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Application of in-situ characterization techniques in modern aqueous batteries

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Rare Metals 2024年第8期43卷 3553-3575页

作者： Jia-Hao wu Hong-wei Cai Zhao-Hui Deng Jean-Jacques Gaumet Yu Bao Wen Luo Department of Physics State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingSchool of Materials Science and EngineeringWuhan University of TechnologyWuhan430070China Laboratoire de Chimie Et Physique:Approche Multi-Echelles Des Milieux Complexes(LCP-A2MC)Institut Jean BarriolUniversitéde Lorraine57070MetzFrance Department of Medicinal Chemistry Hubei College of Chinese MedicineJingzhou 434020China

The development of high-performance aqueous batteries calls for an in-depth knowledge of their chargedischarge redox and failure mechanism,as well as a systematic understanding of the dynamic evolution of microstructure,phase composition,chemical composition,and local chemical environment of the materials for ***-situ characterization technology is expected to understand and reveal the problems faced by aqueous rechargeable batteries,such as the dissolution of electrode materials,the growth of metal negative electrode dendrites,passivation,corrosion,side reactions and a series of *** on this,typical in-situ characterization techniques and their basic mechanisms are summarized,including in-situ optical visualization,in-situ microscopy techniques(in-situ scanning electron microscopy(SEM),in-situ transmission electron microscopy(TEM)),in-situ X-ray techniques(in-situ X-ray diffraction(XRD),in-situ X-ray photoelectron spectroscopy(XPS),in-situ near-edge structural X-ray absorption spectroscopy(XANES)),and in-situ spectroscopy techniques(in-situ Raman spectroscopy,in-situ Fourier transform infrared(FTIR)).Moreover,some emerging techniques concerning aqueous battery research,especially gas evolution and materials dissolution issues,such as in-situ electrochemical quartz crystal microbalance(EQCM).in-situ fiber-optic sensing,in-situ gas chromatography(GC) are *** last,the applications of advanced in-situ characterizations in future research of aqueous batteries are emphasized and discussed,along with some of the remaining challenges and possible solutions.

关键词： Aqueous battery In-situ characterization Phase transformation Solid electrolyte interphase Zinc dendrite growth

Exploring the Mechanism,Advancements,and Application of Thermogalvanic Effect in Hydrogels

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Chinese Journal of Chemistry 2024年第5期42卷 543-556页

作者： Xiaoyu Yang Peng Wang Xiaolong wu Yongli Liao Senyun Liu wei Duan Ying Yue School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBaodingHebei071000 China Hebei Key Laboratory of Electric Machinery Health Maintenance & Failure Prevention North China Electric Power UniversityBaodingHebei071003 China Electric Power Research Institute China South Power GridGuangzhouGuangdong510000 China Key Laboratory of Icing and Anti/De-icing China Aerodynamics Research and Development CenterMianyangSichuan621000 China

The issue of energy consumption has garnered significant interest due to its excessive ***,thermoelectric devices have been getting increased attention,as they can harness waste heat from various sources,such as solar radiation,human body,and industrial ***,the recovery of low-grade heat has been a challenge,resulting in unsustainable energy use and significant *** considerable advances have been made in thermoelectric materials in recent decades,the majority of these devices still primarily employ ***,the emergence of quasi-solid-state thermoelectric materials represents a novel development with profound promise for the environment and *** materials offer several advantages,such as improved energy conversion capacities,cost-effectiveness,versatility,and scalability,to support increased ***,this review explores the application of thermoelectric materials in self-powered sensors,integrated modules,and heat harvesting ***,the potential of high-performance thermocouples based on thermogalvanic effects is assessed,along with the challenges that must be overcome to realize this goal.

关键词： Hydrogel Thermogalvanic effect Thermochemistry Electrolytes Flexible electronics

Dietary supplementation with Neolamarckia cadamba leaf extract improves broiler meat quality by enhancing antioxidant capacity and regulating metabolites

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Animal Nutrition 2024年第2期17卷 358-372页

作者： Cheng Wang Dandan Chen Shou wu wei Zhou Xiaoyang Chen Qing Zhang Li Wang State Key Laboratory of Swine and Poultry Breeding Industry Key Laboratory of Animal Nutrition and Feed Science in South ChinaMinistry of Agriculture and Rural AffairsGuangdong Provincial Key Laboratory of Animal Breeding and NutritionMaoming BranchGuangdong Laboratory for Lingnan Modern AgricultureInstitute of Animal ScienceGuangdong Academy of Agricultural Sciences College of Forestry and Landscape Architecture Guangdong Province Research Center of Woody Forage Engineering TechnologyGuangdong Research and Development Center of Modern Agriculture (Woody Forage) Industrial TechnologyGuangdong Key Laboratory for Innovative Development and Utilization of Forest Plant GermplasmState Key Laboratory for Conservation and Utilization of Subtropical Agro-bioresourcesSouth China Agricultural University

This study was to evaluate the effect of supplementing the diet of broilers with Neolamarckia cadamba leaf extract(NCLE) on meat quality by evaluating antioxidant parameters and the expression of genes in the p38 mitogen-activated protein kinase/nuclear factor-erythroid 2.related factor 2.antioxidant responsive element(p38 MAPK/Nrf2.ARE) signaling pathway, coupled with LC-MS-based metabolomic analysis. A total of 480 one-day-old male broilers were randomly allocated to four treatment groups—a control(CON)group, which was fed a basal diet, and three NCLE treatment groups, which were fed the basal diet supplemented with 100, 2.0, or 400 mg/kg NCLE(N1, N2. and N3 groups, respectively) for 42.d. Compared with the CON group, meat quality was improved in the N2.and N3 groups, as evidenced by the higher p H45min(P 2.ERK1/2., c-Jun N-terminal kinase(JNK), Nrf2. CAT, and GSH-Px(P 2.heme oxygenase, CAT, and superoxide dismutase(SOD)(P < 0.05). Metabolomics analysis revealed that Darabinono-1,4-lactone and lyso-PAF C-16-d4 were negatively correlated with shear force and cooking loss(P < 0.05) and displayed increased abundance in BM of the N3 group. L-Serine levels were upregulated while D-fructose 1,6-diphosphate contents were downregulated in the three NCLE groups. Finally, the differential metabolites in both BM and LM were involved in amino acid metabolism pathwa

关键词： Neolamarckia cadamba leaf extract Broiler Meat quality Antioxidant capacity Metabolomics

WirelessLLM:Empowering Large Language Models Towards Wireless Intelligence

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Journal of Communications and Information Networks 2024年第2期9卷 99-112页

作者： Jiawei Shao Jingwen Tong Qiong wu wei Guo Zijian Li Zehong Lin Jun Zhang Department of Electronic and Computer Engineering The Hong Kong University of Science and TechnologyHong Kong 999077China

The rapid evolution of wireless technologies and the growing complexity of network infrastructures necessitate a paradigm shift in how communication networks are designed,configured,and managed. Recent advancements in large language models (LLMs) have sparked interest in their potential to revolutionize wireless communication systems. However, existing studies on LLMs for wireless systems are limited to a direct application for telecom language understanding. To empower LLMs with knowledge and expertise in the wireless domain, this paper proposes WirelessLLM, a comprehensive framework for adapting and enhancing LLMs to address the unique challenges and requirements of wireless communication networks. We first identify three foundational principles that underpin WirelessLLM:knowledge alignment, knowledge fusion, and knowledge evolution. Then,we investigate the enabling technologies to build WirelessLLM, including prompt engineering, retrieval augmented generation, tool usage, multi-modal pre-training, and domain-specific fine-tuning. Moreover, we present three case studies to demonstrate the practical applicability and benefits of WirelessLLM for solving typical problems in wireless networks. Finally, we conclude this paper by highlighting key challenges and outlining potential avenues for future research.

关键词： large language models multi-modal models wireless communications power allocation spectrum sensing protocol understanding

Attributes of Specialized Households'Resilience and Its Impact on Rural Industrial Advancement:A Case Study of National Musical Instrument Production Specialized Households in Lankao County,Henan,China

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Chinese Geographical Science 2024年第3期34卷 383-400页

作者： wu Nalin wei Yike FAN Sizhe LI Li SUN Yufan ZHANG Yan SHU Yan Key Laboratory of Geospatial Technology for the Middle and Lower Yellow River Regions(Henan University) Ministry of Educa-tion/The College of Geography and Environmental ScienceHenan UniversityKaifeng 475001China College of Urban and Envir-onmental Science Central China Normal UniversityWuhan 430079China Key Laboratory of Ecosystem Network Observation and Modelling Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China

Specialized households serve as the primary units within specialized villages in China,and their capacity to withstand risks and external influences significantly shapes the future trajectory of specialized villages and the overall vitality of the rural *** this study,we established a measurement indicator system based on the definition of specialized households’resilience,elucidating the logical connection between specialized households’resilience and rural industrial development in *** musical instrument industry in Lankao County,Henan Province of China,was employed as a case;survey data,the entropy method,and an obstacle diagnosis model were used to examine how instrument production specialized households responded to the challenges posed by Corona Virus Disease 2.19(COVID-19)and the tightening of national environmental protection policies,yielding the following key findings:1)there exists substantial variation in the comprehensive resilience levels among different specialized households;2.the ability to learn and adapt is the most significant contributor to the overall resilience level of specialized households;3)technological proficiency and access to skilled talent emerge as pivotal factors influencing specialized households’resilience;4)the positioning of specialized households within the industrial supply chain and the stability of their income have a direct bearing on their resilience *** influence of specialized households’resilience on industrial development primarily manifests in the following ways:stronger resilience correlates with increased stability in production and sales,fostering a more proactive approach to future ***,heightened exposure to the external macroeconomic environment can lead to a higher rate of export *** enhance the development resilience of entities like specialized households and family farms,and to invigorate rural economic development,escalating investments in rural science and technology

关键词： resilience specialized households rural industry Lankao County,China

Three-dimensional parametric contact analysis of planetary roller screw mechanism and its application in grouping for selective assembly

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Frontiers of Mechanical Engineering 2024年第1期19卷 53-72页

作者： Huilin HE Peitang wei Huaiju LIU Xuesong DU Rui HU Genshen LIU Yajun wu State Key Laboratory of Mechanical Transmission for Advanced Equipment Chongqing UniversityChongqing 400044China Taiyuan Heavy Machinery Group Co. Ltd.Taiyuan 030024China

The planetary roller screw mechanism(PRSM)is a novel precision transmission mechanism that realizes the conversion between linear and rotary *** contact characteristics of helical surfaces directly determine PRSM’s performance in load-carrying capacity and transmission ***,studying the contact characteristics of PRSM forms the fundamental basis for enhancing its transmission *** this study,a three-dimensional parametric analysis method of contact characteristics is proposed based on the PRSM meshing principle and PyVista(a high-level API to the Visualization Toolkit).The proposed method considers the influence of machining errors among various thread *** effects of key machining errors on contact positions and axial clearance,as well as their sensitivities,are *** excellent solution accuracy,this method exhibits higher calculation efficiency and stronger robustness than the analytical and numerical meshing *** influence of nominal diameter and pitch errors of the screw,roller,and nut on the axial clearance follows a linear relationship,whereas flank angle errors have negligible effects on the axial *** corresponding influence coefficients for these three machining errors on the axial clearance are 0.62.,0.341,and *** variations in contact positions caused by individual errors are *** angle errors and roller diameter errors result in linear displacements of the contact points,whereas pitch errors cause the contact points to move along the arc of the roller *** on the proposed threedimensional parametric contact characteristics analysis method,the Fuzzy C-Means clustering algorithm considering error sensitivity is utilized to establish a component grouping technique in the selective assembly of critical PRSM components,ensuring the rational and consistent clearances based on the given component’s machining *** study provides effective guidance for analyzing conta

关键词： planetary roller screw mechanism(PRSM) contact position axial clearance machining error grouping for selective assembly

Three dimensional discrete element modelling of the conventional compression behavior of gas hydrate bearing coal

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International Journal of Coal Science & Technology 2024年第1期11卷 61-77页

作者： Xia Gao Nannan Wang Baoyong Zhang Qiqi Lin Qiang wu wei Meng Xia Liu Department of Architecture and Civil Engineering Heilongjiang University of Science and TechnologyHarbin150022China School of Qilu Transportation Shandong UniversityJinan250061China Department of Safety Engineering Heilongjiang University of Science and TechnologyHarbin150022China Jining Hongxiang Highway Survey Design and Research Institute Co.Ltd Jining272000China

To analyze the relationship between macro and meso parameters of the gas hydrate bearing coal(GHBC)and to calibrate the meso-parameters,the numerical tests were conducted to simulate the laboratory triaxial compression tests by PFC3D,with the parallel bond model employed as the particle contact constitutive ***,twenty simulation tests were conducted to quantify the relationship between the macro–meso ***,nine orthogonal simulation tests were performed using four meso-mechanical parameters in a three-level to evaluate the sensitivity of the meso-mechanical ***,the calibration method of the meso-parameters were then ***,the contact force chain,the contact force and the contact number were examined to investigate the saturation effect on the meso-mechanical behavior of *** results show that:(1)The elastic modulus linearly increases with the bonding stiffness ratio and the friction coefficient while exponentially increasing with the normal bonding strength and the bonding radius *** failure strength increases exponentially with the increase of the friction coefficient,the normal bonding strength and the bonding radius coefficient,and remains constant with the increase of bond stiffness ratio;(2.The friction coefficient and the bond radius coefficient are most sensitive to the elastic modulus and the failure strength;(3)The number of the force chains,the contact force,and the bond strength between particles will increase with the increase of the hydrate saturation,which leads to the larger failure strength.

关键词： Gas hydrate bearing coal Discrete element method Triaxial compression test Macro-meso mechanical propertie

Advances in ice avalanches on the Tibetan Plateau

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Journal of Mountain Science 2024年第6期21卷 1814-1829页

作者： TANG Minggao LI Guang ZHAO Huanle XU Qiang wu Guangjian YANG wei GUO Daojing State Key Laboratory of Geohazard Prevention and Geoenvironment Protection Chengdu University of TechnologyChengdu 610059China College of Environment and Civil Engineering Chengdu University of TechnologyChengdu 610059China Institute of Tibetan Plateau Research Chinese Academy of SciencesBeijing 100101China

As some of the greatest natural disasters in the cryosphere,ice avalanches(IAs)seriously threaten lives and cause catastrophic damage to the resource environment,but a comprehensive overview of the state of knowledge on IAs remains *** summarized 63 IAs on the Tibetan Plateau(TP)since the 2.th century,of which,over 2. IAs occurred after the 2.st *** distributions of IAs are mainly concentrated in the southeastern and northwestern TP,and the occurrence time of IAs is mostly concentrated from July to *** highlight recent advances in mechanical properties and genetic mechanisms of IAs and emphasize that temperature,rainfall,and seismicity are the inducing *** failure modes of IAs are summarized into 6 categories by examples:slip pulling type,slip toppling type,slip breaking type,water level collapse type,cave roof collapse type,and wedge failure ***,we deliver recommendations concerning the risk assessment and prediction of *** results provide important scientific value for addressing climate change and resisting glacier-related hazards.

关键词： Ice avalanche Global warming Genetic mechanism Risk assessment Tibetan Plateau

PHUI-GA: GPU-based efficiency evolutionary algorithm for mining high utility itemsets

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Journal of Systems Engineering and Electronics 2024年第4期35卷 965-975页

作者： JIANG Haipeng wu Guoqing SUN Mengdan LI Feng SUN Yunfei FANG wei Jiangsu Provincial Engineering Laboratory of Pattern Recognition and Computational Intelligence Department of Computer Science and TechnologyJiangnan UniversityWuxi 214122China China Ship Scientific Research Center Wuxi 214082China Taihu Laboratory of Deepsea Technological Science Wuxi 214082China Department of Mathematics Nanjing UniversityNanjing 210023China

Evolutionary algorithms(EAs)have been used in high utility itemset mining(HUIM)to address the problem of discover-ing high utility itemsets(HUIs)in the exponential search *** have good running and mining performance,but they still require huge computational resource and may miss many *** to the good combination of EA and graphics processing unit(GPU),we propose a parallel genetic algorithm(GA)based on the platform of GPU for mining HUIM(PHUI-GA).The evolution steps with improvements are performed in central processing unit(CPU)and the CPU intensive steps are sent to GPU to eva-luate with multi-threaded *** show that the mining performance of PHUI-GA outperforms the existing *** mining 90%HUIs,the PHUI-GA is up to 188 times better than the existing EAs and up to 36 times better than the CPU parallel approach.

关键词： high utility itemset mining(HUIM) graphics process-ing unit(GPU)parallel genetic algorithm(GA) mining perfor-mance