic and Renewable Energy Engineering The University of New South Wales Sydney New South Wales 2052 Australia

In this work, we demonstrated the successful construction of metal-free zero- dimensional/two-dimensional carbon nanodot （CND）-hybridized protonatedg=C3N4 （pCN）（CND/pCN） heterojunction photocatalysts b; means of electrostatic attraction. We experimentally found that CNDs with an average diameter of 4.4 nm were uniformly distributed on the surface of pCN using electron microscopy analysis. The CND/pCN-3 sample with a CND content of 3 wt.% showed thehighest catalytic activity in the CO2 photoreduction process under visible and simulated solar light. This process results in the evolution of CH4 and CO. Thetotal amounts of CH4 and CO generated by the CND/pCN-3 photocatalyst after 10 h of visible-light activity were found to be 29.23 and 58.82 molgcatalyst-1, respectively. These values were 3.6 and 2.28 times higher, respectively, than thearn＊ounts generated when using pCN alone. The corresponding apparent quantum efficiency （AQE） was calculated to be 0.076%. Furthermore, the CND/pCN-3 sample demonstrated high stability and durability after four consecutive photoreaction cycles, with no significant decrease in the catalytic activity.

关键词： protonated graphiticcarbon nitride carbon nanodots photocatalysis carbon dioxide reduction charge carrier dynamics density functional theory(DFT) calculations