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Journal of Thermal Science 2024年第5期33卷 1867-1882页

作者： LIU Tantao GAO limin LI Ruiyu School of Power and Energy Northwestern Polytechnical UniversityXi'an 710012China School of Aerospace Engineering Xi'an Jiaotong UniversityXi'an 710049China

For complex flows in compressors containing flow separations and adverse pressure gradients,the numerical simulation results based on Reynolds-averaged Navier-Stokes(RANS)models often deviate from experimental measurements more or *** improve the prediction accuracy and reduce the difference between the RANS prediction results and experimental measurements,an experimental data-driven flow field prediction method based on deep learning and l_(1.regularization is proposed and applied to a compressor cascade flow *** inlet boundary conditions and turbulence model parameters are calibrated to obtain the high-fidelity flow *** Saplart-Allmaras and SST turbulence models are used independently for mutual *** contributions of key modified parameters are also analyzed via sensitivity *** results show that the prediction error can be reduced by nearly 70%based on the proposed *** flow fields predicted by the two calibrated turbulence models are almost the same and nearly independent of the turbulence *** corrections of the inlet boundary conditions reduce the error in the first half of the *** turbulence model calibrations fix the overprediction of flow separation on the suction surface near the tail edge.

关键词： experimental data-driven compressor cascade deep learning l_(1.regularization

A universal multifunctional dual cation doping strategy towards stabilized ultra-high nickel cobalt-free lithium layered oxide cathode

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Journal of Energy Chemistry 2024年第8期95卷 296-305,I0007页

作者： Yabin Shen Dongming Yin limin Wang Gang Huang Yong Cheng Henan Institute of Advanced Technology Zhengzhou UniversityZhengzhou 450002HenanChina State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022JilinChina

Ultra-high nickel cobalt-free lithium layered oxides are promising cathode material for lithium-ion batteries(LIBs)because of their relatively high capacity and low ***,the high nickel content would induce bulk structure degradation and interfacial environment deterioration,and the absence of Co element reduces the lithium diffusion kinetics,severely limiting the performance liberation of this kind of ***,a multifunctional Ti/Zr dual cation co-doping strategy has been employed to improve the lithium storage performance of LiNi_(0.9)Mn_(0.1.O_(2)(NM91.*** the one hand,the Ti/Zr co-doping weakens the Li^(+)/Ni^(2+)mixing through magnetic interactions due to the inexistence of unpaired electrons for Ti^(4+)and Zr^(4+),increasing the lithium diffusion rate and suppressing the harmful coexistence of H1.and H2 *** the other hand,they enhance the lattice oxygen stability because of the strong Ti-O and Zr-O bonds,inhibiting the undesired H3 phase transition and lattice oxygen loss,improving the bulk structure and cathode-electrolyte interface *** a result,the Ti/Zr co-doped NM91.NMTZ)exhibits a 91.2%capacity retention rate after 1.0 cycles,while that of NM91.is only82.9%.Also,the NMTZ displays better rate performance than NM91.with output capacities of 1.5 and93 mA h g^(-1.at a high current density of 5 C,***,the designed NMTZ could enable the full battery to deliver an energy density up to 263 W h kg^(-1.,making the ultra-high nickel cobaltfree lithium layered oxide cathode closer to practical applications.

关键词： Lithium-ion battery Ultra-high nickel cobalt-free cathode Ti/Zr co-doping Li^(+)/Ni^(2+)mixing Lattice oxygen stability

Exploring multiple phases and first-order phase transitions in Kármán Vortex Street

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Science China(Physics,Mechanics & Astronomy) 2024年第11期67卷 47-54页

作者： Xu Li Xing Xiang Tingting Xue limin Wang Xiaosong Chen School of Systems Science and Institute of Nonequilibrium Systems Beijing Normal UniversityBeijing 100875China State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy ofSciencesBeijing 100190China School of Chemical Engineering University of Chinese Academy of SciencesBeijing 100049China

Kármán Vortex Street, a fascinating phenomenon of fluid dynamics, has intrigued the scientific community for a long time. Many researchers have dedicated their efforts to unraveling the essence of this intriguing flow pattern. Here, we apply the lattice Boltzmann method with curved boundary conditions to simulate flows around a circular cylinder and study the emergence of Kármán Vortex Street using the eigen microstate approach, which can identify phase transition and its order-parameter. At low Reynolds number, there is only one dominant eigen microstate W_(1. of laminar flow. At Re_(c)^(1.= 53.6, there is a phase transition with the emergence of an eigen microstate pair W^(2,3) of pressure and velocity fields. Further at Re_(c)^(2)= 56, there is another phase transition with the emergence of two eigen microstate pairs W^(4,5) and W^(6,7). Using the renormalization group theory of eigen microstate,both phase transitions are determined to be first-order. The two-dimensional energy spectrum of eigen microstate for W^(1., W^(2,3) after Re_(c)^(1., W^(4-7) after Re_(c)^(2) exhibit-5/3 power-law behavior of Kolnogorov's K41.theory. These results reveal the complexity and provide an analysis of the Kármán Vortex Street from the perspective of phase transitions.

关键词： Kármán Vortex Street first-order phase transition eigen microstate approach renormalization group theory of eigen microstate

Efficient nitrate electroreduction over Mn-doped Cu catalyst via regulating N-containing intermediates adsorption configuration

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Science China Chemistry 2024年第6期67卷 1969-1975页

作者： limin Wu Shunhan Jia Libing Zhang Ruhan Wang Jiaqi Feng Xiaofu Sun Buxing Han Beijing National Laboratory for Molecular Sciences CAS Laboratory of Colloid and Interface and ThermodynamicsCAS Research/Education Center for Excellence in Molecular SciencesCenter for Carbon Neutral ChemistryInstitute of ChemistryChinese Academy of SciencesBeijing100190China School of Chemical Sciences University of Chinese Academy of SciencesBeijing100049China College of Chemical Engineering and Environment China University of PetroleumBeijing102249China Shanghai Key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai200062China

The electrochemical reduction of NO_(3)^(-)to NH_(3)holds promise for economic and environmental benefits,presenting an energyefficient alternative to the traditional Haber-Bosch ***,challenges exist due to its sluggish kinetics,multiple intermediates,and various reaction *** this study,Mn-doped-Cu catalyst was synthesized and employed for electrochemical NO_(3)^(-)-to-NH_(3)*** doping of Mn into Cu resulted in exceptional performance,achieving a FE of 95.8%and an NH_(3)yield rate of 0.91.mol g^(-1.h^(-1.at-0.6 V in a neutral electrolyte at low NO_(3)^(-)*** experimental studies and theoretical calculations revealed that the Mn dopant enhanced the kinetic rate of NO_(2)~--to-NH_(3)and induced a distinct configuration of**** alteration decreased the energy barrier of*NO-to-*NOH,consequently promoting the conversion of NO_(3)^(-)-to-NH_(3).

关键词： nitrate reduction electrocatalysis ammonia synthesis N-intermediate green chemistry

Research on the variation of dielectric properties of oil-paper insulation for power equipment over a wide temperature range

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High Voltage 2024年第3期9卷 648-658页

作者： Mingze Zhang Muhe Yu Wen Zhou Yilin Liang Shengjie Lei Yunbo Shi limin Qu Key Laboratory of Engineering Dielectrics and Its Application Ministry of Education Harbin University of Science and TechnologyHarbinChina School of Measurement and Communication Engineering Harbin University of Science and TechnologyHarbinChina Electric Power Research Institute State Grid Heilongjiang Electric Power Company LimitedHarbinChina

The main part of oil-immersed power equipment is oil-paper *** lower ambient temperatures,transformer oil will become *** a result,compared to those at room temperature or operating temperature,the frequency domain dielectric properties of oil-paper insulation at low temperatures are drastically *** evaluating the insulation condition of electrical equipment,it is essential to accurately determine their dielectric *** paper described the FDS test,the DC conductivity test,and the transformer oil viscosity test,which was carried out in a laboratory environment for different ageing of oil-immersed pressboard and transformer oil at 233–373 *** ef-fects of temperature on the dielectric properties at the competing mechanisms of polarisation and conductivity loss were clarified based on variations of the FDS *** the viscosity change of ageing transformer oil at low temperatures,the Arrhenius and VFT viscosity equations were used to achieve a fitting calculation in the different temperature *** on the molecular/ion transition model in the force field and electric field,the characterisation relationships between the dynamic viscosity,DC conductivity,and test temperature of transformer oil were *** limita-tions of conventional transformer oil equivalent dielectric relaxation models over a wide temperature range were finally clarified by combining the test findings of the DC con-ductivity over a wide temperature range with observed and simulated *** paper provides an essential theoretical reference when using the FDS test to diagnose the insulation performance of oil-immersed power equipment in extremely cold regions.

关键词： insulation viscosity immersed

Unlocking the potential of ultra-thin two-dimensional antimony materials:Selective growth and carbon coating for efficient potassium-ion storage

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Journal of Energy Chemistry 2024年第5期92卷 440-449页

作者： Dongyu Zhang Zhaomin Wang Yabin Shen Yeguo Zou Chunli Wang limin Wang Yong Cheng State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of Sciences(CAS)Changchun 130022JilinChina School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026AnhuiChina

Antimony-based anodes have attracted wide attention in potassium-ion batteries due to their high theoretical specific capacities(∼660 mA h g^(-1.)and suitable voltage ***,severe capacity fading caused by huge volume change and limited ion transportation hinders their practical ***,strategies for controlling the morphologies of Sb-based materials to improve the electrochemical performances have been *** these,the two-dimensional Sb(2D-Sb)materials present excellent properties due to shorted ion immigration paths and enhanced ion ***,the synthetic methods are usually tedious,and even the mechanism of these strategies remains elusive,especially how to obtain large-scale 2D-Sb ***,a novel strategy to synthesize 2D-Sb material using a straightforward solvothermal method without the requirement of a complex nanostructure design is *** method leverages the selective adsorption of aldehyde groups in furfural to induce crystal growth,while concurrently reducing and coating a nitrogen-doped carbon *** to the reported methods,it is simpler,more efficient,and conducive to the production of composite nanosheets with uniform thickness(3–4 nm).The 2D-Sb@NC nanosheet anode delivers an extremely high capacity of 504.5 mA h g^(-1. at current densities of 1.0 mA g^(-1. and remains stable for more than 200 *** characterizations and molecular dynamic simulations,how potassium storage kinetics between 2D Sb-based materials and bulk Sb-based materials are explored,and detailed explanations are *** findings offer novel insights into the development of durable 2D alloy-based anodes for next-generation potassium-ion batteries.

关键词： Antimony Two-dimensional materials Selective growth Nitrogen-doped carbon Potassium-ion batteries

A sponge-based iron-tannic-acid hydrogel interface evaporator designed for clean water production

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Science China(Technological Sciences) 2024年第5期67卷 1579-1591页

作者： ZHANG ZeKun LI ChengLong TAO HuaYu GE Bo ZHANG YongLe ZHAO limin LIU JunChang REN GuiNa ZHANG ZhaoZhu School of Materials Science and Engineering Liaocheng UniversityLiaocheng252059China School of Environmental and Material Engineering Yantai UniversityYantai264405China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China

Due to the rapid advancement of technologies,there has been a significant increase in the discharge of industrial wastewater,and freshwater is becoming a scarce ***,research on solar evaporators is mainly focused on the efficient production of clean water,with less emphasis on the removal of residual pollutants remaining in the original *** this study,problems,including the difficult recovery of catalyst powder and the difficult removal of floating organic matter are solved by co-depositing low-surface-tension zirconia particles and bismuth tungstate onto the floating *** and melamine sponges were combined to solve the problem that traditional hydrogels lack mechanical *** excellent water-repellent effect can be seen from the contact angle between the liquid globule and canvas/felt,which is greater than 1.5°.The steam generation rate of the assembled evaporation system is 1.78 kg m^(-2)h^(-1.,and its purification efficiency for methyl orange and rhodamine B exceeds 99%.This study presents a novel strategy for treating wastewater contaminated with organic dyes,aiming to solve problems including environmental damage,water pollution,and water scarcity.

关键词： oil removal non-wetting interface

Ni/Co bimetallic organic frameworks nanospheres for highperformance electrochemical energy storage

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Nano Research 2024年第6期17卷 5122-5130页

作者： Jianru Guan Minlu Liu limin Zhu Jiamei Wang Qing Han Xiaoxia Yang Weibo Hua Lingling Xie Xiaoyu Cao School of Chemistry and Chemical Engineering Key Laboratory of High Specific Energy Materials for Electrochemical Power Sources of Zhengzhou CityHenan University of TechnologyZhengzhou 450001China School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’an 710049China School of Environmental Engineering Henan University of TechnologyZhengzhou 450001China

In addition to their many well-known advantages(e.g.,ultra-high porosity,good pore size distribution,easy functionalization,and structural tolerability),metal-organic frameworks(MOFs)are a new class of advanced functional ***,their backbones are highly susceptible to deformation after exposure to acidic or alkaline *** a result of lithium-ion batteries embedding or detaching directly from MOFs,they irreversibly *** a result,they fail to maintain their electrochemical *** factors have hindered the development of MOFs as direct electrode materials,making the design of MOF materials with controlled morphology and stable dimensions a new *** this study,we adopted a versatile and effective method to synthesize a novel MOF material(NiCo-BP(BP=BTC/phen and BTC=1.3,5-benzenetricarboxylic acid))using the rigid ligands 1.1.-phenanthroline and homobenzotrizoic acid,and the emergence of the Ni-O/N and Co-O/N coordination layers was observed by extended X-ray absorption fine structure(EXAFS)tests,indicating that Ni and Co were coordinated with heterocyclic N-given atoms to form a stable p-πconjugated ***,the metal-ion is attached to the carboxylic acid ligand on the other side,making the metal-organic skeleton complete and *** nanosphere structure of NiCo-BP(~400 nm)allows for full exposure and utilisation of the active sites,especially the Ni,Co,and phenanthroline units,and exhibit impressively high specific capacity and cycling *** a high current density of 1.0 A·g^(−1.,a high discharge specific capacity of 631.6 mAh·g^(−1.was obtained after 1.00 *** co-participation of two organic ligands in the coordination is in accordance with the theory of soft and hard acids and bases,which contributes to the ability of the material to maintain a high capacity in cycling as well as its cyclic stability.

关键词： lithium-ion batteries metal organic frame electrochemical energy storage dual ligand hard-soft-acid-base

Electric tuning of plasmonic resonances in ultrathin gold nanoribbon arrays

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Photonics Research 2024年第8期12卷 1750-1759页

作者： ZHENXIN WANG ALEXEY VKRASAVIN CHENXINYU PAN JUNSHENG ZHENG ZHIYONG LI XIN GUO ANATOLY VZAYATS limin TONG PAN WANG State Key Laboratory of Extreme Photonics and Instrumentation College of Optical Science and EngineeringZhejiang UniversityHangzhou 310027China Department of Physics and London Centre for Nanotechnology King’s College LondonStrandLondon WC2R 2LSUK Jiaxing Key Laboratory of Photonic Sensing&Intelligent Imaging Intelligent Optics&Photonics Research CenterJiaxing Research Institute Zhejiang UniversityJiaxing 314000China

Ultrathin plasmonic nanostructures offer an unparalleled opportunity for the study of light–matter interactions at the nanoscale and realization of compact nanophotonic *** this study,we introduce an ultrathin gold nanoribbon array and demonstrate an electric approach to actively tuning its plasmonic resonance,which leveraging the extreme light confinement capability in the ultrathin plasmonic nanostructure and a robust nanoscale electro-optical effect in indium tin *** the design(to a total thickness as small as 1. nm for a 2-nmthick gold nanoribbon array),we numerically demonstrate a spectral shift in the plasmonic resonance up to 36 nm along with an approximately 1.%change in the transmission at a gate voltage below 1.7 V at the wavelength of1.47μ*** work presents progress towards electric tuning of plasmonic resonances in ultrathin metallic nanostructures for various applications including surface-enhanced spectroscopy,spontaneous emission enhancement,and optical modulation.

关键词： plasmon tuning realization

Antiglycating effects of citrus flavonoids and associated mechanisms

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Food Science and Human Wellness 2024年第5期13卷 2363-2372页

作者： Yunli Xiao Junfeng Shen Jianfeng Zhan limin Guo Chi-Tang Ho Shiming Li College of Biology and Agricultural Resources Huanggang Normal UniversityHuanggang 438000China Institute of Agro-Products Storage and Processing Xinjiang Academy of Agricultural SciencesUrumqi 830091China Department of Food Science Rutgers UniversityNew Brunswick 08901USA

Glycation of proteins and DNA forms advanced glycation end products(AGEs)causing cell and tissue dysfunction and subsequent various chronic diseases,in particular,metabolic and age-related *** AGE inhibition includes scavengers of reactive carbonyl species(RCS)such as methylglyoxal(MG),glyoxalase-1.enhancers,Nrf2/ARE pathway activators,AGE/RAGE formation inhibitors and other antiglycatng *** flavonoids have demonstrated antioxidant and anti-inflammatory effects and are also found to be effective antiglycating ***,we reviewed the up to date progress of the antiglycation effects of citrus flavonoids and associated *** citrus flavonoids,hesperedin and its aglycone,hesperetin,inhibited glycation by scavenging MG forming mono-or di-flavonoid adducts with MG,enhanced the activity of glyoxase-1.activated Akt/Nrf2 signal pathway while inhibiting AGE/RAGE/NF-κB pathway,reduced the formation of Nε-(carboxylmethyl)lysine(CML)and pentosidine,inhibited aldol reductase activity and decreased the levels of *** antiglycating activity and mechanisms of other flavonoids was also summarized in this *** conclusion,citrus flavonoids possess effective antiglycating activity via different mechanisms,yet there are many challenging questions remaining to be studied in the near future such as in vivo testing and human study of citrus flavonoids for efficacy,effectiveness and adverse effects of citrus flavonoids as a functional food in managing high levels of AGEs and controlling AGE-induced chronic diseases,diabetic complications in particular.

关键词： Citrus flavonoids Hesperedin Advanced glycation end products Antiglycation Diabetic complication