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Pollution characteristics of atmospheric dustfall and heavy metals in a typical inland heavy industry city in China

Pollution characteristics of atmospheric dustfall and heavy metals in a typical inland heavy industry city in China

作     者:Jinhe Wang Xi Zhang Qing Yang Kai Zhang Yue Zheng Guanhua Zhou 

作者机构:School of Municipal and Environmental Engineering Shandong Jianzhu University Jinan 250101 China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3) Shanghai 200433 China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012 China School of Instrument Science and Opto-Electronics Engineering Beihang University Beijing 100083 China 

出 版 物:《Journal of Environmental Sciences》 (环境科学学报(英文版))

年 卷 期:2018年第30卷第9期

页      面:283-291页

核心收录:

学科分类:0830[工学-环境科学与工程(可授工学、理学、农学学位)] 07[理学] 070602[理学-大气物理学与大气环境] 0706[理学-大气科学] 

基  金:supported by the Natural Science Foundation of China (Nos. 41205093, 41305124) the National Department Public Benefit Research Foundation (No. 201109005) the Fundamental Research Funds for Central Public Welfare Scientific Research Institutes of China (No. 2016YSKY-025) funded by Opening Project of Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (No. FDLAP18005) National Key Research & Development Program of China (No. 2016YFE0112200) 

主  题:Atmospheric dustfall Heavy metal Deposition flux Factor analysis Zhuzhou city 

摘      要:Through field sampling of atmospheric dustfall in regions of Zhuzhou City, China for a period of one year, the deposition fluxes of atmospheric dustfall and five heavy metals contained inside, including Cr, As, Cd, Hg and Pb, were analyzed. Meanwhile the enrichment factor and index methods were used to analyze the pollution characteristics of heavy metals of atmospheric dustfall in Zhuzhou. The annual deposition flux of atmospheric dustfall in Zhuzhou was 50.79 g/(m^***), while the annual deposition fluxes of Cr, As, Cd, Hg and Pb were 9.80, 59.69, 140.09, 0.87 and 1074.91 mg/(m^***), respectively. The pollution level of atmospheric dustfall in Zhuzhou was relatively lower compared with most other cities in China, but the deposition fluxes of As, Cd, Hg and Pb in atmospheric dustfall in Zhuzhou were much higher than that in most cities and regions around the world. Cd is the typical heavy metal element in atmospheric dustfall in Zhuzhou, and both the enrichment factor and pollution index of Cd were the highest. Cd, Hg, Pb and As in atmospheric dustfall were mainly from human activities. According to the single-factor index, Nemerow index and pollution load index analyses, the atmospheric dustfall in Zhuzhou could easily cause severe heavy metal pollution to urban soil, and the most polluting element was Cd, followed by Pb, As and Hg. Only the pollution level of Cr lay in the safety region and mainly originated from natural sources.

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