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Environmental characteristics of Mid-Holocene recorded by lacustrine sediments from Lake Daihai, north environment sensitive zone, China

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Science China Earth Sciences 2006年第9期49卷 968-981页

作者： SUN Qianli1,2. ZHOU Jie1, SHEN Ji3. CHEN Peng1,2. WU Feng1,2.& XIE Xiuping1,2.1. State Key Lab of Loess and Quaternary Geology, Institute of Earth Environment, Chinese academy of Sciences, Xi’an 710075, China 2. Graduate University of Chinese academy of Sciences, Beijing 10003., China 3. {2. Institute of Geography and Limnology, Chinese academy of Sciences, {2. 2.0008, China State Key Lab of Loess and Quaternary Geology Institute of Earth Environment Chinese Academy of Sciences Xi’an China Graduate University of Chinese academy of Sciences Beijing China nanjing Institute of Geography and Limnology Chinese Academy of Sciences Nanjing China

Climate proxies, such as total organic carbon and nitrogen (TOC, TN), carbonate content (CaCO3., grain-size and pollen of the sediment core retrieved from enclosed Lake Daihai which lies in the north China environment sensitive zone are analyzed to reconstruct the environment evolution of the area based on high-resolution radiocarbon chronology. The results reveal that the TOC and TN contents of the sediments correlate well with pollen percentage and pollen flux variations during the Holocene, and both reach their peak values simultaneously at 6.7―3.5 ka BP (calendar age, 7.6―3.6 ka BP). Since 6.7 ka BP, both the CaCO3.and organic matter contents of the core have simultaneous variations, and their high values also occur during 6.7―3.5 ka BP. While during 9.0―6.7 ka BP (calendar age, 10―7.6 ka BP) relatively lower level of organic matter content and pollen flux corre- spond to the higher level of carbonate content. The above relations suggest that during 6.7―3.5 ka BP, the productivity and effective precipitation were greatly improved in the lake drainage area, and this would probably strengthen the hydrodynamic conditions, enhancing organic matter, pollen and carbonate inputs from terrestrial sources. Such processes would account for the enrichment of both organic matter and carbonate in the sediments. While during 9.0―6.7 ka BP, the lower level of or- ganic matter, pollen flux but high carbonate content show depressed productivity and declined vege- tation coverage. The higher carbonate content at this stage would have probably resulted from the higher evaporation ratio of the lake water under relatively drier climate conditions. Therefore, it is in- ferred that during 6.7―3.5 ka BP, the climate was more humid with abundant rainfalls and vegetation was more flourishing in the Lake Daihai area. This can be seen as Holocene Climate Optimum (HCO). As a result, this has evident discrepancies with the traditional notion that the HCO occurs at Early Holocene or early Mid

关键词： Lake Daihai, Mid-Holocene, lacustrine sediments, environmental characteristics.

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Geochemical simulation of the formation of brine and salt minerals based on Pitzer model in Caka Salt Lake

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Science China Earth Sciences 2004年第8期47卷 720-726页

作者： LIU Xingqi1, CAI Keqin2.& YU Shengsong3.1. nanjing Institute of Geography and Limnology, Chinese academy of Sciences, nanjing 2.0008, China 2. China University of Geosciences, Beijing 100083. China 3. Institute of Salt Lakes, Chinese academy of Sciences, Xining 810008, China nanjing Institute of Geography and Limnology Chinese Academy of Sciences Nanjing China China University of Geosciences Beijing China Institute of Salt Lakes Chinese Academy of Sciences Xining China

The geochemical simulation of the formation of brine and salt minerals based on Pitzer model was made in Caka Salt Lake. The evolution of the mixed surface-water and the mineral sequences were calculated and compared with the hydrochemical compositions of the brine and the salt minerals of the deposit in Caka Salt Lake. The results show that the formation temperature of the lake is between 0°C and 5°C, which is well identical with other studies. The mixing of salt-karst water with the surface waters, neglected by the former researchers, is very important to the formation of the lake, indicating that the initial waters resulting in the formation of the lake are multi-source. It is the first time to use Pitzer model in China for making geochemical simulation of the formation and evolution of inland salt lake and satisfactory results have been achieved.

关键词： Pitzer model,Caka Salt Lake,geochemical simulation,salt-karst water.

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Two possible mechanisms for vortex self-organization

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Science China Earth Sciences 2006年第2期49卷 202-211页

作者： LUO Zhexian2. ZHOU Xiuji1 & GAO Shouting3.1. Chinese academy of Meteorological Sciences, Beijing 100081, China 2. Department of Space Information Science, {3. University of Information Science and Technology, {3. 2.0044, China 3. Institute of Atmospheric Physics, Chinese academy of Sciences, Beijing 10002., China Department of Environmental Science Nanjing University of Information Science and Technology Nanjing China Chinese academy of Meteorological Sciences Beijing China Institute of Atmospheric Physics Chinese Academy of Sciences Beijing China

The vortex self-organization is investigated in this paper by four groups of numerical experiments within the framework of quasi-geostrophic model, and based on the experimental results two types of possible mechanisms for vortex self-organization are suggested. The meso-scale to-pography may enable separated vortices to merge into a larger scale vortex; and the interaction of meso-γ and meso-β scale systems may make separated vortices to self organize a typhoon-like vor-tex circulation.

关键词： vortex, self-organization, meso-scale topography, interaction of different scales.

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Study on lithogeochemistry of Middle Jurassic basalts from southern China represented by the Fankeng basalts from Yongding of Fujian Province

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Science China Earth Sciences 2006年第10期49卷 1020-1031页

作者： ZHOU Jincheng1,2. JIANG Shaoyong1,2. WANG Xiaolei1,2. YANG Jinghong 1,2.& ZHANG Mengqun 3.1. State Key Laboratory of Mineral Deposit Research, nanjing University, nanjing 2.0093. China 2. Department of Earth Sciences, nanjing University, nanjing 2.0093. China 3. Modern Analysis Center, nanjing University, nanjing 2.0093. China State Key Laboratory of Mineral Deposit Research Nanjing University Nanjing China Department of Earth Sciences Nanjing University Nanjing China Modern Analysis Center Nanjing University Nanjing China

There exists an E-W trending Middle Jurassic volcanic zone in southern China. The Fankeng basalts in the Yongding basin of Fujian Province are considered to be a typical example. The Fankeng basalts have TiO2.contents in the range of 1.92.-3.2.%. They are classified as high-Ti basalts. They also have higher total Fe (averaging FeO* = 11.09%). The Middle Jurassic Fankeng basalts from southwestern Fujian have obvious distinctive lithogeochemical features from early Cre- taceous basalts from southeastern coast of China. They have higher HFSE, such as Th, Nb, Ta, Zr and Ti. Their element ratios related with HFSE, such as Zr/Ba, La/Nb, La/Ta ,Zr/Y, Ti/Y, Ba/Nb, K/Ti and Rb/Zr are similar to those of OIB. The most samples have ε Nd(T) of-0.70-0.2., which are near chondrite. Some samples have higher ε Nd(T) of ***, these basaltic magmas might be derived from depleted asthenospheric mantle. The lithogeochemical characteristics of the Fankeng basalts may be caused by interaction between asthenosphere and lithosphere at the time. The (Early-) Middle Jurassic basalts and gabbros from southeastern Hunan, southern Jiangxi and northern Guangdong provinces show similar geochemical features to those of the Fankeng basalts from the Yongding of Fujian. Occurrence of these OIB-type basalts in the area may be regarded as the petrological mark of upwelling of asthenosphere at the time. Upwelling of asthenosphere has led to tectonic extension and the formation of rifted basin in the area.

关键词： interaction between asthenosphere and lithosphere, lithogeochemistry, basalts, Middle Jurassic, southern China.

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Nitrogen isotopic geochemical characteristics of crude oils in several basins of China

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Science China Earth Sciences 2005年第8期48卷 1211-1219页

作者： CHEN Chuanping1,2. MEI Bowen1 & CAO Yacheng3.1. Jianghan Petroleum University, Jingzhou 43.100, China 2. Huazhong University of Science and Technology, Wuhan 43.047, China 3. nanjing Institute of Soil Science, Chinese {3. of Sciences, nanjing 2.0008, China Jianghan Petroleum University Jingzhou China Huazhong University of Science and Technology Wuhan China nanjing Institute of Soil Science Chinese Academy of Sciences Nanjing China

Nitrogen isotopic ratios of crude oils with different physical and chemical properties in several basins of China have been measured and their geochemistry has been studied ele-mentally combined with molecular organic geochemistry methods. The data indicate that δ 15N is in the range of ?6‰-2.‰. They vary with the oils in different sedimentary types of basins. The oils forming in the limnic environment have lower δ 15N with the value of about 1‰-5‰ whereas the oils in saline or semi-saline environment have higher δ 15N, with most samples being above 10‰ and some exceeding 17‰. The average nitrogen isotopic ratio of oils from the Ordovician formation in the Tarim Basin is the lowest, with most samples having δ 15N below zero, which reflects possibly the characteristic of the oils originating mainly from the organic matter formed in marine carbonate sedimentary environment. The δ 15N distribution can be altered by fractionation. It increases obviously because of biodegradation and decreases during hydrocarbon migration. However, the effect of nitrogen isotopic fractionation in the short distance migration is uncon-spicuous.

关键词： nitrogen isotope, crude oil, sedimentary environment, isotopic fractionation, China.

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Holocene grassland vegetation, climate and human impact in central eastern Inner Mongolia

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Science China Earth Sciences 2005年第7期48卷 1025-1039页

作者： HUANG Fei1, Kealhofer Lisa2. XIONG Shangfa3.& HUANG Fengbao1 1. nanjing Institute of Geology and Paleontology,Chinese academy of Sciences,nanjing 2.0008,China 2. Anthropology and Sociology Department,Santa Clara University,CA 95053.USA 3. Institute of Geology and Geophysics,Chinese academy of Sciences,Beijing 10002.,China nanjing Institute of Geology and Paleontology Chinese Academy of Sciences Nanjing 210008 China Anthropology and Sociology Department Santa Clara University CA 95053 United States Institute of Geology and Geoohysics Chinese Academy of Sciences Beijina 100029 China

Phytolith and pollen preserved in the Taipusi Banner paleosol profile, central eastern Inner Mongolia, provide evidence of Holocene grassland vegetation, climate and human impact. The combined phytolith and pollen records reveal a major change in vegetation composition about 5000 a BP. Before 5000 a BP, the vegetation was dominated by Aneurolepidium Chinese-Stipa grandis grassland of C4 grasses. After 5000 a BP, C4 grasses rapidly retreated, indicating a shift to colder and more arid conditions. The gradual invasion of Stipa krylovii, Ag-ropyron desertorum, Ephedra, Chenopodiaceae and Caragana reveal the onset of grassland degeneration. Between 10000 and 872. a BP, the Aneurolepidium Chinese-Stipa grandis grassland included a small proportion of Artemisia shrub and Echionopos type plants, implying a strong winter monsoon and very weak summer monsoon. From 872. to 7000 a BP, C4 grasses were common, indicating a strengthening of the summer monsoon. Between 7000 and 5000 a BP, the Holocene thermal maximum was evident, with a significant expansion of C4 grasses and the presence of some trees (such as Pinus and Betula, and so on) in or near the study site. From 42.0?000 a BP, a sandy grassland of Artemisia and Agropyron desertorum together with Aster-type taxa occurred. Precipitation amelioration took place between 3.00 and 2.70 a BP, with a rapid development of Echinops type plants and a small expansion of C4 grasses. From 2.70 a BP to present, human activities accelerated the process of grassland degeneration.

关键词： phytolith and pollen records grassland environment change human impact Holocene central eastern Inner Mongolia.

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The reconstruction and interpretations of lake status at 6 ka and 18 ka *** inland mainland Asia

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Chinese Science Bulletin 1998年第14期43卷 1145-1157页

作者： QIN Boqiang 1, SHI Yafeng 1 and YU Ge 2. 3.1. nanjing Institute of Geography & Limnology, Chinese academy of Sciences, nanjing 2.0008, China 2. Dynamic Palaeoclimatology, Lund University, PO Box 117, S 2.1 00, Lund, Sweden 3. Department of nanjing Institute of Geography & Limnolagy Chinese Academy of Sciences Nanjing China Dynamic Palaeoclimatology Lund University Lund Sweden Department of Geology and Ocean Sciences Nanjing University Nanjing China

By means of survey of literature through compilations of sedimentological, biogeological and geomorphologic data, the inland lake level changes in arid or semi arid mainland Asia at 6 and 18 ka B.P. have been reconstructed. The results showed that the lakes from western and northwestern Asia were characterized by very high water levels at 18 ka B.P., but low or intermediate water stands at 6 ka B.P. The high lake level in this region was associated with the southward displacement of westerlies, therefore, the extent of the high lake stand indicated the southern flank of westerlies during the glaciation. Conversely, the lakes from the eastern and southern Asia registered comparative low levels at 18 ka B.P. and significantly high one at 6 ka B.P. The lowering of lake level at 18 ka B.P. was caused by the weakened summer monsoon and the high lake level at 6 ka B.P. by the enhanced summer monsoon induced by the enlarged thermal contrast between land and ocean. The extent of high lake levels indicated the northern boundary of monsoon expansion. Between the above two regions, there is a climatic transitional zone in the Central Asia where the lake behavior was close to that in southeastern Asia at 6 ka B.P. but became similar to that in northwestern Asia at 18 ka B.P. Thus this zone became a transitional sector from the monsoon to the westerlies.

关键词： lake status inland mainland Asia westerlies monsoon.

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Adsorption of surfactants onto acrylic ester resins with different pore size distribution

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Science China Chemistry 2006年第5期49卷 445-453页

作者： YANG Weiben1,2.3.LI Aimin1,3.CAI Jianguo1,3.MENG Guanhua1,3.& ZHANG Quanxing1,3.1. State Key Laboratory of Pollution Control and Resource Reuse,School of the Environment,nanjing University,nanjing 2.0093.China 2. nanjing College of Chemical Technology,nanjing 2.0048,China 3. Jiangsu Engineering & Technology Research Center for Organic Toxicant Control and Resource Reuse,nanjing 2.003.,China State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing China nanjing College of Chemical Technology Nanjing China Jiangsu Engineering & Technology Research Center for Organic Toxicant Control and Resource Reuse Nanjing China

In this study, a series of acrylic ester resins with different pore size distribution were prepared successfully by varying the type and the amount of pore-forming agents. In order to inves-tigate the adsorption behavior and mechanism of surfactants on acrylic ester resins, three kinds of surfactants were utilized as adsorbates that were sodium 6-dodecyl benzenesulfonate (6-NaDBS), sodium 1-dodecyl benzene sulfonate (1-NaDBS) and sodium 1-dodecyl sulfonate, respectively. It was observed that the surface area was available in a particular pore size and an appropriate pore size of resins appeared to be more important for the adsorption of surfactants. As compared to commercial acrylic ester resins XAD-7 and HP2.G, 50# and 3.# resins exhibited more excellent adsorption properties toward 1-NaDBS and 6-NaDBS. The experimental equilibrium data were fitted to the Langmuir, and double-Langmuir models. Two models provided very good fittings for all resins over the temperature range studied. The investigation indicated that electrostatic attraction and hydrogen bond between resins and surfactants were the main forces and had an obvious effect on adsorption proc-ess.

关键词： acrylic ester resin, surfactant, adsorption, pore size distribution, isotherm.

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EPR studies of Mn^(2.) in the Loess Plateau of central China: Implication for variation of the East Asia summer monsoon

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Chinese Science Bulletin 1998年第1期43卷 72-75页

作者： CHEN Jun\+1, JI Junfeng\+1, SU Yuanxia\+2.and LU Huayu\+3.. Department of Earth Sciences, nanjing University, nanjing 2.0093. China 2. Center of Material Analysis, nanjing University, nanjing 2.0093. China 3. Xi’an Laboratory of Loess and Qu Department of Earth Sciences Nanjing University Nanjing China Center of Material Analysis Nanjing University Nanjing China Xi’an Laboratory of Loess and Quaternary Geology Chinese Academy of Sciences Xi’an China

Mn 2. EPR intensity recorded in the Chinese loess_paleosol sequence shows close correlation with magnetic susceptibility and Sr content as well as the oscillation of paleoclimate. Thus Mn 2. EPR signal can serve as an... 详细信息

关键词： paleomonsoon loess paleosol EPR signal of Mn 2.

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Study on growth and properties of novel γ-LiAlO_2.substrate

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Science China(Technological Sciences) 2006年第2期49卷 188-193页

作者： ZOU Jun1,2. ZHOU Shengming1, XU Jun1 & ZHANG Rong3.1. Shanghai Institute of Optics and Fine Mechanics, Chinese academy of Sciences, Shanghai 2.1800, China 2. Graduate School of Chinese academy of Sciences, Beijing 10003., China 3. Laboratory of Solid State Microstructures and Department of Physics, {2. University, {2. 2.0093. China Shanghai Institute of Optics and Fine Mechanics Chinese Academy of Sciences Shanghai China Graduate School of Chinese academy of Sciences Beijing China Laboratory of Solid State Microstructures and Department of Physics Nanjing University Nanjing China

Transparent γ-LiAlO2.single crystal has been grown by Temperature Gradient technique. The surface of the wafer annealed in O2.atmosphere at 1100°C for 70 h became opaque and Li-poor phase (LiAl5O8); while, that annealed in Li-rich atmosphere kept transparent and smooth. The full-width at half maximum value dropped to 3. arcsecs when the wafer was annealed in Li-rich atmosphere. That annealed in O2.atmosphere increased to 78 arcsec. Compared with absorption spectra, we can conclude that the 196 nm absorption peak was caused by Li vacancies and the 73. nm peak was caused by O vacancies.

关键词： γ-LiAlO2 crystal, scanning electron micrograph (SEM), absorption spectra.

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