The leaching behavior of simulated HLW glass under repository condition

作     者：ZHANG Hua YANG Jian-Wen LI Bao-Jun LUO Shang-Geng 

作者机构：China Institute of Atomic Energy Beijing 102413 China 

出 版 物：《Nuclear Science and Techniques》 (核技术（英文）)

年 卷 期：2006年第17卷第3期

页      面：158-163页

核心收录：

学科分类：082704[工学-辐射防护及环境保护] 08[工学] 0827[工学-核科学与技术] 

基　　金：International Atomic Energy Agency IAEA: 10637 

主　　题：滤取测试 花岗岩 斑脱土 多屏障系统 HLW-玻璃 

摘      要：As the multibarrier system has been adopted to dispose HLW glass in geological formation in many coun- tries, it was important to study the leaching behavior of vitrification under geological formation. This article describes the leaching behavior of simulated high level waste glass (90Nd/10), which can incorporate 16 wt.% simulated HLW in five kinds of geological media, such as granite, cement, bentonite, Fe3O4, etc. The durable experimental results show that the glass had less mass loss in granite and more mass loss in bentonite after a two-year leaching test. The SEM/XEDS analysis shows some element distributions on the leached specimen’s surface, i.e., Na, Si and Mg ele- ments were reduced on the specimen’s surface, whereas Ba, Al, and Fe were enriched on the specimen’s surface.