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The unique spontaneous polarization property and application of ferroelectric materials in photocatalysis

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Nano Research 2024年第5期17卷 3571-3585页

作者： Jinghua An Chang Xu lu Li Bo tang College of Chemistry Chemical Engineering and Materials ScienceKey Laboratory of Molecular and Nano ProbesMinistry of EducationCollaborative Innovation Center of Functionalized Probes for Chemical Imaging in University of ShandongInstitute of Molecular and Nano ScienceShandong Normal UniversityJinan 250014China Laoshan Laboratory 168 Wenhai Middle RdAoshanwei JimoQingdao 266237China

The unique spontaneous polarization property of ferroelectric material makes it to be a special catalyst in *** spontaneous polarization property can induce the formation of built-in electric field,which can improve the separation of photoelectrons and holes to affect photocatalytic *** internal electric field induced by spontaneous polarization can be influenced by multiple factors such as the morphology,the concentration of defect,the type of doped heteroatoms,as well as the composition of ***,the preparation method,pretreating temperature,the strength of prepolarized external electric field of ferroelectric-based photocatalysts as well as the strength of external mechanical force or external magnetic field in photocatalytic reactions can influence the photocatalytic effectivity via influencing spontaneous polarization-induced internal electric ***,it is urgently to unveil the mystery of structure-activity relationships for ferroelectric materials-based photocatalysts,which is usually *** this in mind,this review was provided for the role of various complex influencing factors on ferroelectric materials-based photocatalysis based on the latest advancement in the fields of new energy development,environmental *** the beginning,the basic structure and properties of ferroelectric material are ***,popular synthesis methods of ferroelectric-based photocatalysts are *** that,two main mechanisms of ferroelectric photocatalysis are *** research progress of ferroelectric photocatalysis is then given emphatically according to the classification of photocatalytic ***,the problems existing nowadays and the challenges facing in the future on the application of ferroelectric materials-based photocatalysts are outlined in the summary and outlook section.

关键词： spontaneous polarization photocatalysis ferroelectric separation of electrons and holes

A physics-informed neural network for simulation of finite deformation in hyperelastic-magnetic coupling problems

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Applied Mathematics and Mechanics(English Edition) 2024年第10期45卷 1717-1732页

作者： WANG Lei luO Zikun lu Mengkai tang Minghai Department of Engineering Mechanics College of Mechanics and Engineering SciencesHohai UniversityNanjing 211100China School of Mechanical Engineering and Mechanics Ningbo UniversityNingbo 315211Zhejiang ProvinceChina

Recently,numerous studies have demonstrated that the physics-informed neural network(PINN)can effectively and accurately resolve hyperelastic finite deformation *** this paper,a PINN framework for tackling hyperelastic-magnetic coupling problems is *** the solution space consists of two-phase domains,two separate networks are constructed to independently predict the solution for each phase *** addition,a conscious point allocation strategy is incorporated to enhance the prediction precision of the PINN in regions characterized by sharp *** the developed framework,the magnetic fields and deformation fields of magnetorheological elastomers(MREs)are solved under the control of hyperelastic-magnetic coupling *** examples are provided and contrasted with the reference results to validate the predictive accuracy of the proposed ***,the advantages of the proposed framework in solving hyperelastic-magnetic coupling problems are validated,particularly in handling small data sets,as well as its ability in swiftly and precisely forecasting magnetostrictive motion.

关键词： physics-informed neural network(PINN) deep learning hyperelastic-magnetic coupling finite deformation small data set

Review on the Fabrication of Surface Functional Structures for Enhancing Bioactivity of Titanium and Titanium Alloy Implants

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Chinese Journal of Mechanical Engineering 2024年第4期37卷 23-49页

作者： Heng tang Jiaxiang Xu Bin Guo Yansong Xie Yalong Sun Yanjun lu Yong tang Guangdong Provincial Key Laboratory of Micro/Nano Optomechatronics Engineering College of Mechatronics and Control EngineeringShenzhen UniversityShenzhen 518000China School of Mechanical and Power Engineering Zhengzhou UniversityZhengzhou 450001China

Titanium and its alloys have been widely applied in many biomedical fields because of its excellent mechanical properties,corrosion resistance and good ***,problems such as rejection,shedding and infection will occur after titanium alloy implantation due to the low biological activity of titanium alloy *** structures with specific functions,which can enhance osseointegration and antibacterial properties,are fabricated on the surface of titanium implants to improve the biological activity between the titanium implants and human *** paper presents a comprehensive review of recent developments and applications of surface functional structure in titanium and titanium alloy *** applications of surface functional structure on different titanium and titanium alloy implants are introduced,and their manufacturing technologies are summarized and ***,the fabrication of various surface functional structures used for titanium and titanium alloy implants is reviewed and analyzed in ***,the challenges affecting the development of surface functional structures applied in titanium and titanium alloy implants are outlined,and recommendations for future research are presented.

关键词： Surface functional structure Titanium implant Manufacturing technology Bioactivity

Grain-boundary segregation and grain growth in nanocrystalline substitutional solid solution alloys

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Journal of Materials Science & Technology 2024年第1期168卷 239-249页

作者： Fawei tang Chao Hou Hao lu Zhi Zhao Xiaoyan Song Faculty of Materials and Manufacturing Key Laboratory of Advanced Functional MaterialsMinistry of Education of ChinaBeijing University of TechnologyBeijing 100124China

A model for describing solute segregation at grain boundaries has been developed for substitutional solid solution alloys,which integrates multiple factors from atomic to microstructural scales.A concept of mo-lar Gibbs free energy of segregation was introduced to evaluate the segregating capability of the solute elements in a closed system,through which the influences of grain boundary structure,grain size,ma-terial composition,and external conditions were *** on the evaluation of various energy forms related to solute segregation and grain growth processes,the nature of the thermal stabilization of nanograin structures by solute segregation was disclosed.A criterion for the destabilization of nanostruc-tures,which is determined by the competition of the change rates between the molar Gibbs free energy of segregation and the total energy of grain boundaries with grain size,has been *** study provided guideline to achieve high-temperature stability of nanograin structures of solid solution alloys even for the weakly segregating nanocrystalline systems.

关键词： Substitutional solid solution Grain boundary segregation Thermal stabilization Solute concentration Grain size

Optimal Planning of Hybrid AC/DC Low-voltage Distribution Networks Considering DC Conversion of Three-phase Four-wire Low-voltage AC Systems

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Journal of Modern Power Systems and Clean Energy 2024年第1期12卷 141-153页

作者： Bo Zhang lu Zhang Wei tang Gen Li Chen Wang the College of Information and Electrical Engineering China Agricultural UniversityBeijing 100083China the Electric Energy Group Department of Engineering TechnologyTechnical University of Denmark(DTU)2750 BallerupDenmark the Power Distribution Technology Center State Grid Beijing Electric Power Research InstituteBeijing 100075China

The increasing integration of distributed household photovoltaics(PVs)and electric vehicles(EVs)may further ag gravate voltage violations and unbalance of low-voltage distribu tion networks(LVDNs).DC distribution networks can increase the accommodation of PVs and EVs and mitigate mutilple pow er quality problems by the flexible power regulation capability of voltage source *** paper proposes schemes to es tablish hybrid AC/DC LVDNs considering the conversion of the existing three-phase four-wire low-voltage AC systems to DC op *** characteristics and DC conversion constraints of typical LVDNs are *** addition,converter configura tions for typical LVDNs are proposed based on the three-phase four-wire characteristics and quantitative analysis of various DC ***,an optimal planning method of hybrid AC/DC LVDNs is proposed,which is modeled as a bi-level programming model considering the annual investments and three-phase *** are conducted to verify the effectiveness of the proposed optimal planning *** ulation results show that the proposed optimal planning method can increase the integration of PVs while simultaneously reduc ing issues related to voltage violation and unbalance.

关键词： Optimal planning low-voltage distribution net work three-phase unbalance DC conversion

Facile intercalation of alkali ions in WO_(3)for modulated electronic and optical properties:Implications for artificial synapses and chromogenic application

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Science China(Physics,Mechanics & Astronomy) 2024年第2期67卷 149-160页

作者： Changmeng Huan Zihan lu Silin tang Yongqing Cai Qingqing Ke School of Microelectronics Science and Technology Sun Yat-sen UniversityZhuhai 519082China Guangdong Provincial Key Laboratory of Optoelectronic Information Processing Chips and Systems Sun Yat-sen UniversityZhuhai 519082China Institute of Applied Physics and Materials Engineering University of MacaoTaipaMacao 999078China

Tungsten oxides(WO_(3))are widely recognized as multifunctional systems owing to the existence of rich *** diverse phases exhibit distinct octahedra-tilting patterns,generating substantial tunnels that are ideally suited for ***,a quantitative comprehension regarding the impact of distinct phases on the kinetics of intercalated conducting ions remains ***,we employ first-principles calculations to explore the spatial and orientational correlations of ion transport inγ-and h-WO_(3),shedding light on the relationship between diffusion barriers and the size of the conducting *** findings reveal that different types and concentrations of alkali-metals induce distinct and continuous lattice distortions in WO_(3)***,γ-WO_(3)is more appropriate to accommodate Li+ions,exhibiting a diffusion barrier and coefficient of 0.2. eV and 9.31×10^(-8)cm^(2.s^(-1),***,h-WO_(3)features unidirectional and sizeable tunnels that facilitate the transport of K+ions with an even lower barrier and a high coefficient of 0.11 e V and 2.12.10^(-5)cm^(2.s^(-1),***,the introduction of alkali-metal into WO_(3)tunnels tends to introduce n-type conductivity by contributing s-electrons to the unoccupied W 5d states,resulting in enhanced conductivity and tunable electronic *** alkali metals in WO_(3)tunnels are prone to charge transfer,forming small polaronic states and modulating the light absorption in the visible and nearinfrared *** tunable electronic and optical properties,combined with the high diffusion coefficient,underscore the potential of WO_(3)in applications such as artificial synapses and chromogenic devices.

关键词： WO_(3)polymorphs ion insertion kinetic activity tunable electronic and optical properties iontronics

Power optimization of photovoltaic modules under varying environmental conditions based on current equalization collaborating with constant voltage control

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Clean Energy 2024年第4期8卷 169-182页

作者： DaiBin tang Fei lu Siaw Tzer Hwai Gilbert Thio School of Electrical Engineering Anhui Technical College of Mechanical and Electrical EngineeringWuhu 241002China Centre for Sustainability in Advanced Electrical and Electronics Systems(CSAEES) Faculty of EngineeringBuilt Environment and Information TechnologySEGi University47810 Petaling JayaSelangorMalaysia

The performance of photovoltaic(PV)modules is affected by environmental factors such as irradiance and temperature,which can lead to a decrease in output performance or even *** study proposes an improved formula for calculating the real maximum power of PV modules by analysing the influence of irradiance and temperature.A simulation model is developed using PLECS software to simulate the global maximum power of PV modules under different environmental conditions and the results are compared with the calculated real maximum power.A power optimization scheme for PV modules is then proposed based on current equalization and constant voltage *** scheme employs a single-switch multi-winding forward-flyback converter to equalize the mismatched currents between cell strings,thereby enhancing the output *** proportional-integral controllers are utilized to achieve constant voltage control and obtain the real maximum power of PV *** models are built in the PLECS simulation platform to evaluate the performance of a global maximum power point tracking scheme based on the traditional perturb-and-observe(TPO)algorithm with current equalization,a segment perturb-and-observe algorithm without current equalization,and the proposed power optimization *** simulation results demonstrate that the proposed constant voltage control has greater efficiency than the TPO *** proposed scheme achieves a significant improvement in efficiency,with a 2..87%increase compared with the segment perturb-and-observe algorithm without current equalization.

关键词： current equalization constant voltage control forward-flyback converter PV modules perturb-and-observe(P&O)algorithm

Artificial intelligence-assisted design of new chemical materials: a perspective

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Science China(Information Sciences) 2024年第8期67卷 334-336页

作者： Feng QIAN Wenli DU Weimin ZHONG Yang tang Jingyi lu Key Laboratory of Smart Manufacturing in Energy Chemical Process Ministry of EducationEast China University of Science and Technology

New chemical materials are a fresh category of substances created through chemical reactions or by refining existing materials through secondary processes. By using creative methods, advanced technologies, innovative techniques, and state-of-the-art equipment, these materials(e.g., high-end polyolefin, nano materials) [1] are carefully designed and developed to showcase outstanding performance and unique capabilities beyond what traditional chemical materials can offer [2..

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Spatiotemporal variations of ecosystem services and driving factors in the Tianchi Bogda Peak Natural Reserve of Xinjiang,China

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Journal of Arid Land 2024年第6期16卷 816-833页

作者： ZHU Haiqiang WANG Jinlong tang Junhu DING Zhaolong GONG lu Key Laboratory of Sustainable Development of Xingjiang's Historical and Cultural Tourism Xinjiang UniversityUrumqi 830046China College of Tourism Xinjiang UniversityUrumqi 830046China Ecological Postdoctoral Research Station Xinjiang UniversityUrumqi 830046China College of Ecology and Environment Xinjiang UniversityUrumqi 830017China

Nature reserves play a significant role in providing ecosystem services and are key sites for biodiversity *** Tianchi Bogda Peak Natural Reserve(TBPNR),located in Xinjiang Uygur Autonomous Region,China,is an important ecological barrier area in the temperate arid *** evaluation of its important ecosystem services is of great significance to improve the management level and ecological protection efficiency of the *** the present study,we assessed the spatiotemporal variations of four ecosystem services(including net primary productivity(NPP),water yield,soil conservation,and habitat quality)in the TBPNR from 2.00 to 2.2. based on the environmental and social data using the Integrated Valuation of Ecosystem Services and Trade-offs(InVEST)*** addition,the coldspot and hotspot areas of ecosystem services were identified by hotspot analysis,and the trade-off and synergistic relationships between ecosystem services were analyzed using factor analysis in a geographic *** the study period,NPP and soil conservation values in the reserve increased by 48.2.%and 2..56%,respectively;conversely,water yield decreased by 16.56%,and there was no significant change in habitat ***,both NPP and habitat quality values were higher in the northern part and lower in the southern part,whereas water yield showed an opposite *** analysis revealed that NPP showed a synergistic relationship with habitat quality and soil conservation,and exhibited a trade-off relationship with water *** yield and habitat quality also had a trade-off *** and habitat quality were affected by annual average temperature and Normalized Difference Vegetation Index(NDVI),respectively,while water yield and soil conservation were more affected by digital elevation model(DEM).Therefore,attention should be paid to the spatial distribution and dynamics of trade-off and synergistic relationships between ecosystem services in future ec

关键词： net primary productivity(NPP) water yield soil conservation habitat quality Integrated Valuation of Ecosystem Services and Trade-offs(InVEST)model geographic detector Tianchi Bogda Peak Natural Reserve