Degradation of phenol using a combination of granular activated carbon adsorption and bipolar pulse dielectric barrier discharge plasma regeneration

作     者：唐首锋 李娜 綦金榜 袁德玲 李杰 

作者机构：Hebei Key Laboratory of Applied ChemistrySchool of Environmental and Chemical EngineeringYanshan University Institute of Electrostatics and Special PowerDalian University of Technology 

出 版 物：《Plasma Science and Technology》 (等离子体科学和技术（英文版）)

年 卷 期：2018年第20卷第5期

页      面：92-100页

核心收录：

学科分类：083002[工学-环境工程] 0830[工学-环境科学与工程（可授工学、理学、农学学位）] 08[工学] 

基　　金：financially supported by National Natural Science Foundation of China(Project No.51608468) the Natural Science Foundation of Hebei Province(Project Nos.B2015203303 and B2015203300) the China Postdoctoral Science Foundation(Project Nos.2015M580216 and 2016M601285) the Youth Teacher Independent Research Program of Yanshan University(Project No.15LGA013) the Hebei Province Preferred Postdoctoral Science Foundation(B2016003019) the Open Foundation of Key Laboratory of Industrial Ecology and Environmental Engineering(MOE) 

主　　题：granular activated carbon regeneration dielectric barrier discharge plasma phenoldegradation bipolar pulse power 

摘      要：A combined method of granular activated carbon（GAC） adsorption and bipolar pulse dielectric barrier discharge（DBD） plasma regeneration was employed to degrade phenol in *** being saturated with phenol,the GAC was filled into the DBD reactor driven by bipolar pulse power for regeneration under various operating *** results showed that different peak voltages,air flow rates,and GAC content can affect phenol decomposition and its major degradation intermediates,such as catechol,hydroquinone,and *** higher voltage and air support were conducive to the removal of phenol,and the proper water moisture of the GAC was 20%.The amount of H2 O2 on the GAC was quantitatively determined,and its laws of production were similar to phenol *** the optimized conditions,the elimination of phenol on the GAC was confirmed by Fourier transform infrared spectroscopy,and the total removal of organic carbons achieved 50.4%.Also,a possible degradation mechanism was proposed based on the HPLC ***,the regeneration efficiency of the GAC was improved with the discharge treatment time,which attained 88.5% after 100 min of DBD processing.