Construction of novel TiO2/Bi4Ti3O(12)/MoS2 core/shell nanofibers for enhanced visible light photocatalysis
Construction of novel TiO2/Bi4Ti3O12/MoS2 core/shell nanofibers for enhanced visible light photocatalysis作者机构:Department of Materials Science and EngineeringXi'an University of Science and TechnologyXi'an710054China School of Safety Science and EngineeringXi'an University of Science and TechnologyXi'an710054China
出 版 物:《Journal of Materials Science & Technology》 (材料科学技术(英文版))
年 卷 期:2020年第36卷第1期
页 面:97-105页
核心收录:
学科分类:081704[工学-应用化学] 081705[工学-工业催化] 07[理学] 08[工学] 070304[理学-物理化学(含∶化学物理)] 070205[理学-凝聚态物理] 0817[工学-化学工程与技术] 0806[工学-冶金工程] 080501[工学-材料物理与化学] 0805[工学-材料科学与工程(可授工学、理学学位)] 0703[理学-化学] 0802[工学-机械工程] 0801[工学-力学(可授工学、理学学位)] 0702[理学-物理学]
基 金:supported financially by the National Natural Science Foundation of China(Nos.21501140,21403165,51372197) the Outstanding Youth Science Fund of Xi’an University of Science and Technology(No.2019YQ2-06) the Key Innovation Team of Shaanxi Province(No.2014KCT-04)
主 题:Electrospinning Bi4Ti3O12 Nanofibers MoS2 Visible light photocatalysis
摘 要:TiO2/Bi4 Ti3 O12 hybrids have been widely prepared as promising photocatalysts for decomposing organic ***,the insufficient visible light absorption and low charge separation efficiency lead to their poor photocatalytic ***,a robust methodology to construct novel TiO2/Bi4 Ti3 O12/MoS2 core/shell structures as visible light photocatalysts is *** bismuth oxyiodide(BiOI) nanoplates were immobilized on electrospun TiO2 nanofiber surface by successive ionic layer adsorption and reaction(SILAR) ***2/Bi4 Ti3 O12 core/shell nanofibers were conveniently prepared by partial conversion of TiO2 to high crystallized Bi4 Ti3 O12 shells through a solid-state reaction with BiOI nanoplates,which is accompanied with certain transition of TiO2 from anatase to rutile ***,MoS2 nanosheets with several layers thick were uniform decorated on the TiO2/Bi4 TiO3 O12 fiber surface resulting in TiO2/Bi4 Ti3 O12/MoS2 *** enhancement of visible light absorption and photo-generated charge separation of TiO2/Bi4 Ti3 O12 were achieved by introduction of *** a result,the optimized TiO2/Bi4 Ti3 O12/MoS2-2 presents 60% improvement for photodegrading RhB after 120 min irradiation under visible light and 3 times higher of apparent reaction rate constant in compared with the TiO2/Bi4 Ti3 *** synthetic method can also be used to establish other photocatalysts simply at low cost,therefore,is suitable for practical applications.